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At least 595 records · Page 33
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Spectroscopic features of dissolved iodine in pristine and gamma-irradiated nitric acid solutions

While iodine speciation is important for a wide range of nuclear activities, understanding the mechanisms of the transformations of iodine between chemical forms and the sensitivity of these transitions to solution conditions and exposure to radiation remains an active area of research. This work curates spectroscopic data from several experimental techniques and establishes their sensitivity and limitations in detecting changes in iodine speciation in both neutral and acidic regimes. The techniques include Raman spectroscopy, Fourier Transform Infrared (FTIR) spectroscopy, 127 I NMR spectroscopy, and ultraviolet-visible (UV-Vis) spectroscopy. Analysis of these data indicates that these commonly accessible spectroscopies often have dynamic ranges of measurable concentrations that do not always overlap between all techniques. The experimental techniques are disparately sensitive to iodide (I - ), molecular iodine (I 2 ), iodate (IO 3 - ), and periodate (IO 4 - ) species. Raman, FTIR, and NMR spectra were subsequentially analyzed using two-dimensional correlation analyses to generate high-resolution autocorrelation spectra. Here, the use of these spectroscopies is then extended to tracking acidification-induced and gamma irradiation-induced transformations of dissolved sodium iodate in deionized water and concentrated nitric acid. Both dissolution into nitric acid and irradiation with a gamma source are demonstrated to perturb the iodine speciation promoting their assembly into molecular iodine (I 2 ) and/or triiodide (I 3 - ). While I 2 and I 3 - species are undetectable with FTIR spectroscopy and 127 I NMR spectroscopy, the species can be detected with UV-Vis spectroscopy, and in some instances, I 3 - can be detected with Raman spectroscopy in the low wavenumber region. Ultimately, the results of this work provide a path to designing optimal combinations of techniques to detect forms of iodine across a wide range of concentrations and conditions.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2025

Exposing Process‐Level Biases in a Global Cloud Permitting Model With ARM Observations

The emergence of global convective‐permitting models (GCPMs) represents a significant advancement in climate modeling, offering improved representation of deep convection and complex precipitation patterns. In this study, we evaluate the performance of the Simple Cloud‐Resolving E3SM Atmosphere Model (SCREAM) using its doubly periodic configuration (DP‐SCREAM) against large eddy simulations and modern observational data sets from the Atmospheric Radiation Measurement program. We introduce several new transitional cloud regime cases, such as the transition from shallow to deep convection and from stratocumulus to cumulus, as well as cold‐air outbreak scenarios. The results reveal both strengths and limitations of SCREAM, particularly in the accurate simulation of cloud transitions and midlevel convection, with varying degrees of sensitivity to horizontal and vertical resolution. Despite improvements at higher resolutions, key biases remain, including the abrupt transition from shallow to deep convection and the lack of congestus clouds. These findings underscore the need for further refinement in turbulence parameterizations and vertical grid resolution in GCPMs.

Bogenschutz, Peter A. [Lawrence Livermore National↗
DOE OSTI2026

Radiation damage in tungsten under high-energy He-ion irradiation

Tungsten (W) is a primary candidate for plasma-facing components (PFCs) in fusion reactors and hybrid fission-fusion reactors. However, W suffers from severe microstructural damage under Helium (He) ion irradiation in operation conditions. Key irradiation parameters, including incident ion energy, fluence, and irradiation temperature, are known to determine the formation of He bubbles and dislocation loops, which ultimately lead to the degradation of mechanical properties, such as radiation hardening and ductile-to-brittle transition temperature (DBTT) shifts. Various strategies, for instance, interface engineering and alloying, have been developed to enhance He irradiation tolerance in W to address these challenges. Studies in the recent two decades have enhanced the understanding of the underlying mechanisms that drive defect evolution and mechanical performance degradation, thereby offering more insights into the design of more resilient W-based materials for extreme environments.

Liu, Yinghang [Purdue University]↗
DOE OSTI2026

Primordial black hole dark matter: A quantitative parameter sensitivity comparison across formation mechanisms and particle candidates

Primordial black holes (PBHs) in the asteroid-mass window ( 10 17 – 10 22 g ) can account for all of the dark matter without violating any observational constraint, yet are routinely dismissed as fine-tuned. I put that dismissal to the test by applying three complementary sensitivity measures uniformly across a broad landscape: three noninflationary PBH production mechanisms, six classes of inflationary PBH models, and seven particle dark matter benchmarks, all evaluated against the same observable target. Three distinct naturalness universality classes emerge, determined entirely by the analytic structure of the abundance map rather than by the nature of the dark matter candidate. Biased-domain-wall PBHs, in their least model-dependent (free- V b ) form, have the same low sensitivity, Δ = 4.5 , as off-resonance weakly interacting massive particles and freeze-in particles ( Δ = 2 ), a sensitivity that, because it is constant over the entire parameter space of the construction, also coincides trivially with its own Wilson-normalized average within that parameter space (Section Definition and conventions), an equivalence that concerns only the space over which Δ is computed and is not a naturalness statement about the construction as a whole; a further reduction to Δ = 2 is possible only under the additional, independently motivated but not required, assumption that the domain-wall bias is generated by Planck-suppressed operators; early matter-domination PBHs occupy an intermediate tier alongside coannihilating weakly interacting massive particles (WIMPs), unified by a structural identity in which the sensitivity measure equals the logarithm of the ratio of the formation scale to the matter–radiation equality scale; first-order phase transition PBHs, once the more accurate super-exponential collapse probability is used in place of the single-exponential approximation, instead belong to the same highly sensitive tier as resonant WIMP annihilation and single-field inflationary collapse, for a structurally distinct reason; single-field ultraslow-roll inflationary collapse is severely tuned for a distinct reason: a double exponential in which the power spectrum amplitude is itself exponentially sensitive to the inflaton potential coefficients, on top of the exponential collapse sensitivity of the abundance map. My main conclusion is that the claim that PBH dark matter is generically fine-tuned conflates the worst case with a landscape spanning every naturalness tier. The Barbieri-Giudice sensitivity computed here and the Wilson-normalized measure of Iovino and Riotto answer distinct and mutually consistent questions about the same construction, a distinction I clarify within the two-layer decomposition.

Profumo, Stefano [University of California, Santa ↗
NASA NTRS1974

Coordinated analysis of airborne spectrophotometric measurements from the mid-day auroras

Measurements made in the midday auroras are analyzed and compared to measurements from the nighttime auroras. The auroral emission features in the UV spectrum, the N2(+)ING, the N22PG, and N2VK bands, are discussed. Spectral profiles of different bands are presented, and intensity distributions are obtained. Three mechanisms are suggested which can account for the marked differences between the intensity distributions of the N2(+)ING bands of the high altitude midday auroras and the low altitude nighttime auroras: (1) differences in vibrational, rotational, and transitional temperatures; (2) resonant scattering of solar radiation; and (3) excitation of slow ions.

Sivjee, G. G.↗
NASA NTRS1977

A study of the aerothermal environment for the Pioneer Venus multiprobe mission

In December 1978, four Pioneer Venus probe spacecraft are scheduled for almost simultaneous entry into the Venusian atmosphere at widely dispersed points about the planet. In this study, both detailed and approximate flow field analyses are used to define the entry aerothermal environment for the forebody of each of the four probes. The results show that approximate analyses can be used to predict inviscid radiative and laminar convective heating rates with acceptable accuracy. However, the radiative heating rates obtained with inviscid analyses are significantly greater than those obtained with a nonablating viscous-shock-layer (VSL) analysis, because the VSL analysis includes a strongly absorbing boundary layer. Also, the results show that the radiative heating is sensitive to small variations in atmospheric gas composition while the convective heating is not affected. With carbon-phenolic injection, the convective heating is reduced substantially while the overall radiative heating reduction is very small. Most of the radiative blockage occurs in the atomic line transitions which is significant only in the stagnation region.

Moss, J. N.↗
NASA NTRS1984

Uncooled IR Detector

Detector combines liquid crystal film with light-sensitive solid-state array. Liquid-crystal film acts as IR detector when maintained just below temperature of transition from opacity to transparancey. When IR radiation is absorbed by film, resultant heating changes visiblelight transmission, modulating uniform visible light beam as it passes through film.

Shlichta, P. J.↗
NASA NTRS1984

Physical conditions in the cool parts of prominences. II - The Mg triplet lines

The statistical equilibrium of Mg under prominence conditions is considered. It is shown that the principal lines of the triplet system can serve as an equivalent to the Na D lines for spectral diagnostic purposes. Like the Na D lines, these Mg lines are relatively easy to measure in prominences and exhibit small optical depths. It is demonstrated that potential complications due to possible radiative transfer effects in the Mg resonance transition (3 1S0 - 3 1P1) have little consequence for the triplet populations. The results are used to repeat the spectral analysis of Landman (1983) using the Mg multiplets in place of the Na ones. The results of the two analyses are in general agreement. The finding of a low degree of H ionization in the cool prominence regions and a correspondingly high gas pressure is confirmed.

Landman, D. A.↗
NASA NTRS1984

Flare parameters for the 7 September, 1973 two-ribbon flare

A study is made of the relative importance of the various energy loss mechanisms for the long-decay event of September 7, 1973, using spectral scans in the 400 A-1335 A range. This spectral range contains many of the important electron density and temperature diagnostic line ratios for the solar transition zone. Earlier analyses of the flare energy budget are refined, using more detailed emission measure curves and density diagnostics. The constant pressure assumptions used in both coronal loop models and in the interpretation of observations in terms of flare energetics are examined. It is found that much of the upper transition region emission originates in cooling loops. Radiative losses are found to dominate.

Doyle, J. G.↗
NASA NTRS1985

Thermal phases of interstellar and quasar gas

Interstellar gas may be in a variety of thermal phases, depending on how it is heated and ionized; here a unified picture of the equation of state of interstellar and quasar gas is presented for a variety of such mechanisms over a broad range of temperatures, densities, and column densities of absorbing matter. It is found that for select ranges of gas pressure, photoionizing flux, and heating, three thermally stable phases are allowed: coronal gas (T above 100,000 K); warm gas (T about 10,000 K); and cold gas (T less than 100 K). With attenuation of ultraviolet and X-ray radiation, the cold phase may undergo a transition to molecules. In quasar broad-line clouds, this transition occurs at column density N(H) = about 10 to the 23rd/sq cm and could result in warm molecular cores and observable emission from H2 and OH. The underlying atomic physics behind each of these phase transitions and their relevance to interstellar matter and quasars are discussed.

Lepp, S.↗
NASA NTRS1985

IUE spectra of G0 V-G5 V solar-type stars

An atlas of IUE short-wavelength spectra for a set of 14 bright G0 V-G5 V stars are presented, and it is shown that these manifest a range of qualitatively different chromospheric and transition region spectra and significant differences in radiative flux originating at the temperature minimum level. A comprehensive survey of observational data and physical parameters of these stars has been performed, and tabular summaries of the data are presented. It is concluded that the UV continuum longward of about 1600 A is a diagnostic of the temperature minimum. A considerable range of minimum temperature for stars of similar effective temperature and spectral type is found. The temperature minimum of the sun is highly structured on spatial scales of about one arcsec.

Haisch, B. M.↗
NASA NTRS1987

Quantized synchrotron radiation in strong magnetic fields

Spectra from electrons making synchrotron transitions in high magnetic fields are calculated using the exact quantum transition rates for Landau states up to n = 500, and the results are compared with spectra calculated from the classical formula and the asymptotic quantum formula. The behavior of the transition rates are examined at low and high harmonics as a function of the spin state of the electron. The calculations confirm those of Herold, Ruder, and Wunner (1982) for low Landau states, extending them to higher states and individual spin state transitions. The results also confirm the dominance of ground-state transitions at high field strengths noted by White (1976). Single particle emissivities for electrons with both spin-up and spin-down in the initial state are calculated using these transition rates. Spectra for thermal electron distributions at transrelativistic temperatures and for steady state injection of monoenergetic electrons with isotropic pitch angles are also presented.

Harding, Alice K.↗
NASA NTRS1989

Line blanketing without local thermodynamic equilibrium. II - A solar-type model in radiative equilibrium

A statistical solution for the problem of non-LTE radiative transfer in the millions of atomic transitions responsible for line blanketing is proposed which takes into account the influence of scattering on the atomic populations. A multifrequency/multigray algorithm is used to analyze the thermal equilibrium. Although CO is shown to cool the upper atmosphere to a boundary temperature of 2640 K, the molecule has little influence in the region of the solar temperature minimum.

Anderson, Lawrence S.↗
NASA NTRS1989

Cyclotron resonant scattering in the spectra of gamma-ray bursts

Fits of theoretical spectra from Monte Carlo radiation-transfer calculations to dips at approximately 20 and 40 keV in a spectrum of the gamma-ray burst source GB 880 205 give best-fit values and 68 percent-confidence intervals for the magnetic field of (1.71 + or - 0.07) x 10 to the 12th G, the electron density of (1.2 + or - 0.6) x 10 to the 21st electrons/cm-squared, and the cosine of the viewing angle relative to the field of 0.31 + or - 0.05. The dips observed at approximately 20 keV in the spectra are interpreted as cyclotron resonant scattering, in which electrons undergo radiative 0 to 1 to 0 Landau transitions initiated by photons near the first harmonic. Physical self-consistency fixes the temperature, and the equilibrium temperature equals 5.3 + 0.3 or - 0.2 keV. These results suggest that this gamma-ray burst and many others which exhibit a low-energy dip originate from strongly magnetic neutron stars and are galactic in origin.

Wang, J. C. L.↗
NASA NTRS1990

Relic gravitational waves and extended inflation

In extended inflation, a new version of inflation where the transition from an inflationary to a radiation-dominated universe is accomplished by bubble nucleation, bubble collisions supply a potent - and potentially detectable - source of gravitational waves. The energy density in relic gravitons from bubble collisions is expected to be about 0.00005 of closure density. Their characteristic wavelength depends on the reheating temperature. If black holes are produced by bubble collisions, they will evaporate, producing shorter-wavelength gravitons.

Turner, Michael S.↗
NASA NTRS1990

Some comparisons of linear stability theory with experiment at supersonic and hypersonic speed

Measurements of waves initiated by wind-tunnel sounds are obtained for both supersonic and hypersonic speed. Flat-plate experiments carried out at Mach numbers of 4.5, 3.7, and 2.4 under the condition of laminar tunnel-wall boundary layers whereby a low background fluctuation level prevailed are outlined, as well as flat-plate experiments with sound-induced waves at supersonic speeds. Experimental studies of 'natural' wave growth on sharp cones at zero angle of attack and Mach numbers near 8 are discussed. Attention is focused on experimental research needed on boundary-layer receptivity to eddy Mach-wave radiation, hypersonic speed, and the stability-transition relationship in zero-pressure-gradient layers.

Kendall, James M., Jr.↗
NASA NTRS1995

Generation Of 369.4-Nanometers Second Harmonic From A Diode Laser

Experimental laser system features polarization feedback scheme maintaining frequency lock. Generates light at wavelength of 369.4 nanometers by second-harmonic generation from 738.8-nanometers laser diode. System prototype of source of 369.4-nanometers radiation used to optically pump 2S1/2 ' 2P1/2 transition in 171Yb+ ions in lightweight, low-power trapped-ion frequency-standard apparatus.

Williams, Angelyn P.↗