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At least 1,639 records · Page 91
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DOE OSTI2024

Extended Interacting Boson Model with Configuration Mixing Description For 98 Mo

An extended version of the interacting boson model (IBM), encompassing two-particle–two-hole (2p-2h) excitations originating from below a valence shell and one-particle–one-hole (1p-1h) excitations extending to the upper next-nearest major shell, is developed to investigate cross-shell excitation effects in the transitional nucleus 98 Mo. This extended IBM framework is utilized to reproduce experimentally observed properties such as low-lying positive-parity level energies, 𝐵⁡(𝐸⁢2) values, and the electric quadrupole moment of the 2$^{+}_{1}$ state, 𝜌 2 ⁡(𝐸⁢0, 0$^{+}_{2}$ → 0$^{+}_{g}$), as well as the strength functions of the isoscalar giant monopole resonance (ISGMR) and the isoscalar giant quadrupole resonance (ISGQR) in 98 Mo. It is shown that the extended consistent-𝑄 IBM, incorporating configuration mixing of both 2p-2h excitations from below the valence shell and 1p-1h excitations to the upper next-nearest major shell, describes the low-lying structural properties and the ISGMR and ISGQR strength distributions of 98 Mo quite well, with the ISGMR and the ISGQR strength distributions comparable to the results of the self-consistent quasiparticle random-phase approximation with Skyrme interactions.

90 ≤ A ≤ 149↗
DOE OSTI2024

Analog-antianalog isospin mixing in 47 K 𝛽−decay

Here, we have measured the isospin mixing of the 𝐼 𝜋 =1/2 + , 𝐸 𝑥 = 2.599 MeV state in nearly doubly magic 47 Ca with the isobaric analog 1/2 + state of 47 K . Using the TRIUMF atom trap for 𝛽 decay, we have measured a nonzero asymmetry of the progeny 47 Ca with respect to the initial 47 K spin polarization, which together with the 𝛽 asymmetry implies a nonzero ratio of Fermi to Gamow-Teller matrix elements 𝑦 = 0.098 ± 0.037 for the 1/2 + → 1/2 + transition. Interpreting 𝑦 as mixing between this state and the isobaric analog state implies a Coulomb matrix element magnitude 101 ± 37 keV. This relatively large matrix element supports a model from the literature of analog-antianalog isospin mixing, which predicts large matrix elements in cases involving excess neutrons over protons occupying more than one major shell. The result supports pursuing a search for time-reversal odd, parity-even, isovector interactions using a correlation in 47 K 𝛽 decay.

beta decay↗
DOE OSTI2024

𝐵⁡(𝐸⁢2) measurements in the yrast band of 28 Mg: Implications for the 𝑁 = 20 island of inversion

High-precision lifetime measurements in 28 Mg were performed to study neutron shell evolution in Mg isotopes and the onset of the N = 20 island of inversion. Here, using both the recoil distance and Doppler shift attenuation methods, five lifetimes were measured in addition to six upper limits. The observation of two long-lived, negative-parity states demonstrate the importance of studying Mg isotopes for the contribution of intruder configurations to sd-shell nuclei. Lifetimes of the $2^+_1$ and $4^+_1$ states of 1.81(5) ps and 172⁢($^{+11}_{–10}$) stat.⁢ (4) stop. ⁢(8) feed.⁢ (4) targ. fs, respectively, demonstrate a loss of collectivity with increasing spin in the yrast band, permitting for distinguishing between current theoretical models. These measurements also highlight the progression of yrast structure across the Mg isotopic chain from rotational at N = 12 to large shape mixing at N = 16 and back to collective behavior at N = 20 but with dominating intruder configurations.

20 ≤ A ≤ 38↗
DOE OSTI2025

Direct observation of 𝛽 and 𝛾 decay from a high-spin long-lived isomer in 187 Ta

187 Ta (Z = 73, N = 114) is located in the neutron-rich A ≈ 190 region where a prolate-to-oblate shape transition via triaxial softness is predicted to take place. A preceding work on the K π = (25/2 - ) isomer and a rotational band to which the isomer decays carried out by the same collaboration revealed that axial symmetry is slightly violated in this nucleus. Here, this paper focuses on a higher-lying isomer, which was previously identified at 2933(14) keV by mass measurements with the Experimental Storage Ring at GSI. The isomer of interest has been populated by a multinucleon transfer reaction with a 136 Xe primary beam incident on a natural tungsten target, using the KEK Isotope Separation System at RIKEN. New experimental findings obtained in the present paper include the internal and external β-decay branches from the high-spin isomer and a revised half-life of 136(24) s. The evaluated hindrances for K-forbidden transitions put constraints on the spin-parity assignment, which can be interpreted as being ascribed to a prolate shape with a five-quasiparticle configuration by model calculations.

beta decay↗
DOE OSTI2025

Precise mass measurement of the longest odd-odd chain of nuclei with 1+ ground states

Precise mass measurements of the ground and isomeric states of the odd-odd Rh108,110,112,114,116 were performed using the Canadian Penning Trap at Argonne National Laboratory, showing good agreement with recent JYFLTRAP measurements. A new possible isomeric state of Rh114 was also observed. These isotopes are part of the longest odd-odd chain of identical ground-state spin-parity assignment of 1+, spanning Rh104–118, despite being in a region of deformation. Realistic phenomenological mean-field calculations using the “universal” Wood-Saxon Hamiltonian were performed, which explained this phenomenon for the first time. In addition, multiquasiparticle blocking calculations were performed to study the configuration of low-lying states in the odd-odd Rh nuclei, elucidating anomalous isomeric yield ratio observed for Rh114.

Liu, B↗
DOE OSTI2025

Decay spectroscopy of an isomeric state in Md251

Excited states in Md251 have been populated by decay of an isomeric state at Ex≈1174 keV and studied via delayed γ-ray spectroscopy. We observe the population of two rotational bands, one of which we identify as the Nilsson π72[514] ground-state band and the other we propose is based on the π92[624] configuration. From the observed decay pattern, we suggest that the isomer spin parity is 232+, with the three-quasiparticle configuration π72[514]⊗{ν72[624]⊗ν92[734]}Kπ=8−. We compare our results to theoretical predictions of the single- and multi-quasiparticle structure of Md251.

Morse, C↗
DOE OSTI2025

Quenching of the octupole rotational band in 71 Ge

The main goal of this study was to enhance the knowledge of the properties of the known octupole rotational band in 71 Ge, including transition rates, and to investigate whether the band persists to higher spin. An experiment at Florida State University using the 62 Ni ( 14 C, 𝛼⁢𝑛) reaction at 50 MeV was used to produce 71 Ge at high spin. An array of ten Compton-suppressed Ge detectors, consisting of three Clover detectors and seven single-crystal detectors, was used to measure the 𝛾 decays in coincidence. An analysis of the resulting coincidence spectra resulted in the placement of 13 additional transitions in the 71 Ge level scheme, one of which (1092 keV) extends the octupole band to a (35/2 − ) state at 8206 keV. However, calculations of the kinematic moment of inertia show that the 1092-keV transition disrupts the rigid rotational pattern and is likely associated with a band crossing, potentially quenching the octupole deformation. Transition strengths inferred from lifetime measurements in the octupole band are not well reproduced by either shell-model calculations using the JUN45 interaction or a semimicroscopic cluster model, while those for the 𝜈⁢𝑔 9/2 band are in good agreement with the corresponding shell-model predictions. Comparisons between the octupole band in 71 Ge and negative-parity bands based on 3 − octupole states in some neighboring even-even nuclei show both similarities and differences. Systematic trends within the 𝜈⁢𝑔 9/2 bands among odd-𝐴 Ge isotopes point to increased collectivity near 𝑁 = 40.

59 ≤ A ≤ 89↗
DOE OSTI2011

Emergence of the N=16 shell gap in {sup 21}O

The spectroscopy of {sup 21}O has been investigated using a radioactive {sup 20}O beam and the (d,p) reaction in inverse kinematics. The ground and first excited states have been determined to be J{sup {pi}=}5/2{sup +} and 1/2{sup +}, respectively. Two neutron unbound states were observed at excitation energies of 4.77(10) and 6.17(11) MeV. The spectroscopic factor deduced for the lower of these, interpreted as a 3/2{sup +} level, reveals a relatively pure (60%) 0d{sub 3/2} single-particle configuration, in good agreement with shell-model calculations that predict {sup 26}O to be unbound. The large energy difference between the 3/2{sup +} and 1/2{sup +} states is indicative of the emergence of the N=16 shell gap, which is estimated to be 5.1(11) MeV. For the higher-lying resonance, which has a character consistent with a spin-parity assignment of 3/2{sup +} or 7/2{sup -}, a 0.71(22) branching ratio to the first 2{sup +} state in {sup 20}O has been observed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2011

Identification of high-spin states in the stable nucleus {sup 195}Pt

Excited states of the stable nucleus {sup 195}Pt have been studied using an in-beam {gamma}-ray spectroscopic technique following the incomplete fusion of {sup 7}Li on an {sup 192}Os target at 44 MeV. A level scheme built on the I{sup {pi}=}13/2{sup +} isomer has been established up to I{sup {pi}=}33/2{sup -} at an excitation energy of about 2.6 MeV. Spin and parity values of these states have been assigned from an analysis of anisotropy ratios of {gamma} rays and by analogy with the neighboring nuclei. A comparison of the observed structures with the yrast states in the neighboring even-even {sup 196}Pt core indicates that the identified levels may be regarded as arising from the weak coupling of a {nu}i{sub 13/2} neutron hole to the core states.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2011

Production of 26 Al in stellar hydrogen-burning environments: Spectroscopic properties of states in 27 Si

Model predictions of the amount of the radioisotope Al-26 produced in hydrogen-burning environments require reliable estimates of the thermonuclear rates for the Al-26g(p,gamma) Si-27 and Al-26m(p,gamma)Si-27 reactions. These rates depend upon the spectroscopic properties of states in Si-27 within about 1 MeV of the Al-26g + p threshold (S-p = 7463 keV). We have studied the Si-28(He-3,alpha)Si-27 reaction at 25 MeV using a high-resolution quadrupole-dipole-dipole-dipole magnetic spectrograph. For the first time with a transfer reaction, we have constrained J(pi) values for states in Si-27 over E-x = 7.0-8.1 MeV through angular distribution measurements. Aside from a few important cases, we generally confirm the energies and spin-parity assignments reported in a recent gamma-ray spectroscopy study. The magnitudes of neutron spectroscopic factors determined from shell-model calculations are in reasonable agreement with our experimental values extracted using this reaction.

Parikh, A.↗
DOE OSTI2013

Neutron-skin uncertainties of Skyrme energy density functionals

Neutron-skin thickness is an excellent indicator of isovector properties of atomic nuclei. As such, it correlates strongly with observables in finite nuclei that depend on neutron-to-proton imbalance and the nuclear symmetry energy that characterizes the equation of state of neutron-rich matter. A rich worldwide experimental program involving studies with rare isotopes, parity-violating electron scattering, and astronomical observations is devoted to pinning down the isovector sector of nuclear models. We assess the theoretical systematic and statistical uncertainties of neutron-skin thickness and relate them to the equation of state of nuclear matter, and in particular to nuclear symmetry energy parameters. We use the nuclear superfluid density functional theory with several Skyrme energy density functionals and density dependent pairing. To evaluate statistical errors and their budget, we employ the statistical covariance technique. We find that the errors on neutron skin increase with neutron excess. Statistical errors due to uncertain coupling constants of the density functional are found to be larger than systematic errors, the latter not exceeding 0.06 fm in most neutron-rich nuclei across the nuclear landscape. The single major source of uncertainty is the poorly determined slope $L$ of the symmetry energy that parametrizes its density dependence. To provide essential constraints on the symmetry energy of the nuclear energy density functional, next-generation measurements of neutron skins are required to deliver precision better than 0.06 fm.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2013

Electromagnetic properties of the 2+ state in 134Te: Influence of core excitation on single-particle orbits beyond 132Sn

The g factor and B (E2) of the first excited 2+ state have been measured following Coulomb excitation ofthe neutron-rich semimagic nuclide 134Te (two protons outside 132Sn) produced as a radioactive beam. The precision achieved matches related g-factor measurements on stable beams and distinguishes between alternative models. The B(E2) measurement exposes quadrupole strength in the 2+ state beyond that predicted by current large-basis shell-model calculations. This additional quadrupole strength can be attributed to coupling between the two valence protons and excitations of the 132Sn core. However, the wave functions of the low-excitation positive-parity states in 134Te up to 6+ remain dominated by the (g7/2)2 configuration.

Stuchbery, Andrew E↗
DOE OSTI2014

β decay of V 61 , 63 and low-energy level schemes of Cr 61 , 63

Near N = 40, rapid development of collectivity has been inferred based on the low-energy level schemes of the even-even Fe and Cr isotopes and attributed to deformation arising primarily from the influence of the ν g 9/2 intruder orbital. The level schemes of the odd-A Co and Fe isotopes, as well as the odd-odd Co and Mn isotopes, are also influenced by the g 9/2 orbital and suggest prolate deformation. However, scarce information is available regarding the neutron-rich odd-A Cr isotopes. Furthermore the distinct difference between the low-energy level scheme of 61 Cr and the lighter neutron-rich odd-A Cr isotopes is inferred to be due to the influence of the g 9/2 intruder orbital and suggests the possibility of low-energy positive-parity states in 61 Cr, leading to the conclusion that a significant change in deformation and orbital occupancies has taken place when N exceeds 36.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

Search for unbound Be 15 states in the 3 n + Be 12 channel

Background: Be-15 is expected to have low-lying 3/2(+) and 5/2(+) states. A first search did not find the 3/2(+) [A. Spyrou et al., Phys. Rev. C 84, 044309 (2011)]; however, a resonance in Be-15 was populated in a second attempt and determined to be unbound with respect to Be-14 by 1.8(1) MeV with a tentative spin-parity assignment of 5/2(+) [J. Snyder et al., Phys. Rev. C 88, 031303(R) (2013)]. Purpose: Search for the predicted Be-15 3/2(+) state in the three-neutron decay channel. Method: A two-proton removal reaction from a 55 MeV/u C-17 beam was used to populate neutron-unbound states in Be-15. The two-, three-, and four-body decay energies of the Be-12+ neutron(s) detected in coincidence were reconstructed using invariant mass spectroscopy. Monte Carlo simulations were performed to extract the resonance and decay properties from the observed spectra. Results: The low-energy regions of the decay energy spectra can be described with the first excited unbound state of Be-14 (E-x = 1.54 MeV, E-r = 0.28 MeV). Including a state in Be-15 that decays through the first excited Be-14 state slightly improves the fit at higher energies though the cross section is small. Conclusions: A Be-15 component is not needed to describe the data. If the 3/2(+) state in Be-15 is populated, the decay by three-neutron emission through Be-14 is weak,

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗