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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Charge radii of exotic potassium isotopes challenge nuclear theory and the magic character of N = 32

Nuclear charge radii are sensitive probes of different aspects of the nucleon–nucleon interaction and the bulk properties of nuclear matter, providing a stringent test and challenge for nuclear theory. Experimental evidence suggested a new magic neutron number at N = 32 in the calcium region, whereas the unexpectedly large increases in the charge radii open new questions about the evolution of nuclear size in neutron-rich systems. By combining the collinear resonance ionization spectroscopy method with β-decay detection, we were able to extend charge radii measurements of potassium isotopes beyond N = 32. Here we provide a charge radius measurement of 52 K. It does not show a signature of magic behaviour at N = 32 in potassium. The results are interpreted with two state-of-the-art nuclear theories. The coupled cluster theory reproduces the odd–even variations in charge radii but not the notable increase beyond N = 28. This rise is well captured by Fayans nuclear density functional theory, which, however, overestimates the odd–even staggering effect in charge radii. These findings highlight our limited understanding of the nuclear size of neutron-rich systems, and expose problems that are present in some of the best current models of nuclear theory.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

What is ab initio in nuclear theory?

Ab initio has been used as a label in nuclear theory for over two decades. Its meaning has evolved and broadened over the years. We present our interpretation, briefly review its historical use, and discuss its present-day relation to theoretical uncertainty quantification.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Using isotope shift for testing nuclear theory: The case of nobelium isotopes

We calculate field isotope shifts for nobelium atoms using nuclear charge distributions which come from different nuclear models.We demonstrate that comparing calculated isotope shifts with experiment can serve as a testing ground for nuclear theories. It also provides a way of extracting parameters of nuclear charge distribution beyond nuclear root mean square (rms) radius, e.g., parameter of quadrupole deformation β. The measurements of at least two atomic transitions is needed to disentangle the contributions of the changes in deformation and nuclear rms radius into field isotopic shift. We argue that a previous interpretation of the isotope measurements in terms of δ < r 2 > between 252,254 No isotopes should be amended when nuclear deformation is taken into account. As a result, we calculate isotope shifts for other known isotopes and for hypothetically metastable isotope 286 No for which the predictions of nuclear models differ substantially.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Muon capture on Li 6 , C 12 , and O 16 from ab initio nuclear theory

Muon capture on nuclei is one of the most promising probes of the nuclear electroweak current driving the yet-hypothetical neutrinoless double-beta (0νββ) decay. Both processes involve vector and axial-vector currents at finite momentum transfer, q ~ 100 MeV, as well as the induced pseu doscalar and weak-magnetism currents. Comparing measured muon-capture rates with reliable ab initio nuclear-theory predictions could help us validate these currents. To this end, we compute partial muon-capture rates for 6 Li, 12 C and 16 O, feeding the ground and excited states in 6 He, 12 B and 16 N, using ab initio no-core shell model with two- and three-nucleon chiral interactions. Here, we remove the spurious center-of-mass motion by introducing translationally invariant operators and approximate the effect of hadronic two-body currents by Fermi-gas model. We solve the bound-muon wave function from the Dirac wave equations in the Coulomb field created by a finite nucleus. We find that the computed rates to the low-lying states in the final nuclei are in good agreement with the measured counterparts. We highlight sensitivity of some of the transitions to the sub-leading three-nucleon interaction terms. We also compare summed rates to several tens of final states with the measured total capture rates and note that we slightly underestimate the total rate with this simple approach due to limited range of excitation energies

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Testing isospin symmetry breaking in ab initio nuclear theory

In this work we present the first steps towards benchmarking isospin symmetry breaking in ab initio nuclear theory for calculations of superallowed Fermi β decay. Using the valence-space in-medium similarity renormalization group, we calculate b and c coefficients of the isobaric multiplet mass equation, starting from two different Hamiltonians constructed from chiral effective field theory. We compare results to experimental measurements for all T = 1 isobaric analog triplets of relevance to superallowed β decay for masses A = 10 to A = 74 and find an overall agreement within approximately 250 keV of experimental data for both b and c coefficients. A greater level of accuracy, however, is obtained by a phenomenological Skyrme interaction or a classical charged-sphere estimate. Lastly, we show that evolution of the valence-space operator does not meaningfully improve the quality of the coefficients with respect to experimental data, which indicates that higher-order many-body effects are likely not responsible for the observed discrepancies.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Nuclear charge radii of Na isotopes: Interplay of atomic and nuclear theory

The accuracy of atomic theory calculations limits the extraction of nuclear charge radii from isotope shift measurements of odd-proton nuclei. For Na isotopes, though precise spectroscopic measurements have existed for more than half a century, calculations by different methods offer a wide range of values. Here, we present accurate atomic calculations to reliably extract the Na charge radii. By combining experimental matter radii with nuclear coupled-cluster calculations based on nucleon-nucleon and three-nucleon forces, we constrain the parameters obtained from the atomic calculations. Furthermore, this study guides atomic theory and highlights the importance of using accurate atomic and nuclear computations in our understanding of the size of light nuclei.

20 ≤ A ≤ 38↗
DOE OSTI2020

Stringent constraints on neutron-star radii from multimessenger observations and nuclear theory

The properties of neutron stars are determined by the nature of the matter that they contain. These properties can be constrained by measurements of the star’s size. We obtain stringent constraints on neutron-star radii by combining multimessenger observations of the binary neutron-star merger GW170817 with nuclear theory that best accounts for density-dependent uncertainties in the equation of state. We construct equations of state constrained by chiral effective field theory and marginalize over these using the gravitational-wave observations. Combining this with the electromagnetic observations of the merger remnant that imply the presence of a short-lived hypermassive neutron star, we find that the radius of a 1.4 M⊙ neutron star is $R_{1.4M_⊙} = 11.0^{+0.9}_{-0.6} km$ (90% credible interval). Finally, using this constraint, we show that neutron stars are unlikely to be disrupted in neutron star–black hole mergers; subsequently, such events will not produce observable electromagnetic emission.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2026

Computational Workflows for Uncertainty-Quantified Nuclear Reactions: From Nuclear Theory Inputs to Astrophysical Reaction Rates

Reactions on unstable nuclei, particularly those on the neutron-rich side of stability, are important for both fundamental and applied physics. For fundamental science, the most prevalent use case is astrophysi cal nucleosynthesis by rapid neutron capture—the r-process—by which heavy nuclei are formed in extreme astrophysical environments, such as in supernovae and neutron star mergers; see, e.g., Refs. [1–3]. For ap plications, these processes are relevant for the interpretation of radiochemical data from historic nuclear tests, which contribute to our ability to certify the enduring stockpile in the absence of nuclear testing [4]; see Ref. [5] for a broader discussion of applications. However, reaction cross sections involving unsta ble species are generally poorly understood, for the simple reason that useful data become scarce as one moves away from stability. While there are avenues for improving the amount and quality of data for these species [6], one is fundamentally reliant on nuclear theory to make progress on these fields of study.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Toward ab-initio nuclear theory calculations of 𝛿 𝐶

We propose a theory framework to study the isospin-symmetry breaking correction 𝛿 C in superallowed nuclear 𝛽 decays, crucial for the precise determination of |𝑉 𝑢⁢𝑑 |. Based on a general assumptions of the isovector dominance in isospin-symmetry breaking interactions, we construct a set of functions 𝐹 𝑇 𝑧 which involve nuclear matrix elements of isovector monopole operators and the nuclear Green's function. Via the functions 𝐹 𝑇 𝑧 , a connection of 𝛿 C to measurable electroweak nuclear radii is established, providing an experimental gauge of the theory accuracy of 𝛿 C . Here, we outline a strategy to perform ab initio calculations of 𝐹 𝑇 𝑧 based on the Lanczos algorithm, and discuss its similarity with other nuclear-structure-dependent inputs in nuclear 𝛽 decays.

Ab initio calculations↗
DOE OSTI2022

Nuclear Theory from First Principles to Forefront Experiments (Final Report for DE-SC0018638)

The Lee research group is a part of the Nuclear Lattice Effective Field Theory Collaboration, which has developed and performed ab initio lattice simulations of nuclear structure, scattering, reactions, and many-body systems. The other senior members of the collaboration include Ulf-G. Meißner at Bonn/Julich, Evgeny Epelbaum and Hermann Krebs at Bochum, Timo Lahde and Thomas Luu at Julich, and Gautam Rupak at Mississippi State. Our letter “Ab initio alpha-alpha scattering” was featured in a Nature News and Views article. Another letter “Nuclear binding near a quantum phase transition” was highlighted in a Viewpoint article in the online APS journal Physics as well as a news article in the IOP publication Physics World (September 21, 2016). Our letter “Eigenvector continuation with subspace learning” was also highlighted a Synopsis article in Physics. There are many promising ab initio approaches being used to calculate the properties of few-and many-nucleon systems. This includes the no-core shell model, symmetry-adapted no-core shell model quantum Monte Carlo, auxiliary-field diffusion Monte Carlo, self-consistent Green’s functions, many-body perturbation theory, in-medium similarity renormalization group, and coupled cluster methods. Lattice effective field theory is another ab initio approach which combines the framework of effective field theory with lattice Monte Carlo methods to allow favorable scaling from few- to many-body systems. Perhaps the most important aspect of lattice effective field theory is that its strengths and weaknesses are orthogonal to that of other ab initio methods. For example, lattice effective field theory has little difficulty in probing cluster structures and collectivity, while such features are much more difficult using other methods. Furthermore it can be used to compute superfluid condensate fractions as well as the phase diagram of strongly matter and the density and temperature dependence of clustering. Lattice effective field theory was first used in simulations of infinite nuclear matter and infinite neutron matter with pions and without pions. In addition to the efforts by our collaboration, there have been recent efforts by other groups as well.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Quantifying Uncertainties of Microscopic Nuclear Theories

The goal of this project was to produce modernized nuclear data libraries of light ion fusion reactions and actinide fission product yields. Such libraries are essential input in both stockpile science but also fundamental science (nucleosynthesis, superheavy nuclei). When such libraries are used to model complex processes involving exotic, very short-lived nuclei that have not been measured experimentally, the underlying nuclear data come from theoretical models, the predictive power of which needs to be quantified, together with its uncertainties. By teaming up nuclear theorists and statisticians, we built comprehensive theoretical frameworks based on the most fundamental theories of fusion and fission that we coupled for the first time with a Bayesian framework with machine learning techniques for uncertainty quantification. Our results include: (1) statistical emulators for neutron-alpha scattering, and the fission product mass yields of neutron-induced fission of 239 Pu, which will enable developers to generate random realizations of the corresponding data for uncertainty quantification (UQ) in applications; (2) the first complete and most accurate ab initio prediction of the S-factor for proton capture on 7 Be, which – combined with UQ – may become the recommended value at solar energies in the next review of solar fusion cross sections; (3) statistical emulators for fission mass yields in the neutron-induced fission of 239 Pu; (4) the first quantification of how uncertainties in nuclear forces impact fission properties that are relevant in nucleosynthesis simulations to explain how heavy elements are formed in the Cosmos.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Mass measurements of 99–101 In challenge ab initio nuclear theory of the nuclide 100 Sn

The tin isotope 100 Sn is of singular interest for nuclear structure due to its closed-shell proton and neutron configurations. It is also the heaviest nucleus comprising protons and neutrons in equal numbers—a feature that enhances the contribution of the short-range proton–neutron pairing interaction and strongly influences its decay via the weak interaction. Decay studies in the region of 100 Sn have attempted to prove its doubly magic character but few have studied it from an ab initio theoretical perspective, and none of these has addressed the odd-proton neighbours, which are inherently more difficult to describe but crucial for a complete test of nuclear forces. Here we present direct mass measurements of the exotic odd-proton nuclide 100 In, the beta-decay daughter of 100 Sn, and of 99 In, with one proton less than 100 Sn. We use advanced mass spectrometry techniques to measure 99 In, which is produced at a rate of only a few ions per second, and to resolve the ground and isomeric states in 101 In. The experimental results are compared with ab initio many-body calculations. The 100-fold improvement in precision of the 100 In mass value highlights a discrepancy in the atomic-mass values of 100 Sn deduced from recent beta-decay results.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

Dark Matter-Induced Nuclear De-Excitation at SBND with Ab Initio Nuclear Theory

We explore the sensitivity of the Short-Baseline Near Detector (SBND) experiment to light dark matter using MeV-scale electromagnetic activity. Inelastic scattering of dark matter with argon nuclei can excite nuclear states that subsequently de-excite via the emission of MeV-scale photons, producing localized low-energy "blip" signatures in a liquid argon time projection chamber. We perform state-of-the-art ab initio nuclear calculations, including all relevant argon excited states with energies up to 18 MeV, to provide reliable predictions for these signals. After accounting for relevant backgrounds, we find that SBND can probe previously unexplored regions of parameter space for light dark matter.

Dutta, Bhaskar [Bucharest, IFIN-HH; Texas A-M] (OR↗
DOE OSTI2020

Nuclear Theory (Final Technical Report)

This Grant spans a period of 29 years. Achievements of the principal investigator for Task A (F. Iachello), and of the principal investigator for Task B (Y. Alhassid) during this period. Because of the large span in years, the achievements of the P.I. are many, both within the realm of Nuclear Physics and in Interdisciplinary subjects (Hadronic Physics, Molecular Physics, Crystal Physics and Mathematical Physics).

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Discovering the nature of neutrinos: How nuclear theory will advance this grand endeavor. Final report

Why is there more matter than antimatter in the visible universe? Are neutrinos their own antiparticles? These are some of the most profound questions in science. The detection of a (0vββ) neutrinoless doublebeta decay and the measurement of its half-life is one of the most important experimental endeavors in science because it will answer these questions. Paramount to these measurements are accurate predictions with quantified uncertainties of the 0vββ-decay nuclear transitions, especially for the germanium-76 and xeon-136 nuclei, two candidate materials for building the next generation of DOE funded 0vββ-decay experiments. These predictions will guide the Office of Science’s down selection of experiments as well as aid in determining how much material is needed by these experiments. We studied a specific difficult to assess source of uncertainty that will impact coming microscopic predictions, uncertainty which arises from an incomplete yet systematically improvable model of interactions between nucleons and of nucleons with the other particles involved in decay process, referred to as the theory uncertainty. We employed a surrogate model of the germanium-76 nucleus, and its decay products, just detailed enough to adequately mimic the decaying nucleons need for a reasonable measure of this uncertainty and nothing more, avoiding the immense computational expense required in quantifying uncertainties of the full calculation. We found that microscopic calculations of this process can be expected to achieve relative theory uncertainties around 30%, including an unconstrained contribution that had the potential to spoil microscopic calculations. This results in a nearly order of magnitude on previously estimated uncertainties for this rare decay process.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS1989

Testing nuclear theory using the 0.5 ms pulsar

It is argued that a uniformly rotating neutron star with period of 0.5 ms or less may be unable to spin down to become a slowly rotating neutron star if any of the currently proposed equations of state are correct. Asssuming that the neutron star in SN1987A is 'typical' and does not collapse to a black hole as it spins down to a rotational period much larger than 0.5 ms, then its existence may actually invalidate all previously viable nuclear equations of state. An approximate but analytical test that can be used to identify untenable equations of state in the future is proposed.

Shapiro, Stuart L.↗
DOE OSTI2026

Halo Nuclei from Ab Initio Nuclear Theory

A realistic description of halo nuclei, characterized by low-lying breakup thresholds, requires a proper treatment of continuum effects. We have developed an ab initio approach, the No-Core Shell Model with Continuum (NCSMC), capable of describing both bound and unbound states in light nuclei in a unified way. With chiral two- and three-nucleon interactions as the only input, we can predict the structure and dynamics of halo and other light nuclei and, by comparing to available experimental data, test the quality of chiral nuclear forces. We review NCSMC calculations of weakly bound states and resonances of the exotic halo nuclei 6He, 8B, 11Be, and 15C. For the latter, we discuss its production in the capture reaction 14C(n,𝛾 )15C. We highlight the challenges of a description of 6He as a Borromean n-n-4He system. Finally, we present our calculations of excited states in 10Be exhibiting a one-neutron halo structure and a large scale No-Core Shell Model investigation of 11Li as a precursor of a full n-n-9Li NCSMC study.

Navrátil, Petr↗
DOE OSTI2020

Fission of 240 Pu with Symmetry-Restored Density Functional Theory

Nuclear fission plays an important role in fundamental and applied science, from astrophysics to nuclear engineering, yet it remains a major challenge to nuclear theory. Theoretical methods used so far to compute fission observables rely on symmetry-breaking schemes where basic information on the number of particles, angular momentum, and parity of the fissioning nucleus is lost. In this letter, we analyze the impact of restoring broken symmetries in the benchmark case of 240 Pu.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗