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NASA NTRS1993

Planetary and satellite x ray spectroscopy: A new window on solid-body composition by remote sensing

The rings and most of the satellites of the outer planets orbit within the radiation belts of their parent bodies. This is an environment with intense fluxes of energetic electrons. As a result, these objects are strong emitters of X-rays. The characteristic X-ray lines from these bodies depend on atomic composition, but they are not sensitive to how the material is arranged in compounds or mixtures. X-ray fluorescence spectral analysis has demonstrated its unique value in the laboratory as a qualitative and quantitative analysis tool. This technique has yet to be fully exploited in a planetary instrument for remote sensing. The characteristic X-ray emissions provide atomic relative abundances. These results are complementary to the molecular composition information obtained from IR, visible, and UV emission spectra. The atomic relative abundances are crucial to understanding the formation and evolution of these bodies. They are also crucial to the proper interpretation of the molecular composition results from the other sensors. The intensities of the characteristic X-ray emissions are sufficiently strong to be measured with an instrument of modest size. Recent developments in X-ray detector technologies and electronic miniaturization have made possible space-flight X-ray imaging and nonimaging spectrometers of high sensitivity and excellent energy resolution that are rugged enough to survive long-duration space missions. Depending on the application, such instruments are capable of resolving elemental abundances of elements from carbon through iron. At the same time, by measuring the bremsstrahlung intensity and energy spectrum, the characteristics of the source electron flux can be determined. We will discuss these concepts, including estimated source strengths, and will describe a small instrument capable of providing this unique channel of information for future planetary missions. We propose to build this instrument using innovative electronics packaging methods to minimize size and weight.

Chenette, D. L.↗

NASA NTRS1995

Characterization of the Minimum Energy Paths and Energetics for the Reaction of Vinylidene with Acetylene

The reaction of vinylidene (CH2C) with acetylene may be an initiating reaction in soot formation. We report minimum energy paths and accurate energetics for a pathway leading to vinyl-acetylene and for a number of isomers of C4H4. The calculations use complete active space self-consistent field (CASSCF) derivative methods to characterize the stationary points and internally contacted configuration interaction (ICCI) and/or coupled cluster singles and doubles with a perturbational estimate of triple excitations (CCSD(T)) to determine the energetics. We find an entrance channel barrier of about 5 kcal/mol for the addition of vinylidene to acetylene, but no barriers above reactants for the reaction pathway leading to vinyl-acetylene.

Walch, Stephen P.↗

NASA NTRS1995

Characterization of the Minimum Energy Paths and Energetics for the reaction of Vinylidene with Acetylene

The reaction of vinylidene (CH2C) with acetylene may be an initiating reaction in soot formation. We report minimum energy paths and accurate energetics for a pathway leading to vinylacetylene and for a number of isomers Of C4H4. The calculations use complete active space self-consistent field (CASSCF) derivative methods to characterize the stationary points and internally contacted configuration interaction (ICCI) and/or coupled cluster singles and doubles with a perturbational estimate of triple excitations (CCSD(T)) to determine the energetics. We find an entrance channel barrier of about 5 kcal/mol for the addition of vinylidene to acetylene, but no barriers above reactants for the reaction pathway leading to vinylacetylene.

Walch, Stephen P.↗

NASA NTRS1997

Cloud Liquid Water Path Comparisons from Passive Microwave and Solar Reflectance Satellite Measurements: Assessment of Sub-Field-of-View Cloud Effects in Microwave Retrievals

Satellite observations of the cloud liquid water path (LWP) are compared from special sensor microwave imager (SSM/I) measurements and GOES 8 imager solar reflectance (SR) measurements to ascertain the impact of sub-field-of-view (FOV) cloud effects on SSM/I 37 GHz retrievals. The SR retrievals also incorporate estimates of the cloud droplet effective radius derived from the GOES 8 3.9-micron channel. The comparisons consist of simultaneous collocated and full-resolution measurements and are limited to nonprecipitating marine stratocumulus in the eastern Pacific for two days in October 1995. The retrievals from these independent methods are consistent for overcast SSM/I FOVS, with RMS differences as low as 0.030 kg/sq m, although biases exist for clouds with more open spatial structure, where the RMS differences increase to 0.039 kg/sq m. For broken cloudiness within the SSM/I FOV the average beam-filling error (BFE) in the microwave retrievals is found to be about 22% (average cloud amount of 73%). This systematic error is comparable with the average random errors in the microwave retrievals. However, even larger BFEs can be expected for individual FOVs and for regions with less cloudiness. By scaling the microwave retrievals by the cloud amount within the FOV, the systematic BFE can be significantly reduced but with increased RMS differences of O.046-0.058 kg/sq m when compared to the SR retrievals. The beam-filling effects reported here are significant and are expected to impact directly upon studies that use instantaneous SSM/I measurements of cloud LWP, such as cloud classification studies and validation studies involving surface-based or in situ data.

Greenwald, Thomas J.↗

NASA NTRS1998

SeaWiFS Postlaunch Technical Report Series: The SeaWiFS Transfer Radiometer (SXR) - Volume 1

The SeaWiFS Transfer Radiometer (SXR) was built for the Sea-viewing Wide Field-of-view Sensor (SeaWiFS) Project as part of an Interagency Agreement with the National Aeronautics and Space Administration (NASA). The SXR is a multichannel radiometer designed to verify and compare measurements of spectral radiance at six discrete wavelengths in the visible and near infrared for various calibration sources in the SeaWiFS Project. In addition, the SXR is used to compare these sources to standards of spectral radiance maintained at the National Institute of Standards and Technology (NIST). The SXR was designed, built, and thoroughly characterized in the Optical Technology Division at NIST. A unique optical design provides six independent optical paths, each equipped with a temperature stabilized interference filter and silicon photodiode. A separate beam path through the input lens is used to visually align the SXR. The entrance windows for each channel overlap at the source, with each channel sampling a unique solid angle within the field of view of the SXR; this allows for simultaneous sampling of all channels. The combined standard relative uncertainty of spectral radiance measurements with the SXR is estimated to be between 0.6% and 1.3%. This report describes the design and construction of the SXR in detail, and gives the results of the optical characterization and calibrations done at NIST. The SXR has been used for several intercomparisons which include several SeaWiFS Intercalibration Round-Robin Experiments (SIRREXs); those done at the Marine Optical Buoy (MOBY) laboratories in Honolulu, Hawaii; at the NEC Corporation in Yokohama, Japan; and Orbital Sciences Corporation (OSC) in Germantown, Maryland. Thorough optical characterization and calibration of the SXR was essential to the successful application of the radiometer for these measurements.

Johnson, B. Carol↗

NASA NTRS1998

SeaWiFS Postlaunch Technical Report Series: The SeaWiFS Transfer Radiometer (SXR) - Volume 1

Hooker, Stanford B.↗

NASA NTRS2004

Analysis of the Variation of Energetic Electron Flux with Respect to Longitude and Distance Normal to the Magnetic Equatorial Plane for Galileo Energetic Particle Detector Data

In this study we examine ten-minute omni-directional averages of energetic electron data measured by the Galileo spacecraft Energetic Particle Detector (EPD). Count rates from electron channels B1, DC2, and DC3 are evaluated using a power law model to yield estimates of the differential electron fluxes from 1 MeV to 11 MeV at distances between 8 and 51 Jupiter radii. Whereas the orbit of the Galileo spacecraft remained close to the rotational equatorial plane of Jupiter, the approximately 11 degree tilt of the magnetic axis of Jupiter relative to its rotational axis allowed the EPD instrument to sample high energy electrons at limited distances normal to the magnetic equatorial plane. We present a Fourier analysis of the semi-diurnal variation of electron fluxes with longitude.

synchrotron radiation↗

NASA NTRS2011

On Deriving Incident Auroral Particle Fluxes in the Daytime Using Combined Ground-Based Optical and Radar Measurements

Particle energies and fluxes have predominantly been measured from instruments onboard satellites. In this study, we use daytime ground-based oxygen redline emission measurements, along with the ionospheric electron density, and electron temperature profiles measured from the incoherent scatter radar, and a physics-based modeling approach to derive the energy and flux of particles incident over Boston during the storm of 30 October 2003. We find that the characteristic energy and the associated flux vary between 0.07.5.7 keV and 0.5.130 mW/sq m, respectively, during the intense magnetic disturbance that brought aurora to midlatitudes. Such an approach not only offers another method to estimate the incident particle energies and fluxes but also enhances our understanding on the channels of energy deposition in the upper atmospheric region, especially during magnetic disturbances, about which database is poor.

Pallamraju, Duggirala↗

NASA NTRSDate not supplied

The GEOS Neural Network Retrieval (NNR) for Multi-spectral AOD

One of the difficulties in data assimilation is the need for multi-sensor data merging that can account for temporal and spatial biases between satellite sensors. In the Goddard Earth Observing System Model Version 5 (GEOS-5) aerosol data assimilation system, a neural network retrieval (NNR) is used as a mapping between satellite observed top of the atmosphere (TOA) reflectance and AOD, which is the target variable that is assimilated in the model. By training observations of TOA reflectance from multiple sensors to map to a common AOD dataset (in this case AOD observed by the ground based Aerosol Robotic Network, AERONET), we are able to create a global, homogenous, satellite data record of AOD from multiple sensors. In this presentation, I will present recent updates to the GEOS-5 NNR for estimation of spectral AOD from MODIS and VIIRS, and the potential for multi-channel AOD assimilation to provide constraints on aerosol composition.

GEOS↗

NASA NTRSDate not supplied

The GEOS Neural Network Retrieval (NNR) for Multi-spectral AOD

Patricia Castellanos↗

NASA NTRS2013

Conductance of Ion Channels - Theory vs. Experiment

Transmembrane ion channels mediate a number of essential physiological processes in a cell ranging from regulating osmotic pressure to transmission of neural signals. Kinetics and selectivity of ion transport is of critical importance to a cell and, not surprisingly, it is a subject of numerous experimental and theoretical studies. In this presentation we will analyze in detail computer simulations of two simple channels from fungi - antiamoebin and trichotoxin. Each of these channels is made of an alpha-helical bundle of small, nongenomically synthesized peptides containing a number of rare amino acids and exhibits strong antimicrobial activity. We will focus on calculating ionic conductance defined as the ratio of ionic current through the channel to applied voltage. From molecular dynamics simulations, conductance can be calculated in at least two ways, each involving different approximations. Specifically, the current, given as the number of charges transferred through the channel per unit of time, can be obtained from the number of events in which ions cross the channel during the simulation. This method works well for large currents (high conductance values and/or applied voltages). If the number of crossing events is small, reliable estimates of current are difficult to achieve. Alternatively, conductance can be estimated assuming that ion transport can be well approximated as diffusion in the external potential given by the free energy profile. Then, the current can be calculated by solving the one-dimensional diffusion equation in this external potential and applied voltage (the generalized Nernst-Planck equation). To do so three ingredients are needed: the free energy profile, the position-dependent diffusion coefficient and the diffusive flux of ions into the channel. All these quantities can be obtained from molecular dynamics simulations. An important advantage of this method is that it can be used equally well to estimating large and small currents. In addition, once the free energy profile becomes available the full current-voltage dependence can be readily obtained. For both channels we carried out calculations using both approaches. We also tested the main assumptions underlying the diffusive model, such as uncorrelated nature of individual crossing events and Fickian diffusion. The accuracy and consistency of different methods will be discussed. Finally we will discuss how comparisons between calculated and measured ionic conductance and selectivity of transport can be used for determining structural models of the channels.

Pohorille, Andrew↗

DOE OSTI2024

Resilient Consensus State Observer for Nonlinear Systems and Against Attacks

Herein, we investigate the design of a resilient consensus observer that yields correct and continuous state estimates of a nonlinear control system whose state observations are subject to attacks. The observations are assumed to be obtained from multiple sensors and/or communication channels employed to provide redundancy. It is shown that, in an attack-free setting, individual globally convergent observers can be designed for each sensor/channel using the corresponding state-dependent Jacobian system. To counter attacks, a resilient consensus observer is then designed by merging the observers estimates to produce a smooth consensus estimate. Resilient convergence of the consensus estimate to the true state is ensured under the condition that the sparsity of the attacks being less than a half of the number of redundant channels. As an illustrative example, the proposed scheme is successfully applied to the chaotic circuit synchronization problem in which their synchronization has been attacked.

97 MATHEMATICS AND COMPUTING↗

DOE OSTI2026

Dynamics of the water-plasma interface in various discharge modes of atmospheric-pressure plasmas

This paper presents an experimental study of the dynamics of the water-plasma interface during the interaction high-voltage (HV) atmospheric pressure discharge with the water surface. Under the influence of the voltage applied to the pin type electrode, discharges are formed at the air layer between the sharp-tip HV electrode and deionized water. Three discharge regimes were identified from synchronized electrical waveforms and imaging: (i) a weak linear regime at 3–10.6 kV, (ii) a branching streamer regime at the maximum applied voltage of 12.6 kV, and (iii) a continuous arc-like regime occurring during the transition to lower voltage and higher current (e.g., U ≈ 3.2 kV, I ≈ 4.07 mA). High-speed shadowgraph images showed a symmetric interfacial cavity whose depth increased nonlinearly with voltage from h 0 ≈ 0.1 mm at 3 kV to h 0 ≈ 2.7 mm at 10.6 kV, reaching a maximum depth of h 0 ≈ 5.9 mm at 12.6 kV, while the cavity disappeared in the continuous-channel regime and was replaced by outward-propagating wave-like motion. The deformation of the water surface during the discharge-water interaction is governed by the balance between electric field forces, surface tension, gravitational forces, and electrohydrodynamic forces, whose relative contributions vary with the applied voltage. This effect was explained by quantitatively estimating the magnitudes of the acting forces and establishing the force balance. Optical emission spectroscopy in the continuous-channel regime indicated air plasma signatures and yielded a gas temperature of approximately 400 K, while prolonged operation (≈ 20 min) increased the water temperature to ~ 70 °C, reduced the water-layer thickness from 6 mm to 3 mm, and decreased pH from 7 to 4. These regime-resolved, quantitative results clarify how the dominant interfacial forcing shifts with discharge mode and provide a mechanistic basis for controlling plasma-water interactions in atmospheric-pressure applications.

atmospheric pressure plasma↗

NASA NTRS1994

Temperature-moisture biases in ECMWF analyses based on clear sky longwave simulations constrained by SSMI and MSU measurements and comparisons to ERBE estimates

Clear sky longwave radiation fluxes for the summer of 1988 and winter of 1989 have been simulated with a radiative transfer model that includes detailed treatment of atmospheric gas absorption. The input data to the model are humidity and temperature profiles from European Center for Medium-Range Weather Forecasts (ECMWF) analyses and surface temperature measurements from the International Satellite Cloud Climatology Project. To reduce the inherent uncertainties in humidity profiles, the ECMWF moisture fields have been adjusted, based on the climatological relationship between the moisture profile and total precipitable water (PW), so that the ECMWF PW is equal to that derived from Special Sensor Microwave Imager (SSMI) data. SSMI and ECMWF PW patterns are generally similar, but significant differences in magnitude are found in the low latitudes, particularly over the subtropical oceans in the Southern Hemisphere. At the same time the tropospheric brightness temperature (T(sub B)) at 53.74 GHz has been computed using a microwave transfer model with ECMWF temperature and humidity fields as inputs. The comparison of computed T(sub B) with the Microwave Sounding Unit (MSU) channel 2 T(sub B) revealed differences larger than 1.5 K over most of the oceans, suggesting that the ECMWF model atmosphere has a cold bias. Maximum biases greater than 3 K are found in low latitudes. After removing the bias from the ECMWF temperature field, a new set of temperature profiles yielding brightness temperature equal to MSU channel 2 T(sub B) has been obtained. Simulation results clearly demonstrate that inclusion of satellite estimates of PW and T(sub B) enhances the accuracy of the clear sky LW flux simulation, substantially reducing the differences from Earth Radiation Budget Experiment (ERBE) estimates. Global averages indicate that the model-derived top-of-atmosphere (TOA) clear sky fluxes from the adjusted moisture and temperature profiles are in very good agreement with satellite-measured ERBE values, differing by only 1.4 W/sq m. By contrast, the calculation using only ECMWF analyses without any adjustments gives a significant underestimation of TOA clear sky fluxes up to 10.7 W/sq m compared to the satellite measurements, suggesting that the constraint method can significantly improve the accuracy in the radiation budget simulation. The results also indicate that the ECMWF-based simulation errors are, at least for the two seasons studied, mainly attributed to the error in the temperature field rather than to errors in the moisture field.

Sohn, Byung-Ju↗

NASA NTRS1991

Ice water path estimation and characterization using passive microwave radiometry

Model computations of top-of-atmospheric microwave brightness temperatures T(B) from layers of precipitation-sized ice of variable bulk density and ice water content (IWC) are presented. It is shown that the 85-GHz T(B) depends essentially on the ice optical thickness. The results demonstrate the potential usefulness of scattering-based channels for characterizing the ice phase and suggest a top-down methodology for retrieval of cloud vertical structure and precipitation estimation from multifrequency passive microwave measurements. Attention is also given to radiative transfer model results based on the multiparameter radar data initialization from the Cooperative Huntsville Meteorological Experiment (COHMEX) in northern Alabama. It is shown that brightness temperature warming effects due to the inclusion of a cloud liquid water profile are especially significant at 85 GHz during later stages of cloud evolution.

Vivekanandan, J.↗

NASA NTRS2006

FETs Based on Doped Polyaniline/Polyethylene Oxide Fibers

A family of experimental highly miniaturized field-effect transistors (FETs) is based on exploitation of the electrical properties of nanofibers of polyaniline/ polyethylene oxide (PANi/PEO) doped with camphorsulfonic acid. These polymer-based FETs have the potential for becoming building blocks of relatively inexpensive, low-voltage, highspeed logic circuits that could supplant complementary metal oxide/semiconductor (CMOS) logic circuits. The development of these polymerbased FETs offers advantages over the competing development of FETs based on carbon nanotubes. Whereas it is difficult to control the molecular structures and, hence, the electrical properties of carbon nanotubes, it is easy to tailor the electrical properties of these polymerbased FETs, throughout the range from insulating through semiconducting to metallic, through choices of doping levels and chemical manipulation of polymer side chains. A further advantage of doped PANi/PEO nanofibers is that they can be made to draw very small currents and operate at low voltage levels, and thus are promising for applications in which there are requirements to use many FETs to obtain large computational capabilities while minimizing power demands. Fabrication of an experimental FET in this family begins with the preparation of a substrate as follows: A layer of silicon dioxide between 50 and 200 nm thick is deposited on a highly doped (resistivity 0.01 W.cm) silicon substrate, then gold electrodes/contact stripes are deposited on the oxide. Next, one or more fibers of camphorsulphonic acid-doped PANi/PEO having diameters of the order of 100 nm are electrospun onto the substrate so as to span the gap between the gold electrodes (see Figure 1). Figure 2 depicts measured current-versus-voltage characteristics of the device of Figure 1, showing that saturation channel currents occur at source-todrain potentials that are surprisingly low, relative to those of CMOS FETs. The hole mobility in the depletion regime in this transistor was found to be 1.4 10(exp -4) sq cm/(V.s), while the one-dimensional charge density at zero gate bias was estimated to be approximately one hole per 50 two-ring repeat units of polyaniline, consistent with the rather high channel conductivity (approx. 10(exp -3) S/cm). Reducing or eliminating the PEO content of the fibers is expected to enhance the properties of future versions of this transistor.

Theofylaktos, Noulie↗

DOE OSTI2020

Performance simulation of the soft gamma-ray concentrator

The soft gamma-ray concentrator is a telescope mission concept utilizing a suitable arrangement of bent multilayer structures of alternating low- and high-density materials. This lens is able to channel gamma-ray photons via total external reflection and concentrate the incident radiation to a point. The channeling technique offers the potential for concentrating gamma rays with focal lengths <10 m and energies >100 keV, beyond the reach of current grazing-incidence hard x-ray mirrors. For the performance estimation of such an instrument, we have developed a flexible set of computer modeling tools to compute the optical properties of multilayer structures, predict the channeling efficiency for a given multilayer configuration, and aid in the optimization of potential gamma-ray concentrator-based telescope designs. This modeling includes the multilayer optical properties calculated by the IMD software, the ray tracing using an IDL code, and the focal plane detector simulation by MEGAlib. We illustrate the potential of this approach by presenting simulated astronomical observations from a balloon-borne platform. The final result, including simulated effective area, instrument sensitivity, and polarization performance, shows that the gamma-ray concentrator will provide greatly increased sensitivity for next-generation soft gamma-ray missions with modest cost and complexity.

47 OTHER INSTRUMENTATION↗

NASA NTRS1999

A TRMM Microwave Radiometer Rain Rate Estimation Method with Convective and Stratiform Discrimination

Tropical Rainfall Measuring Mission (TRMM) Microwave Imager (TMI) radiometer brightness temperature data in the 85 GHz channel (T85) reveal distinct local minima (T85min) in a regional map containing a Mesoscale Convective System (MCS). This is because of relatively small footprint size (approximately 5.5 km) and strong extinction properties in this channel of the TMI. A map of surface rain rate for that region, deduced from simultaneous measurements made by the Precipitation Radar (PR) on board the TRMM satellite, reveals that these T85(sub min), produced by scattering, correspond to local PR rain maxima. Utilizing the PR rain rate map as a guide, we infer empirically from TMI data the presence of three different kinds of thunderstorms or Cbs. These Cbs are classified as young, mature, and decaying types, and are assumed to have a scale of about 20 km on the average. Two parameters are used to classify these three kinds of Cbs based on the T85 data: a) the magnitude of scattering depression deduced from local T85(sub min) and b) the mean horizontal gradient of T85 around such minima. Knowing the category of a given Cb, we can estimate the rain rate associated with it. Such estimation is done with the help of relationships linking T85min to rain rate in each Cb type. Similarly, a weak background rain rate in all the areas where T85 is less than 260 K is deduced with another relationship linking T85 to rain rate. In our rain retrieval model, this background rain constitutes stratiform rain where the Cbs are absent. Initially, these relationships are optimized or tuned utilizing the PR and TMI data of a few MCS events. After such tuning, the model is applied to independent MCS cases. The areal distribution of light (1-10 mm/hr), moderate (10-20 mm/hr), and intense (>= 20 mm/hr) rain rates are retrieved satisfactorily. Accuracy in the estimates of the light, moderate, and intense rain areas and the mean rain rates associated with such areas in these independent MCS cases is on the average about 15 %. Taking advantage of this ability of our retrieval method, one could derive the latent heat input into the atmosphere over the 760 km wide swath of the TMI radiometer in the tropics.

Prabhakara, C.↗