SEARCH · Engineering Papers
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.
Liquid scintillation counting technique is applied to the direct measurement of carbon-14 in carbon dioxide. This method has high counting efficiency and eliminates many of the basic problems encountered with previous techniques. The technique can be used to achieve a percent substitution reaction and is of interest as an analytical technique.
Next-generation large-scale neutrino detectors, from EOS, at the 1 t scale, to THEIA, at the 10 s-of-kt scale, will utilize differences in both the scintillation and Cherenkov light emission for different particle species to perform background rejection. This manuscript presents measurements of the scintillation light yield and emission time profile of water-based liquid scintillator samples in response to α radiation. These measurements are used as input to simulation models used to make predictions for future detectors. In particular, we present the timing-based particle identification achievable in generic water-based scintillator detectors at the 4 t, 1 kt, and 100 kt scales. We find that α/β discrimination improves with increasing scintillation concentration and we identify better than 80% α rejection for 90% β acceptance in 10% water-based liquid scintillator, at the 4 t scale.
Water Cherenkov and liquid scintillator detectors represent two complementary approaches in neutrino physics. Water Cherenkov detectors provide particle track direction and particle identification (PID) through Cherenkov ring topology, while liquid scintillator detectors offer higher light yield and lower energy thresholds. Water-based liquid scintillator (WbLS) is designed to combine the advantages of both technologies. However, the simultaneous detection of Cherenkov and scintillation light by photosensors introduces significant challenges for event reconstruction. This poster presents event reconstruction studies for WbLS detectors. A likelihood-based reconstruction framework, fiTQun, has been successfully used in Super-Kamiokande to reconstruct water Cherenkov events in cylindrical detectors. We extend and improve this framework to demonstrate event reconstruction in WbLS detectors, enabling the concurrent reconstruction of particle energy, PID, vertex, and direction. The results demonstrate competitive performance in energy resolution, PID separation, and vertex and direction reconstruction, highlighting the strong potential of WbLS for next-generation neutrino experiments.
Liquid scintillator neutron spectrometer using pulse shape discrimination and two parameter analyzer
Liquid scintillator neutron spectrometer using pulse shape discrimination and two parameter analyzer
Water-based liquid scintillator (WbLS) is a hybrid detector medium which has been proposed as a fill material for future large-volume rare event searches, including ν − detectors. This family of scintillating suspensions promises waterlike attenuation and scattering behavior, while offering scintillation light yield for sub-Cherenkov-threshold events. These features may allow for improved vertex and energy resolution, and concomitant improvements in background rejection and particle identification. While subscale measurements of light yield, timing and pulse-shape have been performed in several WbLS formulations, detailed measurements of the attenuation and scattering properties of WbLS remain a critical, unresolved step along the pathway to deployment. In pursuit of a better understanding of these parameters, a “long-arm” attenuation and scattering instrument has been developed at Lawrence Livermore National Laboratory, dubbed LASE (Livermore Attenuation and Scattering Experiment). Optical property measurements have been performed using LASE in DI water, Gd-water, WbLS and Gd-WbLS. Measurements of the optical properties of WbLS (1% LAB-PPO scintillator) provided by Brookhaven National Laboratory demonstrate an attenuation minimum of 4.87 × 10 − 4 ± 1.42 × 10 − 4 cm − 1 at 450 nm, while Gd-loaded WbLS (1% LAB-PPO scintillator, 0.1% Gd) demonstrated a minimum attenuation coefficient of 4.77 × 10 − 4 ± 1.27 × 10 − 4 cm − 1 at the same wavelength. Measurements of scattering in WbLS show a scattering coefficient of 3.39 × 10 − 4 ± 1.98 × 10 − 5 cm − 1 at the 450 nm attenuation minimum, while Gd-WbLS has a scattering coefficient of 2.8 × 10 − 4 ± 1.63 × 10 − 5 cm − 1 at that wavelength. These scattering and attenuation coefficients are significantly larger than measured for DI water at similar wavelengths ( 8.8 × 10 − 5 cm − 1 ± 3.8 × 10 − 5 attenuation at 430 nm, 2.2 × 10 − 5 ± 1.28 × 10 − 6 cm − 1 scattering). Though the WbLS attenuation and scattering coefficients measured are lower than the corresponding values published for ultrapure oils and LAB-PPO liquid scintillator, the material tested attenuates significantly more than water across the blue and green portions of the visible spectrum. This attenuation is markedly stronger at wavelengths under 430 nm. Published by the American Physical Society 2025
Abstract This manuscript describes measurements of water-based liquid scintillators (WbLS), demonstrating separation of the Cherenkov and scintillation components using a low energy $$\beta $$ β source and the fast timing response of a Large Area Picosecond Photodetector (LAPPD). Additionally, the time profiles of three WbLS mixtures, defined by the relative fractions of scintillating compound, are characterized, with improved sensitivity to the scintillator rise-time. The measurements were made using both an LAPPD and a conventional photomultiplier tube (PMT). All samples were measured with an effective resolution $$O\left( 100~\text {ps}\right) $$ O 100 ps , which allows for the separation of Cherenkov and scintillation light (henceforth C/S separation) by selecting on the arrival time of the photons alone. The Cherenkov purity of the selected photons is greater than 60% in all cases, with greater than 80% achieved for a sample containing 1% scintillator. This is the first demonstration of the power of synthesizing low light yield scintillators, of which WbLS is the canonical example, with fast photodetectors, of which LAPPDs are an emerging leader, and has direct implication for future mid- and large-scale detectors, such as Theia , ANNIE, and AIT-NEO.
Liquid scintillator is widely used in particle physics experiments due to its high light yield, good timing resolution, scalability and low cost. Certain liquid scintillators exhibit pulse shape discrimination capabilities because of difference in fluorescence timing properties induced by different particles. Its fluoresence timing properties have been measured mostly for radioactive decay sources at MeV energies. Here, we present a novel measurement of fluorescence time properties of Linear Alkyl Benzene (LAB) based liquid scintillator in response to high-energy ions of hydrogen (Z = 1), helium (Z = 2) and krypton at around 200–300 MeV/u for the first time. We compared the results to those from radioactive sources and observed a distinct dE / dX dependence, regardless of the particle type. These findings are essential for physics searches such as the diffuse supernova neutrino background in large liquid scintillator detectors like JUNO, and are also critical towards understanding the underlying scintillation timing mechanism.
Here, we present the characterization of a novel radiation detector based on an opaque water-based liquid scintillator. Opaque scintillators, also known as LiquidO, are made to be highly scattering, such that the scintillation light is effectively confined, and read out through wavelength-shifting fibers. The 1-liter, 32-channel prototype demonstrates the capability for both spectroscopy and topological reconstruction of point-like events. The design, construction, and evaluation of the detector are described, including modeling of the scintillation liquid optical properties and the detector’s response to gamma rays of several energies. A mean position reconstruction error of 4.4 mm for 1.6 MeV-equivalent events and 7.4 mm for 0.8 MeV-equivalent events is demonstrated using a simple reconstruction approach analogous to center-of-mass.
Abstract The proton light yield of liquid scintillators is an important property in the context of their use in large-scale neutrino experiments, with direct implications for neutrino-proton scattering measurements and the discrimination of fast neutrons from inverse $$\beta $$ β -decay coincidence signals. This work presents the first measurement of the proton light yield of a water-based liquid scintillator (WbLS) formulated from 5% linear alkyl benzene (LAB), at energies below 20 MeV, as well as a measurement of the proton light yield of a pure LAB + 2 g/L 2,5-diphenyloxazole (PPO) mixture (LABPPO). The measurements were performed using a double time-of-flight method and a pulsed neutron beam from the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. The proton light yields were measured relative to that of a 477 keV electron. The relative proton light yield of WbLS was approximately 3.8% lower than that of LABPPO, itself exhibiting a relative proton light yield 15–20% higher than previous measurements of an analogous anoxic sample. The observed quenching is not compatible with the Birks model for either material, but is well described with the addition of Chou’s bimolecular quenching term.
Intrinsic 40 K radioactive backgrounds from impurities of natural K in liquid scintillation cocktails have previously been demonstrated to limit their use in ultra-sensitive applications. Here, this work explores two methodologies in parallel for the reduction of 40 K backgrounds in the cocktails, and lays the groundwork for use in ultra-sensitive applications. In one method, alternative low-K liquid scintillation matrix constituents were identified and in the other, a simple purification method for single components and finished cocktails was developed. Both methods were verified via ICP-MS analysis. Liquid scintillation counting of selected purified cocktails demonstrated background reduction, improved stability, and enhanced performance. The best performing purified cocktail was also counted on a custom-built ultra-low background liquid scintillation counter, with results below the detector background.
The KamLAND-Zen 800 experiment is searching for the neutrinoless double-beta decay of 136 Xe by using 136 Xe-loaded liquid scintillator. The liquid scintillator is enclosed inside a balloon made of thin, transparent, low-radioactivity film that we call Inner Balloon (IB). The IB, apart from guaranteeing the liquid containment, also allows to minimize the background from cosmogenic muon-spallation products and 8B solar neutrinos. Indeed these events could contribute to the total counts in the region of interest around the Q-value of the double-beta decay of 136 Xe. In this paper, we present an overview of the IB and describe the various steps of its commissioning minimizing the radioactive contaminations, from the material selection, to the fabrication of the balloon and its installation inside the KamLAND detector. Finally, we show the impact of the IB on the KamLAND background as measured by the KamLAND detector itself.
Here, this paper describes preparation of 6 Li-loaded liquid scintillators by methods involving direct dissolution of 6Li salts in the commercial diisopropylnaphthalene (DIPN) solvent, without the formation of water-in-oil emulsions. Methods include incorporation of 6 Li that, unlike previously reported formulations, does not require additions of water or a strong acid such as hydrochloric acid (HCl). Results of the conducted experiments show that dissolution of aromatic and aliphatic 6 Li salts in DIPN can be easily achieved at 0.1%–0.3% by weight of atomic 6 Li, using small additions of waterless surfactants, or mild carboxylic acids. An alternative way suggests incorporation of 6 Li as a part of a surfactant molecule that can be dissolved in DIPN without any solubilizing additions. Proposed methods enable preparation of efficient 6 Li-loaded liquid scintillators that, at a large scale of 50 cm, exhibit good pulse shape discrimination (PSD) properties combined with up to 107% of light output and up to 115% of the attenuation length measured relative to standard undoped EJ-309 liquid scintillator.
In this work, an investigation into the direct method for liquid scintillation counting (LSC) quantification of biogenic fuel content in fuel blendstock is presented. This method development intentionally used a colored matrix (~99 wt%), fossil diesel fraction, and low-level biogenic fractions (~1 wt%) to determine the applicability of the LSC technique in colored blend mixtures. LSC procedures for quench correction, including the use of an instrument internal standard (Quantulus SQP values), color quench curves, and an internal 14 C standard spike on samples containing low-level amounts of biogenic gasoline, jet, and diesel mixed with fossil fuel, were compared. Samples were analyzed on both Perkin-Elmer Quantulus and Tri-Carb instruments, and the 14 C contents were compared with those determined by accelerator mass spectrometry (AMS). Results from the Tri-Carb instrument showed that percent differences of <10 % compared to AMS-reported values are achievable at 5-hour count times despite colored samples. A comparison between the impact of chemical and color quenching in the fuel samples showed that color quenching in highly colored samples reduces efficiency significantly more than chemical quenching, indicating that chemical quench curves are not appropriate for highly colored biofuel/fossil-fuel blended samples. Results indicate that both the direct method with internal spike quench correction and the use of a color-quench curve provide accurate results for 1 % biogenic fuel blends. Additionally, we have explored the use of Fourier transform infrared (FTIR) spectroscopy in measuring the biogenic content of the colored blended fuel samples. Preliminary results show the presence of biogenic carbon-derived fingerprints that are absent in fossil-derived sample. However, further work is needed to develop an FTIR-based quantitative method.
The direction of individual B 8 solar neutrinos has been reconstructed using the SNO + liquid scintillator detector. Prompt, directional Cherenkov light was separated from the slower, isotropic scintillation light using time information, and a maximum likelihood method was used to reconstruct the direction of individual scattered electrons. A clear directional signal was observed, correlated with the solar angle. The observation was aided by a period of low primary fluor concentration that resulted in a slower scintillator decay time. This is the first time that event-by-event direction reconstruction in high light-yield liquid scintillator has been demonstrated in a large-scale detector. Published by the American Physical Society 2024
Water-based liquid scintillators (WbLS) are a new class of detector materials that provide efficient and tunable detection of both Cherenkov and scintillation light. A massive WbLS neutrino detector with suitable photosensor coverage for low intensity light detection could therefore reconstruct the momentum of an energetic charged particle and also have enhanced low-energy sensitivity. These materials are also better suited for metal doping broadening the potential scientific utility. Here, we recently constructed and commissioned a 1-ton WbLS detector with good photosensor coverage and a capable data acquisition and calibration system. We intend to use this flexible detector system as a testbed for WbLS R&D. In this paper we give an overview of the 1-ton system and provide some early results.
In this study, the conceptual design and physics simulations of a near-field Water-based Liquid Scintillator (WbLS) detector placed 100 m from the Akkuyu Nuclear Power Plant (ANPP), currently under construction and aiming at being Turkey’s first nuclear power plant, is presented. The ANPP is an excellent opportunity for neutrino studies and the development of an R &D program for neutrino detectors in Turkey. The Reactor Neutrino Experiments of Turkey (RNET) program includes a compact detector with a 2.5-ton volume of WbLS and a ~ 30% photo-coverage, and the program is planned to be expanded with a medium-size 30-ton detector that will be an international testbed for WbLS and new detector technologies through low energy neutrino studies. In the following, the focus will be on the smaller ~2.5 ton detector, instrumented with 8-in. high quantum efficiency PMTs and two layers of cosmic veto paddles, covering all sides of the detector, to track and veto cosmic particles. Inverse Beta Decay (IBD) events from electron anti-neutrinos generated in the reactor core are simulated using the RAT-PAC simulation package and several liquids with different percentages of Liquid Scintillator (LS) and Gadolinium (Gd) are investigated.
Liquid scintillation counting method with sonic oscillations, noting decreased preparation time and increased counting efficiency