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At least 199 records · Page 11

Data Science and Computation for Rapid and Dynamic Compression Experiment Workflows at Experimental Facilities, September 8-11, 2020. Workshop Report

The application of high pressure to materials has enabled discoveries in scientific fields such as planetary science, materials science, and materials synthesis. Recent advances in X-ray user light sources and other facilities, co-location and integration of user facilities with high-pressure drivers, availability of high-performance computing (HPC) platforms, and the development of new data science techniques have created opportunities for, and challenges in, advancing data analytics for rapid and dynamic compression experiments. To address these challenges, harness the emerging technology now available, and expedite scientific discovery, Los Alamos National Laboratory (LANL) hosted a virtual workshop entitled “Data Science and Computation for Rapid and Dynamic Compression Workflows at Experimental Facilities” from September 8 to 11, 2020. The workshop included 95 registered scientists and analytics experts from 15 universities, 9 United States (US) national laboratories, 5 US and European X-ray light sources, neutron sources such as the Los Alamos Neutron Science Center (LANSCE), other big science facilities such as the National Ignition Facility (NIF), and an industry representative. The workshop included 31 invited talks and 4 lightning talks by students and postdocs.

36 MATERIALS SCIENCE↗

Reflectometry with Polarized Neutrons on In Situ Grown Thin Films

Originating from the demand for obtaining depth-resolved magnetization profiles from thin films and heterostructures, polarized neutron reflectometry (PNR) has developed into a unique research tool, which also finds application in the analysis of superconducting or soft matter thin films. While certain in situ sample environments such as gas-loading or humidity cells were quickly realized after PNR first emerged, preparing and growing thin magnetic films directly in the neutron beam could only be realized in recent years. Herein, a dedicated insight is given on the history and development of in situ thin film growth capabilities for PNR, from early pioneering experiments to the present day. The scientific and technological challenges as well as the advances of neutron sources, neutronics, and data treatment that have led to its realization are highlighted together with the unique research opportunities that it provides and recently obtained experimental results.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Neutron-Antineutron Transition Search at DUNE

Neutron-antineutron transition is a baryon number violating process with ΔB=2, providing a unique insight into potential explanations of the baryon asymmetry in our universe, especially in the context of post-sphaleron baryogenesis. Studies have been conducted across various neutron-rich environments, including free neutron sources, neutron stars, and bound neutrons in large underground neutrino detectors, among which large neutrino experiments have historically obtained the most stringent constraints. The forthcoming Deep Underground Neutrino Experiment (DUNE) will offer especially strong prospects for this search, enabled by the high spatial resolution of its liquid argon time projection chamber. This poster presents a recent study on neutron-antineutron transition at DUNE using machine-learning based event classification.

Yu, Kaiwen [UC, Irvine (main)]↗

Search for Neutron-Antineutron Transition in Large Neutrino Detectors

Neutron-antineutron transition is a baryon number violation process with $\Delta B=2$, providing a unique insight into the potential explanation of the baryon asymmetry in our university, especially in the context of post-sphaleron baryogenesis. Studies have been conducted in various neutron-rich environment including free neutron sources, neutron stars, and bound neutrons in large neutrino detectors, among which the large neutrino experiments obtained the most stringent constraints.

Wan, Linyan [Fermilab] (ORCID:0000000155246137)↗

Neutron stars as X-ray sources.

Neutron star structure and evolution from presupernovae stars including gravitational collapse and neutrino emission processes

GRAVITATIONAL COLLAPSE↗

A Moderator Test Station at ORNL

Oak Ridge National Laboratory (ORNL) hosts two world-leading slow neutron sources, the Spallation Neutron Source (SNS) and the High Flux Isotope Reactor (HFIR), and is currently developing the technical design for a Second Target Station (STS) for the SNS. Upon completion of the STS project, ORNL will be uniquely positioned to optimize each of its three neutron sources, the SNS First Target Station (FTS), the STS, and HFIR, in a complementary way. Among the essential aspects of a reimagined FTS and the current STS concept are high-brightness parahydrogen moderators—moderators which are optimized for high per-unit-area neutron brightness rather than integrated-across-large-area neutron intensity. The high-brightness moderators proposed for the STS will significantly outperform the coupled moderators currently on the FTS for appropriately optimized neutron beamlines, provided the moderating hydrogen is converted to near-equilibrium levels of parahydrogen (approximately 99.8% at 20 K). The original FTS moderators, by contrast, were conservatively designed to be relatively insensitive to the exact ortho:para ratio, with a consequent loss in performance. As a result, a redesign of the FTS moderators assuming fully converted parahydrogen could result in significant performance improvements on the FTS coupled moderators, and more consistent performance over time for all hydrogen moderators. This “parahydrogen problem” is a long-standing challenge for the effective implementation of hydrogen cold moderators at high-power neutron sources. In addition, the development of new moderator concepts, whether based on previously unused materials, structured heterogeneous arrays, or even simply on changes in overall shape and size is significantly restricted at a large-scale production facility intended to use the neutron beams so produced. Accordingly, moderators for production neutron sources are often designed in a very conservative, low-risk fashion, even though this compromises the absolute neutronic performance. Advanced moderator concepts worthy of study include features that could not be tested without redesigning and redeploying the entire existing reflector, shielding, and neutron beamline installation, making such development efforts far more expensive than building a stand-alone test facility. We propose a Moderator Test Station (MTS) at the SNS with which we will verify such performance gains and test new moderator concepts. These concepts include both high-brightness and large-volume parahydrogen moderators, as well as moderators with tailored ortho:para hydrogen levels, heterogeneous moderator concepts such as the convoluted moderator or pelletized moderators, and moderators made of materials like ammonia, ethane, and oxygen clathrates, which have not been widely tested let alone deployed at neutron source facilities.

42 ENGINEERING↗

The ORNL Moderator Test Station Science Case

Oak Ridge National Laboratory (ORNL) hosts two world-leading slow neutron sources, the Spallation Neutron Source (SNS) and the High Flux Isotope Reactor (HFIR), and is currently developing the technical design for a Second Target Station (STS) for the SNS. Upon completion of the STS project, ORNL will be uniquely positioned to optimize each of its three neutron sources, the SNS First Target Station (FTS), the STS, and HFIR, in a complementary way. Among the essential aspects of a re-imagined FTS and the current STS design are high-brightness parahydrogen moderators—moderators which are optimized for high per-unit-area neutron brightness rather than integrated-across-large-area neutron intensity. The high-brightness moderators proposed for the STS will, for the brightness metric, significantly outperform the coupled moderators currently on the FTS for appropriately optimized neutron beamlines, provided the moderating hydrogen is converted to near-equilibrium levels of parahydrogen (approximately 99.8% at 20 K). The original FTS moderators, by contrast, were conservatively designed to be relatively insensitive to the exact ortho:para ratio, with a consequent loss in performance. As a result, a redesign of the FTS moderators assuming fully converted parahydrogen could result in significant performance improvements on the FTS coupled moderators, and more consistent performance over time for all hydrogen moderators. This “parahydrogen problem” is a long-standing challenge for the effective implementation of hydrogen cold moderators at high-power neutron sources. In addition, the development of new moderator concepts, whether based on previously unused materials, structured heterogeneous arrays, or even simply on changes in overall shape and size is significantly restricted at a large-scale production facility intended to use the resulting neutron beams. Accordingly, moderators for production neutron sources are often designed in a very conservative, low-risk fashion, even though this compromises the absolute neutronic performance. Advanced moderator concepts worthy of study include features that could not be tested without redesigning and redeploying the entire existing reflector, shielding, and neutron beamline installation, making such development efforts far more expensive than building a stand-alone test facility.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Feasibility study of a compact neutron resonance transmission analysis instrument

Neutron Resonance Transmission Analysis (NRTA) uses resonant absorption of neutrons to infer the absolute isotopic composition of a target object, enabling applications in a broad range of fields such as archaeology, enrichment analysis of nuclear fuel, and arms control treaty verification. In the past, NRTA involved large user facilities and complex detector systems. However, recent advances in the intensity of compact neutron sources have made compact neutron imaging designs increasingly feasible. This work describes the Monte Carlo (MC) based design of a compact epithermal NRTA radiographic instrument which uses a moderated, compact deuterium-tritium (DT) neutron source and an epithermal neutron detector. Such an instrument would have a wide range of applications, and would be especially impactful for such scenarios as nuclear inspection and arms control verification exercises, where system complexity and mobility may be of critical importance. The MC simulations presented in this work demonstrate accurate time-of-flight (TOF) reconstructions for transmitted neutron energies, capable of differentiating isotopic compositions of nuclear material with high levels of accuracy. A new generation of miniaturized and increasingly more intense neutron sources will allow this technique to achieve measurements with greater precision and speed, with significant impact on a variety of engineering and societal problems.

47 OTHER INSTRUMENTATION↗

High deuteron and neutron yields from the interaction of a petawatt laser with a cryogenic deuterium jet

A compact high-flux, short-pulse neutron source would have applications from nuclear astrophysics to cancer therapy. Laser-driven neutron sources can achieve fluxes much higher than spallation and reactor neutron sources by reducing the volume and time in which the neutron-producing reactions occur by orders of magnitude. We report progress towards an efficient laser-driven neutron source in experiments with a cryogenic deuterium jet on the Texas Petawatt laser. Neutrons were produced both by laser-accelerated multi-MeV deuterons colliding with Be and mixed metallic catchers and by d (d,n) 3 He fusion reactions within the jet. We observed deuteron yields of 10 13 /shot in quasi-Maxwellian distributions carrying ~8-10% of the input laser energy. We obtained neutron yields greater than 10 10 /shot and found indications of a deuteron-deuteron fusion neutron source with high peak flux (>10 22 cm -2 s -1 ). The estimated fusion neutron yield in our experiment is one order of magnitude higher than any previous laser-induced dd fusion reaction. Though many technical challenges will have to be overcome to convert this proof-of-principle experiment into a consistent ultra-high flux neutron source, the neutron fluxes achieved here suggest laser-driven neutron sources can support laboratory study of the rapid neutron-capture process, which is otherwise thought to occur only in astrophysical sites such as core-collapse supernova, and binary neutron star mergers.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Differential neutron spectrum generator and related methods and systems

A neutron spectrum generator is disclosed herein including a neutron source, a scatterer positioned in a direct path between the neutron source and a neutron detector, and a material shell configured to have at least one non-uniform characteristic selected from the group consisting of a material, a thickness, a length, an angle, a layer, and combinations thereof to generate a specific spectrum at the neutron detector that is different than the spectrum of the neutron source. A related method includes measuring a first response generated by a first material shell of a neutron spectrum generator interacting with a neutron source, replacing the first material shell with a second material shell, measuring a second response generated by a second material shell of a neutron spectrum generator interacting with the neutron source, and determining a total fission response by determining a difference between the first response and the second response.

Scates, Wade↗

Cosmogenic neutron-capture-produced nuclides in stony meteorites

The complete neutron-flux results and production rates for Cl-36, Ni-59, and Co-60 in stony meteorites of various radii and composition are presented. The relative neutron source strengths and neutron production-versus-depth profiles were determined by using calculated H-3 production rates. The absolute source strengths were normalized to that determined for the moon by Woolum et al. (1975). The energy spectrum of the source neutrons and the neutron transport calculations, which employed the ANISN computer code, were similar to those used for the moon by Lingenfelter et al. (1972). The production rates of the three radionuclides were determined as a function of depth in various spherical meteoroids from the calculated equilibrium neutron-flux distributions and from energy-dependent neutron-capture cross sections. Rates for producing these radionuclides by spallation reactions were also calculated.

Spergel, M. S.↗

AWCC Simulations

Neutron well counters provide a means to measure fissile mass by detecting coincident neutrons, which is a unique signature to fission. For coincidence counting, mass is determined using a calibration curve established with items that have the same material characteristics. Multiplicity analysis solves the point model equations for mass using known detector parameters. In both cases, mass measurements may exhibit a bias due to item characteristics and should be corrected for. Experiments can be done to estimate bias and material effects, but they require having both the well counter and the material well defined. In pursuit of estimating measurement bias and uncertainty in a High Efficiency Neutron Counter (HENC), an MCNP simulation was matched to measurements performed with an Active Well Coincidence Counter (AWCC) to de ne a neutron source term. The neutron source term will be used to predict measurement performance of similar material types in a HENC.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Time-gated fast neutron transmission radiography system and method

The present disclosure relates to a time-gated fast neutron transmission radiography system and method. The system makes use of a pulsed neutron source for producing neutrons in a plurality of directions, with at least a subplurality of the neutrons being directed at an object to be imaged. The system also includes a neutron detector system configured to time-gate the detection of neutrons emitted from the pulsed neutron source to within a time-gated window.

Schmidt, Andrea↗

Numerical Studies of the On-Line Reactivity Monitoring Techniques in Subcritical Systems: Revisit of the Area-Ratio Method, the Neutron Source-Modulation Method, and the Flux-to-Current Ratio Method

In the subcritical systems, the subcriticality level must be monitored continuously to ensure the safe operation of the systems. Techniques such as the neutron source-modulation method and the flux-to-current ratio method have been proposed for on-line reactivity measurements of the subcritical systems. However, the accuracy of these methods is unknown in the actual applications. In this report, the fundamental concepts of these techniques are visited, with numerical simulation techniques developed to validate these on-line reactivity monitoring methodologies. Specifically, the Monte Carlo numerical simulation results show that the neutron source-modulation method is not accurate in determining the reactivity of the subcritical systems. The flux-to-current ratio method can provide on-line reactivity measurements, and its spatial effects have been studied and well understood through the numerical simulations of the fuel loading of the neutron source facility of Ukraine. In addition, a modified version of the area-ratio method is proposed for the on-line measurements of the absolute reactivity of the subcritical systems. Monte Carlo numerical simulations showed that this method can provide the absolute reactivity of the subcritical systems within ~5% error, if the neutron detectors are placed close to the fuel assembly interface with the reflector zone or in the reflector zones away from the neutron source.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Background and Lunar Neutron Populations Detected by LEND and Average Concentration of Near-Surface Hydrogen near the Moon's Poles

Neutron flux measurements by the Lunar Exploration Neutron Detector (LEND) on the Lunar Reconnaissance Orbiter (LRO) enable quantifying hydrogen-bearing volatiles in the lunar surface from orbit. Accurately determining hydrogen abundance requires discriminating between the instrument background detection rate and the population of lunar-sourced neutrons that are sensitive to surficial hydrogen. We have investigated the detection rate for lunar and non-lunar (spacecraft-sourced) neutrons in LEND by modeling maps of measured count rate in three LEND detector systems using linear combinations of maps compiled from LEND detectors and from the Lunar Prospector Neutron Spectrometer. We find that 30% of the global-average 24.926 +/- 0.020 neutron counts per second (cps) detected by the LEND STN3 thermal-energy neutron sensor are lunar-sourced neutrons in the thermal energy range (E < 0.4 eV), 65% are lunar-sourced neutrons in the epithermal and fast energy range (E > 0.4 eV), and 5% are from spacecraft-sourced background signal. In the SETN epithermal neutron detector, 90% of the 10.622 +/- 0.002 neutron detections per second are consistent with a lunar source of epithermal and fast neutrons combined (E > 0.4 eV), with 3% due to lunar-sourced thermal neutron leakage into the detector (E < 0.4 eV), and background signal accounting for 7% of total detections. Background signal due to spacecraft-derived neutrons is substantial in the CSETN collimated detector system, accounting for 57% of the global average detection rate of 5.082 +/- 0.001 cps, greater than the 48% estimated from cruise-phase data. Lunar-sourced epithermal and fast neutrons account for 43% of detected neutrons, including neutrons in collimation as well as neutrons that penetrate the collimator wall to reach the detector. We estimate a lower limit of 17% of lunar-sourced neutrons detected by CSETN are epithermal neutrons in collimation (0.37 cps), with an upper limit estimate of 54 +/- 11% of lunar-sourced neutrons received in collimation, or 1.2 +/- 0.2 cps global average. The pole-to-equator contrast ratio in epithermal and high-energy epithermal neutron flux indicates that the average concentration of hydrogen in the polar regolith above 80deg north or south latitude is ∼105 ppmw (parts per million by weight), or 0.095 +/- 0.01 wt% water-equivalent hydrogen. Above 88deg north or south, the concentration increases to ∼140 ppmw, or 0.13 +/- 0.02 wt% water-equivalent hydrogen. The similar pattern of neutron flux suppression at both poles suggests that hydrogen concentration generally increases nearer the pole and is not closely associated with a specific feature such as Shackleton Crater at the lunar south pole that has no northern counterpart. Epithermal neutron flux decreases with increasing latitude outside the polar regions, consistent with surface hydration that increases with latitude if that hydration extends to ∼13-40 cm into the surface.

T A Livengood↗