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Evaluation of Radiation Transport Through a Nuclear-Grade Sandwich Composite

The development and deployment of microreactors are often synonymous with their transportability; however, designing a shield which is appropriate for both transportation and operations is challenging. A recent approach is the use of composite style shield which combines the reactor pressure vessel and biological shielding into a single unit to enhance the shields effectiveness without degrading the structural properties. To assess the viability of a nuclear grade sandwich composite (NGSC), and understanding of how radiation transports through the shield needs to be understood to select the appropriate materials. This work examines a two-layered NGSC of varying thicknesses with two primary shielding materials (tungsten-tetraboride cermet and boron carbide). To assess the NGSC, quantities of interest including neutron attenuation, photon attenuation, energy deposition, displacements per atom, helium generation, and dose are examined. Altogether, it is found that a combination of both tungsten-tetraboride and boron carbide are necessary to act as an appropriate shield, where the order in which these materials are place in the composite are important to their effectiveness.

22 - GENERAL STUDIES OF NUCLEAR REACTORS↗

Preliminary Analysis of a Nuclear Grade Sandwich Composite for Transportable Micro-Reactor Shielding

Transportable microreactors pose a unique shielding challenge compared with conventional reactors. Many vendors are seeking to transport a microreactor to a site, operate it for a number of years, and then transport it to a secondary site. This involves ensuring the reactor has sufficient shielding during operations and post-irradiation transportation to ensure the safety of those around it, all while ensuring it can be transported via traditional means. This work examines the use of a nuclear grade sandwich composite (NGSC) which seeks to combine the reactor pressure vessel and biological shielding into a single unit. Through this work, it was determined that the NGSC was sufficient to adequately reduce neutron and gamma current exiting the structure to warrant further investigation as a potential shielding option for microreactors.

42 ENGINEERING↗

Streaming in a Nuclear Grade Sandwich Composite for Microreactor Shielding

The NGSC is a new approach to develop a shield structure for microreactors which combines the biological shielding with the reactor pressure vessel. Six layers of SS316 skins and core materials are present in the NGSC, where the core materials are reduce the neutron and gamma dose. Previous work has examined how a simplified NGSC can be optimized for cost, dose, and weight. This work explored the inclusion of SS36 ribs, which helps maintain the structural integrity of the NGSC, affects the transportation of radiation through the NGSC. For B$_4$C layers, the addition of ribs reduces neutron absorption but increase photon absorption. For WB$_4$-cermet layers, the addition of ribs reduces neutron absorption and reduces photon absorption.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Mass Optimization of a Multilayered Shield for Transportable Microreactors

The ability to easily transport microreactors is a major selling point for deploying microreactors to remote areas. However, this creates a unique shielding challenge, especially when the microreactor is being shipped after irradiation. A traditional reactor configuration utilizes a separate biological shield and pressure vessel to meet radiological shielding and pressure needs. The limited space available for transportable microreactors for both shielding and pressure vessels requires a revised assessment of separating out the biological shield and pressure vessel. To address these concerns, we examine a nuclear-grade sandwich composite (NGSC) that combines the reactor pressure vessel and biological shielding functions into a single component. Through a series of optimization problems for both transportation and operational use cases, the NGSC is able to minimize dose, minimize the vessel cost, and ensure that weight requirements are met for transportation. Initial results show that using a tungsten-tetraboride cermet in the first two layers of a six-layer NGSC provides adequate shielding for both use cases. These results show promise that an NGSC has enough overlap between operational and transportation cases to help reduce the design space for future analysis and assessment.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Microstructural Characterization of the Second High Fluence Baffle-Former Bolt Retrieved from a Westinghouse Two-loop Downflow Type PWR

As one of the pressurized water reactor (PWR) internal components, baffle-former bolts (BFBs) are subjected to significant mechanical stress and neutron irradiation from the reactor core during the plant operation. Over the long operation period, these conditions lead to potential degradation and reduced load-carrying capacity of the bolts. In support of evaluating long-term operational performance of materials used in core internal components, the Oak Ridge National Laboratory (ORNL), through the Department of Energy (DOE), Light Water Reactor Sustainability (LWRS) Program, Materials Research Pathway (MRP) has harvested two high fluence BFBs from a commercial Westinghouse two-loop downflow type PWR. The two bolts of interest, i.e. bolts # 4412 and 4416, were withdrawn from service in 2011 as part of a preventative replacement plan. No identification of cracking or potential damage was found for these bolts during their removal in 2011. However, the bolts required a lower torque for removal from the baffle structure than the original torque specified during installation. Irradiation displacement damage levels in the bolts range from 15 to 41 displacements per atom. The goal of this project is to perform detailed microstructural and mechanical property characterization of BFBs following in-service exposures. The information from these bolts will be integral to the LWRS program initiatives in evaluating end of life microstructure and properties. Furthermore, valuable data will be obtained that can be incorporated into model predictions of long-term irradiation behavior and compared to results obtained in high flux experimental reactor conditions. In this report, we present our latest study in FY22 on microstructural characterizations of the second high fluence baffle-former bolt, i.e., bolt # 4412. Analytical electron microscopy and atom probe tomography characterization were performed. The radiation-induced defects in the material add to the large wealth of knowledge for neutron-induced defects in 304/316 grades of stainless steels, specifically for radiation-induced precipitation after high fluence commercial PWR irradiation. The main findings are summarized as follows: 1) The cavity size was considerably larger in the bolt thread section than in the bolt head, with the bolt thread section having a bimodal distribution of cavities greater than ~6 nm in diameter and less than ~3 nm in diameter. The bolt head only had the small-sized cavities. In addition, there was a denuded zone of large cavities near grain boundaries in the thread section of the bolt. 2) Radiation-induced precipitation in the BFB #4412 was highly complex, with the volume fraction, size, and number density of Ni/Si and Cu-rich precipitates depending strongly on the radiation temperature/dose. In many cases, co-precipitates of adjoined clusters were found with Ni/Si-rich precipitates sandwiched between Cu-rich clusters and Mo/Cr/P-rich clusters. 3) Solute segregation out of solution was highest for most solutes in the thread section of the bolt #4412 with the exception of Cu, which experienced more separation out of solution into Curich clusters in the bolt head section. This highlights the difference in the mechanisms for precipitation of Ni/Si clusters, which have the Ni 3 Si phase composition, and precipitation of Cu-rich clusters. 4) There appear to be multiple simultaneous influences that affect the microstructural variation along the length of the bolt that overcomes the ~2X difference in irradiation dose between the bolt head and the bolt thread. The irradiation temperature, thermal/fast neutron ratio variation, potential strain gradient, and exposure to PWR coolant water that each section of the bolt sees may have more influence on the microstructural evolution than the total irradiation dose. The bolt thread and shank, with higher temperature, higher relative fast neutron flux, higher strain, and exposure to coolant but lower dose, underwent more enhanced cavity formation, precipitation, and solute segregation than the bolt head section.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗