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At least 307 records · Page 17

Machine Learning in Safeguards at Pebble Bed Reactors

The goal of this project is to investigate and demonstrate the applicability of machine learning (ML) in safeguards at pebble bed reactors (PBRs). The detailed scope of work includes working with DOE-Nuclear Energy and other domain experts to examine current safeguards approaches at PBRs, defining ML tasks that can potentially strengthen the safeguards at PBRs, selecting ML task(s) for proof of concept based on safeguards needs and availability of testbeds and datasets, and developing ML algorithm(s) to demonstrate the feasibility of ML in PBR safeguards.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Integration of Online Cross-Section Generation Capability with Depletion and Transient Solvers in Griffin

Griffin is a Multiphysics Object-Oriented Simulation Environment (MOOSE)-based reactor multiphysics analysis application jointly developed by Argonne and Idaho National Laboratories under the DOENE Nuclear Energy Advanced Modeling and Simulation (NEAMS) program. In FY25, an online crosssection generation capability based on the Self-Shielding Application Programming Interface (SSAPI) was demonstrated for TRISO-fueled reactor problems under steady-state conditions. This fiscal year, that capability was extended to support depletion and transient multiphysics calculations, enabling high-fidelity analyses that generate self-shielded cross sections on the fly from the actual evolving composition and temperature states rather than from pre-tabulated libraries. For depletion, a two-way coupling was established in which SSAPI computes compact-averaged self-shielded cross sections that the depletion solver then uses to advance the Bateman equations, with the updated compositions returned to SSAPI at each step; the depletion module was refactored to support both library-based and SSAPI-based cross sections, and additional logic was added to track daughter isotopes and to exclude minor isotopes for efficiency. For transient analysis, the SSAPI multigroup library was extended with the kinetics data required for time-dependent calculations, the Improved Quasi-Static (IQS) scheme was coupled with SSAPI, and several supporting capabilities were implemented, including a self-shielding treatment that lets control rods and drums move within a self-shielded model, which had previously been impossible and had ruled out rod- and drum-movement transients with on-the-fly cross sections altogether, a new mixing scheme for delayed-neutron precursor decay constants, a checkpoint-based restart workflow, and performance improvements such as pointwise cross-section interpolation and the bypassing of unnecessary Dancoff factor calculations. The implemented capabilities were verified against Serpent Monte Carlo solutions. For depletion, a prismatic pin-cell problem based on a Next Generation Nuclear Plant (NGNP) Very High Temperature Reactor benchmark showed excellent agreement, with eigenvalue differences within 200 pcm over the entire burnup range (up to 140 MWD/kgU) and fission-product and actinide inventories agreeing to within 0.8% and 2.5%, respectively; a heat-pipe microreactor assembly problem with a much higher fuel loading confirmed the same behavior and quantified the bias introduced when the multigroup equivalence effect is neglected. For transient analysis, a pin-cell problem with a step reactivity insertion and temperature feedback reproduced the analytically expected asymptotic power and showed close agreement between the direct and IQS solutions, and a two-dimensional microreactor core problem with control-drum rotation exercised the new moving-drum self-shielding treatment and demonstrated successful coupling of the online crosssection generation with both the direct and IQS transient methods. The capability was further exercised on a full-core pebble-bed problem, in which Griffin was coupled with the System Analysis Module (SAM) to simulate load-following operation of the gPBR with the Doppler feedback resolved at the TRISO fuel kernel temperature. These developments in Griffin provide a convenient, high-fidelity approach to cross-section generation for advanced thermal reactors with geometrically complex and highly heterogeneous configurations, including TRISO-fueled prismatic and pebble-bed systems, and support steady-state, depletion, and transient multiphysics calculations. They also enable self-shielded cross sections to be evaluated directly at the actual coupled state of the system, thereby establishing a foundation for high-fidelity, fully coupled multiphysics analysis of advanced reactors

Park, H.↗

Demonstrating PyCalphad, ESPEI, and MSTDB-TC for MSR Applications

The utility of thermochemical modeling tools PyCalphad, ESPEI, and MSTDB-TC are demonstrated for applications relevant to molten salt reactor design, safety, and licensing. Given the availability of experimental data, the demonstration is predominantly focused on the use of MSTDB-TC v3.0 to model Li- and Be-bearing fluoride salt mixtures. Nonetheless, the methodology reported in using these tools for such applications can be applied to any salt system given requisite data availability.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Technoeconomic Design Optimization for Fast Reactors. Part I: Workflow Development and Case Study for Small LFR District Energy Application

The nuclear industry is developing small reactor designs that can target a variety of deployment locations and energy products. Smaller nuclear designs have traditionally struggled to handle the steep trade-offs between size and cost that have historically incentivized large reactors. This motivates computational optimization of small reactors to minimize costs and quantify the trade-off between size and cost. In this paper, the cost/size trade-off for a small fast reactor is derived using a multi-objective genetic algorithm optimization, with steady-state, transient, and cost analysis of the fast reactor being performed. Specifically, the method is demonstrated on a small 10- to 120-MW(thermal) U-Pu-Zr–fueled lead-cooled fast reactor with a 10-year core life for district energy applications, which can have a thermal load compatible with this range. The results reinforced that fast reactor cores at the lower end of this power range suffer cost penalties due to critical mass considerations. It was found that high power density cores with strong reactivity swings and many control rods were favored over designing to minimize reactivity swing. Furthermore, this contrasts with some traditional configurations designed using engineering judgment and demonstrates that optimizers can find nontraditional but realistic solutions, along with demonstrating the value of incorporating cost functions into whole-reactor design optimization.

Fast reactor↗

Demonstration of Monte Carlo Reference Equilibrium Core Solutions for Pebble Bed Reactors Using Shift in kugelpy

This report describes how to produce reference solutions for the equilibrium core search of pebble bed reactors using the pyrates Python library. The pyrates library uses the kugelpy methodology to perform running-in calculations to reach an equilibrium core. This approach relies on full-core Monte Carlo neutron transport calculations and the shifting of fuel pebble inventory through the reactor to simulate pebble movement in the core from one step to the next of a running-in scenario. In addition to the use of Serpent for the Monte Carlo neutron transport calculations, as part of this work, updates for the use of the Shift Monte Carlo code were integrated into the official pyrates GitHub repository. Comparisons of running-in simulations for a generic pebble bed reactor produced by using pyrates with Serpent and Shift are shown. Although consistent trends are shown between the use of the two Monte Carlo codes, the limiting factor in either calculation is the computation time due to the need to perform several hundred full-core neutron transport calculations before an equilibrium core is reached.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Demonstration of Monte Carlo Reference Equilibrium Core Solutions for Pebble Bed Reactors Using Shift in kugelpy

This report describes how to produce reference solutions for the equilibrium core search of pebble bed reactors using the pyrates Python library. The pyrates library uses the kugelpy methodology to perform running-in calculations to reach an equilibrium core. This approach relies on full-core Monte Carlo neutron transport calculations and the shifting of fuel pebble inventory through the reactor to simulate pebble movement in the core from one step to the next of a running-in scenario. In addition to the use of Serpent for the Monte Carlo neutron transport calculations, as part of this work, updates for the use of the Shift Monte Carlo code were integrated into the official pyrates GitHub repository. Comparisons of running-in simulations for a generic pebble bed reactor produced by using pyrates with Serpent and Shift are shown. Although consistent trends are shown between the use of the two Monte Carlo codes, the limiting factor in either calculation is the computation time due to the need to perform several hundred full-core neutron transport calculations before an equilibrium core is reached.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Demonstration of Pronghorn’s Subchannel Code Modeling of Liquid-Metal Reactors and Validation in Normal Operation Conditions and Blockage Scenarios

Pronghorn-SC is a subchannel code within the Multiphysics Object-Oriented Simulation Environment (MOOSE). Initially designed to simulate flows in water-cooled, square lattice, subchannel assemblies, Pronghorn-SC has been expanded to simulate liquid-metal-cooled flows in triangular lattices, hexagonal subchannel assemblies. For this purpose, the algorithm of Pronghorn-SC was adapted to solve the subchannel equations as they are applicable to a hexagonal wire-wrapped sodium-cooled fast reactor. Cheng–Todreas models for pressure drop and cross-flow models were adopted and a coolant heat conduction term was added. To solve these equations, an improved implicit algorithm was developed robust enough to deal with the numerical issues, associated with low flow and recirculation phenomena. To confirm the prediction capability of Pronghorn-SC, calculations and comparisons with available experimental data of 19- and 37-pin assemblies were performed, as well as other subchannel codes. Finally, a flow blockage modeling feature was added. This capability was validated for both water-cooled square sub-assemblies and sodium-cooled hexagonal sub-assemblies, using experimental data of partially and fully blocked cases.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Flowable Cementitious Grouts for False Bottoms in Hanford Waste Tanks – 26085

Cementitious grouts with epoxy coatings are being evaluated as an approach to refurbish the bottom of waste tanks at the Hanford Site. This work studies four grout concept materials for this application, two grouts being from commercial vendors and two grouts based off formulations used to close reactors and tanks at the Savannah River Site. All the candidate grouts demonstrate flowability and pumpability at the 0.5 cu ft scale. The commercial vendor products demonstrate the best flow and have lower water/premix ratio and are less likely to have bleed, which would impact epoxy bonding to the grout. The commercial products also demonstrate increased compression strengths compared to the reactor closure grouts. Additional fresh and cured properties for all the grout formulations were similar. The grouts in the tank waste simulant without epoxy coating do not crack but show visual changes to the grout and the surrounding simulant solution, and simulant absorption into the grout. The grout/epoxy bond in ambient conditions has strengths of over 7 MPa and needs to be evaluated for simulant chemical durability. Overall, the results to date justify testing the flowability, pumpability, and placement of the grouts at larger, engineering scale and for further studies of the interactions between the grout and epoxy.

Valdes, Nicholas [Savannah River National Laborato↗

In-Sodium Testing of a Prototype Thermoacoustic Power Sensor for Sodium-Cooled Fast Reactors

The ultimate goal of this project is to develop and demonstrate a thermoacoustic power sensor (TAPS) for Sodium-Cooled Fast Reactors (SFRs), with potential application also envisioned to other nuclear technologies such as Lead-Cooled Fast Reactors (LFRs), Molten Salt Reactors (MSRs), in addition to Light Water Reactors (LWRs). The project was led by Westinghouse Electric Company, LLC (Westinghouse) and carried out in collaboration with Argonne National Laboratory (ANL) and the University of Pittsburgh. A TAPS is a passive (self-powered), non-invasive (wireless) sensor envisioned for measuring key parameters, such as local temperature and neutron flux, in a nuclear reactor core. The sensor generates pressure waves (i.e., sound waves) with a frequency and amplitude dependent upon nuclear operating conditions (coolant temperature or power changes). The acoustic waves are able to travel through the core and associated structures, and reach to the sensor network placed outside and/or inside of the reactor vessel. These sensors require a very small amount of power which, during loss of power events, can be provided, for example, by harvesting gamma radiation energy, thus resulting in a monitoring system that can function both during normal operation and during loss of power events. Westinghouse and the University of Pittsburgh designed and fabricated TAPS prototypes for Argonne National Laboratory (ANL) to carry out in-sodium testing to evaluate the effects of sodium on the TAPS and the performance of the TAPS technique in sodium. Argonne received a TAPS prototype from Westinghouse, and the prototype was modified such that it can be installed into a test vessel and function in sodium at elevated temperature without potentially leaking. A water mockup test apparatus was constructed to validate proper working of the prototype. An instrumentation and control (I&C) system, running on the National Instruments (NI) LabView platform, was developed to: 1) operate both the water mockup test and the in-sodium test facility; and 2) process and analyze the received acoustic signals from an array of accelerometers and the Argonne sodium-submersible high-temperature acoustic sensor. The prototype was successfully tested in a water bath at different temperatures. Water mockup tests demonstrated that the TAPS prototype is working properly and its resonance frequency changes linearly with the coolant (water) temperature. A TAPS test apparatus was constructed and integrated with the upgraded Under-Sodium Viewing (USV) sodium test facility. The integrated USV-TAPS sodium test facility has been operational. The TAPS prototype and a high-temperature sodium-submersible acoustic sensor (SSAS) developed by Argonne were both installed inside the TAPS test vessel. Being operated within argon cover gas under ambient conditions, the TAPS prototype demonstrated that it was functioning properly with a resonance frequency at 1407.2 Hz, which was successfully detected by the accelerometers mounted on the external wall of the vessel and the high-temperature SSAS installed inside the vessel. After successfully transferring sodium into the vessel, in-sodium tests of the prototype were conducted. Tests of the TAPS prototype demonstrated that the resonance frequency of the TAPS changes linearly with respect to the temperature difference between the interior of the TAPS and bulk sodium. The early tests showed that the TAPS prototype could not establish a continuous and consistent resonance in sodium. The resonance diminished before the prototype reached its operating temperature. A signal postprocessor was added to the DAQ module latterly to isolate interferences, enhance signal conditioning, improve peak detection, and generate resonance frequency versus temperature plots. After testing in molten sodium and immersion at higher temperature for several weeks, the TAPS prototype was able to establish a continuous resonance. Performance evaluation of the TAPS prototype was then conducted in sodium. The tests included the investigation of 1) the effects of the temperature difference between the TAPS and bulk sodium, 2) the effects of sodium flowrate; and 3) the performance of the different sensor-receiver systems positioned inside or outside the vessel. Results of a test demonstrated that, with limited sodium circulation, a continuous and consistent resonance of the TAPS prototype was established occasionally. The tests also demonstrated that, because of the nature of detection principles and mounting methods, the high temperature SSAS is more affected by acoustic noise, while accelerometers are more affected by vibrations, in the test environment. It is unknown why the TAPS prototype only occasionally established a continuous and consistent resonance when the TAPS temperature reached its operating temperature in molten sodium, and why it ultimately failed to resonate at all. A failure modes assessment was conducted and a few potential causes of failure were identified. Different post in-sodium tests were conducted to obtain additional information potentially relevant to the cause of the failure. Nondestructive evaluation techniques are suggested to examine the internal integrity as well as the gas mixture of the prototype. If they prove inconclusive, the prototype should be cut open to conduct a thorough inspection of its internal integrity and determine the state of the gas mixture.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Coupled fuel performance calculations in VERA and demonstration on Watts Bar unit 1, cycle 1

As the core simulator capabilities in the Virtual Environment for Reactor Applications (VERA) have become more mature and stable, increased attention has been focused on coupling Bison to provide fuel performance simulations. This technique has been a very important driver for the pellet-clad interaction challenge problem being addressed by the Consortium for Advanced Simulation of Light Water Reactors (CASL). Here, two coupling approaches are demonstrated on quarter core problems based on Watts Bar Nuclear Plant Unit 1, Cycle 1: (1) an inline approach in which a one-way coupling is used between neutronics/thermal hydraulics (through MPACT/CTF) and fuel performance (through Bison) but no fuel temperature information is passed back to MPACT/CTF, and (2) a two-way approach (coupled) in which the fuel temperature is passed from Bison to MPACT/CTF. In both approaches, power and temperature distributions from MPACT/CTF are used to inform the Bison simulations for each rod in the core.The demonstrations presented here are the first integrated fuel performance simulations in VERA, which opens many possibilities for future work, including applications to accident-tolerant fuel efforts and transient simulations, which are of critical importance to CASL. These demonstrations also highlight the potential to move away from the current Bison-informed fuel temperature lookup table approach, which is the default in MPACT/CTF simulations, if performance improvements are made in the near future.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Catalytic Removal of Oxygen and Pollutants in Exhaust Gases from Pressurized Oxy-Combustors

The primary goal of this project was to develop and validate advanced catalytic materials and systems for purifying the flue gas generated from pressurized oxy-combustors in an effort to achieve the purity specifications of carbon dioxide (CO 2 ) streams required by the U.S. Department of Energy (USDOE) for application in enhanced oil recovery. The technology has shown great potential for improving energy efficiency, simplifying process complexity, and lowering costs compared with current state-of-the-art oxy-combustion flue gas purification technologies. Laboratory studies were conducted for the development, characterization, and screening of metal catalysts for residual oxygen (O 2 ) reduction with methane (CH 4 ) and multifunctional carbon catalysts for combined nitrogen oxides (NO x ), sulfur oxides (SO x ), and mercury (Hg) removal. A bench-scale reverse-flow fixed-bed (RFFB) reactor and a trickle-bed direct-contact cooler (DCC) reactor capable of treating 15 standard liters per min of pressurized oxy-combustion flue gas were fabricated and tested with both a simulated flue gas in the laboratory and a slipstream of actual flue gas at a 100 kW th Staged, Pressurized Oxy-Combustion (SPOC) pilot facility. Process simulation and techno-economic studies were performed to evaluate the energy efficiency and cost of the developed catalytic flue gas purification process integrated into a conceptual 550-MWe SPOC power plant. The goal and objectives of the project have been successfully accomplished. A cobalt-manganese (CoMn) oxide catalyst was developed and demonstrated in the bench-scale RFFB reactor in either a reverse-flow or one-direction flow mode of operation that met the success criterion of performance for residual O 2 reduction. A carbon catalyst was developed and demonstrated in the bench-scale DCC reactor that met the success criterion of performance for combined NO x /SO x /Hg removal. Slipstream testing of the integrated DCC-RFFB system at the SPOC pilot facility demonstrated stable operation and verified the superior performance obtained in the laboratory. The techno-economic analysis showed that a 550-MWe SPOC plant integrated with the catalytic flue gas purification process would result in costs of electricity of $\$$96.94/MWh and $\$$80.27/MWh in two assessed cases compared with $\$$91.07/MWh reported for the USDOE’s Current Technology Case, which generated only a partially pure CO 2 stream. On the basis of the results and findings from this project, scale-up studies of materials production and system demonstration and optimization studies of reactors and processes are recommended at the next stage of technology development.

20 FOSSIL-FUELED POWER PLANTS↗

Wireless Instrumented RB Experiment Preliminary Design and Analysis

The ability to deploy new nuclear fuels for current or future reactor concepts requires carefully designed experiments to generate data to support fuel qualification. Ideally these experiments would include state of-the-art sensing to maximize the amount of in situ data that can be collected during operation. Furthermore, advanced reactor systems can take advantage of integrated in-core sensing technologies to maximize fuel utilization, reduce unnecessary conservativism in design margins, and improve operator’s understanding of limiting peaking factors. Before any novel sensing technologies can be readily adopted for nuclear applications, they must first demonstrate acceptable performance in test reactors. This report summarizes the preliminary design and analysis of the most highly instrumented irradiation experiment ever performed in the removable beryllium (RB) positions of the High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory (ORNL). The Wireless Instrumented RB Experiment 2021 (WIRE-21) will test a wide range of sensors including wireless sensors being developed by Westinghouse Electric Company (WEC) that could provide in situ measurements of peak fuel temperatures and fuel rod pressurization due to fission gas release. The ability to wirelessly transmit a signal through the fuel rod’s cladding is critical to improving fuel monitoring capabilities without requiring signal penetrations through the cladding pressure boundary, which would significantly impact fuel fabrication, handling, and operation. Other sensors that will be tested in WIRE-21 include an array of thermocouples, self-powered neutron detectors (SPNDs), and spatially distributed fiber-optic temperature sensors. More generally, WIRE-21 will establish a flexible irradiation vehicle design to allow accelerated, economical testing of advanced sensor technologies while leveraging the extremely high neutron flux that is available in HFIR. This report summarizes the mechanical design for WIRE-21, the experimental test matrix, initial neutronic and thermal design analyses, and the active monitoring and control system enhancements necessary to support testing of advanced sensor technologies. The containment for WIRE-21 is similar to previous RB irradiation vehicles but includes a few modifications, most notably the use of integrated compression seals to pass a larger number of sensor leads through the experiment’s pressure boundary. In addition to the sensor leads, inert gas lines are passed into the experiment to enable active temperature control and the ability to pneumatically actuate a bellows-driven pressure sensor. WIRE-21 is targeting temperatures (300–350°C) and neutron fluence levels (~10 22 n/cm 2 ) relevant to light water reactors (LWRs), but the flexible design of the experiment vehicle allows much higher operating temperatures (>1,100°C). Neutronic calculations determine the neutron flux conditions as well as the nuclear heating within the experiments. These results are used as inputs to detailed thermal finite element calculations, which are required to evaluate the complex, three-dimensional heat transfer that occurs within WEC’s wireless sensor enclosures. Initial results show that the temperatures of the sensors’ enclosures and the metal bellows can be operated near the temperature range of LWR coolants and cladding while simultaneously increasing the temperature of a surrogate fuel material to values in the range of 800–1200°C to simulate centerline fuel temperatures during LWR operation.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Development of a Subchannel Capability for Liquid-Metal Fast Reactors in Pronghorn

This report details the development and demonstration of an entirely new capability in Pronghorn, namely the ability to model liquid-metal fast reactor (LMFR) flow conditions on the engineering scale. We developed two modeling approaches for LMFR that can be used separately or be combined into a hybrid simulation: (1) a modern subchannel capability called Pronghorn-Subchannel for square and hexagonal lattices, and (2) a porous flow capability for LMFR geometries. The report emphasizes the novel aspects of the developed subchannel capability and the interoperability of the subchannel capability, porous flow capability, and multiphysics tools within the multiphysics object oriented simulation environment (MOOSE). Here we demonstrate the ability to: (1) Accurately model subchannel flow in hexagonal lattices; (2) Couple the subchannel flow model to multidimensional finite-element method (FEM) or finite-volume method (FVM) heat conduction models; (3) Model LMFRs using Pronghorn’s porous media FVM approach; (4) Couple porous flow FVM and subchannel models in a single simulation; (5) Explicitly model inter-wrapper flows along with conjugate heat transfer from the intra-element flow; and (6) Demonstrate the numerical robustness of the subchannel algorithm by simulating intra-element flow recirculation in a high-buoyancy, low-flow fuel element.

97 MATHEMATICS AND COMPUTING↗

Advanced Materials and Manufacturing Technologies (AMMT) 2025 Roadmap

The mission of the Advanced Materials and Manufacturing Technologies (AMMT) program is to accelerate the development, qualification, demonstration, and deployment of advanced materials and manufacturing technologies in support of the United States (US) leadership in a broad range of nuclear energy applications. The vision of the AMMT program is the expansion of reliable and economical nuclear energy enabled by advanced materials and manufacturing technologies. Four major goals were set to realize the mission and vision of the AMMT program, including: (1) develop advanced materials and manufacturing technologies that have cross-reactor applications, (2) establish and demonstrate a rapid qualification framework that supports diverse materials and manufacturing technology needs, (3) evaluate materials performance in a range of nuclear environments, and (4) accelerate commercialization of new technologies through technology maturation. The program is designed to deliver solutions that support a wide range of reactor technologies.

36 MATERIALS SCIENCE↗

Screening and qualification methodology for SiC end plug processing methods

Deployment of SiC-ceramic-based fuel cladding for light water reactors requires a hermetic end plug–to–cladding joint that can withstand neutron irradiation during normal operation and maintain integrity during design-basis accidents. Reactor experiments have shown that some SiC composite tubes with SiC end plugs can retain hermeticity after irradiation. However, achieving consistent joint performance under irradiation remains a key challenge. Resolving this issue is essential to enable integral irradiation testing and to demonstrate fuel integrity under commercial-reactor irradiation conditions. This report aims to: (1) provide guidance for designing radiation-tolerant end plug joints for SiC cladding; (2) demonstrate experimental methods to detect processing defects that are unstable under neutron irradiation at light-water-reactor-relevant temperatures and doses; and (3) outline a step-by-step approach for designing and conducting reactor experiments to screen joining methods. The resulting data will be used to improve joint processing and to define critical defect types and sizes that must be detected and eliminated through non-destructive evaluation for quality assurance. Based on prior irradiation experiments at the High Flux Isotope Reactor, differential swelling among the cladding, bonding layer, and end plug was identified as an underlying mechanism for irradiation-induced joint degradation. Accordingly, this effect must be considered in the design of radiation-tolerant joining techniques. In this work, miniature SiC end plug joint specimens irradiated during the previous project were analyzed using X-ray computed tomography to characterize the joint microstructure. Digital volume correlation of the tomography data quantified radiation-induced microstructural changes and enabled evaluation of defect-related risks. Finally, ongoing neutron irradiation efforts using larger specimen volumes are presented. These efforts aim to statistically assess joint performance and to build a microstructure–performance (e.g., leak-tightness) dataset to inform processing improvements and quality control.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Subcritical Neutron and Gamma Noise Measurements at the Seven Percent Critical Experiment (7uPCX)

As part of a collaborative international effort organized by Lawrence Livermore National Laboratory (LLNL), with key participants from L’Institut de radioprotection et de sûreté nucléaire (IRSN), Los Alamos National Laboratory (LANL), and Sandia National Laboratories (SNL), a series of high-multiplication subcritical neutron and gamma noise measurements were planned and executed. The primary aim of this research was to advance detector technology, assess the validity of gamma noise for subcriticality measurements, and nuclear criticality safety, focusing on collecting list-mode or time-series data from various reactor configurations with multiplication values ranging from 20 to 310. This comprehensive dataset enabled a detailed comparative analysis of multiple detector systems and the results of both neutron and gamma noise measurements. In this work we focus on experimentally comparing the results from neutron and gamma noise measurements. We note good agreement between estimations of the prompt neutron decay constant and demonstrate the effects of changing reactor geometry on the efficiency of the differing methods.

Criticality↗

Experimental Investigation of Subcritical Neutron and Gamma Noise Methods at the Seven Percent Critical Experiment (7uPCX)

As part of a collaborative international effort organized by the Lawrence Livermore National Laboratory (LLNL), with key participants from the Institut de radioprotection et de sûreté nucléaire (IRSN), Los Alamos National Laboratory (LANL), and the Sandia National Laboratories (SNL), a series of high-multiplication subcritical neutron and gamma noise measurements was planned and executed. The primary aim of this article was to advance detector technology, assess the validity of gamma noise for subcriticality measurements, and nuclear criticality safety, focusing on collecting list-mode or time-series data from various reactor configurations with multiplication values ranging from 20 to 310. This comprehensive dataset enabled a detailed comparative analysis of multiple detector systems and the results of both neutron and gamma noise measurements. In this work, we focus on experimentally comparing the results from neutron and gamma noise measurements. We note good agreement between estimations of the prompt neutron decay constant and demonstrate the effects of changing reactor geometry on the efficiency of the differing methods. Our results agree well with independent experimental measurements and simulations performed by LLNL.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Real-Time Characterization of Salt Aerosols Generated from Static and Sparged Molten Salt

The formation of radionuclide-bearing aerosols in the respirable size range has the potential to significantly influence offsite dose consequences and is, therefore, an important consideration in nuclear facility safety assessments. Molten salt reactor (MSR) developers will likely need to demonstrate an understanding of the conditions under which radionuclide-bearing aerosols may be generated from their reactor under normal operating and accident conditions, as well as the characteristics and transport behavior of these aerosols, to demonstrate to the U.S. Nuclear Regulatory Commission (NRC) that the facility can be operated safely. Recent reviews of the literature identified a lack of experimental data describing the mechanisms of formation and properties (size, concentration, and composition) of salt aerosol particles that are produced from molten salts. Experiments that identify the conditions that lead to radionuclide-bearing salt aerosol releases and quantify the characteristics of salt aerosols formed by different mechanisms are high-priority needs to support MSR licensing. This report describes tests that were conducted within the Argonne Salt Aerosol Test Stand (a sealed vessel and measurement system) to generate salt aerosols from static and sparged molten salts and measure their size and concentration in real-time. The results provide insight into salt aerosol formation by the vapor condensation and bubble bursting mechanisms and inform the potential radiological consequences of aerosol formation from molten fuel salt. Videos of the salt surface were taken during salt sparge tests to observe surface bubble behavior. The data in this report can be used to develop mechanistic source term and accident progression models for MSRs. The real-time salt aerosol characterization technique used in this study will be employed in future integral effects tests that are conducted at an engineering scale to simulate realistic MSR accidents and in future separate effects tests to address additional variables that may impact salt aerosol characteristics (e.g., presence of fission products in salt and humidity in atmosphere).

22 GENERAL STUDIES OF NUCLEAR REACTORS↗