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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 379 records · Page 21
All sourcesNASA NTRSDOE OSTI
DOE OSTI2019

Effect of the electric field induced birefringence on the slab waveguide evanescent-wave sensor sensitivity

We have investigated the potential of using the E-field induced birefringence for improving the sensitivity of uniaxial anisotropic slab waveguide sensor based on evanescent wave interactions. LiNbO{sub 3} waveguide core was used as an example. We have calculated the sensor sensitivity formulas for the two kinds of modes propagating simultaneously in the waveguide sensor. In our study, we have distinguished between two different cases. The first case when the electric field is applied along the optic axis (+c) of the LiNbO{sub 3} wave guiding film (positive electric field); the second case when the electric field is applied opposite to the optic axis (−c) of such uniaxial crystal (negative electric field). The obtained results showed that, for positive electric field, increasing the electric field induces an increasing of the total anisotropy which causes decreasing on sensor sensitivity. However, for negative electric field, the increase of absolute values of negative electric field induces a decrease of the total anisotropy, the latter increases the sensor sensitivity. On the other hand, the study of the physical parameters on the sensor sensitivity showed that, to maximize the sensor sensitivity, it is advisable to use isotropic substrate that has a refractive index as closer as possible to the measurand index.

42 ENGINEERING↗
DOE OSTI2022

Decarbonization scenarios of the U.S. Electricity system and their costs

Decarbonizing the electricity system to zero-carbon emission is crucial for climate change mitigation. Previous studies have shown that such a transition in the United States (U.S.) may lead to higher system cost compared to a business-as-usual case, but it is not well-known how the cost of electricity generation varies at sub-regional level under the transition, and studies have rarely evaluated the trade-off between the cost and avoided climate damages, as well as the potential roles of negative emission technologies (NETs) in the electricity decarbonization. In this work, we present a regionally resolved national model to quantify the cost of decarbonizing the U.S. electricity system under a set of possible scenarios. The results show that, compared to the reference scenario without a decarbonization policy, reaching zero CO 2 emission by 2050 would incur, depending on the scenarios, 335-494 billion USD additional cost to the U.S. electric power sector during 2020-2050. The regional costs of electricity generation ranges from 2.4 to 4.7 cent/kWh, largely due to the generation profiles and renewable resources availability of those regions. The additional costs can be translated to an average CO 2 abatement cost of 29-59 USD/metric ton CO 2 (with 2%-7% discount rates), which are comparable to the social cost of carbon in the literature at around 4% discount rate. The results also show that the cost of mitigating the last few percent CO 2 emission from the U.S. electricity system may exceed the costs of NETs, indicating an opportunity for NETs to contribute to electricity decarbonization.

24 POWER TRANSMISSION AND DISTRIBUTION↗
DOE OSTI2022

Non-premixed counterflow methane flames in DC/AC/NS electric fields

The response of counterflow diffusion flames to sub-breakdown DC and AC electric fields, as well as their superposition with ns pulse discharge waveforms, is studied in the plane-to-plane electrode geometry. Sub-breakdown DC and low-frequency AC electric fields cause the flame displacement toward the grounded electrode, in the direction of the applied field, indicating that the body force on the positive ions exceeds that on the electrons and negative ions. As the AC frequency increases, the flame response becomes less pronounced, due to the reduction of the electrohydrodynamic (EHD) body force impulse over the AC half-period. The electric field in the electrode gap is determined by ps Electric Field Induced Second Harmonic (E-FISH) generation, with absolute calibration using sub-breakdown ns pulses overlapped with the measured electric field waveform. The results show that the electric field distribution across the flame in the current saturation regime follows the Laplacian field. This indicates that the space charge density in the gap is too low to distort the applied DC or AC field, consistent with the kinetic modeling predictions. Combining a nanosecond pulse discharge with a sub-breakdown DC field generates a diffuse plasma across the entire gap. Time-resolved and spatially resolved measurements of the electric field in the discharge indicate the ionization wave propagation between the electrodes. The present results do not exhibit a detectable flame displacement enhancement by ns discharge pulses combined with a sub-breakdown field, observed previously. Kinetic modeling calculations show that the absence of this effect in the plane-to-plane geometry is due to the rapid plasma self-shielding. This indicates that alternative electrode geometries limiting the self-shielding would be more effective for the plasma / electric field enhanced flameholding and flame stabilization applications.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

Electrical Potential Investigation of Reversible Metastability and Irreversible Degradation of CdTe Solar Cells

In this paper, we report on the stability of CdTe devices with a structure of TCO/MZO/CdSeTe/CdTe/back-contact. The device showed reversible transitions between the light-soak state (LSS) with the best device efficiency and the dark-soak state (DSS) with an inferior efficiency. However, it showed an irreversible degradation state (DgS) driven by long-hour light soaking at an elevated temperature. We have investigated transitions between these three states from the perspective of the electric field by nm-resolution potential imaging across the devices using Kelvin probe force microscopy (KPFM). The results exhibit different anomalous electric field profiles. At the LSS, the electric field exhibits a main peak inside the CdSeTe layer instead of the MZO/CdSeTe heterointerface, illustrating a buried homojunction (BHJ) of the device. At the DSS, a large electric field peak at the MZO/CdSeTe interface was measured, which probably resulted in the inferior fill factor at the DSS. At the DgS, the electric field peak at the MZO/CdSeTe interface increased further and a third electric field was measured at the back contact of the device. Device modeling using COMSOL software, in alignment with both the electric field and device current-voltage curves, elucidates that a low n-doped CdSeTe in the region near the MZO/CdSeTe interface caused the BHJ in the LSS and a loss of MZO doping and/or increase of the conduction band offset spike due to long-term stress caused the increased electric field near the MZO/CdSeTe interface at the DgS.

CdTe solar cell↗
DOE OSTI2023

Electric Field Effects on Water and Ion Structure and Diffusion at the Orthoclase (001)–Water Interface

Understanding the electrochemical properties of mineral–water interfaces tends to rely upon electrical double layer (EDL) models, but these models are based on the assumption that electrostatic equilibrium is constantly maintained. In reality, interfacial reactions, ion diffusion, and their electrochemical signatures are based in nonequilibrium conditions of locally or globally imbalanced electrical fields where current EDL models have limited purview. In this work, we performed molecular dynamics (MD) simulations of the orthoclase (001) surface in contact with a 1 M NaCl aqueous solution under various electric fields, to explore the interplay between EDL structure and dynamics when perturbed by electric fields of different direction and strength, by confinement, and by different distributions of structural surface charge. The simulations showed that confinement between two opposing (001) surfaces led to the development of an induced field when the applied field was perpendicular to the surfaces and, as a result, to ionic diffusion coefficients that were independent of electric field strength. In contrast, when the applied field was parallel to the surfaces, confinement resulted in ionic diffusion coefficients that were more strongly dependent on the magnitude of the electric field than in bulk water. Differences in the density and distribution of aluminol groups on the two surfaces had a significant impact on how the interfacial structure and dynamics varied in the presence of an electric field. Notably, these differences resulted in an electro-osmotic flow with opposite directions at the two surfaces under parallel applied electric field. Overall, the MD simulations highlighted the importance of considering atomic-level structure and heterogeneities when developing models of the electrochemical properties of mineral–water interfaces.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

Electric Field Control of Magnetic Skyrmion Helicity in a Centrosymmetric 2D van der Waals Magnet

Two-dimensional van der Waals magnets hosting topological magnetic textures, such as skyrmions, show promise for spintronics and quantum computing. Electrical control of these topological spin textures is crucial for enhancing operational performance and functionality. Here, using electron microscopy combined with in situ electric and magnetic biasing, we show that the skyrmion helicity in insulating Cr 2 Ge 2 Te 6 can be controlled by the direction of the external electric field applied during the field cooling process. The electric field-tuned helicity remains stable at low temperature, even amid variations in magnetic and electric fields. Our theoretical investigation reveals that nonzero Dzyaloshinskii-Moriya interactions between nearest neighbors, induced by the electric field, change their sign upon reversing the electric field direction, thereby facilitating helicity selection. The electrical control of magnetic helicity demonstrated in this study can be extended to other centrosymmetric skyrmion-hosting magnets, paving the way for future device designs in topological spintronics and quantum computing.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

A numerical solver for investigating the space charge effect on the electric field in liquid argon time projection chambers

This paper reports the development of a numerical solver aimed to simulate the interaction between the space charge (i.e. ions) distribution and the electric field in liquid argon time projection chamber (LArTPC) detectors. The ion transport equation is solved by a time-accurate, cell-centered finite volume method and the electric potential equation by a continuous finite element method. The electric potential equation updates the electric field which provides the drift velocity to the ion transport equation. The ion transport equation updates the space charge density distribution which appears as the source term in the electric potential equation. The interaction between the space charge distribution and the electric field is numerically simulated within each physical time step. The convective velocity in the ion transport equation can include the background flow velocity in addition to the electric drift velocity. The numerical solver has been parallelized using the Message Passing Interface (MPI) library. Numerical tests show and verify the capability and accuracy of the current numerical solver. It is planned that the developed numerical solver, together with a Computational Fluid Dynamics (CFD) package which provides the flow velocity field, can be used to investigate the space charge effect on the electric field in large-scale particle detectors.

42 ENGINEERING↗
DOE OSTI2021

Potential of Utilizing Thermal Energy Storage Integrated Ground Source Heat Pump System to Reshape Electricity Demand in the United States

Each year, more than 20% of electricity generated in the United States is consumed for meeting the thermal demands (e.g., space cooling, space heating, and water heating) in residential and commercial buildings. Integrating thermal energy storage (TES) with building’s HVAC systems has the potential to reshape the electric load profile of the building and mitigate the mismatch between the renewable generation and the demand of buildings. A novel ground source heat pump (GSHP) system integrated with underground thermal energy storage (UTES) has been proposed to level the electric demand of buildings while still satisfying their thermal demands. This study assessed the potential impacts of the proposed system with a bottom-up approach. The impacts on the electricity demand in various electricity markets were quantified. The results show that, within the capacity of the existing electric grids, the maximum penetration rate of the proposed system in different wholesale markets could range from 51% to 100%. Altogether, about 46 million single-family detached houses can be retrofitted into the proposed system without increasing the annual peak demand of the corresponding markets. By implementing the proposed system at its maximum penetration rate, the grid-level summer peak demand can be reduced by 9.1% to 18.2%. Meanwhile, at the grid level, the annual electricity consumption would change by –12% to 2%. The nationwide total electricity consumption would be reduced by 9%.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗
DOE OSTI2020

Electric Vehicle Adoption in Illinois

Over 1.3 million plug-in electric vehicles (PEVs) have been sold in the United States since 2010 when the first Chevy Volt and Nissan Leaf vehicles came on the market. Currently, electric vehicles account for about 2% of monthly light-duty vehicle (LDV) sales. More than 40 different electric vehicle models are actively being marketed, and most of these are LDVs. Over the last few years, automakers have brought more models, with varying mileage ranges, to the market, including medium-duty and heavy-duty trucks and buses. Government agencies at the federal, regional, and state levels, as well as utilities across the United States, have provided financial and non-financial incentives to promote electric vehicle adoption and charging infrastructure deployment. Argonne National Laboratory, sponsored by the U.S. Department of Energy, has developed tools and collected data to quantify the energy, economic, and environmental benefits of electric vehicles. This project has three objectives. First, we summarize the policies and other actions of the federal government, various states/regions, and utilities to promote PEV adoption, and evaluate their relative effectiveness based on a review of the literature. Second, we identify possible PEV adoption paths or scenarios that would result in PEVs making up 15% of all on-road vehicles in Illinois, and we quantify the resulting impacts on petroleum consumption and electricity demand. We also summarize the possible reduction in greenhouse gas (GHG) and criteria pollutant emissions due to PEV adoption. The PEV scenarios include private and public adoption of electric cars, light trucks (e.g., sports utility vehicles [SUVs], vans, pickups), medium-duty vehicles (MDVs), and heavy-duty vehicles (HDVs). Third, we estimate hourly charging loads of light-duty PEVs in 2030 associated with these scenarios, incorporating assumptions about vehicle electric range, efficiency, and travel behavior.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗
DOE OSTI2026

Pilot Development Progress to Demonstrate Electric Thermal Energy Storage (ETES) Using Low-Cost Particles

The rapid growth of future energy demand increases the need to economically store electrical energy over durations up to several days in long-duration energy storage (LDES) applications. LDES can reduce the grid stress for improving the resilience of the grid. The integration of renewable power and storage has several significant and positive impacts including expanding the renewable energy portion of electricity generation, meeting peak-load demand, and coordinating supply and demand. Several energy storage approaches including mechanical, chemical and electrochemical methods are currently deployed or under development. However, LDES requirements pose unique challenges for scalability, energy capacity, and cost. Thermal energy storage (TES) has the ability to store a large capacity of energy with improved site flexibility compared to incumbent LDES technologies (i.e., pumped hydro) and has attracted significant interest. Our development in TES technology using solid particles as the storage medium has shown feasibility and potential in serving LDES purposes. Particle TES has various advantages over commercialized molten nitrate salt TES and has emerged as a promising storage technology originating from Generation 3 concentrating solar power (CSP) development. Stable, inexpensive silica sand produced in the Midwestern U.S. was identified as a suitable storage medium and has been validated through lab heating and cycling tests. We have successfully developed particle TES for bidirectional electric energy storage to broaden the applications for TES beyond CSP technologies and into standalone electric-thermal energy storage (ETES) systems. Key component designs and performance were verified with prototype testing and model simulations. The ETES system uses high-temperature, low-cost particle thermal energy storage coupled with a unique pressurized fluidized bed heat exchanger that supports a high-efficiency, air-Brayton combined power cycle. At times of low energy demand or high renewable production, an electric particle heater heats large quantities of solid particles to high temperatures in excess of 1100 degrees C. The particles are stored in internally insulated silos. At times of high electricity demand, the hot particles are gravity-fed through the heat exchanger where stored thermal energy is transferred to the power cycle working fluid to drive the gas turbine power generation system, thereby converting the thermal energy back into electricity for the grid. The cold particles leaving the heat exchanger are returned to the storage silos by a well-insulated particle conveyor. This ETES technology using particle TES can be sited anywhere and is predicted to be economic and efficient. Moreover, this ETES technology could be co-located with a retired coal or gas plant to leverage existing power generation and grid infrastructure. Our work has focused on the development of each of the key components (e.g., the electric particle heater, particle storage silos, and the particle-to-gas pressurized fluidized bed heat exchanger) through conceptual designs, prototype testing, and computational modeling. These developments demonstrate technological feasibility and are an important step towards the next phase of development of this promising LDES technology. This presentation will show the progress in developing a pilot demonstration of the ETES system on a commercially relevant scale.

25 ENERGY STORAGE↗
NASA NTRS2018

Examining the Conceptual Design Process for Future Hybrid-Electric Rotorcraft

Hybrid-electric propulsion systems introduce immense complexity and numerous design challenges not previously encountered in aircraft design. Traditional conceptual-level rotorcraft design approaches may not adequately capture the level of propulsion system detail desired for hybrid-electric vehicle conceptual design. As part of a NASA Small Business Innovative Research (SBIR) Phase II contract, Empirical Systems Aerospace (ESAero) investigated the implementation of several hybrid-electric propulsion architectures onto three rotorcraft configurations. Unique hybrid-electric variants of these configurations were compared against their conventionally-powered counterparts using typical metrics such as payload, range, and energy efficiency. The feasibility and performance of these vehicles was also investigated in the +15 and +30-year timeframes based on third-party estimations for future component performance. Using the lessons learned during this trade study, ESAero then conducted a conceptual design effort for a hybrid-electric tiltrotor demonstrator based on the XV-15. A detailed integration of the hybrid-electric propulsion system into the vehicle airframe was also performed. The hybrid-electric XV-15 concept vehicle was estimated to achieve a 10% reduction in cruise fuel consumption compared to the original NASA XV-15 at the cost of increasing the vehicle empty weight by almost 25%. The success of this design effort suggests that the design of a manned, hybrid-electric tiltrotor is technically feasible at current technology levels.

Future↗
NASA NTRS2021

Thunderstorm and Fair-weather Quasi-Static Electric Fields Over Land and Ocean

Natural lightning and the associated clouds are known to behave differently over land and ocean, but many questions remain. We expand the related observational datasets by obtaining simultaneous quasi-static electric field observations over coastal land, near-shore water, and deep ocean regions during both fair-weather and thunderstorm periods. Oceanic observations were obtained using two 3-m NOAA buoys that were instrumented with Campbell Scientific electric field mills to measure the quasi-static electric fields. These data were compared to selected electric field records from the existing on-shore electric field mill suite of 31 sensors at Kennedy Space Center (KSC). Lightning occurrence times, locations and peak current estimates for both onshore and ocean were provided by the U.S. National Lightning Detection Network. The buoy instruments were first evaluated on-shore at the Florida coast, and the first system was calibrated for field enhancements and to confirm proper behavior of the system in elevated-field environments. The buoys were then moored 20 mi and 120 mi off the coast of KSC in February (20 mi) and August (120 mi) 2014. Diurnal fair-weather fields at both ocean sites matched will with each other and with those found during the Carnegie cruise, but mean values were 33% smaller, due at least in-part to constraints on the calibration procedure. Diurnal fair-weather fields variations at coastal and inland sites were a poorer match than offshore, likely because the offshore environment is “cleaner” with limited variations in local space charge, lower surface aerosol densities, little surface heating to disturb the surface charge layer during fair weather, and fewer local radioactive sources to modulate the near-surface electrical conductivity. Storm-related static fields were 4-5× larger at both oceanic sites than over land, likely due to decreased screening by near-surface space charge produced by corona current. The time-evolution of the electric field and field changes during storm approach are sufficiently different over land and ocean to warrant further study. This work shows the quality, accuracy, and reliability of these data, and has demonstrated the practicality of off-shore electric field measurements for safety- and launch-related decision making at KSC.

Lightning↗
DOE OSTI2020

Role of Electric Vehicles in the U.S. Power Sector Transition: A System-Level Perspective

After over a century of petroleum dominance many anticipate that electrification could disrupt the transportation energy landscape. At the same time, the electric power systems are undergoing profound changes: variable renewables are displacing conventional generation sources; distributed generation is disrupting utility business models; energy storage and other new technologies are emerging; and the traditional system based on the premise that generation is dispatched to match an inelastic demand is evolving to create a system with greater participation in power system planning and operations from traditionally passive consumers. In this context, it is important to understand how transportation electrification will impact electricity demand and in turn electricity supply, including changes in the load shapes that characterize the system and the opportunity to leverage flexible electric vehicle (EV) charging to better integrate demand and supply. Assessing the impacts of electrification on the energy system requires an understanding of how it might impact the amount and shape of electricity consumption, and how this electricity can be supplied. In particular, increased adoption of electric vehicles introduces a new source of demand altogether, potentially very flexible. Moreover, electrification could shift the consumption of natural gas between sectors, thereby affecting the economics for natural gas-fired generation relative to other electricity generation options. Several factors will impact the evolution of the power system under a widespread electrified future, which, in turn, could have far-reaching effects on future energy costs and emissions.

47 OTHER INSTRUMENTATION↗
DOE OSTI2020

Can Polyelectrolyte Mechanical Properties be Directly Modulated by an Electric Field? A Molecular Dynamics Study

Multifunctionality in polymers facilitates their application in emerging technologies. Electrical fields are a preferred stimulus because of the speed and ease of application to bulk polymers. While a wide range of electrically triggered actuators are developed, and electrically controlled adhesion between gels is demonstrated, modification of bulk mechanical properties via electrical stimuli remains elusive. Polymers with covalently incorporated ionic charge (polyelectrolytes) should be well suited to achieving this goal since the mechanical properties depend on electrostatic interactions and these charges are intrinsically susceptible to electric fields. Molecular dynamics simulations are utilized here to investigate whether electric fields can modulate the mechanical properties of polyelectrolytes and to understand the governing mechanisms. Mechanical property modulation by electric field is found to be sensitive to the charge distribution—charges must be tightly attached to the polymer backbone, and responsivity is greater if a single backbone contains both positive and negative charges. The dominant mechanisms are reorientation and stretching of the polymer chains, which also elongate the ionic clusters to maintain strong electrostatic interactions throughout deformation. Furthermore, these insights are critical for future experimental realization of polymers with electric field regulated mechanical properties.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Deep Reinforcement Learning Based Smart Water Heater Control for Reducing Electricity Consumption and Carbon Emission

Water heating is the third largest electricity consumer in U.S. households, after space heating and cooling. Thus, water heaters represent a significant potential for reducing electricity consumption and associated CO2 emissions of residential buildings. To this end, this study proposes a model-free deep reinforcement learning (RL) approach that aims to minimize the electricity consumption and the CO2 emissions of a heat pump water heater without affecting user comfort. In this approach, a set of RL agents focusing on either electricity saving or emission reduction, with different look ahead periods, were trained using the deep Q-networks (DQN) algorithm and their performance was tested on different hot water usage and Marginal Operating Emissions Rate (MOER) profiles. The testing results showed that the RL agents that focus on electricity saving can save electricity in the range of 12–22% by operating the water heater with maximum heat pump efficiency and minimum electric element utilization. On the other hand, the RL agents that focus on emission reduction reduced emissions in the range of 18–37% by making use of the variable MOER values. These RL agents used the heat pump and/or an element when the MOER values are low due to the availability of renewable energy sources (e.g., solar and wind) and mostly avoided the periods of carbon-intensive periods. Overall, these results showed that the proposed RL approach can help minimize the electricity consumption and the CO2 emissions of a heat pump water heater without having any prior knowledge about the device.

Amasyali, Kadir↗
DOE OSTI2023

Modeling the Water Systems of the Western US to Support Climate‐Resilient Electricity System Planning

Abstract Electricity and water systems in the Western US (WUS) are closely connected, with hydropower comprising 20% of total annual WUS generation, and electricity related to water comprising about 7% of total WUS electricity use. Because of these interdependencies, the threat of climate change to WUS resources will likely have compounding electricity impacts on the Western Interconnect grid. This study describes a WUS‐wide water system model with a particular emphasis on estimating climate impacts on hydropower generation and water‐related electricity use, which can be linked with a grid expansion model to support climate‐resilient electricity planning. The water system model combines climatically‐driven physical hydrology and management of both water supply and demand allocation, and is applied to an ensemble of 15 climate scenarios out to 2050. Model results show decreasing streamflow in key basins of the WUS under most scenarios. Annual water‐related electricity use increases up to 4%, and by up to 6% during the summer months, driven by growing agricultural demands met increasingly through a shift toward energy‐intensive groundwater to replace declining surface water. Total annual hydropower generation changes by +5% to −20% by mid‐century but declines in most scenarios, with decreases in summer generation by up to nearly −30%. Water‐related electricity use increases tend to coincide with hydropower generation declines, annually and seasonally, demonstrating the importance of concurrently evaluating the climate signal on both water‐for‐energy and energy‐for‐water to inform planning for grid reliability and decarbonization goals.

13 HYDRO ENERGY↗
DOE OSTI2024

Estimating the Electric Fields Driving Lightning Dart Leader Development With BIMAP‐3D Observations

Abstract In this paper, a numerical dart leader model has been implemented to understand the leader's development and the corresponding electric field changes observed by the 3D broadband mapping and polarization (BIMAP‐3D) system. The model assumes the extending leader channel is equipotential and has a linear charge distribution induced by an ambient electric field. The charge distribution induced by the ambient field can be used to model the electric field change at the ground. We then find the ambient electric field which best fits the field change measurements at the two BIMAP stations. The estimated ambient electric field decreases in the direction of dart leader propagation. Our observations and modeling results are consistent with our earlier hypothesis that dart leader speed is proportional to the electric field at the leader tip. The model also supports our earlier analysis that leader speed variations near branch junctions were due to previous charge deposits near the junctions. The modeled tip electric field is generally lower than the breakdown field unless the pre‐dart‐leader channel has a significant temperature of 3,000 K. This is consistent with the fact that dart leaders typically do not form new branches into the virgin air. Furthermore, the tip field is generally close to the negative streamer stability field at ambient temperatures, explaining the nature of the narrow and well‐defined channel structure. In addition to the charge distribution and the ambient and tip electric field, the development of the channel potential and current distribution are also presented.

3D lightning mapping↗
DOE OSTI2020

Coherent electrical control of a single high-spin nucleus in silicon

Nuclear spins are highly coherent quantum objects. In large ensembles, their control and detection via magnetic resonance is widely exploited, for example, in chemistry, medicine, materials science and mining. Nuclear spins also featured in early proposals for solid-state quantum computers and demonstrations of quantum search and factoring algorithms. Scaling up such concepts requires controlling individual nuclei, which can be detected when coupled to an electron. However, the need to address the nuclei via oscillating magnetic fields complicates their integration in multi-spin nanoscale devices, because the field cannot be localized or screened. Control via electric fields would resolve this problem, but previous methods relied on transducing electric signals into magnetic fields via the electron–nuclear hyperfine interaction, which severely affects nuclear coherence. In this work, we demonstrate the coherent quantum control of a single 123 Sb (spin-7/2) nucleus using localized electric fields produced within a silicon nanoelectronic device. The method exploits an idea proposed in 1961 but not previously realized experimentally with a single nucleus. Our results are quantitatively supported by a microscopic theoretical model that reveals how the purely electrical modulation of the nuclear electric quadrupole interaction results in coherent nuclear spin transitions that are uniquely addressable owing to lattice strain. The spin dephasing time, 0.1 seconds, is orders of magnitude longer than those obtained by methods that require a coupled electron spin to achieve electrical driving. These results show that high-spin quadrupolar nuclei could be deployed as chaotic models, strain sensors and hybrid spin-mechanical quantum systems using all-electrical controls. Integrating electrically controllable nuclei with quantum dots could pave the way to scalable, nuclear- and electron-spin-based quantum computers in silicon that operate without the need for oscillating magnetic fields.

42 ENGINEERING↗