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All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Bringing weak transitions to light

Abstract Weak transitions between quantum states are of fundamental importance for a broad range of phenomena from analytical biochemistry to precision physics, but generally challenge experimental detection. Due to their small cross sections scaling with the absolute square of their transition matrix elements, spectroscopic measurements often fail in particular in the presence of competing background processes. Here we introduce a general concept to break this scaling law and enhance the transition probability by exploiting a stronger laser-coupled pathway to the same excited state. We demonstrate the concept experimentally by attosecond transient absorption spectroscopy in helium atoms. The quasi-forbidden transitions from the ground state 1s 2 to the weakly coupled doubly excited 2p3dandsp 2,4− states are boosted by an order of magnitude. Enhancing single-photon-suppressed transitions can find widespread applicability, from spectral diagnostics of complex molecules in life and chemical sciences to precision spectroscopy of weak transitions in metastable atomic nuclei in the search for new physics.

Science & Technology - Other Topics↗
DOE OSTI2020

Chiral effective field theory calculations of weak transitions in light nuclei

In this work, we report quantum Monte Carlo calculations of weak transitions in A≤10 nuclei, based on the Norfolk two- and three-nucleon chiral interactions, and associated one- and two-body axial currents. Furthermore, we find that the contribution from two-body currents is at the 2–3% level, with the exception of matrix elements entering the rates of 8Li, 8B, and 8He β decay. These matrix elements are suppressed in impulse approximation based on the (leading order) Gamow Teller transition operator alone; two-body currents provide a 20–30% correction, which is, however, insufficient to bring theory in agreement with experimental data. For the other transitions, the agreement with the data is satisfactory, and the results exhibit a negligible to mild model dependence when different combinations of Norfolk interactions are utilized to construct the nuclear wave functions. We report a complete study of two-body weak transition densities which reveals the expected universal behavior of two-body currents at short distances throughout the range of A=3 to A=10 systems considered here.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Weak Transitions in Light Nuclei

Nuclei are used for high-precision tests of the Standard Model and for studies of physics beyond the Standard Model. Without a thorough understanding of nuclei, we will not be able to meaningfully interpret the growing body of experimental data nor will we be able to disentangle new physics signals from underlying nuclear effects. This calls for accurate calculations of nuclear structure and reactions. In this work, we focus on electroweak decays in nuclei with mass number A ≤ 10 and report on ab initio Quantum Monte Carlo calculations of reduced matrix elements entering beta decays and electron captures in nuclei with mass number A ≤ 10. The many-body wave functions are calculated using selected Norfolk two- and three-nucleon potential models and associated one- and two-body axial currents at tree-level obtained from a chiral effective field theory with pions, nucleons, and Δ. The agreement with the experimental data is satisfactory except for transitions in A = 8 nuclei. In this specific case, the theory significantly underpredicts the experimental data, which indicates the need of further improvements in the corresponding nuclear wave functions. In this study, emphasis is placed on the contributions of two-body axial currents that are carefully analyzed using two-body transition densities. This allow us to study the spatial distribution and short-range behavior of two-body dynamics. In particular, the transition densities when scaled to peak at 1.0 exhibit universal short-range behavior across the considered nuclei, while they differ in the long-range tails.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Modified Brink-Axel hypothesis for astrophysical Gamow-Teller transitions

Weak interaction charged current transition strengths from highly excited nuclear states are fundamental ingredients for accurate modeling of compact object composition and dynamics, but are difficult to obtain either from experiment or theory. For lack of alternatives, calculations have often fallen back upon a generalized Brink-Axel hypothesis, that is, assuming the strength function (transition probability) is independent of the initial nuclear state but depends only upon the transition energy and the weak interaction properties of the parent nucleus ground state. Here we present numerical evidence for a modified “local” Brink-Axel hypothesis for Gamow-Teller transitions for pf-shell nuclei relevant to astrophysical applications. Specifically, while the original Brink-Axel hypothesis does not hold globally, strength functions from initial states nearby in energy are similar within statistical fluctuations. This agrees with previous work on strength function moments. Using this modified hypothesis, we can tackle strength functions at previously intractable initial energies, using semiconverged initial states at arbitrary excitation energy. Our work provides a well-founded method for computing accurate thermal weak transition rates for medium-mass nuclei at temperatures occurring in stellar cores near collapse. We finish by comparing results to previous calculations of astrophysical rates.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS1994

Time-dependent evolution of cosmic-ray-modified shock structure: Transition to steady state

Steady state solutions to the two-fluid equations of cosmic-ray-modified shock structure were investigated first by Drury and Volk (1981). Their analysis revealed, among other properties, that there exist regions of upstream parameter space where the equations possess three different downstream solutions for a given upstream state. In this paper we investigate whether or not all these solutions can occur as time-asymptotic states in a physically realistic evolution. To do this, we investigate the time-dependent evolution of the two-fluid cosmic-ray equations in going from a specified initial condition to a steady state. Our results indicate that the time-asymptotic solution is strictly single-valued, and it undergoes a transition from weakly to strongly cosmic-ray-modified at a critical value of the upstream cosmic ray energy density. The expansion of supernova remnant shocks is considered as an example, and it is shown that the strong to weak transition is in fact more likely. The third intermediate solution is shown to influence the time-dependent evolution of the shock, but it is not found to be a stable time-asymptotic state. Timescales for convergence to these states and their implications for the efficiency of shock acceleration are considered. We also investigate the effects of a recently introduced model for the injection of seed particles into the shock accelerated cosmic-ray population. The injection is found to result in a more strongly cosmic-ray-dominated shock, which supports our conclusion that for most classes of intermediate and strong cosmic-ray-modified shocks, the downstream cosmic-ray pressure component is at least as large as the thermal gas pressure, independent of the upstream state. As a result, cosmic rays almost always play a significant role in determining the shock structure and dissipation and they cannot be regarded as test particles.

Donohue, D. J.↗
DOE OSTI2025

Transition from weak to strong coupling in thermal gauge theories: Lessons from 𝒩 = 4 SYM theory

We investigate the transition between weak and strong coupling in thermal 𝒩 =4 supersymmetric Yang-Mills theory as a function of ’t Hooft coupling 𝜆 for several quantities of phenomenological interest for which next-to-leading order calculations are available in both regimes. We use Padé approximants to interpolate between the weak and strong coupling expansions and determine the location and width of the transition between the asymptotic regimes.

Gauge Theories↗
DOE OSTI2024

Identification of the weak-to-strong transition in Alfvénic turbulence from space plasma

Abstract Plasma turbulence is a ubiquitous dynamical process that transfers energy across many spatial and temporal scales in astrophysical and space plasma systems. Although the theory of anisotropic magnetohydrodynamic (MHD) turbulence has successfully described natural phenomena, its core prediction of an Alfvénic transition from weak to strong MHD turbulence when energy cascades from large to small scales has not been observationally confirmed. Here we report evidence for the Alfvénic weak-to-strong transition in small-amplitude, turbulent MHD fluctuations in Earth’s magnetosheath using data from four Cluster spacecraft. Our observations demonstrate the universal existence of strong turbulence accompanied by weak turbulent fluctuations on large scales. Moreover, we find that the nonlinear interactions of MHD turbulence are crucial to the energy cascade, as they broaden the cascade directions and fluctuating frequencies. The observed connection between weak and strong MHD turbulence systems may be present in many astrophysical environments, such as star formation, energetic particle transport, turbulent dynamos, and solar corona or solar wind heating.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

Identification of the weak-to-strong transition in Alfvénic turbulence from space plasma

Plasma turbulence is a ubiquitous dynamical process that transfers energy across many spatial and temporal scales in astrophysical and space plasma systems. Although the theory of anisotropic magnetohydrodynamic (MHD) turbulence has successfully described natural phenomena, its core prediction of an Alfvénic transition from weak to strong MHD turbulence when energy cascades from large to small scales has not been observationally confirmed. Here we report evidence for the Alfvénic weak-to-strong transition in small-amplitude, turbulent MHD fluctuations in Earth’s magnetosheath using data from four Cluster spacecraft. Our observations demonstrate the universal existence of strong turbulence accompanied by weak turbulent fluctuations on large scales. Moreover, we find that the nonlinear interactions of MHD turbulence are crucial to the energy cascade, as they broaden the cascade directions and fluctuating frequencies. The observed connection between weak and strong MHD turbulence systems may be present in many astrophysical environments, such as star formation, energetic particle transport, turbulent dynamos, and solar corona or solar wind heating.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS2018

The Impact of Stellar Variability on the Detection of Transiting Earth-like Planets

Stellar variability represents a key limitation on the detectability of weak transit signatures of small, Earth-size planets with space-based missions such as NASA's Kepler Mission or ESA's PLATO Mission. The expectations for the performance of the Kepler Mission in the face of solar-like variability were predicated on observations of the Sun with the Variability of Solar Irradiance and Gravity Oscillations (VIRGO) instrument aboard NASA and ESA's joint Solar and Heliospheric Observatory (SOHO) mission, which was launched in December 1995. Analyses of SOHO data indicated that solar-like variability would contribute approx.10 ppm to Kepler's noise budget at 6.5 ours, a typical grazing transit timescale. This proved to be optimistic as the typical 12th mag G2V star in the Kepler field of view exhibited 20 ppm of stellar variability-related noise at 6.5 hours, making the detection of true Earth-Sun analogs more difficult. While the consequent increase in the total noise at 6.5 hours from 20 ppm to 30 ppm could have been overcome by extending the mission to a total duration of 7 to 8 years. Unfortunately, a second reaction wheel failed in May 2013, ending the Kepler primary mission. Nevertheless, Kepler proved to be a veritable cornucopia of science results, both for exoplanets and for astrophysics. The phenomenal photometric precision and continuous observations required in order to identify small, rocky transiting planets enables the study of a large range of phenomena contributing to stellar variability for many thousands of solar-like stars in Kepler's field of view in exquisite detail. These effects range from less than 1 ppm acoustic oscillations on timescales from a few minutes and longward, to flares on timescales of hours, to spot-induced modulation on timescales of days to weeks to activity cycles on timescales of months to years. Kepler discovered over 2600 validated and confirmed exoplanets, and measured the pressure-mode oscillations of over 15000 stars over the course of its mission and the reconstituted K2 mission. We present the adaptive, wavelet-based matched filter used for both the Kepler and the TESS missions, and discuss the connections between this detection algorithm and fundamental detection theory, which allows the detector to function as a noise characterization engine. This provides a dynamical measurement of the photometric noise at transit timescales and thus, a key performance metric for missions like PLATO and Kepler. We give an overview of the stellar variability we see across the full range of spectral types observed by Kepler, from the cool, small red M stars to the hot, large late A stars, both in terms of amplitude as well as timescale.

transit surveys↗
NASA NTRS2018

The Impact of Stellar Variability on the Detection of Transiting Earth-Like Planets

Stellar variability represents a key limitation on the detectability of weak transit signatures of small, Earth-size planets with space-based missions such as NASA's Kepler Mission or ESA's PLATO Mission. The expectations for the performance of the Kepler Mission in the face of solar-like variability were predicated on observations of the Sun with the Variability of Solar Irradiance and Gravity Oscillations (VIRGO) instrument aboard NASA and ESA's joint Solar and Heliospheric Observatory (SOHO) mission, which was launched in December 1995. Analyses of SOHO data indicated that solar-like variability would contribute ~10 ppm to Kepler's noise budget at 6.5 ours, a typical grazing transit timescale. This proved to be optimistic as the typical 12th mag G2V star in the Kepler field of view exhibited 20 ppm of stellar variability-related noise at 6.5 hours, making the detection of true Earth-Sun analogs more difficult. While the consequent increase in the total noise at 6.5 hours from 20 ppm to 30 ppm could have been overcome by extending the mission to a total duration of 7 to 8 years. Unfortunately, a second reaction wheel failed in May 2013, ending the Kepler primary mission. Nevertheless, Kepler proved to be a veritable cornucopia of science results, both for exoplanets and for astrophysics. The phenomenal photometric precision and continuous observations required in order to identify small, rocky transiting planets enables the study of a large range of phenomena contributing to stellar variability for many thousands of solar-like stars in Kepler's field of view in exquisite detail. These effects range from <1 ppm acoustic oscillations on timescales from a few minutes and longward, to flares on timescales of hours, to spot-induced modulation on timescales of days to weeks to activity cycles on timescales of months to years. Kepler discovered over 2600 validated and confirmed exoplanets, and measured the pressure-mode oscillations of over 15000 stars over the course of its mission and the reconstituted K2 mission. We present the adaptive, wavelet-based matched filter used for both the Kepler and the TESS missions, and discuss the connections between this detection algorithm and fundamental detection theory, which allows the detector to function as a noise characterization engine. This provides a dynamical measurement of the photometric noise at transit timescales and thus, a key performance metric for missions like PLATO and Kepler. We give an overview of the stellar variability we see across the full range of spectral types observed by Kepler, from the cool, small red M stars to the hot, large late A stars, both in terms of amplitude as well as timescale.

exoplanets↗
NASA NTRS2014

The Evolution of Transition Region Loops Using IRIS and AIA

Over the past 50 years, the model for the structure of the solar transition region has evolved from a simple transition layer between the cooler chromosphere to the hotter corona to a complex and diverse region that is dominated by complete loops that never reach coronal temperatures. The IRIS slitjaw images show many complete transition region loops. Several of the "coronal" channels in the SDO AIA instrument include contributions from weak transition region lines. In this work, we combine slitjaw images from IRIS with these channels to determine the evolution of the loops. We develop a simple model for the temperature and density evolution of the loops that can explain the simultaneous observations. Finally, we estimate the percentage of AIA emission that originates in the transition region.

Winebarger, Amy R.↗
NASA NTRS1982

Laser-excitation technique for the measurement of absolute transition probabilities of weak atomic lines

A new technique is presented for the measurement of transition probabilities for weak allowed, intersystem, and forbidden lines. The method exploits the fact that oscillator strength is proportional to the number of stimulated absorptions and emissions produced by a narrow-band laser pulse of known energy which is in resonance with an atomic transition. The method is tested for a particular transition of Mg I with a known oscillator strength value and of appropriate magnitude. The number densities are measured using a Mach-Zehnder interferometer and the hook method for the lower level population and by measuring an absorption-equivalent width for the other. The apparatus consisted of a high-power tunable laser and a magnesium oven to produce excited Mg vapor, and a laser-plasma background continuum. The results are in good agreement with theoretical and other experimental data.

Kwong, H. S.↗
DOE OSTI2021

Spontaneous emission dynamics of Eu 3+ ions coupled to hyperbolic metamaterials

We show that sub-wavelength nanostructured systems with tunable electromagnetic properties, such as hyperbolic metamaterials (HMMs), provide a useful platform to tailor spontaneous emission processes. Here, we investigate a system comprising Eu 3+ (NO 3 ) 3 ·6H 2 O nanocrystals on an HMM structure featuring a hexagonal array of Ag nanowires in a porous Al2O 3 matrix. The HMM-coupled Eu 3+ ions exhibit up to a 2.4 fold increase in their decay rate, accompanied by an enhancement of the emission rate of the 5 D 0 → 7 F 2 transition. Using finite-difference time-domain modeling, we corroborate these observations with the increase in the photonic density of states seen by the Eu 3+ ions in the proximity of the HMM. Our results indicate that HMMs can serve as a valuable tool to control the emission from weak transitions and, hence, hint at a route toward more practical applications of rare-earth ions in nanoscale optoelectronics and quantum devices.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRSDate not supplied

Chasing Shadows in the Night: How NASA's Kepler and TESS Missions Are Revolutionizing Exoplanet Science

The first planet outside our own solar system was discovered almost thirty years ago in an extremely unlikely place, orbiting a pulsar, and the first exoplanet orbiting a Sun-like star was discovered nearly 26 years ago. In the time since, we’ve detected over 5000 planets and over 75% of these have been detected by transit surveys. The Kepler Mission, launched in 2009, has found the lion’s share of these exoplanets, and demonstrated that each star in the night sky has, on average, at least one planet. Kepler’s success spurred NASA and ESA to select several exoplanet-themed missions to move the field of exoplanet science forward from discovery to characterization: How do these planets form and evolve? What is the structure and composition of the atmospheres and interiors of these planets? Can we detect biomarkers in the atmospheres of these planets and learn the answer to the fundamental question, are we alone? NASA selected the Transiting Exoplanet Survey Satellite (TESS) in 2014 to conduct a nearly all-sky survey for transiting planets with the goal of identifying at least 50 small planets with measured masses that can be followed up by large telescopic assets, such as the upcoming James Webb Space Telescope. TESS has discovered 266 exoplanets so far, 100 of which are smaller than earth with measured masses. In this talk I will describe how we detect weak transit signatures in noisy but beautiful transit survey data sets and present some of the most compelling discoveries made so far by Kepler and TESS.

TESS↗
DOE OSTI2024

Regulating the Electron Distribution of Metal-Oxygen for Enhanced Oxygen Stability in Li-rich Layered Cathodes

Li-rich Mn-based layered oxides (LLO) hold great promise as cathode materials for lithium-ion batteries (LIBs) due to their unique oxygen redox (OR) chemistry, which enables additional capacity. However, the LLOs face challenges related to the instability of their OR process due to the weak transition metal (TM)-oxygen bond, leading to oxygen loss and irreversible phase transition that results in severe capacity and voltage decay. Herein, a synergistic electronic regulation strategy of surface and interior structures to enhance oxygen stability is proposed. In the interior of the materials, the local electrons around TM and O atoms may be delocalized by surrounding Mo atoms, facilitating the formation of stronger TM—O bonds at high voltages. Besides, on the surface, the highly reactive O atoms with lone pairs of electrons are passivated by additional TM atoms, which provides a more stable TM—O framework. Hence, this strategy stabilizes the oxygen and hinders TM migration, which enhances the reversibility in structural evolution, leading to increased capacity and voltage retention. This work presents an efficient approach to enhance the performance of LLOs through surface-to-interior electronic structure modulation, while also contributing to a deeper understanding of their redox reaction.

25 ENERGY STORAGE↗
DOE OSTI2020

Exact sum rules with approximate ground states

Electromagnetic and weak transitions tell us a great deal about the structure of atomic nuclei. Yet modeling transitions can be difficult: it is often easier to compute the ground state, if only as an approximation, than excited states. One alternative is through transition sum rules, in particular the non-energy-weighted and energy-weighted sum rules, which can be computed as expectation values of operators. We investigate by computing sum rules for a variety of nuclei, comparing the numerically exact full configuration-interaction shell model, as a reference, to Hartree-Fock, projected Hartree-Fock, and the nucleon pair approximation. Furthermore, these approximations yield reasonable agreement, which we explain by prior work on the systematics of transition moments.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS1990

Photophysical behavior of doubly bridged d7-d7 metal-metal bonded compounds - The crystal structure and the excited- and ground-state electronic spectra of Re2(CO)6(dmpm)2 (dmpm = bis/dimethylphosphino/ methane)

Re2(CO)6(dmpm)2 shows photophysical behavior in a rigid medium that differs dramatically from that observed in fluid solution. In a hydrocarbon glass at 77 K, metal-metal bond homolysis is suppressed and an intense phosphorescence is observed. The transient absorption spectrum, which shows only weak transitions to the red of the ground state 1(sigma-sigma asterisk) transition, permits assignment of the emitting state to a 3(sigma-sigma asterisk) transition. The crystal structure of Re2(CO)6(dmpm)2 is also reported. The ground-state electronic structure is discussed relative to the structural data.

Milder, Steven J.↗