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At least 811 records · Page 45

High Temperature Steam Oxidation of Irradiated FeCrAl in the Severe Accident Test Station

FeCrAl-UO2 test capsules were fabricated at Oak Ridge National Laboratory (ORNL) and irradiated at the Advanced Test Reactor. Following irradiation, samples were sectioned from the irradiated rod and oxidation kinetics were evaluated to access the candidate cladding high-temperature oxidation performance following irradiation. The irradiation was performed at approximately 400°C to a burnup of 10 GWd/MT. The high-temperature oxidation tests were conducted in the ORNL Severe Accident Test Station at 1200 and 1300°C. Weight measurements were taken before and after oxidation testing. Cross-sections of the cladding were metallographically mounted and optical microscopy was performed. Measurements of the oxidation layer before and after high-temperature testing were collected. The results indicate the irradiated FeCrAl C35M alloy provided good thermal stability up to 1200°C.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Effects of 18 O Exchange on Neutron Emission Rates of Aging 238 PuO 2 LWRHUs

The Lightweight Radioisotope Heater Unit (LWRHU) provides about 1 Watt of thermal power to critical electrical and mechanical systems in the extreme temperatures of space, maintaining the operating temperature of the spacecraft’s scientific and general operating equipment. Los Alamos National Laboratory (LANL) designed and tested the LWRHU in the 1970s through early 1980s. The first production campaign at LANL was in the early 1980s in support of the Galileo mission in which over 100 LWRHUs were manufactured. In the mid-1990s, almost 200 LWRHUs were manufactured in support of the Cassini mission. After the primary Cassini manufacturing campaign, the Department of Energy (DOE) approved the fabrication of more than 10 additional LWRHUs as spares in 1998. The LWRHU assembly contains the following components: a fuel pellet, a vented capsule, a pyrolytic graphite insulator, and a fine-weave pierced fabric (FWPF) graphite aeroshell. The fuel pellet is a hot-pressed 238 PuO 2 cylindrical pellet that is sintered to create a ceramic pellet. The pellet is encapsulated in a platinum-rhodium encapsulation. The welded fueled clad is placed inside a pyrolytic graphite thermal insulation to protect the fuel from the heat produced in reentry events. The exterior layer of the LWRHU assembly is the FWPF aeroshell. Before sintering, PuO 2 granules are heated in a furnace at temperatures greater than or equal to 700°C under an enriched 16 O atmosphere in order to reduce trace quantities of 18 O. Because 18 O undergoes an (α,n) reaction, 18 O needs to be removed as much as possible to meet radiation emission requirements set by the Jet Propulsion Laboratory (JPL) and the National Aeronautics and Space Administration (NASA), as well as other agencies. The relative abundances of the oxygen isotopes are indicated by neutron emission rate (NER) measurements. LWRHUs are vented with a sintered platinum frit vent (George 1986). During extraterrestrial operation, the vent in the cladding allows helium from the decay of plutonium to escape and relieves pressure from the system while preventing the solids from escaping (Rinehart 1996, Tate 1982 & 1985). This vent is protected during manufacture by a platinum-30 rhodium cover. The capsule vent is activated by milling a 0.025-inch diameter hole through the protective cover to a nominal depth of 0.015 inches, generally immediately before the LWRHU is loaded into the aeroshell (George 1986). Prior to long-term storage, LWRHUs are vented and thus potentially allow infiltration of 18 O from the ambient atmosphere. Although NER decreases with age due to the reduction in emitted alpha particles, it might be expected that NER reduction is mitigated by the exchange of 18 O. However, this is not necessarily the case and no trend was observed relating NER to age other than the natural decay of 238 Pu (Mulford 2021). The most probable and dominant factor for determining specific NER was manufacturing discrepancies between individual units. It is important to understand the lack of observed 16 O- 18 O exchange and to compare LWRHU pellets as much as possible.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Microstructural Analysis of Iron-Chromium-Aluminum Samples Exposed to Loca-Type Conditions Followed by Quench

The QUENCH-19 experiment was performed to examine the behavior of FeCrAl-alloy B1236Y3 as a potential nuclear fuel cladding and accident conditions. Over the course of the test, a surrogate bundle achieved a temperature of just over 1400°C. Post-test characterization revealed that the FeCrAl formed a thin layer of aluminum oxide that protected most of the underlying cladding and surrogate fuel pin. However, a few pins were heavily corroded and even destroyed primarily by thermocouple-FeCrAl interactions and subsequent steam, FeCrAl, and ZrO 2 interactions. Absent these effects, it is suggested that FeCrAl’s performance may be acceptable under these conditions.

36 MATERIALS SCIENCE↗

Advanced Low-Temperature Chlorination of Zirconium

Recovery of Zr from nuclear fuel is of high interest because the Zr cladding material comprises up to 50% of the high-level radioactive waste (HLW) that requires disposition. An ideal Zr-recovery process would not only recover the bulk Zr from the fuel or cladding but would also provide decontamination from the components that give rise to the HLW designation. A simplified decontamination pathway providing recovered Zr in compliance with low-level radioactive waste acceptance criteria could significantly reduce the burden of HLW requiring geologic disposition. A newly developed advanced low-temperature chlorination process presents an opportunity to recover a ZrCl4 product that is effectively decontaminated from the elements of concern. This advanced low-temperature chlorination process uses a mixture of the sulfur-containing chlorination compounds sulfur monochloride (S 2 Cl 2 ) and thionyl chloride (SOCl 2 ).

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Dissolution Flowsheet for Skull Oxide Generated during U-Mo Alloy Casting for High Performance Research Reactor Fuel

The Savannah River National Laboratory was requested to develop dissolution flowsheets for high assay low enriched U scrap generated during the fabrication of high performance research reactor fuel. The scrap streams include U-10Mo and U-10Mo-Zr foils, rejected Al-clad fuel plates, and skull oxide from casting molds. Flowsheets for the dissolution of the U-10Mo-Zr foils and Al-clad U-10Mo-Zr mini-plates received from BWX Technologies, Inc were developed and demonstrated in the first phase of this project. In the second phase (this work), the skull oxide from a U-10Mo casting mold was obtained from the Y-12 National Security Complex (Y-12) and small-scale experiments were performed to demonstrate dissolution flowsheets.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Transverse Rupture Strength of Uranium Dioxide

Uranium dioxide (UO 2 ) fuel is used as fuel in light water reactors (LWRs). While the fuel pellet is technically the first engineering barrier for radionuclide release, pellet fracturing at intermediate- to high-burnup values releases fission gases into the fuel rod plenum [1, 2]. Therefore, the true engineering barrier is the fuel cladding, which performs very well in LWR environments [3]. The extreme temperature gradients generated by fission energy and the low thermal conductivity of UO 2 quickly induce radial cracking in UO 2 during operation [4]. Cracks in the fuel provide opportunities for fuel relocation, increased fission gas release, and pellet-cladding mechanical interaction (PCMI) [5]. The ability to predict and engineer the fracture of UO 2 fuel pellets using modern computational tools is therefore a key engineering goal that has been the focus of ongoing experimental and computational efforts [6, 7]. Accurate predictions of fuel pellet cracking during operation requires knowledge of more complex phenomena, but improved understanding of the fundamental fracture behavior of unirradiated UO 2 is first necessary.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Update on the Investigation of Commercial Drying Cycles Using the Advanced Drying Cycle Simulator

The purpose of this report is to document updates on the apparatus to simulate commercial vacuum drying procedures at the Nuclear Energy Work Complex at Sandia National Laboratories. Validation of the extent of water removal in a dry spent nuclear fuel storage system based on drying procedures used at nuclear power plants is needed to close existing technical gaps. Operational conditions leading to incomplete drying may have potential impacts on the fuel, cladding, and other components in the system during subsequent storage and disposal. A general lack of data suitable for model validation of commercial nuclear canister drying processes necessitates well-designed investigations of drying process efficacy and water retention. Scaled tests that incorporate relevant physics and well-controlled boundary conditions are essential to provide insight and guidance to the simulation of prototypic systems undergoing drying processes. This report documents a new test apparatus, the Advanced Drying Cycle Simulator (ADCS). This apparatus was built to simulate commercial drying procedures and quantify the amount of residual water remaining in a pressurized water reactor (PWR) fuel assembly after drying. The ADCS was constructed with a prototypic 17×17 PWR fuel skeleton and waterproof heater rods to simulate decay heat. These waterproof heaters are the next generation design to heater rods developed and tested at Sandia National Laboratories in FY20. This report describes the ADCS vessel build that was completed late in FY22, including the receipt of the prototypic length waterproof heater rods and construction of the fuel basket and the pressure vessel components. In addition, installations of thermocouples, emissivity coupons, pressure and vacuum lines, pressure transducers, and electrical connections were completed. Preliminary power functionality testing was conducted to demonstrate the capabilities of the ADCS. In FY23, a test plan for the ADCS will be developed to implement a drying procedure based on measurements from the process used for the High Burnup Demonstration Project. While applying power to the simulated fuel rods, this procedure is expected to consist of filling the ADCS vessel with water, draining the water with applied pressure and multiple helium blowdowns, evacuating additional water with a vacuum drying sequence at successively lower pressures, and backfilling the vessel with helium. Additional investigations are expected to feature failed fuel rod simulators with engineered cladding defects and guide tubes with obstructed dashpots to challenge the drying system with multiple water retention sites.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Research and Test Reactor Fuels

PRO-RR is the research reactor focused program element of the broader Proliferation Resistance Optimization program (PRO-X) under the National Nuclear Safety Administration (NNSA) in the U.S. Department of Energy (DOE). PRO-X provides a framework for integrating proliferation resistance in nuclear system designs to minimize weapons usable nuclear materials (WUNM) production and diversion pathways while optimizing systems performance for peaceful use missions. PRO-RR applies the PRO-X mission objectives to research reactor system design. This document serves as one of the foundational documents for the PRO-RR-Fuel System Design technical team by documenting current research reactor fuels usage. The PRO-RR-Fuel System Design technical team consists of subject matter experts from Argonne National Laboratory (Argonne) and Savannah River National Laboratory (SRNL). In order to determine the preferred fuel of use in upcoming research and test reactors to optimize proliferation resistance, performance, and safety, it is useful to assess the fuels that have been used in the past, or are currently in use. This report reviews the historical and current fuels used in research and test reactors to inform future fuel selection. Chapter 2 discusses the low-enriched uranium (LEU) fuels currently in use in terms of thermal power level and utilization of the reactor. Chapter 3 summarizes the fabrication processes for common fuel types. Chapter 4 discusses in detail the fuel types in use in research and test reactors. A review of the cladding types in use is presented in Chapter 5, and a historical review of research and test reactor fuel fabricators is presented in Chapter 6. The data collection strategy used the International Atomic Energy Agency (IAEA) research reactor database [1] as a starting point. Information on the fuel used was gathered on research reactors (other than critical assemblies) that were listed as operational, planned, or in temporary shutdown in the IAEA database. Data on the fuel type, geometry, enrichment, uranium loading, cladding type, and fabricator were collected for each of the reactors available in the public domain. Sources of data included conference papers, journal articles, and facility and fabricator websites. Data on research reactors operating on LEU fuels are presented in Appendix A, while Appendix B presents data collected on all reactors at the time of publication of this report. Appendix C presents data collected on reactors that were part of the M3 research and test reactor conversion program.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Implementation of an Orificing Optimization Algorithm in the DASSH Subchannel Analysis Code

The Ducted Assembly Steady-State Heat transfer code (DASSH) performs full-core subchannel thermal hydraulics calculations in liquid metal fast reactors. One of the applications of subchannel codes is to optimize coolant flow orificing. As a design activity, the primary task is to determine the best way to divide assemblies into groups and distribute coolant flow rates among them. This report documents an algorithm implemented in DASSH to automatically optimize coolant orificing. Over the course of multiple iterations, DASSH determines the orifice grouping and flow distribution that minimizes peak coolant, clad, or fuel temperatures across all timesteps for a user-specified number of assembly groups. The total coolant flow rate in the reactor is constrained to achieve the specified core-average outlet temperature. The flow rate to each orifice group may also be constrained by the allowable pressure drop. The distribution of coolant flow among groups is accelerated using a predictor-corrector algorithm based on interpolated results from single-assembly parametric calculations. The assembly orificing grouping is initially predicted based on assembly power but can be refined if results demonstrate that an assembly would fit better in another group. The algorithm is demonstrated with two case studies. The first is a simple model for a reactor core consisting of just fuel assemblies; the pin power distributions are specified to create a situation where the initial assembly grouping prediction is suboptimal. This example is used to describe the initial grouping, demonstrate convergence over multiple iterations, and highlight the impact of regrouping. Then, the algorithm is applied to minimize peak clad and fuel temperatures in an example sodium-cooled fast reactor, the Versatile Test Reactor. The multicycle optimization confirms prior calculations for the reference core design. The example highlights how optimizing for different peak temperatures affects the results and demonstrates the use of the pressure drop constraint to limit the maximum flow rate.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

FY22 Progress Report on BISON Metallic Fuel Model Development and V&V Using EBR-II Legacy Data

In this report, the activities and achievements made by Argonne National Laboratory for the Nuclear Energy Advanced Modeling and Simulation (NEAMS) BISON code metallic fuel validation and verification project in FY2022 are summarized. The FIPD-BISON integration powered metallic fuel low-burnup swelling framework has been enhanced to cover both radial and axial swelling analyses. Axial-dependent as-fabricated fuel radius profiles have been used to improve the accuracy in evaluating radial swelling strain. The simulations of the IFR experiment X447, which was focused on FCCI/CCCI induced cladding degradation and failure, have been converted into a BISON metallic fuel assessment case with detailed documentation, which is also the first FIPD-BISON integration powered assessment case in BISON. A FIPD-BISON integration repository has been established to be an optional submodule of BISON to support FIPD-BISON integration powered assessment cases. Preliminary trials to simulate the in-cell out-of-pile transient experiment have been made after implementing some essential models such as cladding plasticity models and liquid phase penetration models. The initial results are promising and help identify gaps that need to be filled in FY2023 and beyond, to eventually achieve OPTD-BISON integration powered assessment cases.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Second Target Station High-Fidelity Target Activation Comparison

The development of the Second Target Station (STS) target system at the Spallation Neutron Source (SNS) at Oak Ridge National Laboratory (ORNL) is well underway. The target system at STS consists of a rotating target disk that contains 21 segments of tungsten clad in tantalum clad in steel. A key aspect of the design of the target system is to account for the delayed heating and material damage caused by the delayed dose from decaying radionuclides. These radionuclides are a product of either spallation reactions or transmutation of the nuclei in the target system. These radionuclides build up in the target system components over the lifetime of the facility, and the radiation that is emitted can deposit energy in the components causing significant component heating and material damage. Monte Carlo N-Particle (MCNP) Version 6.2 transports the various particle species and calculates the spallation products and neutron fluxes throughout the target system. These spallation products and neutron fluxes along with the material definition of each component are relayed to the CINDER2008 transmutation code to calculate the radionuclide inventories and the corresponding decay gamma emission spectra. MCNP6.2 coupled with CINDER2008 is the computational method-of-choice for the analysis discussed in the following sections of this report. The analysis focuses on validating major assumptions in calculating the radionuclide inventory in the STS target system: all of the target segments are fresh, unirradiated material when the protons are incident on the segment, the average of the 21 segments of the target is sufficient to represent a single segment, and that averaging the proton pulse structure over time does not significantly affect the radionuclide inventory. The position-averaged, high-fidelity, and single-tally computational methods are used to validate the assumptions and provide a point of comparison to evaluate how the assumptions impact the radionuclide inventories. A more detailed explanation of the three computational methods is provided in Section 2. The position-averaged and single-tally methods are less computationally expensive when compared with the high-fidelity method where 54,000 individual calculations are needed to calculate 1 hr of STS operation. Section 3 details the comparison of the three methods to show that the assumptions made in the position-averaged method do not significantly impact the radionuclide inventory after 1 hr of operation. The discussions and results in this report are for 1 hr of operation. Due to the computational cost associated with calculating the transmutation and activation using the high-fidelity method, only 1 hr of operation has been calculated. The discrepancies observed after 1 hr of operation are not extrapolated out to longer operational times, and this report does not address how the discrepancies between the computational methods may manifest for longer operational periods.

43 PARTICLE ACCELERATORS↗

Preliminary Thermal-Hydraulic Analysis of the UTA–2 Subcritical Linear Accelerator–Driven System

The National Nuclear Security Administration’s mission includes establishing a reliable supply of 99 Mo without highly enriched uranium. Oak Ridge National Laboratory (ORNL) supports this objective through collaborative research and development with industrial partners. Niowave Inc., a current partner, is currently designing a subcritical linear accelerator-driven system (ADS) and preparing for the US Nuclear Regulatory Commission’s licensing process. Niowave’s system has the potential to efficiently supply medical radioisotopes. The technology includes a superconducting electron accelerator and a pile of both natural and low-enriched uranium (LEU) targets. The process fissions uranium and many valuable isotopes can then be extracted from the targets. Niowave is currently iterating through conceptual and detailed design processes for several system sizes. This report discusses UTA–2, which is at the demonstration stage. UTA–2 will validate numerical modeling results with experimental measurements before progressing to the detailed design of UTA–3, the commercial-sized ADS. The thermal-hydraulic behavior of the UTA–2 core design was numerically investigated using STAR-CCM+, as described in this report. STAR-CCM+, a state-of-the-art computational fluid dynamics (CFD) software that was commercially developed by Siemens, has an extensive user base and a set of validation studies. It is also compliant with the American Society of Mechanical Engineers’ Nuclear Quality Assurance 1 standard. Three cases are investigated in this report. Case 1 quantified the temperature field within the UTA–2 assembly and water tank using only conduction as the method of thermal energy transport. This simplified approach was overly conservative and yielded wetted cladding temperatures above the coolant saturation temperature. In this case, the maximum temperature of the wetted cladding surface of the highest power rod exceeded the saturation temperature of water by 63.8°C. Because of the overly conservative approach taken in Case 1 and its negative subcooled margin, buoyancy-driven natural circulation flow physics were implemented in Case 2. Adding coolant motion significantly distributed the thermal energy of the system through convective heat transfer. This relatively small amount of convective heat transfer significantly reduced system temperatures and increased the subcooled margin from –63.8 to 61.3°C. This margin confirmed that no boiling was expected during normal operation of UTA–2 at 230 W. Case 3 had no additional physics models but considered an overpower event during which the power of each LEU and natural uranium rod was at its respective peak values. This resulted in a study with the total assembly power equal to 176% of the nominal power of 230 W considered in Cases 1 and 2. The resulting natural circulation flows were slightly enhanced. The subcooled margin decreased slightly to 46.3°C, which is still a significant margin to local boiling of the water within the tank. This margin confirmed that no boiling was expected during an abnormal operation of UTA–2 at 406 W.

07 ISOTOPE AND RADIATION SOURCES↗

Benchmark Specifications for TREAT Tests M5, M6, and M7

Detailed information describing three TREAT tests performed on metallic fuels has been collected and organized for use as a benchmark in evaluating the performance of metallic fuel models and codes. The tests, designated M5, M6, and M7, subjected EBR-II-irradiated fuel pins to a single type of overpower transient (at prototypical conditions with full coolant flow and an exponential power rise on an 8 second period) in flowing sodium loops. Six fuel pins were tested; five were ternary (U-19Pu-10Zr) alloy fuel clad in D9 with burnup ranging from 0.8 to 9.8 at. %, and one was binary alloy fuel (U-10Zr) clad in HT9 with 2.9 at. % burnup. The information gathered from the test records is expected to be useful for pre-transient characterization of the irradiated fuel pins as well as the transient analysis of the metallic fuel when subjected to severe accident conditions. This report presents benchmark specifications for the M5, M6, and M7 TREAT tests, identifies where primary sources of benchmark-related information can be found, and includes background information to help a user of the data understand their applicability and limitations.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Modeling of Radiolytic Hydrogen Generation of Irradiated Surrogate Aluminum Plates

The hydrogen generation from oxyhydroxide layers under irradiation is an important effect to understand for the long-term storage of aluminum-clad spent nuclear fuel. The original chemical model shows steady production of hydrogen from aluminum oxyhydroxide layers, with no roll-over effect in the curves of the hydrogen concentration until significant pressure has built up within the canister. This study uses a variety of kinetic fits to adjust the old chemical model to have roll-over effects that are consistent with new high-dose experiments. The data from aluminum 6061 coupon tests at high doses were used to fit several kinetic models. The 6061 aluminum samples are representative of the aluminum-clad fuel from the ATR. The fitted kinetic models were then used in a model of a mini-canister with much higher packing density to determine which kinetic rates would fit both sets of experimental tests. The rate constants for the kinetic mechanisms that were close were then tweaked such that the chemical models fit both the experimental data from the capsule tests and the data from the mini-canister tests. The kinetic models which fit the best are either inhibition by hydrogen, or a back reaction wherein H radical is reabsorbed onto the oxyhydroxide layer. The H back reaction rolls over quicker and may fit future collected data.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Milestone 1.2.10: Steady-state H 2 “roll over” point data for aluminum alloys 1100 and 6061

Extended (> 50 years) dry storage is being evaluated by the U.S. Department of Energy (DOE) for the disposition of ~ 18 metric tons of aluminum-clad spent nuclear fuel (ASNF). Transition of the current ASNF inventory into dry storage—using the standard DOE canister—necessitates a rigorous, predictive understanding of the long-term physical and chemical factors that may influence the integrity of the proposed storage canister, including radiolytic molecular hydrogen (H 2 ) generation. Current model predictions employ initial radiolytic yields of H 2 , the values of which change as the cladding’s H 2 -precursor inventory is depleted and H 2 itself becomes progressively more involved in radiolytic and surface dissociation processes. Consequently, the absorbed radiation dose that this steady-state H 2 yield corresponds to is essential for the evaluation and improvement of model predictions. Here, we report our findings on the long-term generation of H 2 from the gamma irradiation (≤ 36 MGy) of corroded AA1100 and AA6061 coupons in helium environments at ambient temperature and ~ 50% RH. Our findings show that AA1100 systems reached steady-state by ~ 36 MGy, while higher doses were necessary for AA6061 systems. This discrepancy was attributed to the AA6061 coupons developing a thicker corrosion layer that led to the trapping of H 2 and its precursors, and potentially additional chemistries, ultimately delaying the depletion of H 2 precursors and the system’s “roll over” point. Further, current model predictions—based on previous AA1100 data—do not show steady-state attainment until above 120 MGy, which is not the case for the AA1100 data collected here. Consequently, the new alloy dependent data presented here are important for the continued improvement of predictive computer models for evaluating the feasibility of extended storage of ASNF in helium backfilled canisters.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Sister Rod Destructive Examinations (FY22) Appendix E: Mechanical Testing - Spent Fuel and Waste Disposition

As a part of the DOE NE High Burnup Spent Fuel Data Project, Oak Ridge National Laboratory (ORNL) is performing destructive examinations (DEs) of high burnup (HBU) (>45 GWd/MTU) spent nuclear fuel (SNF) rods from the North Anna Nuclear Power Station operated by Dominion Energy. The SNF rods, called sister rods or sibling rods, are all HBU and include four different kinds of fuel rod cladding: standard Zircaloy-4 (Zirc-4), low-tin Zirc-4, ZIRLO, and M5. The DEs are being conducted to obtain a baseline of the HBU rod’s condition before dry storage and are focused on understanding overall SNF rod strength and durability. Composite fuel and defueled cladding will be tested to derive material properties. Although the data generated can be used for multiple purposes, one primary goal for obtaining the post-irradiation examination data and the associated measured mechanical properties is to support SNF dry storage licensing and relicensing activities by (1) addressing identified knowledge gaps and (2) enhancing the technical basis for post-storage transportation, handling, and subsequent disposition. This report documents the status of the ORNL Phase 1 DE activities related to the mechanical testing of selected sister rods in Phase 1 of the sister rod test program.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Sister Rod Destructive Examinations (FY22) Appendix C: Rod Internal Pressure, Void Volume, and Gas Transmission Tests

As a part of the DOE NE High Burnup Spent Fuel Data Project, Oak Ridge National Laboratory (ORNL) is performing destructive examinations (DEs) of high burnup (HBU) (>45 GWD/MTU) spent nuclear fuel (SNF) rods from the North Anna Nuclear Power Station operated by Dominion Energy [C-1]. The SNF rods, called the sister rods or sibling rods, are all HBU and include four different kinds of fuel rod cladding: standard Zircaloy-4 (Zirc-4), low-tin (LT) Zirc-4, ZIRLO, and M5. The DEs are being conducted to obtain a baseline of the HBU rod’s condition before dry storage and are focused on understanding overall SNF rod strength and durability. Both fuel rods and empty cladding will be tested to derive material properties. Although the data generated can be used for multiple purposes, one primary goal for obtaining the postirradiation examination data and the associated measured mechanical properties is to support SNF dry storage licensing and relicensing activities by (1) addressing identified knowledge gaps and (2) enhancing the technical basis for post-storage transportation, handling, and consolidation activities. This appendix documents the status of the ORNL Phase 1 DE activities [C-2, C-3] related to rod internal pressure and void volume measurement techniques, fission gas stack flow measurements applied to selected sister rods, and fission gas release calculations in Phase 1 of the sister rod test program.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗