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At least 19 records

How Well Satellite Remote Sensing Can Inform Surface Level Ozone Production Sensitivity to Precursor Trace Gas Emissions?

Surface-level ozone (O3) pollution mitigation strategies rely on a clear understanding of the atmospheric chemical processes involving O3, NOx (nitric oxide (NO) + nitrogen dioxide (NO2)) and volatile organic compounds (VOCs). A robust spatiotemporal classification of O3 photochemical regimes with relative chemical sensitivity of local O3 formation to emission reductions of NOx (NOx-limited regime) versus VOCs (radical-limited regime) is required to design anthropogenic emission reduction policies in order to improve surface air quality. Numerous studies found that the ratio of satellite-retrieved Vertical Column Densities (VCDs) of formaldehyde (HCHO) to NO2 can diagnose O3 production sensitivity. However, uncertainty still remains about the accuracy of such estimates using satellite-based retrievals. This study conducts an investigation to identify how well satellite data can inform surface-level O3 sensitivity by validating satellite-based estimates against aircraft-based retrievals taken during the Long Island Sound Tropospheric Ozone Study (LISTOS-2018) and Ozone Water-Land Environmental Transition Study (OWLETS-2) field campaigns. For this study, we use HCHO and NO2 retrievals from the Ozone Monitoring Instrument (OMI) onboard the Aura satellite, and high spatiotemporal resolution TROPOspheric Monitoring Instrument (TROPOMI) onboard the Sentinel-5 Precursor (S5P) satellite. The Community Multiscale Air Quality (CMAQ) modelling system is used to provide trace gas vertical profiles to recalculate air mass factor for deriving consistent satellite-based VCDs. To demonstrate the ability of satellites to diagnose O3 production regimes, we validate satellite-derived O3 sensitivity regimes, along with the OMI and TROPOMI products applied, using HCHO and NO2 retrievals from the aircraft-based instruments: Geostationary Trace gas and Aerosol Sensor Optimization (GeoTASO) spectrometer and Geostationary Coastal and Air Pollution Events Airborne Simulator (GCAS) instruments deployed during the LISTOS-2018 and OWLETS-2 campaigns. The results of this work will advance our fundamental knowledge of the spatiotemporal evolution of the complex O3-NOx-VOC chemistry, and will advance our understanding about the quality of remote-sensing, suborbital, and satellite data for accurately observing surface-level O3 production sensitivity.

Satellite↗

Statistical relation between monthly mean precipitable water and surface-level humidity over global oceans

Monthly summaries of atmospheric soundings taken over 17 years from 49 midocean stations at small islands and weather ships distributed over major oceans are examined. Over tropical oceans, precipitable water is found to be a better predictor of surface-level humidity than surface-level air temperature. A statistical relation in the form of a polynomial is derived; from this relation, the monthly-mean, surface-level mixing ratio can be computed from monthly-mean precipitable water. The root-mean-square differences between the measured and derived values were found to be less than 8 x 10 to the -4th over most ocean areas. Such a relation is useful in deriving large-scale evaporation and latent heat flux data from the ocean, using spaceborne observations. The temporal and spatial variabilities of data deviations from this relation are examined. This relation is found to be applicable to all major ocean basins and can be used to monitor interannual variability. Boundary-layer thermodynamics of different air masses are suggested as an explanation of some characteristics of this relation.

Liu, W. T.↗

Investigating the Sensitivity of Surface-Level Nitrate Seasonality in Antarctica to Primary Sources Using a Global Model

Determining the sources of total nitrate (TNIT NO-3 + HNO3) reaching Antarctica is a long-standing challenge. Here we analyze the monthly sensitivity of surface-level TNIT in Antarctica to primary sources using a global 3-D chemical transport model, GEOS-Chem, and its adjoint. Modeled seasonal variation of TNIT concentrations shows good agreement with several measurement studies, given that the lack of post-depositional processing in the model leads to an expected underestimate of maximum values in November through January. Remote NOx sources have the greatest impact May-July, during when the model background concentrations are sensitive to NOx emissions from fossil fuel combustion, soil, and lightning originating from 25S to 65S. In this season, NOx is transported to Antarctica as TNIT, which is formed above continental source regions at an altitude of 5-11 km. In other seasons, more NOx is transported as a reservoir species (e.g., peroxyacetyl nitrate, PAN) through the free troposphere, transforming into TNIT within a cone of influence that extends to 35S and above 4 km altitude. Photolysis of PAN over Antarctica is the main driver of modeled NOx seasonality. Stratospheric production and loss of tracers are relatively unimportant in monthly sensitivities in GEOS-Chem, driving only a few percent of surface level variability of TNIT. A small peak concentration in August is captured by the model, although some measured values in August fall outside the range of simulated concentrations. Modifications to the model to represent sedimentation of polar stratospheric clouds (PSCs) lead to increased surface level August TNIT concentrations. However, this simple representation does not explicitly account for PSC particle deposition or disappearance of the tropopause in the middle of winter, and thus the influence of stratospheric nitrate sources estimated in this study is likely a lower bound.

stratosphere↗

A predictive monsoon signal in the surface level thermal field over India

The mean monthly surface thermal field over India during the premonsoon months March-May, based on mean monthly-temperature/minimum-temperature/maximum-temperature data from the network of 119 stations, was examined with the objective of locating significant predictor parameters for forecasting Indian monsoon rainfall. The results of linear correlation analysis bring out three areas for which the relationships between Indian monsoon rainfalls and the area average of mean monthly minimum temperature for April or for May were found to be significant. The best correlation was found for the southern peninsular area, where the mean May minimum temperature is significantly related to the 500 mB April ridge, a tendency in the Southern Oscillation Index, and a tendency in eastern equatorial Pacific SST.

Mooley, D. A.↗

Generation of topographic terrain models utilizing synthetic aperture radar and surface level data

Topographical terrain models are generated by digitally delineating the boundary of the region under investigation from the data obtained from an airborne synthetic aperture radar image and surface elevation data concurrently acquired either from an airborne instrument or at ground level. A set of coregistered boundary maps thus generated are then digitally combined in three dimensional space with the acquired surface elevation data by means of image processing software stored in a digital computer. The method is particularly applicable for generating terrain models of flooded regions covered entirely or in part by foliage.

Imhoff, Marc L.↗

Experiments in Transitional Boundary Layers With Emphasis on High Free-Stream Disturbance Level, Surface Concave Curvature and Strong Favorable Streamwise Pressure Gradient Effects

Experiments on boundary layer transition with flat, concave and convex walls and various levels of free-stream disturbance and with zero and strong streamwise acceleration have been conducted. Measurements of both fluid mechanics and heat transfer processes were taken. Examples are profiles of mean velocity and temperature; Reynolds normal and shear stresses; turbulent streamwise and cross-stream heat fluxed; turbulent Prandtl number; and streamwise variations of wall skin friction and heat transfer coefficient values. Free-stream turbulence levels were varied over the range from about 0.3 percent to about 8 percent. The effects of curvature on the onset of transition under low disturbance conditions are clear; concave curvature leads to an earlier and more rapid transition and the opposite is true for convex curvature This was previously known but little documentation of the transport processes in the flow was available

Simon, T. W.↗

Using Machine Learning to Estimate Surface-Level SO2 Concentrations from Satellite-Based Measurements

Sulfur dioxide (SO2) is a criteria air pollutant due to its contributions to aerosol formation, rainfall acidification, and harm to human health. The placement of air quality monitoring sites is typically biased towards urban areas, leaving large areas with very limited monitoring data. The Ozone Monitoring Instrument (OMI) has been used to provide estimates of SO2 vertical column densities (VCDs) globally at spatial resolution of 10s of kms once per day. OMI SO2 VCDs have been previously used to estimate surface SO2 concentrations using chemical transport model (CTM) simulations. The CTMs use estimated emissions and assimilated meteorological data, and simulate the chemical and physical processes that determine the vertical profile of SO2, which can be used to derive a ratio between the surface concentrations and VCDs. These models are complex, computationally expensive, and have large uncertainties in the simulated surface-to-VCD ratio due to biases in emissions and relatively coarse resolution. Machine learning techniques are comparatively easier to use, much less computationally expensive to use after training, and can produce more accurate estimations of surface concentrations than the CTM-based method. The interpretation of machine learning models often poses challenges, and in some cases, non-physical variables unrelated to SO2 are used as predictors. In this work, we create an artificial neural network (ANN) to relate OMI retrievals and archived GEOS-FP boundary layer heights to surface SO2 concentrations from the ChinaHighAirPollutants ChinaHighSO2 dataset (CHAP; Wei et al., 2023) on a seasonal average timescale from 2013-2018. Our model only utilizes five variables that are directly relevant to the satellite retrieval, lifetime, and spatial distribution of SO2. The model was trained on 16 seasons (four of each) with independent validation (one of each season) and testing datasets (one of each season) to avoid overfitting. Our ANN generates surface SO2 concentrations that are sensitive (slope = 0.51) and consistent (r = 0.74) with the CHAP data, but are underpredicted by an average of 1.2 ppbv with a mean absolute error of 2.2 ppbv. These results are better than recent studies utilizing the CTM method. To our knowledge, this is the best performing machine learning model that only uses physical variables to predict surface SO2. Our work demonstrates that a carefully constructed, simple ML model can accurately estimate surface-based SO2 concentrations from satellite VCD measurements, and this technique has future promise to expend to newer, higher resolution satellites and other air pollutants.

SO2, air quality, OMI, machine learning↗

Bayesian Geostatistical Modelling of PM10 and PM2.5 Surface Level Concentrations in Europe Using High-Resolution Satellite-Derived Products

Air quality monitoring across Europe is mainly based on in situ ground stations which are too sparse to accurately assess the exposure effects of air pollution for the entire continent. The demand for precise predictive modelsthat estimate gridded geophysical parameters of ambient air at high spatial resolution has rapidly grown. Here, we investigate the potential of satellite derived products to improve particulate matter (PM) estimates. Bayesiangeostatistical models addressing confounding between the spatial distribution of pollutants and remotely sensed predictors were developed to estimate yearly averages of both, fine (PM2.5) and coarse (PM10) surface PM concentrations at 1 sq.km spatial resolution over 46 European countries and were compared to geostatistical, geographically weighted and land-use regression formulations. Rigorous model selection identified the Earth observation data which contribute most to pollutants' estimation. Geostatistical models outperformed the predictive ability of the frequently employed land-use regression. The resulting estimates of PM10 and PM2.5, which represent the main air quality indicators for the urban Sustainable Development Goal, indicate that in 2016, 66.2% of the European population was breathing air above the WHO Air Quality Guidelines thresholds. Our estimates are readily available to policy makers and scientists assessing the effects of long-term exposure to pollution on human and ecosystem health.

Beloconi, Anton↗

ISOLEV - A level surface cutting plane program for fluid flow data

A computer program, ISOLEV, allows interactive visualization of CFD scalar and vector functions by means of user-specified sections of the data. The application is based on table lookups which govern both isosurface generation on hexahedral grid cells and recursive subdivision of the cells. The program supports Gouraud-shaded color maps of the data, surface-on-surface maps, and deformation surfaces of vector fields. The execution of the code for animated sweeps is improved by resorting to the cells in the database and maintaining an active set of cells to be rendered.

Kerlick, G. David↗

An Experimental Investigation of the Dynamics of the MSL Rover Landing Event

A developmental test program was conducted for the touchdown event of the Mars Science Laboratory rover. The test hardware consisted of a full-size 3/8th mass scaled test rover, a descent stage mass mock-up, and a Vectran triple-bridle system over 6 meters in length. More than eighty landing tests were performed on terrains of various types, including level rigid surfaces, level and sloped sand surfaces, and level and sloped surfaces with rocks. Landing velocities ranged between 0.4 m/s and 1.4 m/s. A computational model of the landings was developed using the ADAMS analysis program, and validation of this model has been performed through test-analysis comparisons.

Planetary Landing↗

Analysis of Ultra High Resolution Sea Surface Temperature Level 4 Datasets

Sea surface temperature (SST) studies are often focused on improving accuracy, or understanding and quantifying uncertainties in the measurement, as SST is a leading indicator of climate change and represents the longest time series of any ocean variable observed from space. Over the past several decades SST has been studied with the use of satellite data. This allows a larger area to be studied with much more frequent measurements being taken than direct measurements collected aboard ship or buoys. The Group for High Resolution Sea Surface Temperature (GHRSST) is an international project that distributes satellite derived sea surface temperatures (SST) data from multiple platforms and sensors. The goal of the project is to distribute these SSTs for operational uses such as ocean model assimilation and decision support applications, as well as support fundamental SST research and climate studies. Examples of near real time applications include hurricane and fisheries studies and numerical weather forecasting. The JPL group has produced a new 1 km daily global Level 4 SST product, the Multiscale Ultrahigh Resolution (MUR), that blends SST data from 3 distinct NASA radiometers: the Moderate Resolution Imaging Spectroradiometer (MODIS), the Advanced Very High Resolution Radiometer (AVHRR), and the Advanced Microwave Scanning Radiometer ? Earth Observing System(AMSRE). This new product requires further validation and accuracy assessment, especially in coastal regions.We examined the accuracy of the new MUR SST product by comparing the high resolution version and a lower resolution version that has been smoothed to 19 km (but still gridded to 1 km). Both versions were compared to the same data set of in situ buoy temperature measurements with a focus on study regions of the oceans surrounding North and Central America as well as two smaller regions around the Gulf Stream and California coast. Ocean fronts exhibit high temperature gradients (Roden, 1976), and thus satellite data of SST can be used in the detection of these fronts. In this case, accuracy is less of a concern because the primary focus is on the spatial derivative of SST. We calculated the gradients for both versions of the MUR data set and did statistical comparisons focusing on the same regions.

sea surface temperature SST)↗

The effect of the sea breeze circulation on surface ozone levels at Wallops Island, Virginia

Surface measurements of windspeed, direction, and ozone concentration collected at Wallops Island, Virginia, during the summers of 1977 and 1978 are analyzed to study the effects of the dominant mesoscale sea breeze circulation on the local photochemical oxidant levels. A bimodality in the atmospheric dynamics is linked to systematic variations in ozone concentration. It is concluded that during certain phases of the two circulation modes, increased wind speed reduces the resistance of the earth's surface to the deposition of ozone, and decreased ozone concentration levels result. For other phases, light winds occur, signifying high resistance to deposition and high ozone levels. This modulation by the local dynamics is a major impediment for pollutant studies in coastal environments, especially those centering on transport, because it tends to mask other processes that may be occurring.

Parsons, C. L.↗

Illustrating Surface Shape in Volume Data via Principal Direction-Driven 3D Line Integral Convolution

The three-dimensional shape and relative depth of a smoothly curving layered transparent surface may be communicated particularly effectively when the surface is artistically enhanced with sparsely distributed opaque detail. This paper describes how the set of principal directions and principal curvatures specified by local geometric operators can be understood to define a natural 'flow' over the surface of an object, and can be used to guide the placement of the lines of a stroke texture that seeks to represent 3D shape information in a perceptually intuitive way. The driving application for this work is the visualization of layered isovalue surfaces in volume data, where the particular identity of an individual surface is not generally known a priori and observers will typically wish to view a variety of different level surfaces from the same distribution, superimposed over underlying opaque structures. By advecting an evenly distributed set of tiny opaque particles, and the empty space between them, via 3D line integral convolution through the vector field defined by the principal directions and principal curvatures of the level surfaces passing through each gridpoint of a 3D volume, it is possible to generate a single scan-converted solid stroke texture that may intuitively represent the essential shape information of any level surface in the volume. To generate longer strokes over more highly curved areas, where the directional information is both most stable and most relevant, and to simultaneously downplay the visual impact of directional information in the flatter regions, one may dynamically redefine the length of the filter kernel according to the magnitude of the maximum principal curvature of the level surface at the point around which it is applied.

Interrante, Victoria↗