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At least 37 records · Page 2

Demonstration of low-level biogenic fuel content using quench curve and direct liquid scintillation counting (LSC) methods

In this work, an investigation into the direct method for liquid scintillation counting (LSC) quantification of biogenic fuel content in fuel blendstock is presented. This method development intentionally used a colored matrix (~99 wt%), fossil diesel fraction, and low-level biogenic fractions (~1 wt%) to determine the applicability of the LSC technique in colored blend mixtures. LSC procedures for quench correction, including the use of an instrument internal standard (Quantulus SQP values), color quench curves, and an internal 14 C standard spike on samples containing low-level amounts of biogenic gasoline, jet, and diesel mixed with fossil fuel, were compared. Samples were analyzed on both Perkin-Elmer Quantulus and Tri-Carb instruments, and the 14 C contents were compared with those determined by accelerator mass spectrometry (AMS). Results from the Tri-Carb instrument showed that percent differences of <10 % compared to AMS-reported values are achievable at 5-hour count times despite colored samples. A comparison between the impact of chemical and color quenching in the fuel samples showed that color quenching in highly colored samples reduces efficiency significantly more than chemical quenching, indicating that chemical quench curves are not appropriate for highly colored biofuel/fossil-fuel blended samples. Results indicate that both the direct method with internal spike quench correction and the use of a color-quench curve provide accurate results for 1 % biogenic fuel blends. Additionally, we have explored the use of Fourier transform infrared (FTIR) spectroscopy in measuring the biogenic content of the colored blended fuel samples. Preliminary results show the presence of biogenic carbon-derived fingerprints that are absent in fossil-derived sample. However, further work is needed to develop an FTIR-based quantitative method.

09 BIOMASS FUELS↗

Event-by-event direction reconstruction of solar neutrinos in a high light-yield liquid scintillator

The direction of individual B 8 solar neutrinos has been reconstructed using the SNO + liquid scintillator detector. Prompt, directional Cherenkov light was separated from the slower, isotropic scintillation light using time information, and a maximum likelihood method was used to reconstruct the direction of individual scattered electrons. A clear directional signal was observed, correlated with the solar angle. The observation was aided by a period of low primary fluor concentration that resulted in a slower scintillator decay time. This is the first time that event-by-event direction reconstruction in high light-yield liquid scintillator has been demonstrated in a large-scale detector. Published by the American Physical Society 2024

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Design, construction, and operation of a 1-ton Water-based Liquid scintillator detector at Brookhaven National Laboratory

Water-based liquid scintillators (WbLS) are a new class of detector materials that provide efficient and tunable detection of both Cherenkov and scintillation light. A massive WbLS neutrino detector with suitable photosensor coverage for low intensity light detection could therefore reconstruct the momentum of an energetic charged particle and also have enhanced low-energy sensitivity. These materials are also better suited for metal doping broadening the potential scientific utility. Here, we recently constructed and commissioned a 1-ton WbLS detector with good photosensor coverage and a capable data acquisition and calibration system. We intend to use this flexible detector system as a testbed for WbLS R&D. In this paper we give an overview of the 1-ton system and provide some early results.

47 OTHER INSTRUMENTATION↗

Low energy neutrino detection with a compact water-based liquid scintillator detector

In this study, the conceptual design and physics simulations of a near-field Water-based Liquid Scintillator (WbLS) detector placed 100 m from the Akkuyu Nuclear Power Plant (ANPP), currently under construction and aiming at being Turkey’s first nuclear power plant, is presented. The ANPP is an excellent opportunity for neutrino studies and the development of an R &D program for neutrino detectors in Turkey. The Reactor Neutrino Experiments of Turkey (RNET) program includes a compact detector with a 2.5-ton volume of WbLS and a ~ 30% photo-coverage, and the program is planned to be expanded with a medium-size 30-ton detector that will be an international testbed for WbLS and new detector technologies through low energy neutrino studies. In the following, the focus will be on the smaller ~2.5 ton detector, instrumented with 8-in. high quantum efficiency PMTs and two layers of cosmic veto paddles, covering all sides of the detector, to track and veto cosmic particles. Inverse Beta Decay (IBD) events from electron anti-neutrinos generated in the reactor core are simulated using the RAT-PAC simulation package and several liquids with different percentages of Liquid Scintillator (LS) and Gadolinium (Gd) are investigated.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

First measurement of the yield of 8 He isotopes produced in liquid scintillator by cosmic-ray muons at Daya Bay

Here, Daya Bay presents the first measurement of cosmogenic 8 He isotope production in liquid scintillator, using an innovative method for identifying cascade decays of 8 He and its child isotope, 8 Li. We also measure the production yield of 9 Li isotopes using well-established methodology. The results, in units of 10 –8 μ –1 ⁢g –1 cm 2 , are 0.307 ± 0.042, 0.341 ± 0.040, and 0.546 ± 0.076 for 8 He, and 6.73 ± 0.73, 6.75 ± 0.70, and 13.74 ± 0.82 for 9 Li at average muon energies of 63.9 GeV, 64.7 GeV, and 143.0 GeV, respectively. The measured production rate of 8 He isotopes is more than an order of magnitude lower than any other measurement of cosmogenic isotope production. It replaces the results of previous attempts to determine the ratio of 8 He to 9 Li production that yielded a wide range of limits from 0% to 30%. The results provide future liquid-scintillator-based experiments with improved ability to predict cosmogenic backgrounds.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Development of a bi-solvent liquid scintillator with slow light emission

One of the most promising approaches for the next generation of neutrino experiments is the realization of large hybrid Cherenkov/scintillation detectors made possible by recent innovations in photodetection technology and liquid scintillator chemistry. The development of a potentially suitable future detector liquid with particularly slow light emission is discussed in the present publication. This cocktail is compared with respect to its fundamental characteristics (scintillation efficiency, transparency, and time profile of light emission) with liquid scintillators currently used in large-scale neutrino detectors. In addition, the optimization of the admixture of wavelength shifters for a scintillator with particularly high light emission is presented. Furthermore, the pulse-shape discrimination capabilities of the novel medium was studied using a pulsed particle accelerator driven neutron source. Beyond that, purification methods based on column chromatography and fractional vacuum distillation for the co-solvent DIN (Diisopropylnaphthalene) are discussed.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

High-precision Measurement of the 16 O($n, n'γ$) Cross Section using $γ$-ray Detection in Liquid Scintillators with H 2 O and BeO Targets

The 16 O($n, n'γ$) reaction was measured at the Los Alamos Neutron Science Center white neutron source using γ-ray detection in liquid scintillators present in the upper hemisphere of the Correlated Gamma-Neutron Array for sCattering (CoGNAC). Separate measurements of this reaction were performed using H 2 O and BeO targets in successive years. The unique high energies of γ rays emitted from the 16 O($n, n'γ$) reaction facilitated a clean selection of this reaction from threshold to 9.8 MeV incident neutron energy without the need for precise measurements of the γ-ray energy or the scattered neutrons. The precise time resolution of the liquid scintillator detectors was then exploited to obtain high-resolution incident neutron energy measurements, and good agreement was obtained between the H 2 O and BeO results reported here. The dominant literature data sets for this reaction have systematic differences between them, but the present results improve upon the neutron energy resolution of earlier measurements and show important discrepancies in recent data. Finally, tentative data are also shown up to 20 MeV incident neutron energy but are potentially subject to improved understanding of the relative γ-ray and α decay branches from 16 O excited states.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Performance of a ton-scale water-based liquid scintillator detector

This study reports the performance and light yield of 1% concentration water-based liquid scintillator (WbLS) deployed in a 1000-liter detector. A light yield of 99± 15 photons per MeV is determined by comparing data with simulation. This result aligns with our previous light yield determination using smaller detectors, thus establishing a solid foundation for the ongoing development and deployment of WbLS in larger-scale detectors. In conclusion, the feasibility of in situ preparation and the stability of light yield in WbLS are demonstrated, reinforcing its suitability for long-term experimental endeavors.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Optimization of the JUNO liquid scintillator composition using a Daya Bay antineutrino detector

To maximize the light yield of the liquid scintillator (LS) for the Jiangmen Underground Neutrino Observatory (JUNO), a 20 t LS sample was produced in a pilot plant at Daya Bay. The optical properties of the new LS in various compositions were studied by replacing the gadolinium-loaded LS in one antineutrino detector. The concentrations of the fluor, PPO, and the wavelength shifter, bis-MSB, were increased in 12 steps from 0.5 g/L and 0.01 mg/L to 4 g/L and 13 mg/L, respectively. The numbers of total detected photoelectrons suggest that, with the optically purified solvent, the bis-MSB concentration does not need to be more than 4 mg/L. In order to bridge the one order of magnitude in the detector size difference between Daya Bay and JUNO, the Daya Bay data were used to tune the parameters of a newly developed optical model. Then, the model and tuned parameters were used in the JUNO simulation. Overall, this enabled to determine the optimal composition for the JUNO LS: purified solvent LAB with 2.5 g/L PPO, and 1 to 4 mg/L bis-MSB.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Radon emanation rate measurements using liquid scintillation counting

This article describes a radon emanation measurement technique using liquid scintillator counting. A model for radon loading and transport is described, along with its calibration. Detector background and blank have been studied and quantified. The Minimal detectable activity has been determined for the counting setup using a toy Monte Carlo simulation. Here, the measurement technique is validated using a butyl rubber sample previously used for cross-calibration between different radon counting facilities.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Results of low energy background measurements with the Liquid Scintillation Detector (LSD) of the Mont Blanc Laboratory

The 90 tons liquid scintillation detector (LSD) is fully running since October 1984, at a depth of 5,200 hg/sq cm of standard rock underground. The main goal is to search for neutrino bursts from collapsing stars. The experiment is very sensitive to detect low energy particles and has a very good signature to gamma-rays from (n,p) reaction which follows the upsilon e + p yields n + e sup + neutrino capture. The analysis of data is presented and the preliminary results on low energy measurements are discussed.

Aglietta, M.↗

Determination of the nat Ti(d,x) 49 V excitation function by liquid scintillation analysis

Here, the experimental cross-sections for deuteron-induced nuclear reactions on natural titanium were measured using the stacked-foil method. Deuteron beams were provided by a Pelletron tandem accelerator at incident energies up to 8 MeV. The cross-sections for the production of 49 V were determined by liquid scintillation analysis, with the highest measured value of 522(32) mb occurring at 5.59(9) MeV. Additionally, the cross-sections for the production of 44m,46,47,48 Sc and 48 V were evaluated using gamma-ray spectroscopy and compared to some available literature.

43 PARTICLE ACCELERATORS↗

Measurement of the light yield response of the Gd-compatible water-based liquid scintillator with the Brookhaven one-ton testbed

The water-based liquid scintillator (WbLS) enables hybrid detection by combining scintillation and Cherenkov signals, providing superior event reconstruction capabilities compared to conventional neutrino detectors. For this work, we measured the light yield of Gd-compatible WbLS at varying concentrations from 0.35% to 1% by mass, using cosmic-ray muons in a 1-ton scale detector at Brookhaven National Laboratory. The light yield is measured as (69.2 ± 6.9) ph/MeV at 0.35% concentration, which increased to (87.3 ± 8.7) ph/MeV at 1%. These results establish a quantitative basis for optimizing future WbLS-based detectors in neutrino physics.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Comparison of neutron spectra measured with three sizes of organic liquid scintillators using differentiation analysis

Proton recoil distributions were obtained by using organic liquid scintillators of different size. The measured distributions are converted to neutron spectra by differentiation analysis for comparison to the unfolded spectra of the largest scintillator. The approximations involved in the differentiation analysis are indicated to have small effects on the precision of neutron spectra measured with the smaller scintillators but introduce significant error for the largest scintillator. In the case of the smallest cylindrical scintillator, nominally 1.2 by 1.3 cm, the efficiency is shown to be insensitive to multiple scattering and to the angular distribution to the incident flux. These characteristics of the smaller scintillator make possible its use to measure scalar flux spectra within media high efficiency is not required.

Shook, D. F.↗

The research program of the Liquid Scintillation Detector (LSD) in the Mont Blanc Laboratory

A massive (90 tons) liquid scintillation detector (LSD) has been running since October 1984 in the Mont Blanc Laboratory at a depth of 5,200 hg/sq cm of standard rock. The research program of the experiment covers a variety of topics in particle physics and astrophysics. The performance of the detector, the main fields of research are presented and the preliminary results are discussed.

Dadykin, V. L.↗

Exploring solar neutrino oscillation parameters with the liquid scintillator counter at Yemilab with a comparison to JUNO

We investigate the sensitivities of the liquid scintillator counter (LSC) at Yemilab and JUNO to solar neutrino oscillation parameters, focusing on θ 12 and Δ m 21 2 . We compare the potential of JUNO with LSC at Yemilab utilizing both reactor and solar data in determining those parameters. We find that the solar neutrino data of LSC at Yemilab is highly sensitive to θ 12 enabling its determination with a higher precision compared to reactor experiments. Our study also reveals that if Δ m 21 2 is larger, with a value close to the best-fit value of KamLAND, JUNO reactor data will have about two times better precision than the reactor LSC at Yemilab. On the other hand, if Δ m 21 2 is smaller and closer to the best-fit value of solar neutrino experiments, the precision of the reactor LSC at Yemilab will be better than JUNO. Published by the American Physical Society 2024

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗