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Cr-Be Pushered Single Shell (PSS) Capsule Development

Pushered single shell (PSS) has emerged as an alternative platform of implosion to ease the stability issue at the ablation front. The design consists of a thin inner Be layer, a 50% Cr:Be plateau region, an S-curve gradient, a low Cr (1.5%) tamper layer, and followed by a pure Be outer layer. General Atomics has developed a way to fabricate the higher-Z Cr to lower-Z Be gradients on glow discharge polymer mandrels with a designed S-shape profile for optimal implosion stability using magnetron sputtering. Microstructure analysis of the gradient coating indicated that at lower Cr concentration a short order or amorphous structure was formed. Here, these fabricated PSS capsules were subsequently built into capsule fill tube assemblies, verified to be leak tight at both ambient and cryogenic conditions, and delivered to Lawrence Livermore National Laboratory for the shots. The capsule thermal stability was demonstrated by invariable Cr profiles before and after pyrolysis. However, cracking at inner Cr layers was observed, which has been attributed to thermal stress.

Capsule

Using radiochemistry to diagnose fuel-ablator mix in inertial confinement fusion studies at the National Ignition Facility: measurement of Tc/Mo isotopic ratios for the Pushered Single Shell campaign

The development of radiochemical measurement techniques as a diagnostic for fusion experiments at the National Ignition Facility enables a new method for assessing fuel-ablator mix and the impact of this mix on capsule performance. Diagnosing capsule mix in internal confinement fusion studies is difficult due to the small spatial scales (10s of µm) and short-time frames (100s of ps) over which the mix typically evolves in these experiments. For the Pushered Single Shell campaign, radiochemical measurements on debris collected from fusion experiments can be used to determine isotopic ratios of activation products, particularly 96g Tc/ 99 Mo and 95g Tc/ 99 Mo, to provide vital information on nuclear reactions in the burning plasma that can inform simulations that seek to understand the degree of capsule-fuel mix and the impact on the capsule performance. These radiochemical measurements have been conducted regularly since November 2023 providing data on a range of capsule designs and neutron yields. Data from eight NIF experiments is presented, the measured 96g Tc/ 99 Mo and 95g Tc/ 99 Mo range from (0.5–5) × 10 –4 to (0.3–3) × 10 –4 , respectively. The development of radiochemical diagnostics aids in understanding and optimizing the design of fusion experiments, providing unique and valuable insights into capsule behavior and directly measuring fuel-ablator mix.

and nuclear chemistry

Completion document for MRT 8824 - Upgrade NIF’s gaseous radiochemistry diagnostics (RAGS) to support weapons science

This milestone highlights the successful upgrade and deployment of the Radiochemical Analysis of Gaseous Samples (RAGS) system, which delivers high-quality measurements (<20% uncertainty) of activated gaseous species from NIF implosions. These measurements are critical for supporting Stockpile Stewardship Program (SSP) relevant platforms, including LANL’s Double Shell and LLNL’s Pushered Single Shell campaigns. The RAGS diagnostic technique enables analysis of short-range mixing in implosions using high-Z shells, which are otherwise inaccessible to conventional x-ray diagnostic methods. By facilitating the investigation of high-Z material mixing into fusion burn, this system provides essential data for quantifying and interpreting results in high-energy density (HED) experiments. This report details the physics motivation, diagnostic fundamentals, planned and enacted upgrade work, and the quantification of uncertainty for the upgraded system.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA

Improving indirect-drive ablator performance through pulse shaping and material selection in double shell implosions

The double shell path to inertially confined volumetric thermonuclear burn relies on efficient kinetic energy transfer from an outer ablator shell to an inner shell containing DT fuel at implosion velocities near 250 km/s. In order to experimentally realize adequate compression, target imperfections and assembly features must be tightly controlled. Pulse shape and ablator material are critical design choices that impact all aspects of the implosion. In this article, we evaluate three designs: an Al ablator with single-shock radiation drive, a CH ablator with single-shock drive, and a CH ablator with reduced-adiabat 2-shock drive. All designs use the same W inner (pusher) shell overcoated with a glow discharge polymer tamper and filled with liquid-density DT. One-dimensional HYDRA simulations revealed that the plastic ablator design required the use of the 2-shock drive to match the performance of the Al design. Two-dimensional simulations resolving broadband surface roughness up to modes of several hundred placed only on the ablator showed plastic to greatly outperform Al. The plastic ablator designs did exhibit higher levels of inner shell instability growth when surface roughness was only placed at the pusher/tamper interface, which was mitigated with higher foam cushion densities. A unique and additional benefit of a plastic ablator is also discussed, where heating of the ablator by Au M-band radiation is predicted to rapidly expand the hemi-shell surfaces, closing the equatorial joint gap ahead of the first shock. Taken together, the properties of the plastic ablator for indirect-drive double shell implosions appear promising in removing several long-standing fabrication challenges.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY