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At least 361 records · Page 20

Irradiation in the Swiss Spallation Neutron Source and its Applications

In high power (∼ 1 MW or higher) spallation targets being operated or developed for different attractive applications such as neutron scattering science and technology or accelerator driven systems (ADS) for nuclear waste transmutation, both target and structural materials are exposed to intensive irradiation of high energy protons and spallation neutrons. Since spallation reactions induced by high energy protons can produce helium (He) and hydrogen (H) and other transmutation elements at very high rates, the behavior of materials used in a spallation irradiation environment can be much different from those observed from materials irradiated with neutrons in fission reactors. Therefore, the damage induced by spallation irradiation cannot be simply simulated by fission neutron irradiation experiments. Seven irradiation experiments have been conducted in the targets of the Swiss Spallation Neutron Source (SINQ) at the Paul Scherrer Institute (PSI) since 1998 within a broad international collaboration with Commissariat a L'energie Atomique Centre d'Etudes de Saclay (CEA), Forschungszentrum Juelich (FZJ), Japan Atomic Energy Agency (JAEA), Los Alamos National Laboratory (LANL), Oak Ridge National Laboratory (ORNL), University California Santa Barbara (UCSB) and several institutes of Chinese Academy of Sciences. More than 7000 samples from various Al-, Ti-, Fe-, Ni-, Zr-, and W-alloys and SiC/SiC, C/SiC and MAX-phase ceramics composites have been irradiated to doses up to ∼25 dpa (in Fe) and ∼2000 appm He at temperatures up to ∼800 deg. C. In addition, quite many specimens were irradiated in contact with stagnant liquid metals such as Hg, PbBi, PbLi etc. Dedicated post-irradiation examinations (PIE) have been performed, together with the international collaborators. Various mechanical tests including tensile, bend, Charpy-impact, small punch and hardness have been carried out to obtain the mechanical properties of the materials after irradiation. The microstructural changes in the irradiated specimens have been investigated by means of transmission electron microscopy, positron annihilation spectroscopy, atom probe tomography etc. Many novel results have been obtained from the PIE conducted by PSI and other STIP partner laboratories. The DBTT-shift of different FM steels increases more or less linearly with dose after irradiation in the SINQ target, while it saturates at a level of few dpa in fission neutron irradiation cases. This phenomenon can be mostly attributed to helium effects. In addition to the strong embrittlement effect, pronounced hardening effect was also detected in high dose specimens, which was contributed by high density helium bubbles.

36 MATERIALS SCIENCE↗

PANDA-FES: Portable and Adaptable Neutron Diagnostics for Advancing Fusion Energy Science

Nuclear fusion is a potential source of carbon-free electricity with many concepts in development. The Portable and Adaptable Neutron Diagnostics for Advancing Fusion Energy Science (PANDA-FES) suite has been deployed since 2021 to measure neutron yield, energy, and spatiotemporal source location at two different Z-pinch fusion devices. This diagnostic can be used at a variety of facilities pursuing fusion in the magnetic, inertial, and magneto-inertial regimes. These different regimes have a wide range of time scales from less than 100 ns to a few μ s, neutron yields from 10 6 to 10 11 , and noise environments. Neutron yield is measured through activation of 79 Br and 89 Y with calibrated detectors. Temporal, spatial, and energy dependence of neutrons is measured with scintillators coupled to photomultiplier tubes (PMTs). Experimental setups and data analysis methods have been developed for these conditions. Finally, neutron yield, neutron energy anisotropy, and spatiotemporal evolution of the source have been measured.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Advances in detection for neutron reflectometry with time-resolved imaging detectors

Thermal neutron detection in neutron scattering science is a challenging endeavour due to a limited number of technologies which are sensitive to these weakly interacting particles. While many improvements to conventional detectors are underway at various facilities, there is a great opportunity to make a leap in performance by combining the spatial resolution benefits of imaging and the temporal resolution and background discrimination of event-driven radiation detectors. This idea has been realized by using a neutron sensitive scintillator read out by a single-photon sensitive camera based on a Timepix3 ASIC. We demonstrate how such data-driven imaging sensors can enable unprecedented performance in neutron reflectometry using the ASTERIX instrument at the Los Alamos Neutron Scattering Center. Several samples were measured with both the new and a conventional 3 He detector systems. The results from this work demonstrate that these imaging based systems can satisfy performance parameters for the future QIKR reflectometer to be built at the Second Target Station at Oak Ridge National Laboratory. Further improvements to the detector are already underway which will allow streamlined and expedited experiments. We demonstrate at least a two order of magnitude increase in detection rate at an acceptable dead time and introduce a new way of tuning the detector efficiency using light collecting optics to accommodate highly intense direct beams which cannot be measured with any current detectors without severe attenuation. This will allow measurements of complete reflectometry profiles and using a single sample measurement combined with fewer direct beam calibration measurements on QIKR and potentially other reflectometers.

36 MATERIALS SCIENCE↗

Portable and Adaptable Neutron Diagnostics for Advancing Fusion Energy Science Addendum

Activation detectors developed at LLNL for measuring real-time neutron fluence from fusion sources are used in the broader fusion community. The recommended fluence operating range of this diagnostic is 5x10 2 – 1x10 6 n/cm2. The upper limit on this fluence range is set by the dead time caused by data transfer between the detector and data acquisition computer. Delaying the start of counting is a possible strategy to operate these detectors in higher fluences.

42 ENGINEERING↗

Supporting Data for "On the magnetic contribution of itinerant electrons to neutron diffraction in the topological antiferromagnet CeAlGe"

Contents of this DOI are data for the research paper "On the magnetic contribution of itinerant electrons to neutron diffraction in the topological antiferromagnet CeAlGe" by the authors: V. Pomjakushin et al. The dataset contains raw data from neutron scattering experiments of CeAlGe powder performed at the CNCS spectrometer at Spallation Neutron Source at ORNL.

36 MATERIALS SCIENCE↗

MENUS—Materials engineering by neutron scattering

Materials engineering by neutron scattering (MENUS) at the second target station will be a transformational high-flux, versatile, multiscale materials engineering diffraction beamline with unprecedented new capabilities for the study of complex materials and structures. It will support both fundamental and applied materials research in a broad range of fields. MENUS will combine unprecedented long-wavelength neutron flux and unique detector coverage to enable real-time studies of complex structural and functional materials under external stimuli. The incorporated small angle neutron scattering and transmission/imaging capabilities will extend its sensitivity to larger length scales and higher spatial resolution. Multimodal MENUS will provide crystallographic and microstructure data to the materials science and engineering community to understand lattice strain/phase transition/microstructure/texture evolution in three orthogonal directions in complex material systems under combined extreme applied conditions. Finally, the capabilities of MENUS will open new scientific opportunities and meet the research needs for science challenges to enable studies of a range of phenomena and answer the key questions in material design/exploration, advanced material processing, transformative manufacturing, and material operations of national impacts in our daily life.

47 OTHER INSTRUMENTATION↗

Reactivation of the Transient Reactor Test (TREAT) Facility Neutron Radiography Program

Reactivation of the Transient Reactor Test (TREAT) Facility Neutron Radiography Program The Transient Reactor Test (TREAT) Facility is a 19,000 MW reactor located at the Idaho National Laboratory designed to perform transient testing on nuclear fuel experiments and materials. A neutron radiography facility was installed with the first radiograph being produced in 1967 that utilized the indirect (or transfer) method of neutron radiography to examine irradiated nuclear fuels and experiment test loops. The TREAT neutron radiography facility performed approximately 5,000 radiographs by the spring of 1977. The original radiography facility was upgraded in 1974-1975 to correct previous deficiencies and to improve capabilities. In 1986, an upgraded aperture was installed to increase the resolution of images followed by a major reactor upgrade completed in 1988. Overall, the existing neutron radiography system was in good working order. Originally built in 1958, the TREAT Facility was in operation until it was placed in a shutdown status in 1994. Following the Fukishima disaster and seeing a need for enhanced accident tolerant fuels, the United Stated Department of Energy decided to restart the TREAT facility and resume transient operations. In November 2017, the TREAT reactor was successfully restarted and is currently performing operational testing in preparation for initial experiment irradiations and transient testing. This paper reports on efforts to reactivate the TREAT neutron radiography station. A few minor shielding and system improvement upgrades have been completed along with the installation of a dedicated room for computed radiography equipment. Detailed beam characterization work was not performed following the last reactor upgrade. To characterize the neutron beam, gold foil activation measurements were made to determine an average neutron flux and flux profile. Additional multi-foil activation measurements will be made to calculate the energy spectrum. An open beam image will be taken that will provide the information about variations in the beam profile. A series of system qualification shots will also take place to accurately determine the effective image quality and image acquisition parameters. Full operational status of the TREAT neutron radiography system is scheduled for late summer of 2018.

36 MATERIALS SCIENCE↗

A neutron tomography study: probing the spontaneous crystallization of randomly packed granular assemblies

We study the spontaneous crystallization of an assembly of highly monodisperse steel spheres under shaking, as it evolves from localized icosahedral ordering towards a packing reaching crystalline ordering. Towards this end, real space neutron tomography measurements on the granular assembly are carried out, as it is systematically subjected to a variation of frequency and amplitude. As expected, we see a presence of localized icosahedral ordering in the disordered initial state (packing fraction ≈ 0.62). As the frequency is increased for both the shaking amplitudes (0.2 and 0.6 mm) studied here, there is a rise in packing fraction, accompanied by an evolution to crystallinity. The extent of crystallinity is found to depend on both the amplitude and frequency of shaking. We find that the icosahedral ordering remains localized and its extent does not grow significantly, while the crystalline ordering grows rapidly as an ordering transition point is approached. In the ordered state, crystalline clusters of both face centered cubic (FCC) and hexagonal close packed (HCP) types are identified, the latter of which grows from stacking faults. Our study shows that an earlier domination of FCC gives way to HCP ordering at higher shaking frequencies, suggesting that despite their coexistence, there is a subtle dynamical competition at play. This competition depends on both shaking amplitude and frequency, as our results as well as those of earlier theoretical simulations demonstrate. It is likely that this involves the very small free energy difference between the two structures.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Spectrostropy

ORNL researchers talk about their research in chemical spectroscopy.

36 MATERIALS SCIENCE↗

Comparison of graphite, aluminum, and TransHab shielding material characteristics in a high-energy neutron field

Space radiation transport models clearly show that low atomic weight materials provide a better shielding protection for interplanetary human missions than high atomic weight materials. These model studies have concentrated on shielding properties against charged particles. A light-weight, inflatable habitat module called TransHab was built and shown to provide adequate protection against micrometeoroid impacts and good shielding properties against charged particle radiation in the International Space Station orbits. An experiment using a tissue equivalent proportional counter, to study the changes in dose and lineal energy spectra with graphite, aluminum, and a TransHab build-up as shielding, was carried out at the Los Alamos Nuclear Science Center neutron facility. It is a continuation of a previous study using regolith and doped polyethylene materials. This paper describes the results and their comparison with the previous study. Published by Elsevier Science Ltd.

NASA Center JSC↗

Alterations in dose and lineal energy spectra under different shieldings in the Los Alamos high-energy neutron field

Nuclear interactions of space radiation with shielding materials result in alterations in dose and lineal energy spectra that depend on the specific elemental composition, density and thickness of the material. The shielding characteristics of materials have been studied using charged-particle beams and radiation transport models by examining the risk reduction using the conventional dose-equivalent approach. Secondary neutrons contribute a significant fraction of the total radiation exposure in space. An experiment to study the changes in dose and lineal energy spectra by shielding materials was carried out at the Los Alamos Nuclear Science Center neutron facility. In the energy range of about 2 to 200 MeV, this neutron spectrum is similar in shape within a factor of about 2 to the spectrum expected in the International Space Station habitable modules. It is shown that with a shielding thickness of about 5 g cm(-2), the conventional radiation risk increases, in some cases by as much as a factor of 2, but decreases with thicknesses of about of 20 g cm(-2). This suggests that care must be taken in evaluating the shielding effectiveness of a given material by including both the charged-particle and neutron components of space radiation.

NASA Discipline Radiation Health↗

Recent developments in plastic scintillators with pulse shape discrimination

The paper reports results of studies conducted to improve scintillation performance of plastic scintillators capable of neutron/gamma pulse-shape discrimination (PSD). Compositional modifications made with the polymer matrix improved physical stability, allowing for increased loads of the primary dye that, in combination with selected secondary dyes, provided enhanced PSD especially important for the lower energy ranges. Additional measurements were made with a newly-introduced PSD plastic EJ-276, that replaces the first commercially produced EJ-299. Comparative studies conducted with the new materials and EJ-309 liquids at large scale (up to 10 cm) show that current plastics may provide scintillation and PSD performance sufficient for the replacement of liquid scintillators. In conclusion, comparison to stilbene single crystals compliments the information about the status of the solid-state materials recently developed for fast neutron detection applications.

36 MATERIALS SCIENCE↗

Neutron irradiation effects on the mechanical properties of powder metallurgical processed tungsten alloys

Neutron irradiation effects on the tensile properties of Pure W, K-doped W, W–3%Re, and K-doped W–3%Re were examined under the US-Japan collaboration project PHENIX. The fission neutron irradiation experiments were carried out up to 0.74 dpa at 600 °C and 800 °C. Pure W (SR) showed irradiation hardening and loss of ductility after irradiation at 600 °C and 800 °C. K-doped W–3%Re (SR) also exhibited irradiation hardening but was ductile after irradiation. Characteristic points of the K-doped W–3%Re (SR) are small grain size and layered structure. Finally, the stress-relief treatment and the layered structure may improve the ductility of powder-metallurgy W alloys after neutron irradiation, so a combination of K-doping and Re addition would be beneficial to improve irradiation resistance.

36 MATERIALS SCIENCE↗