Advanced airborne DIAL system capabilities for ozone and multiwavelength aerosol measurements
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Carter, A. F.↗
Engineering topics
Browell, E. V.
Publications and source records attributed to Browell, E. V..
The Amazon Boundary Layer Experiment (ABLE 2A) - Dry season 1985
The Amazon Boundary Layer Experiment (ABLE 2A) used data from aircraft, ground-based, and satellite platforms to characterize the chemistry and dynamics of the lower atmosphere over the Amazon Basin during the early-to-middle dry season, July and August 1985. This paper reports the conceptual framework and experimental approach used in ABLE 2A and serves as an introduction to the detailed papers which follow in this issue. The results of ABLE 2A demonstrate that isoprene, methane, carbon dioxide, nitric oxide, dimethylsulfide, and organic aerosol emissions from soils and vegetation play a major role in determining the chemical composition of the atmospheric mixed layer over undisturbed forest and wetland environments. As the dry season progresses, emissions from both local and distant biomass burning become an important source of carbon monoxide, nitric oxide and ozone in the atmosphere over the central Amazon Basin.
Harriss, R. C.↗
Tropospheric ozone and aerosol distributions across the Amazon Basin
As a part of the NASA Global Tropospheric Experiment to study the Amazon boundary layer, ozone and aerosol distributions were made measured in July-August 1985 by a NASA Electra aircraft on several long-range flights spanning different areas between Tabatinga and Belem, Brazil. Both positive and negative correlations were found in PBL between aerosol concentrations and O3 mixing ratios. The negative correlations result from the downward transport of relatively clean O3-rich air from the upper troposphere into PBL (which normally has higher aerosol loading and lower O3 concentrations than troposphere); positive correlations are found in biomass-burning plumes, where the aerosols are emitted into the air and O3 is photochemically produced. It was found that, in the dry season, a significant portion of the ozone over the rain forest is a result of biomass burning and that the distribution of photochemically produced O3 is strongly affected by synoptic-scale transport from large fires to the south/southeast.
Browell, E. V.↗
Biomass-burning emissions and associated haze layers over Amazonia
The characteristics of haze layers, which were visually observed over the central Amazon Basin during many of the Amazon Boundary Layer Experiment 2A flights in July/August 1985, were investigated by remote and in situ measurements, using the broad range of instrumentation and sampling equipment on board the Electra aircraft. It was found that these layers strongly influenced the chemical and optical characteristics of the atmosphere over the eastern Amazon Basin. Relative to the regional background, the concentrations of CO, CO2, O3, and NO were significantly elevated in the plumes and haze layers, with the NO/CO ratio in fresh plumes much higher than in the aged haze layers. The haze aerosol was composed predominantly of organic material, NH4, K(+), NO3(-), SO4(2-), and organic anions (formate, acetate, and oxalate).
Andreae, M. O.↗
Raman-shifted dye laser for water vapor DIAL measurements
For improved DIAL measurements of water vapor in the upper troposphere or lower stratosphere, narrowband (about 0.03/cm) laser radiation at 720- and 940-nm wavelengths was generated by stimulated Raman scattering (SRS), using the narrow linewidth (about 0.02/cm) output of a Nd:YAG-pumped dye laser. For a hydrogen pressure of 350 psi, the first Stokes conversion efficiencies to 940 nm were 20 percent and 35 percent, when using a conventional and waveguide Raman cell, respectively. The linewidth of the first Stokes line at high cell pressures, and the inferred collisional broadening coefficients, agree well with those previously measured in spontaneous Raman scattering.
Grossmann, B. E.↗
Tropopause fold structure determined from airborne lidar and in situ measurements
Airborne differential absorption lidar and in situ data obtained during the April 20, 1984 flight experiment conducted over Nevada and California are analyzed. The O3 and aerosols profiles and in situ measurements reveal a 2.0-km-deep layer (with high O3 concentrations and enhanced aerosol backscattering) and a correlation of 0.8 between O3 and aerosol backscatter (with both values decreasing about 25 percent along the central axis of the fold). It is observed that the cold boundary of the fold has weaker gradients, larger-scale undulations, and more irregularity than the warm boundary. The potential vorticity distribution along the flight path was derived from radiosonde data. A positive correlation between the O3 mixing ratio and the potential vorticity values in the fold is detected; the average ratio between O3 and potential vorticity is 50.2 ppbv/10 to the -5th sq cm deg per g s.
Browell, E. V.↗
Linewidth characteristics of Raman-shifted dye laser output at 720 and 940 nm
Raman conversion efficiency and line broadening are reported for Stokes operation at 720 and 940 nm, with hydrogen and deuterium as the Raman source, and using an Nd:YAG pumped Quanta-Ray PDL-2 dye laser. The dye laser linewidth is 0.2/cm (FWHM) with the grating alone as an intracavity element, and the conversion efficiency at 400 psi was found to be 40 and 20 percent for outputs of 720 and 940 nm, respectively. Pressure broadening coefficients of (9.2 + or - 0.9) x 10 to the -5th per cm/psi for hydrogen, and 7.7 x 10 to the -5th per cm/psi for deuterium, were obtained in good agreement with previous results. The linewidth at the first Stokes wavelength was shown to be determined by pressure broadening in the Raman medium.
Grossmann, B. E.↗
Development of a high-altitude airborne dial system: The Lidar Atmospheric Sensing Experiment (LASE)
The ability of a Differential Absorption Lidar (DIAL) system to measure vertical profiles of H2O in the lower atmosphere was demonstrated both in ground-based and airborne experiments. In these experiments, tunable lasers were used that required real-time experimenter control to locate and lock onto the atmospheric H2O absorption line for the DIAL measurements. The Lidar Atmospheric Sensing Experiment (LASE) is the first step in a long-range effort to develop and demonstrate an autonomous DIAL system for airborne and spaceborne flight experiments. The LASE instrument is being developed to measure H2O, aerosol, and cloud profiles from a high-altitude ER-2 (extended range U-2) aircraft. The science of the LASE program, the LASE system design, and the expected measurement capability of the system are discussed.
Browell, E. V.↗
Wavelength dependence of aerosol backscatter coefficients obtained by multiple wavelength Lidar measurements
Aerosols are often classified into several general types according to their origins and composition, such as maritime, continental, and stratospheric aerosols, and these aerosol types generally have different characteristics in chemical and physical properties. The present study aims at demonstrating the potential for distinguishing these aerosol types by the wavelength dependence of their backscatter coefficients obtained from quantitative analyses of multiple wavelength lidar signals. Data from the NASA Airborne Differential Abosrption lidar (DIAL) S ystems, which can measure aerosol backscatter profiles at wavelenghts of 300, 600, and 1064 nm and ozone profiles of backscatter coefficients for these three wavelength were derived from the observations of aerosols of different types. Observations were performed over the Atlantic Ocean, the Southwestern United States, and French Guyana.
Sasano, Y.↗
Assesment of dial data collection and analysis techniques
The key issues in all areas of Differential Absorption Lidar (DIAL) data collection and analysis techniques were examined. This included consideration of the practical and theoretical limitations of DIAL and the range of possible DIAL measurements.
Browell, E. V.↗
Influence of Rayleigh-Doppler broadening on the selection of H2O dial system parameters
Computer simulations have enabled the performance of a H2O Differential Absorption Lidar (DIAL) system to be studied by spectrally analyzing the forward propagating and backscattered laser energy. The simulations were done for a high altitude (21 km) DIAL system operating in a nadir-viewing mode. The influence of Rayleigh Doppler broadening on DIAL measurement accuracies were evaluated and show that the Rayleigh broadening influence, which can be corrected to first order in regions free of large aerosol gradients, reduces the sensitivity of DIAL H2O measurement errors in the upper tropospheric region. The ability to correct the Rayleigh broadening and the selection of H2O DIAL parameters when all the systematic effects are combined, were discussed.
Ismail, S.↗
Air chemistry over the tropical forest of Guyana
A comparison is made of the atmospheric chemistry within and above the atmospheric boundary layer over the tropical forest of Guyana. The data were gathered by NASA during the Global Tropospheric Experiment program in 1984, with an instrumented aircraft being used to collect data at altitudes of 3.5 km and between 150-450 m. The synoptic data covered concentrations of O3, CO, dimethylsulfide (DMS), halocarbons and isoprene and three different aerosol particulate measurements (DIAL system). The forest boundary layer proved to be a significant sink for O3, and a source for substantial emissions of DMS. Isoprene emitted by the forest was photochemically oxidized and became a source of CO.
Gregory, G. L.↗
Distribution and geochemistry of aerosols in the tropical North Atlantic troposphere - Relationship to Saharan dust
Estimates of global aerosol production suggest that mobilization of natural eolian material greatly exceeds anthropogenic-related emissions, and it appears that soil material transported from arid regions by wind might be mainly responsible for the distribution of certain clay materials in oceanic sediments. In connection with studies related to an investigation of these possibilities, the present paper provides a discussion of the aerosol spatial distribution and its water-soluble chemical composition in the tropical North Atlantic troposphere during the ABLE-Barbados mission. Particular attention is given to the composition of the water-soluble fraction, since its chemical reactivity is important with respect to various atmospheric and biogeochemical processes. On the basis of the obtained results, it is suggested that Saharan dust has also a significant impact on the aerosol chemistry over the tropical North Atlantic.
Talbot, R. W.↗
A lidar instrument to measure H2O and aerosol profiles from the NASA ER-2 aircraft
Plans to develop the Lidar Atmospheric Sensing Experiment (LASE) instrument to conduct scientific experiments aboard a NASA U-2 (ER-2) aircraft are described. The LASE measurement objectives are listed, and the design of the LASE instrument is discussed, including performance criteria for the laser transmitter, wavemeter, telescope, optical receiver, and associated electronics. The instrument function is depicted with a block diagram, and layouts of various components are presented.
Vaughan, W. R.↗
Airborne Lidar measurements of aerosols, mixed layer heights, and ozone during the 1980 PEPE/NEROS summer field experiment
A detailed summary of the NASA Ultraviolet Differential Absorption Lidar (UV DIAL) data archive obtained during the EPA Persistent Elevated Pollution Episode/Northeast Regional Oxidant Study (PEPE/NEROS) Summer Field Experiment Program (July through August 1980) is presented. The UV dial data set consists of remote measurements of mixed layer heights, aerosol backscatter cross sections, and sequential ozone profiles taken during 14 long-range flights onboard the NASA Wallops Flight Center Electra aircraft. These data are presented in graphic and tabular form, and they have been submitted to the PEPE/NEROS data archive on digital magnetic tape. The derivation of mixing heights and ozone profiles from UV Dial signals is discussed, and detailed intercomparisons with measurements obtained by in situ sensors are presented.
Browell, E. V.↗
Error caused by using a constant extinction/backscattering ratio in the lidar solution
The Bernoulli solution of the lidar equation with the assumption of a constant extinction/backscattering ratio can lead to errors in the derived aerosol extinction and backscattering profiles. This paper presents a general theoretical analysis of the errors that result from differences between the assumed and actual extinction/backscattering ratio profiles. Examples of the influence of the constant extinction/backscattering ratio assumption on the lidar derived aerosol extinction profile are presented for various laser wavelengths.
Sasano, Y.↗
Airborne DIAL System for Remote Tropospheric Sensing
Spatial distribution of gases and of aerosols measured. Airborne DIAL system uses two frequency-doubled Nd:YAG lasers and mounted in NASA Wallops Electra aircraft. Multipurpose airborne differential absorption lidar (DIAL) system, developed at Langley Research Center, remotely measures profiles of various gases and aerosols in diverse atmospheric investigations. Capability to rapidly determine spatial distribution of gases such as ozone, water vapor, sulfur dioxide, and nitrogen dioxide and to measure simultaneously distribution of aerosols at several laser wavelengths provides opportunity for developing extensive data base for examining complex interaction of atmospheric dynamics and chemistry.
Browell, E. V.↗
Spaceborne lidar system for measurements of atmospheric water vapor and aerosols
The inclusion of a differential absorption lidar (DIAL) system as part of the NASA Earth Observing System (EOS) is proposed. Functioning at 720 nm, the DIAL could provide atmospheric water vapor profiles in the troposphere and stratosphere, and provide data for characterizing the physical properties of clouds. The use of frequency doubling of the laser could also open a window on the 355 nm region, and thereby molecular density and temperature profiles. The date would be of use in studies of the global hydrological cycle, the global radiation balance, climate, meteorology, and atmospheric structure and transport phenomena.
Browell, E. V.↗