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Next Generation Noble Liquid Detectors

The research program here combines Generic and Directed R\&D for Liquid Noble Gas detectors for neutrino physics and dark matter. In neutrino physics and dark matter research, we are addressing some of the most fundamental questions in particle physics today by studying these tiny particles in the electron family. To study them, detectors must be large, high precision, and ideally have the ability to collect detailed information from both charge and light from neutrino and dark matter interactions. Precision detection combined with large scales can be challenging. Liquid Argon detectors mitigate some of these challenges given the nature of its interaction medium and it’s relatively inexpensive cost per ton. Significant progress has been made in the last 15 years in developing these kinds of detectors to be built and operated at large scales. However there are still challenges and new ideas in moving these detectors from ton scale to kiloton scale. To be able to get the most out of these kinds of detectors directed questions with respect to specific components running and colleting data in the detectors must be understood. As well, new ideas on how to best combine charge and light measurements may lead to new ways to learn new things with these detectors. Experimental test stands to conduct this work, as is done in this proposal, to accomplish both of these goals are critical to address both of these questions. In the test stand enabled under this grant at Yale University’s Wright lab, new developments in efficient small scale setups were developed, instrumentation developed for running and future experiments (the SBND experiment at Fermilab at present, the DUNE experiment in the future) were and will be tested, and new ideas for charge and light determination for new measurements are under study. The long term impact of this work in neutrino physcis is both for the short and long baseline programs originating at Fermi National Accelerator Laboratory. At long baselines, the US flagship DUNE experiment will measure neutrino properties through neutrino oscillations using a beam originating at Fermilab and a massive LArTPC detector sited about a mile underground at the Sanford Underground Research Facility in Lead, South Dakota. Studies here on the high voltage for thes detectors, and ongoing work on charge and light production and collection in the TPC are relevant for the design and data taking of this and other LArTPC detectors to enable them to best measure the neutrinos created at Fermilab that then pass through the detector in South Dakota. What we learn in these detectors may ultimately change the course of how we understand neutrino’s impact in the early universe. What we learn about how to improve this detection technology and develop new ideas in Lar detectors in general may impact both future neutrino experiments and dark matter experiments.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Rocks, water, and noble liquids: Unfolding the flavor contents of supernova neutrinos

Measuring core-collapse supernova neutrinos, both from individual supernovae within the Milky Way and from past core collapses throughout the Universe (the diffuse supernova neutrino background, or DSNB), is one of the main goals of current and next generation neutrino experiments. Detecting the heavy-lepton flavor (muon and tau types, collectively v x ) component of the flux is particularly challenging due to small statistics and large backgrounds. Further, while the next galactic neutrino burst will be observed in a plethora of neutrino channels, allowing us to measure a small number of v x events, only upper limits are anticipated for the diffuse v x flux even after decades of data taking with conventional detectors. However, paleo detectors could measure the time-integrated flux of neutrinos from galactic core-collapse supernovae via flavor-blind neutral current interactions. In this work, we show how combining a measurement of the average galactic core-collapse supernova flux with paleo detectors and measurements of the DSNB electron-type neutrino fluxes with the next-generation water Cherenkov detector Hyper-Kamiokande and the liquid noble gas detector DUNE will allow to determine the mean supernova vx flux parameters with precision of order ten percent. Realizing this potential requires both the cosmic supernova rate out to z~1 and the integrated Galactic supernova rate over the last ~1 Gyr to be established at the ~10% level.

79 ASTRONOMY AND ASTROPHYSICS↗

Design of a high voltage delivery system for noble liquid time projection chambers

Noble liquid time projection chambers (TPCs) are a leading technology in the detection of ionizing radiation, particularly in applications such as accelerator neutrino physics, dark matter detection, and neutrinoless double beta decay. This work addresses the design considerations for implementing stable high voltage (HV) systems within large noble liquid TPCs, with a focus on the nEXO experiment. Utilizing insights from prior HV research and experimental investigations, we outline factors influencing HV stability and discuss design choices to improve stability and prevent electrical discharges. A novel HV delivery system concept is presented, tailored for the nEXO TPC, which incorporates these design considerations while also meeting the stringent radiopurity requirements of the nEXO neutrinoless double beta decay search. These design considerations and their specific implementation towards a HV delivery system offer guidance to future experiments applying high voltage in noble liquid environments.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Development of Improved Noble Liquid Purity Measurements (Final Technical Report)

The main goal of the Detector R&D project supported by this grant, “Development of Improved Noble Liquid Purity Measurements”, was to perform a scoping study of the feasibility of trapping ions in a liquid argon medium using a radiofrequency (RF) quadrupole trap, and to subsequently use the population of trapped ions to make measurements of the properties of the liquid medium. Using RF quadrupole traps immersed in a noble liquid to trap ions may yield new capabilities to detect and quantify the presence of impurities, as well as enabling other measurements of the microphysics in a noble liquid environment. The major activities undertaken during this project include: the development of a simulation of ions in a liquid argon medium; the designing of a prototype RF quadrupole trap; and the setup of hardware to be used in testing the prototype in vacuum and gas conditions. The summary of these major activities is reported here.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Development of a novel, windowless, amorphous selenium based photodetector for use in liquid noble detectors

Detection of the vacuum ultraviolet (VUV) scintillation light produced by liquid noble elements is a central challenge in order to fully exploit the available timing, topological, and calorimetric information in detectors leveraging these media. Here in this paper, we characterize a novel, windowless amorphous selenium based photodetector with direct sensitivity to VUV light. We present here the manufacturing and experimental setup used to operate this detector at low transport electric fields (2.7–5.2 V/μm) and across a wide range of temperatures (77 K–290 K). This work shows that the first proof-of-principle windowless amorphous selenium device is robust under cryogenic conditions, responsive to VUV light at cryogenic temperatures, and preserves argon purity. These findings motivate a continued exploration of amorphous selenium devices for simultaneous detection of scintillation light and ionization charge in noble element detectors.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Noble Liquid Test Facility at Fermilab

The Noble Liquid Test Facility (NLTF) at Fermilab is a liquid argon detector R\&D facility open to the national and international HEP community. The facility consists of 4 permanent cryostats, ranging from 250L up to 3000L, open space for small open dewar testing, and an optical test stand facility capable of measuring the optical properties of materials and characterizing photon detectors. NLTF’s strongest advantage is its capability to provide ultra-pure LAr in a reliable manner. Its inline filters are capable of filtering all of the three biggest contaminants for standard LAr detectors, O$_2$ and H$_2$O down to $< 1$ppb and N$_2$ $< 1$ppm. This is critical for the users of the test stands as small levels of impurities can dramatically change the efficiency of LArTPCs for the collection of charge and light. The smallest cryostat is mainly used for material testing, a service provided to the international HEP community interested in understanding how the introduction of a specific material might affect the electron lifetime in LAr. The test stands can be equipped with a purity monitor, which allows measuring the electron lifetime in real time, as well as gas sampling and analyzing, and in the near future, local recirculation and filtering. The facility has hosted many successful R\&D projects, which have published their results in well-known journals and talks. A few examples of such projects are: NIR light production in LAr and GAr, the characterization of VUV metalenses, the testing of new filter media capable of filtering N$_2$ from LAr, high voltage studies and direct charge amplification in LAr, and various doping studies.

Blaszczyk, Flor María [Fermilab]↗

Performance of black silicon photodiodes for VUV detection in noble liquids

Black silicon (b-Si) photodiodes are an emerging technology that employs silicon nanostructures to enhance the efficiency of photon detection. Recently, we demonstrated nearly 100% quantum efficiency at <200 nm vacuum ultraviolet (VUV) wavelengths at ambient and in noble liquids, making such devices particularly useful for direct detection of scintillation light in noble liquid detectors. This is important in nuclear science experiments like DarkSide, LUX, XENON, and nEXO, where detection of weak VUV scintillation photons in noble liquids are used to identify rare physics radiation events. Here, we measured the response of b-Si photodiode to the scintillation light generated by alpha particles, all immersed in a LAr and LXe test cell. We established a guideline for future development of b-Si photodetectors with internal gain to reach single-photon sensitivity.

47 OTHER INSTRUMENTATION↗

Snowmass 2021 Scintillating Bubble Chambers: Liquid-noble Bubble Chambers for Dark Matter and CE$\nu$NS Detection

The Scintillating Bubble Chamber (SBC) Collaboration is developing liquid-noble bubble chambers for the quasi-background-free detection of low-mass (GeV-scale) dark matter and coherent scattering (CE$\nu$NS) of low-energy (MeV-scale) neutrinos. The first physics-scale demonstrator of this technique, a 10-kg liquid argon bubble chamber dubbed SBC-LAr10, is now being commissioned at Fermilab. This device will calibrate the background discrimination power and sensitivity of superheated argon to nuclear recoils at energies down to 100 eV. A second functionally-identical detector with a focus on radiopure construction is being built for SBC's first dark matter search at SNOLAB. The projected spin-independent sensitivity of this search is approximately $10^{-43}$ cm$^2$ at 1 GeV$/c^2$ dark matter particle mass. The scalability and background discrimination power of the liquid-noble bubble chamber make this technique a compelling candidate for future dark matter searches to the solar neutrino fog at 1 GeV$/c^2$ particle mass (requiring a $\sim$ton-year exposure with non-neutrino backgrounds sub-dominant to the solar CE$\nu$NS signal) and for high-statistics CE$\nu$NS studies at nuclear reactors.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Cryogenic electronics for noble liquid neutrino detectors

In this paper we present the general features of cryogenic (or “cold”) electronics for noble liquid time projection chambers, with design principles and details for neutrino physics, a brief history of the technology and details of recent research and development that is driving the design of the detectors under construction. Finally, some comments on future R&D envisioned and the impact of this work on other fields is described. “Cold” in the context of this work applies to CMOS devices operated at 77 K and above, at liquids temperatures of LAr (89 K), LKr (125 K) and LXe (165 K), with most of the tests performed in, or at LN 2 (77 K). Additionally, the paper is concentrated on the design of cold electronics for large liquid argon TPCs, those that have been successfully operated, MicroBooNE and ProtoDUNE, and those designed or under construction, such as SBND and DUNE first and second 10 kton modules. The high performance achieved with MicroBooNE and ProtoDUNE – a high signal-to-noise ratio combined with high stability of response – is mainly due to the integral approach to design and construction of sensing electrodes with cold readout electronics in a modular approach with the cryostat signal feed-throughs incorporating warm interface electronics into a Faraday cage with the cryostat. The integral concept is described in some detail in this paper.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Highly efficient photon detection systems for noble liquid detectors based on perovskite quantum dots

Abstract Wavelength shifting photon detection systems (PDS) are the critical functioning components in noble liquid detectors used for high energy physics (HEP) experiments and dark matter search. The vacuum ultraviolet (VUV) scintillation light emitted by these Liquid argon (LAr) and liquid Xenon (LXe) detectors are shifted to higher wavelengths resulting in its efficient detection using the state-of-the-art photodetectors such as silicon photomultipliers (SiPM). The currently used organic wavelength shifting materials [such as 1,1,4,4 Tetraphenyl Butadiene (TPB)] have several disadvantages and are unreliable for longterm use. In this study, we demonstrate the application of the inorganic perovskite cesium lead bromide (CsPbBr 3 ) quantum dots (QDs) as highly efficient wavelength shifters. The absolute photoluminescence quantum yield of the PDS fabricated using these QDs exceeds 70%. CsPbBr 3 -based PDS demonstrated an enhancement in the SiPM signal enhancement by up to 3 times when compared to a 3 µm-thick TPB-based PDS. The emission spectrum from the QDs was optimized to match the highest quantum efficiency region of the SiPMs. In addition, we have demonstrated the deposition of the QD-based wavelength shifting material on a large area PDS substrate using low capital cost and widely scalable solution-based techniques providing a pathway appropriate for meter-scale PDS fabrication and widespread use for other wavelength shifting applications.

47 OTHER INSTRUMENTATION↗

Cryogenic User Facilities for R&D on Noble Liquid Detectors and Low Temperature Devices

Cryogenic test facilities are critical infrastructure for physics experiments in a variety of fields, perhaps most notably for particle detection with noble liquid detectors, low-temperature device development, and quantum information research. However, considerable investment and technical knowledge are required to construct and operate such facilities. This white paper discusses proposals for user facilities aimed at broadening the availability of testing capabilities for the scientific community.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Status of weak scale supersymmetry after LHC Run 2 and ton-scale noble liquid WIMP searches

After completion of LHC Run 2, the ATLAS and CMS experiments had collected of order 139 fb –1 of data at √s = 13 TeV. While discovering a very Standard Model-like Higgs boson of mass m h ≃ 125 GeV, no solid signal for physics beyond the Standard Model has emerged so far at LHC. In addition, no WIMP signals have emerged so far at ton-scale noble liquid WIMP search experiments. For the case of weak scale supersymmetry (SUSY), which is touted as a simple and elegant solution to the gauge hierarchy problem and likely low energy limit of compactified string theory, LHC has found rather generally that gluinos are beyond about 2.2 TeV whilst top squark must lie beyond 1.1 TeV. These limits contradict older simplistic notions of naturalness that emerged in the 1980s–1990s, leading to the rather pessimistic view that SUSY is now excluded except for perhaps some remaining narrow corners of parameter space. Yet, this picture ignores several important developments in SUSY/string theory that emerged in the 21st century: 1. the emergence of the string theory landscape and its solution to the cosmological constant problem, 2. a more nuanced view of naturalness including the notion of “stringy naturalness”, 3. the emergence of anomaly-free discrete R-symmetries and their connection to R-parity, Peccei-Quinn symmetry, the SUSY μ problem and proton decay and 4. the importance of including a solution to the strong CP problem. Rather general considerations from the string theory landscape favor large values of soft terms, subject to the vacuum selection criteria that electroweak symmetry is properly broken (no charge and/or color breaking (CCB) minima) and the resulting magnitude of the weak scale is not too far from our measured value. Then stringy naturalness predicts a Higgs mass m h ~ 125 GeV whilst sparticle masses are typically lifted beyond present LHC bounds. Lastly, in light of these refinements in theory perspective confronted by LHC and dark matter search results, we review the most likely LHC, ILC and dark matter signatures that are expected to arise from weak scale SUSY as we understand it today.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Scintillating Bubble Chambers for Rare Event Searches

The Scintillating Bubble Chamber (SBC) collaboration is developing liquid-noble bubble chambers to detect sub-keV nuclear recoils, allowing the search for low-mass (GeV-scale) dark matter and coherent elastic neutrino-nucleus scattering from low-energy (MeV-scale) neutrinos. The scintillating bubble chamber detectors benefit from the energy reconstruction that the scintillation signal gives in addition to the superior electron-recoil insensitivity that bubble chambers naturally provide. The high level of superheat achievable in noble liquids while being electron-recoil insensitive allows for lower nuclear recoil thresholds than in existing freon-based bubble chambers, potentially reaching the 100 eV threshold desired for reactor CEvNS measurements. To validate this lower threshold, the SBC collaboration is constructing two 10 kg detectors that are functionally identical. The SBC-LAr10, which is being commissioned at Fermilab, is intended for engineering and calibration research and has additional possibilities in assessing coherent elastic neutrino-nucleus scattering in argon. SBC-SNOLAB, the second detector for a low-background dark matter search, will be run at SNOLAB underground.

Pyda, Daniel [Unlisted, US]↗

A Scintillating Xenon Bubble Chamber for Dark Matter Detection. Final Report

This report describes the progress in the search for particle dark matter achieved under DOE award DE-SC0012161, as well as the invention of a new dark matter and neutrino detection technique. Work supported by this award follows in three distinct thrusts: (1) the successful completion of the Generation-1 Direct Detection experiment PICO-60, which set the world-leading limit on the spin-dependent coupling of dark matter to protons and achieved a precise understanding of the response of bubble chambers to nuclear-recoil signals and electron-recoil backgrounds; (2) the construction of the Generation-2 Direct Detection experiment LZ, which will soon be the world's most sensitive dark matter detector; and (3) the demonstration of the first scintillating bubble chamber. The development of a scintillating liquid noble bubble chamber was the primary goal of the proposed work, with the aim of combining the excellent background rejection of a PICO-style bubble chamber with the event-by-event energy resolution of a liquid-noble detector such as LZ. This work produced the first ever observation of coincident scintillation and bubble nucleation by a nuclear recoil in a superheated fluid and also revealed an unexpected benefit to the use of noble liquids in a bubble chamber, namely the ability to increase the degree of superheat by an order of magnitude beyond that achievable in PICO-style detectors while maintaining PICO's world-leading background rejection. This discovery has led to new projects in the US and Canada, developing noble liquid bubble chambers both as detectors for low-mass dark matter and as detectors of coherent elastic neutrino-nucleus scattering (CEvNS) by neutrinos produced at nuclear reactors.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Study of dielectric breakdown in liquid xenon with XeBrA: The xenon breakdown apparatus

Maintaining the electric fields necessary for the current generation of noble liquid time projection chambers (TPCs), with drift lengths exceeding 1 m, requires a large negative voltage applied to their cathode. Delivering such high voltage is associated with an elevated risk of electrostatic discharge and electroluminescence, which would be detrimental to the performance of the experiment. The Xenon Breakdown Apparatus (XeBrA) is a 5-l, high voltage test chamber built to investigate the contributing factors to electrical breakdown in noble liquids. Here, in this work, we present the main findings after conducting scans over stressed electrode areas, surface finish, pressure, and high voltage ramp speed in the medium of liquid xenon. Area scaling and surface finish were observed to be the dominant factors affecting breakdown, whereas no significant changes were observed with varying pressure or ramp speed. A general rise in both the anode current and photon rate was observed in the last 30 s, leading up to a breakdown, with a marked increase in the last couple of seconds. In addition, the position of breakdowns was reconstructed with a system of high-speed cameras and a moderate correlation with the Fowler–Nordheim field emission model was found. Tentative evidence for bubble nucleation being the originating mechanism of breakdown in the liquid was also observed. We deem the results presented in this work to be of particular interest for the design of future, large TPCs, and practical recommendations are provided.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Studies of event burst phenomenon with SiPMs in liquid nitrogen

Silicon photomultiplier (SiPM) are used to collect scintillation photons in many cryogenic noble liquid detectors deployed around the world, such as DarkSide, nEXO, MEGII, ProtoDUNE and DUNE. An event burst phenomenon was observed during routine characterization on many models of SiPMs operated in liquid nitrogen. These bursts of consecutive pulses are initiated by an intense dark photoelectron pulse with an event rate much lower than the time-uncorrelated thermal dark pulse. Although the rate of these burst events is very low, it can potentially compromise some dedicated rare physics event searches which are also anticipated to be of extremely low rate. Here, we systematically studied the behavior of the event burst phenomenon and identified the probable cause of the phenomenon. Here, this investigation is important for the selection of SiPMs for use in noble liquid detectors, high energy physics experiments, and industrial applications where SiPMs are used in cryogenic environment.

47 OTHER INSTRUMENTATION↗

Installation and Commissioning of the SBC-LAr10 Detector at Fermilab

This report describes the progress towards a scalable detector capable of quasi-background-free detection of sub-keV nuclear recoils under DOE award DE-SC0024254. Work supported by this award follows two distinct thrusts: (1) the first calibration of sensitivity to sub-keV nuclear recoils in a liquid-noble bubble chamber, based on data taken in a prototype liquid xenon bubble chamber run previously at Northwestern University, and (2) the successful assembly and installation of the 10-kg liquid argon bubble chamber SBC-LAr10 in the MINOS underground area at Fermilab. These accomplishments have paved the way for the precision calibration of SBC-LAr10 in the MINOS underground area at Fermilab in the coming year, which will use novel calibration techniques to measure the potential of the liquid noble bubble chamber technology for the detection of GeV-scale dark matter particles and the measurement of coherent elastic nuclear scattering by reactor anti-neutrinos (CEvNS).

47 OTHER INSTRUMENTATION↗