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Reference Model Development
Presentation from the 2011 Water Peer Review in which principal investigator discusses project progress to develop a representative set of Reference Models (RM) for the MHK industry to develop baseline cost of energy (COE) and evaluate key cost component/system reduction pathways.
Photoelectrochemical Hydrogen Production (Final Report)
The objectives of this project, covering two phases and an additional extension phase, were the development of thin film-based hybrid photovoltaic (PV)/photoelectrochemical (PEC) devices for solar-powered water splitting. The hybrid device, comprising a low-cost photoactive material integrated with amorphous silicon (a-Si:H or a-Si in short)-based solar cells as a driver, should be able to produce hydrogen with a 5% solar-to-hydrogen conversion efficiency (STH) and be durable for at least 500 hours. Three thin film material classes were studied and developed under this program: silicon-based compounds, copper chalcopyrite-based compounds, and metal oxides . With the silicon-based compounds, more specifically the amorphous silicon carbide (a-SiC), we achieved a STH efficiency of 3.7% when the photoelectrode was coupled to an a-Si tandem solar cell, and a STH efficiency of 6.1% when using a crystalline Si PV driver. The hybrid PV/a-SiC device tested under a current bias of -3~4 mA/cm 2 , exhibited a durability of up to ~800 hours in 0.25 M H 2 SO 4 electrolyte. Other than the PV driver, the most critical element affecting the photocurrent (and hence the STH efficiency) of the hybrid PV/a-SiC device was the surface energetics at the a-SiC/electrolyte interface. Without surface modification, the photocurrent of the hybrid PEC device was ~1 mA/cm 2 or lower due to a surface barrier that limits the extraction of photogenerated carriers. We conducted an extensive search for suitable surface modification techniques/materials, of which the deposition of low work function metal nanoparticles was the most successful. Metal nanoparticles of ruthenium (Ru), tungsten (W) or titanium (Ti) led to an anodic shift in the onset potential. We have also been able to develop hybrid devices of various configurations in a monolithic fashion and optimized the current matching via altering the energy bandgap and thickness of each constituent cell. As a result, the short-circuit photocurrent density of the hybrid device (measured in a 2-electrode configuration) increased significantly without assistance of any external bias, i.e. from ≤1 mA/cm 2 to ~5 mA/cm 2 . With the copper chalcopyrite compounds, we have achieved a STH efficiency of 3.7% in a coplanar configuration with 3 a-Si solar cells and one CuGaSe 2 photocathode. This material class exhibited good durability at a photocurrent density level of -4 mA/cm 2 (“5% STH” equivalent) at a fixed potential (-0.45 V RHE ). A poor band-edge alignment with the hydrogen evolution reaction (HER) potential was identified as the main limitation for high STH efficiency. Three new pathways have been identified to solve this issue. First, PV driver with bandgap lower than that of amorphous silicon were investigated. Crystalline silicon was identified as possible bottom cell. Mechanical stacks made with one Si solar cell and one CuGaSe 2 photocathode were built. A 400 mV anodic shift was observed with the Si cell, leading to photocurrent density of -5 mA/cm 2 at 0V RHE (compared to 0 mA/cm 2 at the same potential without PV driver). We also investigated the use of p-n junctions to shift CuGaSe 2 flatband potential anodically. Reactively sputtered zinc oxy-sulfide thin films was evaluated as n-type buffer and deposited on CuGaSe 2 . Ruthenium nanoparticles were then added as HER catalyst. A 250 mV anodic shift was observed with the p-n junction, leading to photocurrent density at 0V RHE of -1.5 mA/cm 2 . Combining this device with a Si solar cell in a mechanical stack configuration shifted the onset potential further (+400 mV anodically), leading to photocurrent density of -7 mA/cm 2 at 0V RHE . Finally, we developed wide bandgap copper chalcopyrite thin film materials. We demonstrated that Se can be substituted with S using a simple annealing step. Photocurrent densities in the 5-6 mA/cm 2 range were obtained with red 2.0eV CuInGaS 2 photocathodes. With the metal oxide compounds, we have demonstrated that a WO 3 -based hybrid photoelectrode was feasible. Specifically, we showed that WO 3 paired with an a-Si tandem solar cell can generate short circuit photocurrent density of 2.5 mA/cm 2 , equivalent to STH efficiency of 3.1%. Long-term durability tests demonstrated WO 3 ability to split water over extended periods, for up to 600 hours at current density levels of 2.0-2.5 mA/cm 2 . Efforts have been done to decrease WO 3 bandgap using foreign elements incorporation. We did not manage to reduce the bandgap of WO 3 with this method. However, more promising results have been achieved with bilayered systems, where only the top part of WO 3 films was modified. Also, we have demonstrated that alloying WO 3 with CuO can form 2.2eV bandgap CuWO 4 . Incorporating conductive carbon nanotubes in CuWO 4 reduced its intrinsic bulk resistance. Saturation photocurrent densities in the 0.4-0.5 mA/cm 2 range were achieved. Recently, in collaboration with University of Texas at Arlington, we have identified new quaternary metal oxides with CuWO 4 as primary material host. Our experimental work on ceramics confirmed the theoretical calculations that crowned bismuth as a possible candidate to improve CuWO 4 water splitting efficiency.
Ultrasonic Bat Deterrent Technology
The project objective was to advance the development and testing of a near commercial bat-deterrent system with a goal to increase the current GE deterrent system effectiveness to over 50% with broad species applicability. Additionally, the research supported by this program has provided insights into bat behavior and ultrasonic deterrent design that had not previously been explored. Prior research and development had demonstrated the effectiveness of a commercial-grade, air-powered, ultrasonic bat deterrent to be between 30-50% depending upon the species of bat. However, the previous research provided limited insight into the behavioral responses of bats in the presence of ultrasonic deterrent sound fields that could be utilized to improve effectiveness. A unique bat flight room was utilized to observe the behavioral characteristics of bats in the presence of ultrasonic sound fields. Behavioral testing in the bat flight facility demonstrated that ultrasonic sounds similar to those produced by the GE deterrent influenced the activities and behaviors, primarily those associated with foraging, of the species exposed. The study also indicated that continuous and pulsing ultrasonic signals had a similar effect on the bats, and confirmed that as ultrasonic sounds attenuate, their influence on the bats’ activities and behavior decreases. Ground testing at Wolf Ridge Wind, LLC and Shawnee National Forest assessed both continuous and pulsing deterrent signals emitted from the GE deterrent system and further enhanced the behavioral understanding of bats in the presence of the deterrent. With these data and observations, the existing 4-nozzle continuous, or steady, emission ultrasonic system was redesigned to a 6-nozzle system that could emit a pulsing signal covering a larger air space around a turbine. Twelve GE 1.6-100 turbines were outfitted with the deterrent system and a formal three-month field study was performed using daily carcass searches beneath the 12 turbines. Additionally, a unique 3D bat flight path visualization system was utilized to monitor for and identify any changes in bat activity caused by the operation of the deterrent system. Both the carcass search and flight path visualization data indicated that the pulsed deterrent system was effective, but not more effective, than the steady system tested in prior years. However, an unanticipated byproduct of the pulsing system was the emission of intermittent water vapor from the deterrent devices due to the air compression process that powered the devices. This water vapor may have altered the ultrasonic signal and obscured the results in an unknown way. While a qualitative analysis of the effect of the water vapor on the deterrent signal had indicated there was not dramatic change in the expected ultrasonic signal, it was not possible to conclusively determine if the pulse signal would have been more effective in the absence of the water vapor. A mid-season installation of a desiccant system was performed and the dataset divided into two groups to account for the change. Prior to the system change, the deterrent was not effective (-23%, P = 0.8617, α = 0.05) at reducing eastern red bat fatalities and effective (38%, P = 0.0169, α = 0.05) for the non-eastern red bat species, combined. After the installation of the desiccant system, the pulsed deterrent system showed similar results, although not statistically significant, with a point estimates of 23% (P = 0.2924, α = 0.05) observed for eastern red bats and 54% (P = 0.0926, α = 0.05) for the other combined bat species.
Zero-power wireless system for crop water content monitoring
Zero power wireless sensors, devices, and systems are used for crop water content monitoring. The sensors consume no power while monitoring for the presence of dry crop conditions. Infrared reflectance from plants is measured and when selected spectral conditions are met, a circuit is closed, activating an alarm, an RFID tag, or a radio transmitter. The deployed sensors consume no power while monitoring, reducing or eliminating the need to change batteries.
Hierarchical design and development of nanostructured trifunctional catalysts for electrochemical oxygen and hydrogen reactions
Trifunctional catalysts show a great potential for use in a power-to-gas water-splitting devices for hydrogen gas production, powered by an integrated rechargeable zinc-air battery. None of the currently available commercial electrocatalysts is low cost, and they do not possess excellent catalytic activity and durability at the same time, which is the main barrier to the broad implementation of these technologies. Herein, we design and develop a novel nanostructured trifunctional electrocatalyst that is capable of catalyzing oxygen/hydrogen evolution and oxygen reduction reactions. The combination of non-precious Co, Co 9 S 8 , and S, N co-doped graphitic carbon synergistically provides highly active sites for efficient catalytic reactions, while the unique tubular morphology and hierarchically porous microstructure not only benefit fast access to active sites but also ensure a robust composite structure for durability. As a result, when applied to zinc-air batteries and water splitting, these systems exhibit performance superior to those of commercial precious electrocatalysts (e.g., Pt/C and Ir/C).
Optimization and Annual Average Power Predictions of a Backward Bent Duct Buoy Oscillating Water Column Device Using the Wells Turbine.
This Technical Report presents work completed by The Applied Research Laboratory at The Pennsylvania State University, in conjunction with Sandia National Labs, on the optimization of the power conversion chain (PCC) design to maximize the Average Annual Electric Power (AAEP) output of an Oscillating Water Column (OWC) device. The design consists of two independent stages. First, the design of a floating OWC, a Backward Bent Duct Buoy (BBDB), and second the design of the PCC. The pneumatic power output of the BBDB in random waves is optimized through the use of a hydrodynamically coupled, linear, frequency-domain, performance model that links the oscillating structure to internal air-pressure fluctuations. The PCC optimization is centered on the selection and sizing of a Wells Turbine and electric power generation equipment. The optimization of the PCC involves the following variables: the type of Wells Turbine (fixed or variable pitched, with and without guide vanes), the radius of the turbine, the optimal vent pressure, the sizing of the power electronics, and number of turbines. Also included in this Technical Report are further details on how rotor thrust and torque are estimated, along with further details on the type of variable frequency drive selected.
Optimization and annual average power predictions of a backward bent duct buoy oscillating water column device using the wells turbine.
Abstract not provided.
Water reactive hydrogen fuel cell power system
A water reactive hydrogen fueled power system includes devices and methods to combine reactant fuel materials and aqueous solutions to generate hydrogen. The generated hydrogen is converted in a fuel cell to provide electricity. The water reactive hydrogen fueled power system includes a fuel cell, a water feed tray, and a fuel cartridge to generate power for portable power electronics. The removable fuel cartridge is encompassed by the water feed tray and fuel cell. The water feed tray is refillable with water by a user. The water is then transferred from the water feed tray into a fuel cartridge to generate hydrogen for the fuel cell which then produces power for the user.
Water reactive hydrogen fuel cell power system
A water reactive hydrogen fueled power system includes devices and methods to combine reactant fuel materials and aqueous solutions to generate hydrogen. The generated hydrogen is converted in a fuel cell to provide electricity. The water reactive hydrogen fueled power system includes a fuel cell, a water feed tray, and a fuel cartridge to generate power for portable power electronics. The removable fuel cartridge is encompassed by the water feed tray and fuel cell. The water feed tray is refillable with water by a user. The water is then transferred from the water feed tray into the fuel cartridge to generate hydrogen for the fuel cell which then produces power for the user.
Dynamometer Facts
The National Renewable Energy Laboratory's (NREL's) Flatirons Campus features four dynamometers that can perform research validation on wind turbine systems and ocean energy devices. These dynamometers can validate wave and water power systems over capacity ratings ranging from 1 kilowatt (kW) to 5 megawatts (MW) by replacing water with a controllable, electric motor. By combining these capabilities with other tools, such as the controllable grid interface (https://www.nrel.gov/grid/controllable-grid-interface.html), researchers can verify how their device interacts with the grid or integrates with other technologies.
Wave Energy Prize -- Carderock Test Design and Rigging to Accommodate Diversity of Device Types
Wave Energy Prize Carderock Test Design and Rigging to Accommodate Diversity of Device Types presentation from the Water Power Technologies Office Peer Review, FY14-FY16. The challenge was to determine testing conditions, develop processing algorithms, and execute tests for equitable and consistent evaluation of different wave energy converter (WEC) technologies.
HNEI Role at US Navy Wave Energy Test Site
U.S. Navy established the Wave Energy Test Site (WETS) in the waters off Marine Corps Base Hawaii, the United States’ first grid-connected site, to the nascent commercial wave energy sector which is critically dependent on available test infrastructure to address challenges with developing Wave Energy Conversion (WEC) devices. WETS consists of test berths at 30m, 60m, and 80m water depths, and can host point absorber and oscillating water column devices to a peak power of 1 MW. HNEI provides key research support to this national effort in the form of environmental monitoring, independent WEC device performance analysis, and critical marine logistical support.
A comparison of WEC control strategies
The operation of Wave Energy Converter (WEC) devices can pose many challenging problems to the Water Power Community. A key research question is how to significantly improve the performance of these WEC devices through improving the control system design. This report summarizes an effort to analyze and improve the performance of WEC through the design and implementation of control systems. Controllers were selected to span the WEC control design space with the aim of building a more comprehensive understanding of different controller capabilities and requirements. To design and evaluate these control strategies, a model scale test-bed WEC was designed for both numerical and experimental testing (see Section 1.1). Seven control strategies have been developed and applied on a numerical model of the selected WEC. This model is capable of performing at a range of levels, spanning from a fully-linear realization to varying levels of nonlinearity. The details of this model and its ongoing development are described in Section 1.2.
Separation of gaseous hydrogen from a water-hydrogen mixture in a fuel cell power system operating in a weightless environment
A fuel cell power system for use in a weightless environment, such as in space, includes a device for removing water from a water-hydrogen mixture condensed from the exhaust from the fuel cell power section of the system. Water is removed from the mixture in a centrifugal separator, and is fed into a holding, pressure operated water discharge valve via a Pitot tube. Entrained nondissolved hydrogen is removed from the Pitot tube by a bleed orifice in the Pitot tube before the water reaches the water discharge valve. Water discharged from the valve thus has a substantially reduced hydrogen content.
Biological Consequences of Marine Energy Development on Marine Animals
Marine energy devices harness power from attributes of ocean water to form a sustainable energy source. Knowledge gaps remain about whether marine energy systems can affect the environment, adding another threat to animal populations and habitats already under pressure from climate change and anthropogenic activities. To date, potential environmental effects have been studied under the scope of stressor–receptor interactions, where moving parts of, or emissions from, a system could harm the animals, habitats, and natural processes. While crucial for understanding effects and identifying knowledge gaps, this approach misses a holistic view of what animals may experience in the presence of marine energy systems. We look at six biological consequences and forces that drive the health of an animal population and the effects expected from marine energy development: success of early life stages; changes in competitive capabilities; growth and survival based on food availability; susceptibility to predators; injury or death; and reproductive success. We use case studies to develop this approach, focusing on a variety of marine animals. An approximate level of risk is assigned for each interaction based on the biological consequences. This work highlights the need to examine the effects of marine energy development on animal populations within their natural habitats.
Construction bidding cost of KSC's space shuttle facilities
The bidding cost of the major Space Transportation System facilities constructed under the responsibility of the John F. Kennedy Space Center (KSC) is described and listed. These facilities and Ground Support Equipment (GSE) are necessary for the receiving, assembly, testing, and checkout of the Space Shuttle for launch and landing missions at KSC. The Shuttle launch configuration consists of the Orbiter, the External Tank, and the Solid Rocket Boosters (SRB). The reusable Orbiter and SRB's is the major factor in the program that will result in lowering space travel costs. The new facilities are the Landing Facility; Orbiter Processing Facility; Orbiter Approach and Landing Test Facility (Dryden Test Center, California); Orbiter Mating Devices; Sound Suppression Water System; and Emergency Power System for LC-39. Also, a major factor was to use as much Apollo facilities and hardware as possible to reduce the facilities cost. The alterations to existing Apollo facilities are the VAB modifications; Mobile Launcher Platforms; Launch Complex 39 Pads A and B (which includes a new concept - the Rotary Service Structure), which was featured in ENR, 3 Feb. 1977, 'Hinged Space Truss will Support Shuttle Cargo Room'; Launch Control Center mods; External Tank and SRB Processing and Storage; Fluid Test Complex mods; O&C Spacelab mods; Shuttle mods for Parachute Facility; SRB Recovery and Disassembly Facility at Hangar 'AF'; and an interesting GSE item - the SRB Dewatering Nozzle Plug Sets (Remote Controlled Submarine System) used to inspect and acquire for reuse of SRB's.
Theoretical limits of multiple exciton generation and singlet fission tandem devices for solar water splitting
Photoelectrochemical (PEC) water splitting is one of the most important approaches being investigated for solar fuel generation. In this study, we determine the maximum thermodynamic power conversion efficiencies (PCEs) of PEC water splitting two-bandgap tandem devices that produce multiple carriers per photon absorbed via Multiple Exciton Generation (MEG) or Singlet Fission (SF) and in the presence of solar concentration. Here, we employ a detailed balance thermodynamic analysis to determine the effects of top cell thickness, solar concentration, carrier multiplication, electrode overvoltage (VO), and water absorption on PEC power conversion efficiency for water splitting cells. We have found a maximum PEC power conversion efficiency of 62.9% in cells using two ideal tandem MEG absorbers with bandgaps of 0.3 and 1.2 eV at 1000-suns solar concentration and 0 overvoltage; the maximum PCE for two tandem SF absorbers under the same conditions is nearly the same at 59% with the same values for the absorption thresholds. A very interesting and important result was that, upon thinning the top cell, the range of viable bandgaps for both the top and bottom cells is extended by as much as 0.5-1 eV while still maintaining high maximum conversion efficiency (60-63%). The effects of imposing different solar concentrations from 1X to 1000X and having different tandem configurations of SF and MEG layers were also studied.