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Method and apparatus for efficient operation of optically pumped laser
An optically pumped single mode laser, e.g., Nd:YAG crystal (20) with planoconcave mirrors is increased in efficiency by an order of magnitude to about 8% by optics (25, 27) for focusing the high power multimode output of laser diode arrays (21, 22) into the mode volume (20') of the laser medium (20). A plurality of these optically pumped single mode lasers (1-4) may be cascaded in a ring with dichroic mirrors (M.sub.1 -M.sub.4) at the corners for coupling in the laser diode arrays, each having its own means for spatially tailoring its beam to concentrate pump distribution inside the lasing mode volume of the medium. An InGaAlAs pump diode (30) with its wavelength the same as the lasing medium makes the ring unidirectional.
Method and apparatus for efficient operation of an optically pumped laser
An optically pumped single mode laser, e.g. Nd:YAG crystal (20) with planoconcave mirrors is increased in efficiency by an order of magnitude to about 8% by optics (25, 27) for focusing the high power multimode output of laser diode arrays (21, 22) into the mode volume (20') of the laser medium (20). A plurality of these optically pumped single mode lasers (1-4) may be cascaded in a ring with dichroci mirrors (M.sub.1 -M.sub.4) at the corners for coupling in the laser diode arrays, each having its own means for spatially tailoring its beam to concentrate pump distribution inside the lasing mode volume of the medium. An InGaAlAs pump diode (30) with its wavelength of the same as a lasing medium makes the ring unidirectional. The questions raised in reexamination request No. 90/002,473, filed Oct. 10, 1991, have been considered and the results thereof are reflected in this reissue patent which constitutes the reexamination certificate required by 35 U.S.C. 307 as provided in 37 CFR 1,570(e).
Terahertz Optical Gain Based on Intersubband Transitions in Optically-Pumped Semiconductor Quantum Wells: Coherent Pumped-Probe Interactions
Terahertz optical gain due to intersubband transitions in optically-pumped semiconductor quantum wells (QW's) is calculated nonperturbatively. We solve the pump- field-induced nonequilibrium distribution function for each subband of the QW system from a set of rate equations that include both intrasubband and intersubband relaxation processes. The gain arising from population inversion and stimulated Raman processes is calculated in a unified manner. We show that the coherent pump and signal wave interactions contribute significantly to the THz gain. Because of the optical Stark effect and pump-induced population redistribution, optical gain saturation at larger pump intensities is predicted.
A versatile electrical shutter for optical pumping experiments
Electro-optical shutter for optical pumping experiments using Kerr cell controlled by high voltage modulator
Ultrafast perturbation of magnetic domains by optical pumping in a ferromagnetic multilayer
Ultrafast optical pumping of systems with spatially nonuniform magnetic textures is known to cause far-from-equilibrium spin transport effects, such as the broadening of domain-walls. Here, we study the dynamics of labyrinth domain networks in ferromagnetic CoFe/Ni multilayers subject to a femtosecond optical pump and find an ultrafast domain dilation by 6% within 1.6 ps. This surprising result is based on the unambiguous determination of a harmonically-related shift of ultrafast magnetic X-ray diffraction for the first- and third-order rings. Domain dilation is plausible from conservation of momentum arguments, whereby inelastic scattering from a hot, quasi-ballistic, radial current transfers momentum to the magnetic domains. Our results suggest a potentially rich variety of unexpected physical phenomena associated with far-from-equilibrium inelastic electron-magnon scattering processes in the presence of spin textures.
A path to scaling helium-3 spin-exchange optical pumping
Polarized 3 He has contributed to breakthroughs in particle physics, neutron scattering, and lung imaging, mostly by optical pumping of liter quantities in valved cells or in sealed cells pumped in situ. Only metastability exchange optical pumping currently meets the demand for delivering large quantities of highly polarized 3 He to external volumes. Our development program is under way to achieve medium to large-scale spin-exchange optical pumping of 3 He. Thin-walled aluminosilicate cells placed in contact with thermal reservoirs inside a pressure vessel were optically pumped with kilowatt-scale lasers spectrally narrowed to match pressure-broadened absorption linewidths. We report here the key elements of this program and significant milestones: multi-liter volume valved cells that provide long longitudinal lifetimes that reached polarization as high as 85% inside a thermally stable and pressurized environment.
Studies on Emission Processes in Optically Pumped Mercury Vapor
Electron transitions in optically pumped mercury vapor emission
Magnetic‐Field‐Switchable Laser via Optical Pumping of Rubrene
Abstract Volumetric optical imaging of magnetic fields is challenging with existing magneto‐optical materials, motivating the search for dyes with strong magnetic field interactions, distinct emission spectra, and an ability to withstand high photon flux and incorporation within samples. Here, the magnetic field effect on singlet‐exciton fission is exploited to demonstrate spatial imaging of magnetic fields in a thin film of rubrene. Doping rubrene with the high‐quantum yield dye dibenzotetraphenylperiflanthene (DBP) is shown to enable optically pumped, slab waveguide lasing. This laser is magnetic‐field‐switchable: when operated just below the lasing threshold, application of a 0.4 T magnetic field switches the device between nonlasing and lasing modes, accompanied by an intensity modulation of +360%. This is thought to be the first demonstration of a magnetically switchable laser, as well as the largest magnetically induced change in emission brightness in a singlet‐fission material to date. These results demonstrate that singlet‐fission materials are promising materials for magnetic sensing applications and could inspire a new class of magneto‐optical modulators.
Optical Pumping of Mesospheric Sodium: a New Measurement Capability
The first observation of laser-induced optical pumping in a remote sensing application is reported. We have observed a large variation in the amount of laser light resonantly backscattered from the earth's mesospheric sodium layer depending on the laser polarization. This is consistent with optical pumping of the mesospheric sodium atoms. A new lidar capability is being developed based on measurements of the rethermalization rate of the optically pumped sodium atoms. These measurements have potential applications in the fields of global warming research, spacecraft re-entry, and upper atmospheric dynamics.
Polarizing 3 He via metastability exchange optical pumping using a 1.2 mbar sealed cell at magnetic fields up to 5 T
Here, we report high nuclear polarization of 1.2 mbar 3 He gas in a sealed cell in magnetic fields up to 5 T using Metastability Exchange Optical Pumping (MEOP). The creation of a highly polarized 3 He gas target for use in the 5 T field of Jefferson Lab’s CLAS12 spectrometer would enable new studies of spin-dependent asymmetries on the neutron. We describe a systematic study which was conducted for the first time up to the full 5 T field required for the final target design to evaluate the effects of discharge intensity, pump laser power, and optical pumping transition schemes on nuclear polarization and pumping rates. Steady-state polarizations up to 86% in magnetic fields between 2 and 5 T were achieved, with a discharge-on relaxation time of 898 s at 5 T. These results underscore the potential of MEOP for high-field applications in nuclear physics experiments.
Development of an optically-pumped cesium standard at the Aerospace Corporation
We have initiated a research program to study the performance of compact optically-pumped cesium (Cs) frequency standards, which have potential for future timekeeping applications in space. A Cs beam clock apparatus has been assembled. Basic functions of the frequency standard have been demonstrated. Clock signals are observed with optical pumping schemes using one or two lasers. With two laser pumping, we are able to selectively place up to 80 percent of the atomic population into one of the clock transition states. The observed pattern of clock signal indicates that the velocity distribution of the Cs atoms contributing to the microwave signal is beam-Maxwellian. Thus, in the optically-pumped Cs frequency standards, the entire Cs population in the atomic beam could be utilized to generate the clock signals. This is in contrast to the conventional Cs beam standards where only approx. 1 percent of the atoms in the beam are used. More efficient Cs consumption can lead to improved reliability and increased useful lifetime of the clock. Our preliminary results are summarized in this paper
Elimination of the light shift in rubidium gas cell frequency standards using pulsed optical pumping
Changes in the intensity of the light source in an optically pumped, rubidium, gas cell frequency standard can produce corresponding frequency shifts, with possible adverse effects on the long-term frequency stability. A pulsed optical pumping apparatus was constructed with the intent of investigating the frequency stability in the absence of light shifts. Contrary to original expectations, a small residual frequency shift due to changes in light intensity was experimentally observed. Evidence is given which indicates that this is not a true light-shift effect. Preliminary measurements of the frequency stability of this apparatus, with this small residual pseudo light shift present, are presented. It is shown that this pseudo light shift can be eliminated by using a more homogeneous C-field. This is consistent with the idea that the pseudo light shift is due to inhomogeneity in the physics package (position-shift effect).
Ultrafast perturbation of magnetic domains by optical pumping in a ferromagnetic multilayer
Ultrafast optical pumping of spatially nonuniform magnetic textures is known to induce far-from-equilibrium spin transport effects. Here, we use ultrafast x-ray diffraction with unprecedented dynamic range to study the laser-induced dynamics of labyrinth domain networks in ferromagnetic CoFe/Ni multilayers. We detected azimuthally isotropic, odd order, magnetic diffraction rings up to fifth order. The amplitudes of all three diffraction rings quench to different degrees within 1.6 ps. In addition, all three of the detected diffraction rings both broaden by 15% and radially contract by 6% during the quench process. We are able to rigorously quantify a 31% ultrafast broadening of the domain walls via Fourier analysis of the order-dependent quenching of the three detected diffraction rings. Here, the broadening of the diffraction rings is interpreted as a reduction in the domain coherence length, but the shift in the ring radius, while unambiguous in its occurrence, remains unexplained. In particular, we demonstrate that a radial shift explained by domain-wall broadening can be ruled out. With the unprecedented dynamic range of our data, our results provide convincing evidence that labyrinth domain structures are spatially perturbed at ultrafast speeds under far-from-equilibrium conditions, albeit the mechanism inducing the perturbations remains yet to be clarified.
An optically pumped submillimeter wavelength regenerative amplifier
An optically pumped regenerative submillimeter laser amplifier is described. The amplifier uses a waveguide cavity resonator, and a Fabry-Perot interferometer composed of two dielectric-coated mirrors serves as input and output port for the submillimeter signal. Use of two mirrors enabled obtaining variations of up to 6:1 in transmission by varying the mirror spacing. When the 373-micron transition in CH3CN is excited in the oscillator by the CO2 laser pump beam, the received signal with amplification is about nine times the unamplified signal.
Energy-transfer mechanisms in the CH3F-SF6 optically pumped laser
The power of an optically pumped CH3F laser operating on the 496-micron line has been doubled with the addition of SF6 without any corresponding increase in pump absorption. It is suggested that a near-resonant energy transfer between CH3F and SF6 followed by SF6 deactivation is the mechanism responsible for the enhancement.
Cross modulation of optical rf and microwave signals with optical pumping.
Cross modulation of cesium vapor at radio, microwave and optical frequencies by means of optical pumping
Diode laser 87Rb optical pumping in an evacuated wall-coated cell
The evacuated wall coated sealed cell coupled with diode laser optical pumping offers a number of attractive potential advantages for use in Rb or Cs atomic frequency standards. An investigation of systematic effects is required to explore possible limitations of the technique. The use of diode laser optical pumping of 87 Rb in an evacuated wall coated sealed cell is presented. Experimental results/discussion to be presented include the signal strength and line broadening of the 0 - 0 hyperfine resonance as a function of light intensity for the D1 optical transitions (F - F prime) - (2 1 prime) and (2 - 2 prime), shift of the 0 - 0 hyperfine frequency as a function of laser intensity and de-tuning from optical resonance, and diode laser frequency stabilization techniques.