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Advancing nuclear forensics competencies at the National Nuclear Center of the Republic of Kazakhstan and conceptual development of a National Nuclear Forensics Library

Since 2021, the National Nuclear Center (NNC) of the Republic of Kazakhstan has been successfully developing a project dedicated to nuclear forensics. The relevance of this project is underscored by Kazakhstan’s leading position in the global uranium mining and export market. The country operates research reactors and is involved in the production of experimental nuclear fuel. The nuclear forensics project is being implemented in several key areas: the project will develop competencies in laboratory research of samples, interpretation of results, and develop a prototype concept for the National Nuclear Forensics Library. In implementing these challenges, the NNC experts draw on the experience of colleagues from world-leading scientific and research centers. Designing a prototype National Nuclear Forensics Library (NNFL) is a challenging project. In conclusion, the solution to this task is based on the IAEA’s approaches, recommendations, and the experience gained from the construction of similar systems in other countries.

and nuclear chemistry

Baryon number violation: from nuclear matrix elements to BSM physics

Processes that violate baryon number, most notably proton decay and $n\bar{n}$ transitions, are promising probes of physics beyond the Standard Model (BSM) needed to understand the lack of antimatter in the Universe. To interpret current and forthcoming experimental limits, theory input from nuclear matrix elements to UV complete models enters. Thus, an interplay of experiment, effective field theory, lattice QCD, and BSM model building is required to develop strategies to accurately extract information from current and future data and maximize the impact and sensitivity of next-generation experiments. Here, we briefly summarize the main results and discussions from the workshop ‘INT-25-91W: Baryon Number Violation: From Nuclear Matrix Elements to BSM Physics,’ held at the Institute for Nuclear Theory, University of Washington, Seattle, WA, 13–17 January 2025.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS

Recommendations to Improve Nuclear Licensing: Update to INL/RPT-23-72206, Recommendations to Improve the Nuclear Regulatory Commission Reactor Licensing and Approval Process

In 2023, various stakeholders had asked for BEA’s thoughts and recommendations to improve the U.S. Nuclear Regulatory Commission’s (NRC) licensing review and approval process. This included an April 14, 2023 request from the House Committee on Energy and Commerce on “information and recommendations to improve the licensing review and approval process, . . . as well as the siting, licensing, construction, and oversight of advanced nuclear reactor technologies.” In response to these requests, BEA prepared and published INL/RPT-23-72206, Recommendations to Improve the Nuclear Regulatory Commission Reactor Licensing and Approval Process (2023 Report). The 2023 Report included 13 recommendations related to streamlining NRC hearings, expediting NRC safety and environmental reviews, otherwise improving NRC licensing, and providing financial benefits to new reactor projects. Many of these earlier recommendations were addressed through various legislative actions or changes made by the NRC. Section 2 of this report addresses the current status of those earlier recommendations. BEA recently received a new request from the House Committee on Energy and Commerce seeking any suggestions for additional areas to examine or potential reforms “that may assist in modernizing the licensing and regulatory process that affects civil nuclear deployment.” Additionally, the new Secretary of Energy has identified initial DOE actions to support unleashing the golden era of American energy dominance, including “Unleash Commercial Nuclear Power in the United States” and “Streamline Permitting and Identify Undue Burdens on American Energy.” Given these developments, BEA has prepared a new set of updated recommendations in this report. The recommendations include updated versions of recommendations from the 2023 Report which have not been fully adopted, as well as entirely new recommendations. This set of recommendations has a slightly broader focus with some recommendations focused on DOE authorizations and some recommendations related to nuclear licensing beyond new reactors. Each recommendation below also identifies whether the recommendation would require legislative action or could be addressed directly by the respective agency.

22 GENERAL STUDIES OF NUCLEAR REACTORS

Extraction of ground-state nuclear deformations from ultrarelativistic heavy-ion collisions: Nuclear structure physics context

The collective-flow-assisted nuclear shape-imaging method in ultrarelativistic heavy-ion collisions (UHICs) has recently been used to characterize nuclear collective states. In this paper, we assess the foundations of the shape-imaging technique employed in these studies. We argue that some current UHIC nuclear imaging techniques neglect fundamental aspects of spontaneous symmetry breaking and symmetry restoration in colliding ions and incorrectly infer one-body multipole moments from studies of nucleonic correlations. Therefore, the impact of this approach on nuclear structure research has been overstated. Conversely, efforts to incorporate existing knowledge on nuclear shapes into analysis pipelines can be beneficial for benchmarking tools and calibrating models used to extract information from ultrarelativistic heavy-ion experiments.

Nuclear data analysis & compilation

The inertial confinement fusion experimental platform and diagnostics for studies of nuclear reactions relevant to nuclear astrophysics

High energy density plasmas generated in laser-driven inertial confinement fusion implosions provide unparalleled laboratory conditions for studying stellar-relevant nuclear reactions: plasma environment; hot and dense; uniquely high achievable neutron flux. These experiments have the potential to address long-standing questions about plasma effects on nuclear reactions hitherto experimentally inaccessible, including nuclear rates with thermally distributed reactants, plasma screening, and reactions involving nuclei in excited states. The National Ignition Facility (NIF) and OMEGA lasers are two primary facilities for executing experiments of this type. Existing and future nuclear diagnostics, along with supporting diagnostics to characterize the platform, enable exploitation of these plasmas for such nuclear astrophysics-relevant experiments. Here, this review describes the nuclear diagnostic capabilities currently available for these types of experiments at the NIF and OMEGA, including neutron time-of-flight spectrometers, charged-particle detectors, gamma detectors and radiochemistry diagnostics, and briefly summarizes other available diagnostic capabilities used for platform characterization. Enabling tools not yet available are also identified, including a rapid radioactive sample retrieval system, a low-energy neutron spectrometer and a high-efficiency gamma spectrometer.

National Ignition Facility

International Nuclear Security Nuclear Material Accounting and Control Instructions for Use and Supplementary Documentation

This document describes the use of exercise kits (called NMAC Kits) developed to support training and technical engagements sponsored by DOE/NNSA Office of Nuclear Security (INS) in the use of nuclear material accounting and control (NMAC) methodologies in support of nuclear security. INS has previously used other similar kits that were originally designed to support NMAC training for international safeguards purposes. These new kits are specifically designed to be used in nuclear security training and emphasis the role NMAC plays in nuclear security as well as security against the insider threat. Planning for the development of these kits is described in LA-UR-24-30063, FY24 NMAC Kits Upgrade and served as the initial framework for the development of the new NMAC Kit material in FY25.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P

Role of Nuclear Science User Facilities (NSUF) in Nuclear Energy Materials Research

The Nuclear Science User Facilities (NSUF) is one of a diverse number of U.S. Department of Energy (DOE) user facilities established to provide researchers with the most advanced tools of modern science. The NSUF is unique and represents a consortium of capabilities distributed across the U.S. at twenty-one institutions. The NSUF is centered at and managed from the Idaho National Laboratory (INL), where it was originally founded, but it coordinates activities at twenty “partner” institutions that include universities, the Center for Advanced Energy Studies (CAES), national laboratories, and a nuclear industry vendor. These institutions have capabilities that include neutron, ion, and gamma irradiation, hot cells, advanced materials characterization equipment, and high-performance computing resources. Many of these capabilities were beyond reach for most researchers before NSUF. The NSUF provides researchers to access these capabilities at no cost to nuclear energy researchers to produce the highest quality research results to increase understanding of advanced nuclear energy technologies important to DOE-NE and support national priorities by adapting to the needs of DOE-NE programs, industry, and new innovative concepts for sustainable nuclear future.

22 GENERAL STUDIES OF NUCLEAR REACTORS

Genetic algorithm optimization of nuclear criticality experiment for reduction of intermediate-energy 239 Pu nuclear data uncertainties

Nuclear criticality experiments are conducted to investigate specific nuclear data important for safe handling and storage of fissile materials, reactor design and operation, and the validation of radiation transport codes. Incorrect or uncertain nuclear data can prohibitively impact operational safety limits, reactor licensing, and predictive simulation capability; therefore, integral measurements from criticality experiments are necessary and should be performed frequently. To maximize the impact of the integral measurements, it is important to consider experiment geometry, material selection, and component dimensions. When taking these considerations into account, the experiment design process becomes iterative and very time intensive. This work utilizes a genetic algorithm to efficiently explore potential nuclear criticality experiment designs for the Laboratory Directed Research & Development project PARADIGM (PARallel Approach of Differential and InteGral Measurements) at Los Alamos National Laboratory. In this paper, the building blocks of the genetic algorithm are discussed in detail, the genetic algorithm methodology is verified, and the genetic algorithm is used to produce three candidate experiment models for the final PARADIGM design. The three candidate models produced by the genetic algorithm consist of copper-reflected assemblies containing 14 repeating units of alumina, graphite, boron, and plutonium plates. Furthermore, in addition to the optimization results, final design considerations are also discussed for designs with a height and/or weight very close to or slightly above assembly machine operational limits.

22 GENERAL STUDIES OF NUCLEAR REACTORS

Automated Resonance Fitting for Nuclear Data Evaluation

Global and national efforts to deliver high-quality nuclear data to users have a wide-ranging impact, affecting applications in national security, reactor operations, basic science, medicine, and more. Cross section evaluation is a major part of this effort, combining theory and experimentation to produce recommended values and uncertainties for reaction probabilities. Resonance region evaluation is a specialized type of nuclear data evaluation that can require significant manual effort and months of time from expert scientists. In this article, non-convex non-linear optimization methods are combined with concepts of inferential statistics to infer a resonance model from experimental data in an automated manner that is not dependent on prior evaluation(s). This methodology aims to enhance the workflow of a resonance evaluator by minimizing time, effort, and the potential for bias from prior assumptions, while enhancing reproducibility and documentation, thereby addressing well-known challenges in the field.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS

DOE Challenges and Opportunities Associated with Accountable Nuclear Material Needs for Development and Commercialization of Fusion Nuclear Energy

Fusion energy represents a transformative opportunity to deliver a safe, plentiful, and carbon-free source of reliable primary power. In recent years, fusion research and development have accelerated significantly, particularly within the US, driven by decades of foundational public investment. Notably, in 2024 the US Department of Energy (DOE) established a comprehensive Fusion Energy Strategy aimed at collaborating with industry partners to enable the deployment of fusion power plants and grid integration by the 2030s. This strategy is chiefly implemented through the DOE Office of Science (SC) Fusion Energy Sciences program. This project was initiated to identify potential approaches for the Office of Environment, Safety, and Health (NA-ESH-12) within DOE’s National Nuclear Security Administration to begin engagement with the fusion community on future accountable material needs. The goal of the project is to inform and influence the supply of and demand for accountable nuclear materials as fusion energy is developed and commercialized. NA-ESH-12 must proactively engage with the fusion community regarding the production and management of accountable nuclear materials. Given the complexity and scale of materials required for research, pilot projects, and eventual commercial reactors, early coordination is vital. The project’s objective is to provide insights that will shape the supply and demand landscape for critical nuclear materials, ensuring that DOE is prepared to effectively support fusion energy development and commercialization. In FY 2025, an initial limited review was conducted to identify the status of the fusion energy community’s progress toward full-scale energy production and the need for accountable nuclear material. This included communications with SC, NA-ESH-12, Savannah River National Laboratory, and Oak Ridge National Laboratory, and attending the Rutgers University–sponsored Supply Chain Workshop: Scaling the Fusion Industry and the International Atomic Energy Agency’s Ninth DEMO Programme Workshop. The review to date indicates that the amounts of tritium, lithium-6, and deuterium required by the fusion industry will be dependent on fuel type, breeding technology, blankets, and R&D improvements. One concern is that the commercial sector does not have a sufficient supply chain to meet the demand for development and commercialization for fusion energy production. The supply and demand estimates for these materials should be routinely reviewed as fusion technologies mature.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY

Benchmark of the Chlorine Worth Study Experiments in Support of Chlorine Nuclear Data Validation for Nuclear Criticality Safety

The Chlorine Worth Study (CWS) was a critical experiment to address an urgent need for thermal chlorine nuclear data validation in plutonium systems. This urgent need is tied directly to plutonium recycle and recovery operations in the plutonium facility at Los Alamos National Laboratory, where exceptionally conservative criticality safety limits are used because no credit is taken for the neutron capture by chlorine. The experiment used weapons-grade plutonium metal plates clad in stainless steel, known as the PANN (plutonium aluminum no nickel) ZPPR (zero power physics reactor) plates. The plutonium was reflected and moderated by high-density polyethylene and included combinations of polyvinyl chloride (PVC) and chlorinated polyvinyl chloride (CPVC) as absorbers. The experiment and benchmark included three configurations mimicking 30 g 239 Pu/L plutonium, 300 g 239 Pu/L plutonium, and 600 g 239 Pu/L plutonium in an aqueous chloride solution. Uncertainties in the benchmark included five broad categories: (1) criticality measurement, (2) mass and density, (3) dimensions, (4) material compositions, and (5) positioning. The largest contribution to the overall uncertainties for all three cases came from the material compositions, in particular the PVC and CPVC absorber compositions. A detailed model was created to be a near match (that is within expectations of transport code users) and a simplified model was created to minimize offset dimensions and expedite modeling for code validation. Sample calculations were completed in MCNP6.3 with ENDF/B-VIII.0 and ENDF/B-VII.1 nuclear data. For the detailed and simplified models, the average difference between the computed and experimental k eff was 951 pcm. CWS will serve as the key validation experiment for nuclear criticality safety in support of aqueous chloride operations. The sensitivity to the chlorine capture cross section is orders of magnitude greater than other existing benchmarks. The current limits, as defined by nuclear criticality safety, are 520 g Pu per batch, i.e. the minimum critical mass of the Pu solution infinitely reflected by water [Criticality Handbook: Volume II, (1969)]. This extremely conservative critical mass limit does not credit any neutron capture by chlorine (in particular neutron capture by 35 Cl) and greatly impedes the throughput required for current and future operations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS

Artificial Intelligence for (AI) Nuclear Security: Expert Perspectives on AI Priorities for the Office of International Nuclear Security

Artificial intelligence (AI) has the potential to transform nuclear security operations, offering opportunities to enhance effectiveness while simultaneously introducing new challenges. As AI technologies rapidly evolve, agencies across the United States Government (USG) are researching, implementing, and evaluating various AI models and systems. Given the broad capabilities and applications of these technologies, it is essential for each agency to identify and articulate those areas where it can make meaningful contributions aligned with its mission and expertise. To address this need for strategic focus, in late Fiscal Year 2025 (FY2025), the Office of International Nuclear Security (INS) established an AI Task Force (AITF) to gather input from subject matter experts (SMEs) regarding the most appropriate role INS could serve in researching, evaluating, or implementing AI for nuclear security. The AITF engaged 15 experts from national laboratories with backgrounds in cyber security, physical security, transport security, insider threat mitigation, nuclear engineering, human-systems engineering, and AI/ML development. This white paper summarizes the insights gathered from these SMEs and presents a potential roadmap for INS engagement with AI technologies. The recommendations outlined here are intended to inform INS leadership as they make strategic decisions about resource allocation and program direction in this rapidly evolving technological domain.

97 MATHEMATICS AND COMPUTING

Advanced Characterization Capabilities for Nuclear Materials via Nuclear Science User Facilities (NSUF)

Advanced post-irradiation examination (PIE) techniques are required to design new or improved nuclear materials, characterize, and understand in-core behavior of fuel and materials, and support the qualification of new reactor materials. The Nuclear Science User Facilities (NSUF) is the U.S. Department of Energy Office of Nuclear Energy's only designated nuclear science user facility. NSUF provides researchers access to PIE capabilities at Idaho National Laboratory and at a diverse mix of university, national laboratory and industrial partner institutions. The PIE capabilities include novel destructive and non-destructive techniques for radiation damage characterization, such as advanced diffraction techniques (X-ray, electron, or neutron) coupled to extreme environments; in-situ observation of microstructural evolution under irradiation; in-situ irradiation to monitor corrosive attack in coolant environments; in-situ irradiation and mechanical testing; and test methods for synergistic effects of superimposed extreme environments (temperature, irradiation, stress, corrosion) on materials behaviors. This talk will provide an overview of NSUF PIE capabilities.

36 MATERIALS SCIENCE

Computational Workflows for Uncertainty-Quantified Nuclear Reactions: From Nuclear Theory Inputs to Astrophysical Reaction Rates

Reactions on unstable nuclei, particularly those on the neutron-rich side of stability, are important for both fundamental and applied physics. For fundamental science, the most prevalent use case is astrophysi cal nucleosynthesis by rapid neutron capture—the r-process—by which heavy nuclei are formed in extreme astrophysical environments, such as in supernovae and neutron star mergers; see, e.g., Refs. [1–3]. For ap plications, these processes are relevant for the interpretation of radiochemical data from historic nuclear tests, which contribute to our ability to certify the enduring stockpile in the absence of nuclear testing [4]; see Ref. [5] for a broader discussion of applications. However, reaction cross sections involving unsta ble species are generally poorly understood, for the simple reason that useful data become scarce as one moves away from stability. While there are avenues for improving the amount and quality of data for these species [6], one is fundamentally reliant on nuclear theory to make progress on these fields of study.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS

Intern Poster Session 08/13: Autonomous Nuclear Robotics: Applications in nuclear waste inspection and hot cell experiments

The nuclear industry is experiencing renewed interest in autonomous robotics, yet most deployed systems remain teleoperated with limited autonomy. This work presents two contributions toward fully autonomous nuclear robotic systems: autonomous waste inspection at the Hanford Site and an autonomous hot cell laboratory framework. Inspections of Hanford's underground waste storage tanks are performed manually at significant cost and personnel exposure. We developed a reinforcement-learning (RL) training pipeline for a custom-built inspection arm. In parallel, we are designing an autonomous laboratory framework for post-irradiation examination in hot cells at the Specimen Preparation Laboratory (SPL) that integrates computer vision, task and motion planning, hardware execution, and operator-in-the-loop control. These systems demonstrate a path toward safer, more efficient nuclear operations by reducing human exposure while maintaining rigorous human oversight at critical decision points.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS

Determining hexavalent chromium transport properties in alkaline nuclear waste using nuclear magnetic resonance spectroscopy

This study focuses on the transport properties of hexavalent chromium, specifically the chromate anion, to improve predictive models and environmental remediation strategies for Cr(VI) migration. Using 53 Cr Nuclear Magnetic Resonance (NMR) spectroscopy, the research quantifies chromate in multicomponent electrolytes replicating nuclear waste conditions at the Hanford Site in Washington State. The consistency of the 53 Cr NMR signal integral with chromate concentration, despite varying matrix compositions, establishes it as a reliable concentration indicator. The transport properties of chromate in an alkaline solution were assessed using relaxation-based measurements via saturation recovery and Carr-Purcell-Meiboom-Gill experiments, determining spin-lattice and spin-spin relaxation times. These measurements, combined with the Bloembergen-Purcell-Pound equation, helped estimate the rotational correlation time and the 53 Cr self-diffusion coefficient using Stokes-Einstein-Debye and Stokes-Einstein equations. Direct measurements were obtained through pulsed field gradient stimulated echo 53 Cr NMR spectroscopy. Monte Carlo simulations further estimated uncertainty propagation. The results enhance comprehension of chromate transport and highlight prospects for identifying transport properties of NMR-active nuclei, traditionally considered unreachable.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W