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Turco, R. P.

Publications and source records attributed to Turco, R. P..

At least 37 records · Page 2

Climate and smoke - An appraisal of nuclear winter

A reevaluation is presented of the 'nuclear winter' scenario of Turco et al. (1983). New pertinent data have emerged from laboratory studies, field experiments, and numerical models on the smoke-plume, mesoscale, and global scales. A full-scale nuclear exchange's probable soot injections lead, in three-dimensional climate simulations, to midsummer land temperature decreases averaging 10-20 C in northern midlatitudes, with local cooling of as much as 35 C. Anomalous circulation patterns due to solar heating of the soot could stabilize the upper atmosphere against overturning, thereby prolonging the soot's residence time in the atmosphere. Monsoon disruptions and severe ozone layer depletion are also foreseen.

Turco, R. P.

Physical processes in polar stratospheric ice clouds

The formulation and evolution of polar stratospheric ice clouds are simulated using a one-dimensional model of cloud microphysics. It is found that the optical thickness and particle size of ice clouds depend on the cooling rate of the air in which the cloud formed. It is necessary that there be an energy barrier to ice nucleation upon the preexisting aerosols in order to account for the cooling rate dependence of the cloud properties.

Toon, Owen B.

Theory and observations: Model simulations of the period 1955-1985

The main objective of the theoretical studies presented here is to apply models of stratospheric chemistry and transport in order to understand the processes that control stratospheric ozone and that are responsible for the observed variations. The model calculations are intended to simulate the observed behavior of atmospheric ozone over the past three decades (1955-1985), for which there exists a substantial record of both ground-based and, more recently, satellite measurements. Ozone concentrations in the atmosphere vary on different time scales and for several different causes. The models described here were designed to simulate the effect on ozone of changes in the concentration of such trace gases as CFC, CH4, N2O, and CO2. Changes from year to year in ultraviolet radiation associated with the solar cycle are also included in the models. A third source of variability explicitly considered is the sporadic introduction of large amounts of NO sub x into the stratosphere during atmospheric nuclear tests.

Isaksen, Ivar S. A.

Trends in aerosol abundances and distributions

The properties of aerosols that reside in the upper atmosphere are described. Special emphasis is given to the influence these aerosols have on ozone observation systems, mainly through radiative effects, and on ambient ozone concentrations, mainly through chemical effects. It has long been appreciated that stratospheric particles can interfere with the remote sensing of ozone distribution. The mechanism and magnitude of this interference are evaluated. Separate sections deal with the optical properties of upper atmospheric aerosols, long-term trends in stratospheric aerosols, perturbations of the stratospheric aerosol layer by volcanic eruptions, and estimates of the impacts that such particles have on remotely measured ozone concentrations. Another section is devoted to a discussion of the polar stratospheric clouds (PSC's). These unique clouds, recently discovered by satellite observation, are now thought to be intimately connected with the Antarctic ozone hole. Accordingly, interest in PSC's has grown considerably in recent years. This chapter describes what we know about the morphology, physical chemistry, and microphysics of PSC's.

Turco, R. P.

On the growth of nitric and sulfuric acid aerosol particles under stratospheric conditions

A theory for the formation of frozen aerosol particles in the Antarctic stratosphere was developed and applied to the formation of polar stratospheric clouds. The theory suggests that the condensed ice particles are composed primarily of nitric acid and water, with small admixtures of sulfuric and hydrochloric acids in solid solution. The proposed particle formation mechanism is in agreement with the magnitude and seasonal behavior of the optical extinction observed in the winter polar stratosphere.

Hamill, Patrick

A multidimensional model for aerosols - Description of computational analogs

The numerical algorithms used to simulate the advection, diffusion, sedimentation, coagulation, and condensational growth of atmospheric aerosols are described. The model can be used in one, two, or three spatial dimensions. The continuity equation in a generalized horizontal and vertical coordinate system is developed, which allows the model to be quickly adapted to a wide variety of dynamical models of global or regional scale. Algorithms are developed to treat the various physical processes, and the results of simulations are presented, which show the strengths and weaknesses of these algorithms. Although the emphasis is on the modeling of aerosols, the work is also applicable to the simulations of the transport of gases.

Toon, O. B.

Heterogeneous physicochemistry of the winter polar stratosphere

Present chemical theories of the Antarctic ozone hole assume that heterogeneous reactions involving polar stratospheric clouds (PSCs) are the precursor of springtime ozone depletions. However, none of the theories quantify the rates of proposed heterogeneous processed, and none utilize the extensive data base on PSC's. Thus, all of the theories must be considered incomplete until the heterogeneous mechanisms are properly defined. A unified treatment developed of the cloud related processes, both physical and chemical, and the importance of these processes using observation data is calibrated. The rates are compared competitive heterogeneous processes to place reasonable limits on critical mechanisms such as the denitrification and dechlorination of the polar winter stratosphere. Among the subjects addressed here are the physical/chemical properties of PSC's including their relevant microphysical, optical and compositional characteristics, mass transfer rates of gaseous constituents to cloud particles, adsorption, accommodation and sticking coefficients on cloud particles, time constants for condensation, absorption and other microphysical processes, effects of solubility and vapor pressure on cloud composition, the statistics of cloud processing of chemically active condensible species, rate limiting steps in heterogeneous chemical reactions, and the nonlinear dependence of ozone loss on physical and chemical parameters.

Turco, R. P.

The ozone hole - The role of polar stratospheric cloud particles

The role of polar stratospheric clouds in the formation of the Antarctic ozone hole is considered. Several researchers have suggested that the decrease in ozone over Antarctica is related to the polar stratospheric clouds (PSCs) which had been observed in the antarctic winter stratosphere. Some of the pertinent characteristics of polar stratospheric clouds are discussed, and it is shown how these clouds may participate in the ozone destruction process. The satellite data for PSCs is analyzed, and statistical information regarding the number and maximum extinctions of these clouds is presented. Evidence that the polar stratospheric clouds are composed of frozen nitric acid is considered. It is suggested that the evaporation of the clouds, in late August and September, will release HOCl and HNO3 to the environment. This could be followed by the photodissociation of HOCl to OH and Cl, which would very effectively destroy ozone. However, the ozone destruction mechanism could be halted when enough of the evaporated nitric acid is photolized.

Hamill, Patrick

Characteristics of polar stratospheric clouds during the formation of the Antarctic ozone hole

Measured properties of Antarctic polar stratospheric clouds are described, and the possible relationship between the clouds and the formation of the ozone hole is considered. It is shown that the ozone hole develops and the clouds dissipate in the same place and at the same time. There may be a causal relationship between cloud particle evaporation and ozone depletion. A heterogeneous mechanism involving chemical reactions in the cloud droplets is suggested.

Hamill, Patrick

Ozone, dust, smoke and humidity in nuclear winter

Recent correspondence on nuclear winter is commented on. Reasons are given for why the Tunguska meteor explosion may not be useful in calibrating the effects of a major nuclear exchange. The relationship between the optical depth of an aerosol cloud, the composition of the cloud, and its effect on sunlight intensity and climate are clarified. The significance of the Tambora eruption of 1815 and of historical fires for the nuclear winter theory are briefly discussed. The dispersion of smoke plumes from large fires is addressed, and water condensation and smoke scavenging are considered.

Turco, R. P.

The climatic effects of nuclear war

The effects of various US-USSR nuclear-exchange scenarios on global climate are investigated by means of computer simulations, summarizing the results of Turco et al. (1983) and follow-up studies using 3D global-circulation models. A nuclear-scenario model is used to determine the amounts of dust, smoke, radioactivity, and pyrotoxins generated by a particular type of nuclear exchange (such as a general 5,000-Mt exchange, a 1,000-Mt limited exchange, a 5,000-Mt hard-target counterforce attack, and a 100-Mt attack on cities only): a particle-microphysics model predicts the evolution of the dust and smoke particles; and a radiative-convective climate model estimates the effects of the dust and smoke clouds on the global radiation budget. The findings are presented in graphs, diagrams, and a table. Thick clouds blocking most sunlight over the Northern Hemisphere midlatitudes for weeks or months and producing ground-temperature reductions of 20-40 C, disruption of global circulation patterns, and rapid spread of clouds to the Southern Hemisphere are among the 'nuclear-winter' effects predicted for the 5,000-Mt baseline case. The catastrophic consequences for plant, animal, and human populations are considered, and the revision of superpower nuclear strategies is urged.

Turco, R. P.

Nuclear winter - Global consequences of multiple nuclear explosions

The results of a computerized simulation of the potential global environmental effects of dust and smoke clouds that would be generated by a nuclear war are presented. Short term effects of blast, fire, and radiation are neglected in the series of physical models that include a nuclear war scenario, a particle microphysics model, and a radiative convective model. Account is taken of the altitude-dependent dust, smoke, radioactivity, and NO(x) injections, the temporal evolution of dust and smoke clouds, land and ocean environments, and temperature contrasts. A nuclear exchange would produce thousands of individual smoke and dust clouds rising up to 30 km altitude in the midlatitudes. The smoke, dust, and radioactive debris would cover the entire midlatitudes within 1-2 weeks. The smoke would arise from conflagrations of forests, suburbs, and urban areas. Obscuration of sunlight would induce subfreezing temperatures for several months, disruption of the global circulation patterns, and the arrival of a nuclear winter, followed and accompanied by radioactive fallout, pyrogenic air pollution, and UV-B flux enhancements. It is estimated that a total of only 100 Mtons would be sufficient to plunge the Northern Hemisphere summer to subfreezing temperatures lasting months. Since the probable exchange in a nuclear war would exceed 5000 Mtons, it is expected that many species, including humans, may not survive the war.

Turco, R. P.

A two-dimensional model simulation of the EL Chichon volcanic eruption cloud

Using a two-dimensional model of sulfate photochemistry, transport, and aerosol microphysics, a 2-year period following the eruptions of El Chichon have been simulated. Present calculations suggest that the residence time of the cloud in the stratosphere exceeds 2 years. The model reproduces the observed optical depth, lidar backscatter, and infrared extinction coefficients, if about 10 megatonnes of SO2 are injected. The major deficiency of the model is a somewhat too rapid transport.

Capone, L. A.

The 1980 eruptions of Mount St. Helens - Physical and chemical processes in the stratospheric clouds

The large and diverse set of observational data collected in the high-altitude plumes of the May 18, May 25, and June 13, 1980 eruptions is organized and analyzed with a view to discerning the processes at work. The data serve to guide and constrain detailed model simulations of the volcanic clouds. For this purpose, use is made of a comprehensive one-dimensional model of stratospheric sulfate aerosols, sulfur precursor gases, and volcanic ash and dust. The model takes into account gas-phase and condensed-phase (heterogeneous) chemistry in the clouds, aerosol nucleation and growth, and cloud expansion. Computational results are presented for the time histories of the gaseous species concentrations, aerosol size distributions, and ash burdens of the eruption clouds. Also investigated are the long-term buildup of stratospheric aerosols in the Northern Hemisphere and the persistent effects of injected chlorine and water vapor on stratospheric ozone. It is concluded that SO2, water vapor, and ash were probably the most important substances injected into the stratosphere by the Mount St. Helens volcano, both with respect to their widespread effects on composition and their effect on climate.

Turco, R. P.

Environmental effects of an impact-generated dust cloud - Implications for the Cretaceous-Tertiary extinctions

A model of the evolution and radiative effects of a debris cloud from a hypothesized impact event at the Cretaceous-Tertiary boundary suggests that the cloud could have reduced the amount of light at the earth's surface below that required for photosynthesis for several months and, for a somewhat shorter interval, even below that needed for many animals to see. For 6 months to 1 year, the surface would cool; the oceans could cool only a few degrees Celsius at most, but the continents might cool a maximum of 40 Kelvin. Extinctions in the ocean may have been caused primarily by the temporary cessation of photosynthesis, but those on land may have been primarily induced by a combination of lowered temperatures and reduced light.

Pollack, J. B.

Venus -Mesospheric hazes of ice, dust, and acid aerosols

Four distinct types of particles are suggested to be present in the upper atmosphere of Venus. The lowest and densest haze may consist of a submicron sulfuric acid aerosol which extends above the cloud tops, up to about 80 km, representing an extension of the upper cloud deck. Temperature structure measurements in the 70-120 km altitude range indicate the occasional appearance of two independent water ice layers, of which the lower may form between 80 and 100 km and is probably the detached haze layer noted in high contrast limb photography. A nucleation of this ice layer on sulfuric acid aerosols is hypothesized. Temperatures of the Venus mesopause, near 120 km altitude, are frequently cold enough to allow ice nucleation on meteoric dust or ambient ions, yielding a haze (analogous to noctilucent clouds on earth) which is expected to be tenuous to the point of optical invisibility.

Turco, R. P.

The clouds are hazes of Venus

Pioneer Venus and Venera probe data for the clouds of Venus are considered. These clouds consist of a main cloud deck at 45-70 km altitude, with thinner hazes above and below, although the microphysical properties of the main cloud are further subdivided into upper, middle and lower cloud levels. Much of the cloud exhibits a multimodal particle size distribution, with the mode most visible from the earth being H2SO4 droplets having 2-3 micron diameters. Despite variations, the vertical structure of the clouds indicates persistent features at sites separated by years and by great distances. The clouds are more strongly affected by radiation than by latent heat release, and the small particle size and weak convective activity observed are incompatible with lightning of cloud origin.

Esposito, L. W.

Noctilucent clouds - Simulation studies of their genesis, properties and global influences

A numerical model is presented for testing theories of the physical mechanisms of noctiluminescent clouds. The time-dependent, one-dimensional model describes the formation, evolution, and properties of the clouds as interactive ice crystals, meteoric dust, water vapor, and ionized air. Mesopause temperatures below 140 K are found to be necessary for the formation of the clouds, conditions existing only at high latitudes in the summer. No predominant nucleation particle could be identified for the formation of the clouds, although a time period of up to a day was determined as necessary for materialization, which lasts several days. Several atmospheric and environmental conditions were characterized which enhance the appearance of the noctiluminescent clouds. One conclusion reached is that the numerous launches necessary to build a solar power satellite system would not significantly exacerbate noctiluminescent cloud formation.

Turco, R. P.