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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2014

Communication: slow relaxation, spatial mobility gradients, and vitrification in confined films

Two decades of experimental research indicate that spatial confinement of glass-forming molecular and polymeric liquids results in major changes of their slow dynamics beginning at large confinement distances. A fundamental understanding remains elusive given the generic complexity of activated relaxation in supercooled liquids and the major complications of geometric confinement, interfacial effects, and spatial inhomogeneity. For this research, we construct a predictive, quantitative, force-level theory of relaxation in free-standing films for the central question of the nature of the spatial mobility gradient. The key new idea is that vapor interfaces speed up barrier hopping in two distinct, but coupled, ways by reducing near surface local caging constraints and spatially long range collective elastic distortion. Effective vitrification temperatures, dynamic length scales, and mobile layer thicknesses naturally follow. In conclusion, our results provide a unified basis for central observations of dynamic and pseudo-thermodynamic measurements.

36 MATERIALS SCIENCE↗
DOE OSTI2019

Theory of Alfvén-slow frequency gaps and discovery of Alfvén-slow eigenmodes in tokamaks

An analytical theory based on the MHD model is presented for understanding the coupling between the shear Alfvén wave and the slow magnetosonic wave (or the so called slow mode) in the frequency range below the Toroidal Alfvén Eigenmode (TAE) continuum spectrum gap. In tokamak plasmas, coupling of the Alfvén m poloidal harmonic and the slow mode m ± 1 harmonics causes the Alfvén m harmonic continuous spectrum to be uplifted from the uncoupled Alfvén spectrum by an amount related to the plasma pressure and the geodesic magnetic field curvature. However, the frequency of one of the slow mode m ± 1 harmonics is reduced by the same pressure-curvature coupling effect. But the frequency of the other slow mode harmonic is relatively unaffected. As a result, the Alfvén-slow (AS) mode continuous spectrum is broken up into two Alfvén-Slow (AS) gaps below the TAE continuum gap. Coupling of the Alfvén m harmonic with the slow mode m ± 2 harmonics also creates additional AS gaps if their frequencies cross each other. The AS gap widths increase with the plasma pressure. The creation of AS gaps allows the existence of several new types of Alfvén-Slow Eigenmodes (ASEs). The radial structure of these new ASEs does not intersect with the continuous spectrum and thus does not suffer from continuum damping. The Beta-induced Alfvén-Acoustic Eigenmode (BAAE) is one type of ASEs with frequency in the lowest AS frequency gap. However, the BAAE usually interacts with the Alfvén-Slow continuum and suffers from continuum damping. The existence of ASEs is ubiquitous for normal and reserve safety factor profiles, broad range of plasma β values, different plasma shapes, and many different toroidal mode numbers. The newly discovered ASEs provide explanation for the experimentally observed Beta-induced Alfvén Eigenmodes destabilized by fast ions with frequencies below the TAE frequency gap.

Cheng, C. Z. (ORCID:0000000166187806)↗
DOE OSTI2018

Fail-Slow at Scale: Evidence of Hardware Performance Faults in Large Production Systems

Fail-slow hardware is an under-studied failure mode. We present a study of 114 reports of fail-slow hardware incidents, collected from large-scale cluster deployments in 14 institutions. We show that all hardware types such as disk, SSD, CPU, memory, and network components can exhibit performance faults. We made several important observations such as faults convert from one form to another, the cascading root causes and impacts can be long, and fail-slow faults can have varying symptoms. From this study, we make suggestions to vendors, operators, and systems designers.

fail-slow↗
DOE OSTI2013

Slow light enhanced singlet exciton fission solar cells with a 126% yield of electrons per photon

Singlet exciton fission generates two triplet excitons per absorbed photon. It promises to increase the power extracted from sunlight without increasing the number of photovoltaic junctions in a solar cell. We demonstrate solar cells with an external quantum efficiency of 126% by enhancing absorption in thin films of the singlet exciton fission material pentacene. The device structure exploits the long photon dwell time at the band edge of a distributed Bragg reflector to achieve enhancement over a broad range of angles. Measuring the reflected light from the solar cell establishes a lower bound of 137% for the internal quantum efficiency.

14 SOLAR ENERGY↗
DOE OSTI2018

Unconventional slowing down of electronic recovery in photoexcited charge-ordered La1/3Sr2/3FeO3

We report the coupled slowing down of electronic and structural dynamics in a charge-ordered antiferromagnetic insulating oxide directly measured in the time domain. Following optical excitation, the recovery time of both transient optical reflectivity and x-ray diffraction intensity from a charge-ordered superstructure in a La1/3Sr2/3FeO3 thin film increases by orders of magnitude when the sample temperature approaches the phase transition temperature. The recovery time becomes much longer than the independently measured lattice cooling time, indicating a nonthermal origin of the slowing down. The combined experimental and theoretical investigations show that the slowing down of electronic recovery corresponds to the pseudo-critical dynamics that originates from magnetic interactions close to a weakly first-order phase transition.

Zhu, Yi↗
DOE OSTI2014

Slowing of Femtosecond Laser-Generated Nanoparticles in a Background Gas

The slowing of Pt nanoparticles in argon background gas was characterized by Rayleigh scattering imaging using a plume of nanoparticles generated by femtosecond laser through thin film ablation (fs-TTFA) of 20 nanometers-thick Pt films. The ablation was performed at threshold laser energy fluences for complete film removal to provide a well-defined plume consisting almost entirely of nanoparticles traveling with a narrow velocity distribution, providing a unique system to unambiguously characterize the slowing of nanoparticles during interaction with background gases. Nanoparticles of ~200 nm diameter were found to decelerate in background Ar gas with pressures less than 50 Torr in good agreement with a linear drag model in the Epstein regime. Based on this model, the stopping distance of small nanoparticles in the plume was predicted and tested by particle collection in an off-axis geometry, and size distribution analysis by transmission electron microscopy. These results permit a basis to interpret nanoparticle propagation through background gases in laser ablation plumes that contain mixed components.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2018

Scalar bispectrum beyond slow-roll in the unified EFT of inflation

We introduce a complete formulation of the scalar bispectrum in the unified effective field theory(EFT) of inflation, which includes the Horndeski and beyond-Horndeski Gleyzes-Langlois-Piazza-Vernizzi classes, in terms of a set of simple one-dimensional integrals. These generalized slow-rollexpressions remain valid even when slow-roll is transiently violated and encompass all configurationsof the bispectrum. We demonstrate analytically that our expressions explicitly preserve the squeezed-limitconsistency relation beyond slow-roll. As an example application of our results, we compute thescalar bispectrum in a model in which potential-driven G-inflation at early times transitions tochaotic inflation at late times, showing that our expressions accurately track the bispectrum whenslow-roll is violated and conventional slow-roll approximations fail

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

A slow neutron polarimeter for the measurement of parity-odd neutron rotary power

We present the design, description, calibration procedure, and an analysis of systematic effects for an apparatus designed to measure the rotation of the plane of polarization of a transversely polarized slow neutron beam as it passes through unpolarized matter. This device is the neutron optical equivalent of a crossed polarizer/analyzer pair familiar from light optics. This apparatus has been used to search for parity violation in the interaction of polarized slow neutrons in matter. Given the brightness of existing slow neutron sources, this apparatus is capable of measuring a neutron rotary power of dϕ/dz = 1 × 10{sup −7} rad/m.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2017

Primordial black holes and slow-roll violation

For primordial black holes (PBH) to be the dark matter in single-field inflation, the slow-roll approximation must be violated by at least O(1) in order to enhance the curvature power spectrum within the required number of efolds between CMB scales and PBH mass scales. Power spectrum predictions which rely on the inflaton remaining on the slow-roll attractor can fail dramatically leading to qualitatively incorrect conclusions in models like an inflection potential and misestimate the mass scale in a running mass model. We show that an optimized temporal evaluation of the Hubble slow-roll parameters to second order remains a good description for a wide range of PBH formation models where up to a 10 7 amplification of power occurs in 10 e-folds or more.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2017

Resonance treatment using pin-based pointwise energy slowing-down method

A new resonance self-shielding method using a pointwise energy solution has been developed to overcome the drawbacks of the equivalence theory. The equivalence theory uses a crude resonance scattering source approximation, and assumes a spatially constant scattering source distribution inside a fuel pellet. These two assumptions cause a significant error, in that they overestimate the multi-group effective cross sections, especially for {sup 238}U. The new resonance self-shielding method solves pointwise energy slowing-down equations with a sub-divided fuel rod. The method adopts a shadowing effect correction factor and fictitious moderator material to model a realistic pointwise energy solution. The slowing-down solution is used to generate the multi-group cross section. With various light water reactor problems, it was demonstrated that the new resonance self-shielding method significantly improved accuracy in the reactor parameter calculation with no compromise in computation time, compared to the equivalence theory.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

Rapid selective sweep of pre-existing polymorphisms and slow fixation of new mutations in experimental evolution of Desulfovibrio vulgaris

To investigate the genetic basis of microbial evolutionary adaptation to salt (NaCl) stress, populations of Desulfovibrio vulgaris Hildenborough (DvH), a sulfate-reducing bacterium important for the biogeochemical cycling of sulfur, carbon and nitrogen, and potentially the bioremediation of toxic heavy metals and radionuclides, were propagated under salt stress or non-stress conditions for 1200 generations. Whole-genome sequencing revealed 11 mutations in salt stress-evolved clone ES9-11 and 14 mutations in non-stress-evolved clone EC3-10. Whole-population sequencing data suggested the rapid selective sweep of the pre-existing polymorphisms under salt stress within the first 100 generations and the slow fixation of new mutations. Population genotyping data demonstrated that the rapid selective sweep of pre-existing polymorphisms was common in salt stress-evolved populations. In contrast, the selection of pre-existing polymorphisms was largely random in EC populations. Consistently, at 100 generations, stress-evolved population ES9 showed improved salt tolerance, namely increased growth rate (2.0-fold), higher biomass yield (1.8-fold) and shorter lag phase (0.7-fold) under higher salinity conditions. The beneficial nature of several mutations was confirmed by site-directed mutagenesis. All four tested mutations contributed to the shortened lag phases under higher salinity condition. In particular, compared with the salt tolerance improvement in ES9-11, a mutation in a histidine kinase protein gene lytS contributed 27% of the growth rate increase and 23% of the biomass yield increase while a mutation in hypothetical gene DVU2472 contributed 24% of the biomass yield increase. Our results suggested that a few beneficial mutations could lead to dramatic improvements in salt tolerance.

Zhou, Aifen↗
DOE OSTI2014

Time-resolved analysis of Fermi gamma-ray bursts with fast- and slow-cooled synchrotron photon models

Time-resolved spectroscopy is performed on eight bright, long gamma-ray bursts (GRBs) dominated by single emission pulses that were observed with the Fermi Gamma-Ray Space Telescope. Fitting the prompt radiation of GRBs by empirical spectral forms such as the Band function leads to ambiguous conclusions about the physical model for the prompt radiation. Moreover, the Band function is often inadequate to fit the data. The GRB spectrum is therefore modeled with two emission components consisting of optically thin non-thermal synchrotron radiation from relativistic electrons and, when significant, thermal emission from a jet photosphere, which is represented by a blackbody spectrum. To produce an acceptable fit, the addition of a blackbody component is required in five out of the eight cases. We also find that the low-energy spectral index α is consistent with a synchrotron component with α = –0.81 ± 0.1. This value lies between the limiting values of α = –2/3 and α = –3/2 for electrons in the slow- and fast-cooling regimes, respectively, suggesting ongoing acceleration at the emission site. The blackbody component can be more significant when using a physical synchrotron model instead of the Band function, illustrating that the Band function does not serve as a good proxy for a non-thermal synchrotron emission component. The temperature and characteristic emission-region size of the blackbody component are found to, respectively, decrease and increase as power laws with time during the prompt phase. In addition, we find that the blackbody and non-thermal components have separate temporal behaviors as far as their respective flux and spectral evolutions.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2017

Generalized slow roll in the unified effective field theory of inflation

In this paper, we provide a compact and unified treatment of power spectrum observables for the effective field theory (EFT) of inflation with the complete set of operators that lead to second-order equations of motion in metric perturbations in both space and time derivatives, including Horndeski and GLPV theories. We relate the EFT operators in ADM form to the four additional free functions of time in the scalar and tensor equations. Using the generalized slow roll formalism, we show that each power spectrum can be described by an integral over a single source that is a function of its respective sound horizon. With this correspondence, existing model independent constraints on the source function can be simply reinterpreted in the more general inflationary context. By expanding these sources around an optimized freeze-out epoch, we also provide characterizations of these spectra in terms of five slow-roll hierarchies whose leading order forms are compact and accurate as long as EFT coefficients vary only on timescales greater than an e-fold. Finally, we also clarify the relationship between the unitary gauge observables employed in the EFT and the comoving gauge observables of the post-inflationary universe.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2017

On Kinetic Slow Modes, Fluid Slow Modes, and Pressure-balanced Structures in the Solar Wind

Observations in the solar wind suggest that the compressive component of inertial-range solar-wind turbulence is dominated by slow modes. The low collisionality of the solar wind allows for nonthermal features to survive, which suggests the requirement of a kinetic plasma description. The least-damped kinetic slow mode is associated with the ion-acoustic (IA) wave and a nonpropagating (NP) mode. We derive analytical expressions for the IA-wave dispersion relation in an anisotropic plasma in the framework of gyrokinetics and then compare them to fully kinetic numerical calculations, results from two-fluid theory, and magnetohydrodynamics (MHD). This comparison shows major discrepancies in the predicted wave phase speeds from MHD and kinetic theory at moderate to high β . MHD and kinetic theory also dictate that all plasma normal modes exhibit a unique signature in terms of their polarization. We quantify the relative amplitude of fluctuations in the three lowest particle velocity moments associated with IA and NP modes in the gyrokinetic limit and compare these predictions with MHD results and in situ observations of the solar-wind turbulence. The agreement between the observations of the wave polarization and our MHD predictions is better than the kinetic predictions, which suggests that the plasma behaves more like a fluid in the solar wind than expected.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1989

The radio signatures of a slow coronal mass ejection - Electron acceleration at slow-mode shocks?

The evolution of a coronal mass ejection (CME) event observed on February 17, 1985 is studied using two-dimensional radio imaging observations along with simultaneously obtained coronagraph observations. This event shows that a slow CME can be associated with type II and type IV radio bursts. The implications of the spatial association of the radio bursts with the CME are discussed. It is argued that the CME is due to an instability of the large-scale magnetic field in a helmet streamer and that the radio bursts are some of the responses to this instability. The new feature of this event is the clear association of the moving type IV burst with a CME traveling slower than the coronal Alfven speed. The structure of slow shocks driven by such a CME is discussed, and it is shown that shock drift and diffusive acceleration are ineffective. An acceleration mechanism involving current-driven lower hybrid waves is proposed.

Kundu, M.↗
DOE OSTI2016

Slow Organic-to-Inorganic Sub-Lattice Thermalization in Methylammonium Lead Halide Perovskites Observed by Ultrafast Photoluminescence

We examine carrier dynamics in polycrystalline methylammonium lead iodide (CH3NH3PbI3) perovskite thin films as functions of temperature and excitation wavelength. At room temperature, long-lived (nanosecond) transient absorption signals indicate negligible carrier trapping. Conversely, in ultrafast photoluminescence, we observe a heretofore unreported large amplitude (50-60%), 45-ps decay process prior to slower recombination. This fast feature persists for temperatures down to the orthorhombic phase transition near 150 K, below which phase coexistence manifests as rapid energy transfer between domains. At 3 K, a transient photoluminescence red-shift indicates formation of bound excitons from photogenerated free carriers with a 16 meV binding energy for the orthorhombic phase. Finally, we show that the fast PL decay component depends on pump photon energy, which we suggest relates excitation of high energy phonon modes associated with the organic component that alters wavefunction overlap. High-level electronic structure and dynamics calculation support the experimental findings. Hence, the fast PL decay relates a characteristic organic-to-inorganic sub-lattice equilibration timescale at optoelectronic-relevant excitation energies.

Chang, Angela Y.↗