Secondary ion mass spectrometry signatures for verifying declarations of fissile‐material production
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The Department of Energy’s National Nuclear Security Administration (DOE/NNSA) provides advanced capabilities to simulate the uranium enrichment process to support international negotiations on the peaceful use of nuclear energy. Uranium isotope separation centrifuges connected in a cascade configuration can produce the low-enriched uranium needed for nuclear power. However, those same centrifuges connected in a different configuration can also produce highly enriched uranium for nuclear weapons. Having the capability to assess cascade operations and identify nefarious activities promotes the peaceful uses of nuclear energy while restricting nuclear weapons proliferation. DNN R&D's Nonproliferation Stewardship Program Adaptive Computing Environment and Simulations (ACES) project is creating a modern, sustainable ecosystem of physics-based models and data-analytics tools that enables analysts to model uranium enrichment systems, simulate operational scenarios, and apply various policy options to explore potential outcomes.
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This presentation begins by discussing the importance and significance of cross section fluctuations. It also discusses the motivation and overarching goals which are to establish the highest fidelity nuclear evaluated data. In conclusion, a procedure to accurately model the measured cross section fluctuations for inclusion into evaluated nuclear data files was developed and tested on 239 Pu total cross sections. The procedure consisted of defining population of levels as well as related amplitudes extrapolated from the systematics of the resonance parameters in the resolved resonance region. By using realistic population of extrapolated levels, the fit of measured total cross section produced a continuous S-matrix function S( E ) in Reich-Moore approximation. The S-matrix function averaged over a suitable energy interval was used to obtain averaged cross sections consistent with the measured data. Transmittable formatted files (ENDF, GNDS) with LSSF=1 will consist of File 3 which are smoothed cross sections and File 2 which are average resonance parameters fitted to the energy bins defined in File 3. The capability to store probability tables is a way to show the fluctuating cross sections.
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