Large-scale plane wave shock experiments designed for sample recovery
Prototype explosive assembly for large scale plane wave shock experiments on rock specimen in laboratory
SHOCK WAVE GENERATOR↗
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A study of microkinetic adjustments required to match shock wave experiments and Monte Carlo Direct Simulation for a wide Mach number range
Shock wave thickness predictions from Monte Carlo Direct Simulations, using differential scattering and the Maitland-Smith-Aziz interatomic potential, underpredict experiments as shock Mach numbers increase above about 4. Examination of several sources of data has indicated that at relatively high energies the repulsive portion of accepted potentials such as the Maitland-Smith-Aziz may be too steep. An Exponential-6 potential due to Ross, based on high energy molecular beam scattering data and shock velocity measurements in liquid argon, has been combined with the lower energy portion of the Maitland-Smith-Aziz potential. When this hybrid potential is used in Monte Carlo Direct Simulations, agreement with experiments is improved over the previous predictions using the pure Maitland-Smith-Aziz form.
Pham-Van-diep, Gerald C.↗
Large-scale plane wave shock experiments designed for sample recovery
Planar shock wave test assembly for simulating meteoritic impact on planetary rock surface
METEORITE COLLISION↗
Gasdynamics and shock dynamics of weak shock waves
Experiments in weak-shock dynamics were conducted using a 17-in. diameter shock tube. Weak shocks were generated in air by a compressed nitrogen driver gas; the incident shock waves were brought to a focus by reflecting them from concave cylindrical reflectors at the endwall of the tube. It was found that the behavior of a shock discontinuity at a focus is determined by nonlinear gasdynamic processes. Consideration is also given to nonlinear resonance phenomena, i.e., phenomena associated with oscillatory motion in ducts, with amplitude so large that weak shocks occur. Attention is given to nonlinear resonance in open and closed tubes and to thermal and relaxation effects.
Sturtevant, B.↗
Particle velocity experiments in anorthosite and gabbro
Shock wave experiments were conducted in San Gabriel anorthosite and San Marcos gabbra 10 11 GPa using a 40 mm-borne propellant gun. Particle velocities were measured directly at several points in each target by means of electromagnetic gauges. Hugoniot states were calculated by determining shock-transit time from the gauge records. Sound speeds indicate a loss of shear strength upon sock compression for both rocks, with the strength loss persisting upon release to zero stress om the anorthosite. Stress-density release paths in the anorthosite indicate possible transformation of albite to jadeite + (quartz or coesite), with the amount of material transformed increasing as a function of shock stress. Electrical interferene effects in the gabbro precluded the determination of accurate release paths for the rock.
Boslough, M. B.↗
The role of high pressure experiment and theory in our understanding of gaseous and icy planets
High pressure experiments provide essential data for modeling planetary structure. Shock wave experiments are often especially suitable because they sample the same region of pressure-temperature space that is achieved naturally within the planet during its evolution. A very brief overview of planetary properties is given, followed by a summary of the issues of current interest: the behavior of hydrogen and hydrogen-rich mixtures; C, N, and O at high pressure, and rock-ice mixtures.
Stevenson, David J.↗
Shock wave equation of state of serpentine to 150 GPa - Implications for the occurrence of water in the earth's lower mantle
The shock wave equation of state of Mg end-member serpentine was determined to 150 GPa by examining the shock properties of three polycrystalline serpentines: (1) a lizardite serpentine found near Globe (Arizona), (2) an antigorite serpentine from Thurman (New York), and (3) a chrysotile serpentine from Quebec (Canada). The shock wave experiments were carried out using either a two-stage light gas gun or a 40-mm bore propellant. The shock equation of state that was obtained is shown to exhibit four distinct regions: a low-pressure phase, a mixed phase region, a high-pressure phase, and a very high-pressure phase. The high-pressure density and sound speed of an H2O-rich magnesium silicate determined from these experiments indicate that the observed seismic properties of the lower mantle allow the existence of several weight percent of water in the lower mantle.
Tyburczy, James A.↗
Feasibility studies for light scattering experiments to determine the velocity relaxation of small particles in a fluid
An approach for measuring the non-Markoffian component in the relaxation mechanism of a Brownian particle is proposed which combines desirable features of both the shock wave experiment and conventional light scattering experiments. It is suggested that the radiation pressure generated by a C.W. laser be used to guide an individual spherical particle to terminal velocity. At an appropriate time, the beam intensity is suddenly lowered to a value at which the radiation pressure is negligible, and the ensuing velocity relaxation is measured directly.
Acquista, C.↗
A magma ocean and the Earth's internal water budget
There are lines of evidence which relate bounds on the primordial water content of the Earth's mantle to a magma ocean and the accompanying Earth accretion process. We assume initially (before a magma ocean could form) that as the Earth accreted, it grew from volatile- (H2O, CO2, NH3, CH4, SO2, plus noble) gas-rich planetesimals, which accreted to form an initial 'primitive accretion core' (PAC). The PAC retained the initial complement of planetesimal gaseous components. Shock wave experiments in which both solid, and more recently, the gaseous components of materials such as serpentine and the Murchison meteorite have demonstrated that planetesimal infall velocities of less than 0.5 km/sec, induce shock pressures of less than 0.5 GPa and result in virtually complete retention of planetary gases.
Ahrens, Thomas J.↗
Experimental Shock Transformation of Gypsum to Anhydrite: A New Low Pressure Regime Shock Indicator
The shock behavior of gypsum is important in understanding the Cretaceous/Paleogene event and other terrestrial impacts that contain evaporite sediments in their targets (e.g., Mars Exploration Rover Spirit detected sulfate at Gusev crater, [1]). Most interest focuses on issues of devolatilization to quantify the production of SO2 to better understand its role in generating a temporary atmosphere and its effects on climate and biota [2,3]. Kondo and Ahrens [4] measured induced radiation emitted from single crystal gypsum shocked to 30 and 40 GPa. They observed greybody emission spectra corresponding to temperatures in the range of 3,000 to 4,000 K that are a factor of 2 to 10 times greater than calculated pressure-density energy equation of state temperatures (Hugoniot) and are high enough to melt gypsum. Chen et al. [5] reported results of shock experiments on anhydrite, gypsum, and mixtures of these phases with silica. Their observations indicated little or no devolatilization of anhydrite shocked to 42 GPa and that the fraction of sulfur, by mass, that degassed is approx.10(exp -2) of theoretical prediction. In another report of shock experiments on calcite, anhydrite, and gypsum, Badjukov et al. [6] observed only intensive plastic deformation in anhydrite shock loaded at 63 GPa, and gypsum converted to anhydrite when shock loaded at 56 GPa but have not experimentally shocked gypsum in a step-wise manner to constrain possible incipient transformation effects. Schmitt and Hornemann [7] shock loaded anhydrite and quartz to a peak pressure of 60 GPa and report the platy anhydrite grains were completely pseudomorphed by small crystallized anhydrite grains. However, no evidence of interaction between the two phases could be observed and they suggested that recrystallization of anhydrite grains is the result of a solid-state transformation. They concluded that significant decomposition of anhydrite requires shock pressures higher than 60 GPa. Gupta et al. [8] reanalyzed the calcite and anhydrite shock wave experiments of Yang [9] using improved equations of state of porous materials and vaporized products. They determined the pressures for incipient and complete vaporization to be 32.5 and 122 GPa for anhydrite GPa which is a factor of 2 to 3 lower than reported earlier by Yang [9]. These studies are not in agreement regarding the onset of sulfate decomposition and documentation of shock effects in gypsum is incomplete.
Bell, Mary S.↗
Shockwave determination of the shear velocity at very high pressures
A shock wave experiment is described for confirming changes in density, from seismic interpretation, for determining the properties of planet interiors. The experiment focuses on the problem of measurements in a pressure region, where the shear velocity tends to vanish, or become very small. Pressure-sensitive lattice stability, and the equations for an atomic model of the NaCl lattice are discussed along with the particle velocity shock technique.
Anderson, O. L.↗
A planetary ultra hypervelocity impact mechanics and shock wave science facility
Using the concept of intercepting orbits from a pair of Space Station serviced free flyers, a class of impact and shock wave experiments pertinent to planetary science can be performed. One proposed free flying vehicle is an impactor dispensor, and the second is the impact laboratory. How collision is achieved by utilizing essentially twice orbital velocity is demonstrated. The impactor dispensor contains a series of small flyer plates or other projectiles which are launched into the trajectory of the impactor laboratory at appropriate positions. The impactor laboratory is a large impact tank similar to those in terrestrial gun laboratories, except that it contains a supply of targets and instrumentation such as high speed cameras, flash X-ray apparatus and digital recorders. Shock and isentropic pressures of up to 20 Mbar are achievable with such a system which provides 15 km/sec impact velocities for precisely oriented projectiles.
Ahrens, T. J.↗
A planetary ultra hypervelocity impact mechanics and shock wave science facility
Using the concept of intercepting orbits from a pair of Space Station serviced free flyers, a class of impact and shock wave experiments pertinent to planetary science can be performed. One proposed free flying vehicle is an impactor dispensor, and the second is the impact laboratory. How collision is achieved by utilizing essentially twice orbital velocity is demonstrated. The impactor dispensor contains a series of small flyer plates or other projectiles which are launched into the trajectory of the impactor laboratory at appropriate positions. The impactor laboratory is a large impact tank similar to those in terrestrial gun laboratories, except that it contains a supply of targets and instrumentation such as high speed cameras, flash X-ray apparatus, and digital recorders. Shock and isentropic pressures of up to 20 Mbar are achievable with such a system which provides 15 km/sec impact velocities for precisely oriented projectiles.
Ahrens, Thomas J.↗
Relative Shock Effects in Mixed Powders of Calcite, Gypsum, and Quartz: A Calibration Scheme from Shock Experiments
The shock behavior of calcite and gypsum is important in understanding the Cretaceous/Tertiary event and other terrestrial impacts that contain evaporite sediments in their targets. Most interest focuses on issues of devolatilization to quantify the production of CO2 or SO2 to better understand their role in generating a temporary atmosphere and its effects on climate and biota [e.g., papers in 1,2,3,4]. Devolatilization of carbonate is also important because the dispersion and fragmentation of ejecta is strongly controlled by the expansion of large volumes of gas during the impact process as well [5,6]. Shock recovery experiments for calcite yield seemingly conflicting results: early experimental devolatilization studies [7,8,9] suggested that calcite was substantially outgassed at 30 GPa (> 50%). However, the recent petrographic work of [10,11,12] presented evidence that essentially intact calcite is recovered from 60 GPa experiments. [13] reported results of shock experiments on anhydrite, gypsum, and mixtures of those phases with silica. Their observations indicate little or no devolatilization of anhydrite shocked to 42 GPa and that the fraction of sulfur, by mass, that degassed is approx.10(exp -2) of theoretical prediction. In another (preliminary) report of shock experiments on calcite, anhydrite, and gypsum, [14] observe calcite recrystallization when shock loaded at 61 GPa, only intensive plastic deformation in anhydrite shock loaded at 63 GPa, and gypsum converted to anhydrite when shock loaded at 56 GPa. [15] shock loaded anhydrite and quartz to a peak pressure of 60 GPa. All of the quartz grains were trans-formed to glass and the platy anhydrite grains were completely pseudomorphed by small crystallized anhydrite grains. However, no evidence of interaction between the two phases could be observed and they suggest that recrystallization of anhydrite grains is the result of a solid state transformation. [16] reanalyzed the calcite and anhydrite shock wave experiments of [17] using improved equations of state of porous materials and vaporized products. They determined the pressures for incipient and complete vaporization to be 32.5 and 122 GPa for anhydrite and 17.8 and 54.1 GPa for calcite, respectively, a factor of 2 to 3 lower than reported earlier by [17].
Bell, Mary S.↗
Thermodynamics of dense molecular hydrogen-helium mixtures at high pressure
Effective intermolecular pair potentials derived from liquid hydrogen and helium shock wave experiments are presently used in Monte Carlo simulations of mixtures of hydrogen and helium, at densities of up to 1.2 g/cu cm. The model interaction Helmholtz free energy derived accurately reproduces both the Monte Carlo calculation results and the experimental data obtained for densities of up to about 0.6 g/cu cm. An equation of state is derived from the free energy expression that could be useful in interior models of such Jovian planets as Saturn.
Marley, Mark S.↗
Ultrahigh-pressure melting of lead - A multidisciplinary study
Measurements of the melting temperatures of lead, carried out to pressures of 1 megabar and temperatures near 4000 kelvin by means of a laser-heated diamond cell are in excellent agreement with the results of previous shock-wave experiments. The data are analyzed by means of first principles quantum mechanical calculations, and the agreement documents the reliability of current experimental and theoretical techniques for studies of melting at ultrahigh pressures. These studies have potentially wide-ranging applications from planetary science to condensed matter physics.
Godwal, B. K.↗
The high-pressure melting curve of iron - A technical discussion
The melting curve of iron is reliably determined to 105 GPa using the laser-heated diamond cell, in close agreement with independent measurements using piston-cylinder and large-volume presses or shock-wave experiments. In order to obtain reliable melting data from the internally heated diamond cell, whether by laser or Joule heating, temperature gradients across the sample must be quantitatively measured; otherwise, such 'wire heating' experiments can lead to significant underestimates of the melting temperature and its pressure dependence. The best estimate of the high-pressure melting curve of iron, as derived from the laser-heated diamond cell and Hugoniot temperature measurements, yields melting temperatures of 4800 + or - 200 K and 6700 + or - 400 K at 133 GPa and 243 GPa, respectively.
Williams, Quentin↗
High temperature kinetic study of the reactions H + O2 = OH + O and O + H2 = OH + H in H2/O2 system by shock tube-laser absorption spectroscopy
The reactions: (1) H + O2 = OH + O; and (2) O + H2 = OH + H are the most important elementary reactions in gas phase combustion. They are the main chain-branching reaction in the oxidation of H2 and hydrocarbon fuels. In this study, rate coefficients of the reactions and have been measured over a wide range of composition, pressure, density and temperature behind the reflected shock waves. The experiments were performed using the shock tube - laser absorption spectroscopic technique to monitor OH radicals formed in the shock-heated H2/O2/Ar mixtures. The OH radicals were detected using the P(1)(5) line of (0,0) band of the A(exp 2) Sigma(+) from X(exp 2) Pi transition of OH at 310.023 nm (air). The data were analyzed with the aid of computer modeling. In the experiments great care was exercised to obtain high time resolution, linearity and signal-to-noise. The results are well represented by the Arrhenius expressions. The rate coefficient expression for reaction (1) obtained in this study is k(1) = (7.13 +/- 0.31) x 10(exp 13) exp(-6957+/- 30 K/T) cu cm/mol/s (1050 K less than or equal to T less than or equal to 2500 K) and a consensus expression for k(1) from a critical review of the most recent evaluations of k(1) (including our own) is k(1) = 7.82 x 10(exp 13) exp(-7105 K/T) cu cm/mol/s (960 K less than or equal to T less than or equal to 5300 K). The rate coefficient expression of k(2) is given by k(2) = (1.88 +/- 0.07) x 10(exp 14) exp(-6897 +/- 53 K/T) cu cm/mol/s (1424 K less than or equal to T less than or equal to 2427 K). For k(1), the temperature dependent A-factor and the correlation between the values of k(1) and the inverse reactant densities were not found. In the temperature range of this study, non-Arrhenius expression of k(2) which shows the upward curvature was not supported.
Ryu, Si-Ok↗