Engineering topics

Clarke, Shaun D.

Publications and source records attributed to Clarke, Shaun D..

21 records · Page 2

DOE OSTI2021

New Experiments for Detecting Emissions from Fission

Ensuring that nuclear science and technology is used solely for peaceful purposes is one of the most pressing challenges facing our society. The Consortium for Monitoring, Technology, and Verification (MTV) mission is to help meet this challenge by providing advanced technology and trained talent for careers in nuclear security and nonproliferation. The study of nuclear fission is one area of interest in the MTV. We are performing new experiments for the characterization of neutron and gamma ray emissions from fission fragments. These emissions are signatures for the detection and characterization of nuclear materials. To perform these experiments, we have developed Fission Sphere (FS-3), an array of forty organic stilbene detectors operated in time-coincidence. The FS-3 is used to measure the prompt emissions of neutrons and gamma rays from Cf-252 spontaneous fission. These new data will be used to validate physics-based prediction codes, including CGMF and FREYA, and will be useful in future ENDF and ENSDF evaluations. This paper will present results from the first experiments using FS-3 and a Cf-252 spontaneous fission source. It will compare the experimental results with predictions from theory and Monte Carlo simulation. Specifically, we will describe the correlations among energy, multiplicity, and angles of emitted particles. We will also discuss the application of these correlations in multiplicity counting techniques, which are widely used in nuclear safeguards.

Pozzi, S. A.↗

DOE OSTI2021

Organic glass scintillator bars with dual-ended readout

Organic glass scintillator (OGS) bars (6 × 6 × 50 mm 3 ) were melt-cast and characterized with dual-ended readout by silicon photomultiplier arrays. The results were compared to trans-stilbene bars of the same size. Energy resolution was measured via a 137 Cs Compton-coincidence experiment. Time resolution was determined via a 22 Na coincidence-timing experiment. Depth-of-interaction resolution was measured by moving a gamma ray fan beam along the major axis of the bars. Pulse shape discrimination capability and neutron light output were determined via a time-of-flight measurement of a 252 Cf source. The OGS bars exhibited better energy resolution at 478 keV (10.3 ± 0.5% vs. 11.2 ± 0.5%), better time resolution from 200–341 keVee (270 ps vs. 340 ps FWHM), slightly poorer depth-of-interaction resolution, poorer PSD performance, and higher neutron light output than the stilbene bars. Here, the low cost, ease of manufacturing, brightness, and excellent time resolution make OGS a strong candidate for use in compact radiation imaging systems.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2021

On the Feynman-alpha method for reflected fissile assemblies

The Feynman-alpha method is a neutron noise technique that is used to estimate the prompt neutron period of fissile assemblies. The method and quantity are of widespread interest including in applications such as nuclear criticality safety, safeguards and nonproliferation, and stockpile stewardship; the prompt neutron period may also be used to infer the k eff multiplication factor. The Feynman-alpha method is predicated on time-correlated neutron detections that deviate from a Poisson random variable due to multiplication. Traditionally, such measurements are diagnosed with one-region point kinetics, but two-region models are required when the fissile assembly is reflected. This paper presents a derivation of the two-region point kinetics Feynman-alpha equations based on a double integration of the Rossi-alpha equations, develops novel propagation of measurement uncertainty, and validates the theory. Validation is achieved with organic scintillator measurements of weapons-grade plutonium reflected by various amounts of copper to achieve k eff values of 0.83–0.94 and prompt periods of 5–75 ns. The results demonstrate that Feynman-alpha measurements should use the two-region model instead of the one-region model. The simplified one-region model deviates from the validated two-region models by as much as 10% in the estimate of the prompt neutron period, and the two-region model reduces to the one-region model for small amounts of reflector. The Feynman-alpha estimates of the prompt neutron period are compared to those of the Rossi-alpha approach. The comparative results demonstrate that the Feynman-alpha method is more precise than the Rossi-alpha method and more accurate for k eff < 0.92, whereas the Rossi-alpha method is generally more accurate for higher multiplications. Here, the uncertainty propagation developed in this work should be used for all Feynman-alpha measurements and will therein improve fitting accuracy and appropriate precision estimates.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗