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Graphite waste classification and disposal cost estimation for high temperature gas and salt reactors

As high-temperature reactor designs progress to demonstration, managing the radioactive wastes from these systems presents unique challenges. This work explores the irradiated graphite source term produced by three reactor designs: The Modular High Temperature Gas reactor (MHTGR), a pebble-bed High Temperature Gas Reactor (pb-HTGR), and a Fluoride-cooled High-temperature Reactor (FHR). We predicted a C-14 concentration of 4.3 Ci/m 3 for the MHTGR, 1.2 Ci/m 3 for the pebble bed HTGR, and 2.5 Ci/m 3 for the gFHR after 20 years of operation. The final C-14 concentration highly depended on the graphite nitrogen impurity, a major precursor for C-14. The C-14 concentration in all reactor types exceeded the 0.8 Ci/m3 threshold, resulting in a Class C waste classification. The costs associated with accepting the graphite after 20 years in a low-level waste disposal facility were projected to be 255 dollars per kWe for the MHTGR, 248 dollars per kWe for the pb-HTGR, and 56.8 dollars per kWe for the FHR.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Modeling of Prismatic High Temperature Reactors in Pronghorn

Pronghorn is a MOOSE based thermal-hydraulics code developed at Idaho National Laboratory (INL) for advanced nuclear reactor analysis. It has been previously applied to model pebble-bed high temperature reactors (HTRs), liquid-metal cooled reactors, and molten salt reactors, among others. This work leverages the coarse-mesh modeling capabilities in Pronghorn to model the Oregon State University (OSU)'s High Temperature Test Facility (HTTF). The HTTF is a 1:4 height scaled-down facility of General Atomics' Modular High Temperature Gas-cooled Reactor (MHTGR). The facility is primarily built to generate data for code and model validation, and does not precisely replicate MHTGR conditions. Nevertheless, it encompasses the main physics associated with MHTGR transients.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Progress Towards the Validation of a new RELAP5-3D model of the High Temperature Test Facility

Validation is a key step in the development of any type of systems model. As the next generation of reactors approaches, the need for codes that have been validated for these new types of systems continues to grow. An example of a prominent option is the Reactor Excursion Leak Analysis Program (RELAP5-3D), developed by Idaho National Laboratory. This code was developed for the purpose of systems level thermal-hydraulic modeling of light water reactors (LWRS) and postulated transients that can occur in LWRS.RELAP5-3D has been substantially validated against LWR data. Due to its long history as a reactor safety analysis tool, there has been an effort to adapt RELAP5-3D for the purposes of advanced reactor concepts such as prismatic high-temperature gas-cooled reactors (HTGRs). However, RELAP5-3D has not nearly been validated and verified for HTGRs to the degree of LWRs, warranting verification and validation opportunities with computational benchmarks and existing experimental facilities. Examples of such facilities include the modular high-temperature gas-cooled reactor (MHTGR) 350 and the high temperature engineering test reactor (HTTR) from Japan. The MHTGR 350 is a benchmark design concept for code-to-code verification purposes; therefore, it does not provide any experimental data for validation opportunities The HTTR provides useful multiphysics validation data but does not have the in-core instruments to generate thermal-hydraulic experimental data to help with RELAP5-3D validation. Consequently, a facility that could provide key in-core temperatures for thermal-hydraulic validation was still needed. The High Temperature Test Facility (HTTF) is an integral effects facility for HTGR thermal hydraulics developed and operated by Oregon State University. HTTF represents ¼ length scale of the General Atomics MHTGR and is rated for a total power of 2.2 MW. Axially, the core consists of an upper and lower reflector and 10 blocks, numbered from bottom to top (Block 1 is right above lower reflector). The core is heated via graphite resistive heater rods, with respective channels distributed throughout the core. The primary coolant is helium and heat can radiate out of the core to the reactor cavity cooling system (RCCS), which is cooled by water. The primary purpose of the facility is to investigate pressurized conduction cooldown (PCC) and depressurized conduction cooldown (DCC) transients, which are also referred to as the pressurized and depressurized loss of forced cooling respectively. Two experiments were chosen to perform the validation study with a RELAP5-3D model of HTTF. These experiments are PG-27 (PCC) and PG-29 (DCC). These were chosen based off of the quality of available experimental data before and during the experiment which led to their inclusion in the HTGR Thermal Hydraulics Benchmark.

22 - GENERAL STUDIES OF NUCLEAR REACTORS↗

Representativity error scaling of models of the high temperature test facility

Error scaling is a critical step toward the validation of modeling capabilities for high-temperature gas-cooled reactors (HTGRs). Extensive effort is being made to bring HTGRs into the validation basis of numerous thermal-hydraulics codes. Here, this paper demonstrates how systems-level codes can be leveraged to perform error scaling analyses between an experimental facility and a plant-to-be facility. Specifically, we focus on two conduction cooldown experiments from the High Temperature Test Facility (HTTF) and the General Atomics 350 MW th modular high-temperature gas-cooled reactor (MHTGR-350). The error scaling methodology employed in this study is representativity, which in the context of this work was used to quantify how well experiments captured the physics of the plant facility by comparing sensitivity vectors between the two facilities. In addition, two different RELAP5–3D models of the HTTF were included in the comparison to determine if modeling methodologies notably impact the representativity results. The key figures of merit are the maximum block temperature and the coolant outlet temperature. The time-dependent maximum block temperature had a low representativity of below 0.1 for both models across both transients. The coolant outlet temperature had a higher representativity of around 0.6 for both models during the pressurized conduction cooldown, but it was below 0.2 for the depressurized conduction cooldown. Overall, the HTTF experiments were not representative of the transients in the MHTGR-350. However, these results can play a significant role in informing future potential experiments for HTGR systems that iterate on what the HTTF accomplished.

22 - GENERAL STUDIES OF NUCLEAR REACTORS↗

Assessing the Impact of Effective Thermal Conductivity on Gas-cooled Reactor Transients in RELAP5-3D

High-temperature gas-cooled reactors (HTGRs) are a relatively mature advanced reactor concept that are of interest to industry and government for near-term deployment. These systems feature passive safety through low power density, coated particle fuels, and large graphite volumes that lead to slow heatup. In loss of flow transients, cooldown is achieved through conduction and radiation heat transfer. In prismatic block-type reactors, such as the mHTGR-350, the presence of coolant holes and fuel compacts alters the flow of heat through the blocks. To capture this effect in systems codes like RELAP5-3D, relationships for effective thermal conductivity (ETC) must be used to appropriately degrade the thermal conductivity. This work presents an assessment of the impact of ETC on performance of block-type gas-cooled reactors in a pressurized conduction cooldown (PCC) and depressurized conduction cooldown (DCC) transients. Models for PCC and DCC with bulk material thermal conductivity and ETC were run for both the mHTGR-350 and the High-Temperature Test Facility (HTTF) to determine the impact of ETC on transient performance.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

High Fidelity Simulations of Air-Cooled Reactor Cavity Cooling System

Nuclear energy is increasingly acknowledged as pivotal in the global shift towards cleaner energy solutions. Advanced nuclear technologies, including High Temperature Gas-cooled Reactors (HTGRs), stand out as appealing options among Generation IV reactors due to their high temperature heat output and potential for cogeneration. HTGR designs incorporate passive safety systems, such as the Reactor Cavity Cooling System (RCCS), which utilize natural principles to manage heat dissipation from the reactor pressure vessel (RPV) during accidents or routine shutdowns. Regulatory bodies require thorough validation of safety systems like the RCCS to ensure they meet specified standards. Consequently, there is a pressing need within the industry for advanced simulation tools capable of assessing these systems’ performance accurately. There is a knowladge gap in the literature concerning high-fidelity data for the RCCS, which motivates the focus of this study. This research focuses on a specific RCCS designed for the Modular High-Temperature Gas Reactor developed by General Atomics (GA- MHTGR). Experimental studies on a scaled version of the air-cooled RCCS of GA-MHTGR were conducted by the University of Wisconsin-Madison. This work contributes to a broader initiative aimed at establishing a numerical benchmark based on the UW-Madison experiments. As first step we performed high fidelity simulations of the experimental facility setup, to analyze flow physics in such systems and validate NekRS and the MOOSE heat transfer and radiation modules.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

High Fidelity Simulations of Air-Cooled Reactor Cavity Cooling System

High Temperature Gas Reactor (HTGR) designs incorporate passive safety systems (e.g., the Reactor Cavity Cooling System [RCCS]) that utilize natural principles to manage heat dissipation from the reactor pressure vessel (RPV) during accidents or routine shutdowns. The industry community is experiencing a pressing need for advanced simulation tools that can accurately assess the performance of these types of systems. In the literature, a knowledge gap exists concerning high-fidelity data for the RCCS, and this gap is one of the areas of focus of the present study. This research focuses on a specific RCCS designed for General Atomics' Modular High-Temperature Gas Reactor (GA-MHTGR). Experimental studies on a scaled version (can be seen in Figure 1) of the air-cooled RCCS used in GA-MHTGR were conducted by the University of Wisconsin-Madison (UW-Madison). This work contributes to a broader initiative aimed at establishing a numerical benchmark based on the UW-Madison experiments.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Effects of break geometry and orientation on helium-air mixing in simulated reactor cavities of high temperature gas reactors

Here, this study experimentally examined the spatial and temporal variations in air and helium concentrations and temperature fields within simulated reactor cavities of a High Temperature Gas Reactor (HTGR) following helium discharge into an initially air-filled reactor cavity system. Detailed temperature maps were generated using a combination of fiber optics temperature sensor and multiple thermocouple probes within the simulated reactor cavities. The research scenario involved a hypothetical small pipe break in the Reactor Pressure Vessel, resulting in the release of high-temperature helium into the surrounding cavity. A scaled multi-compartment experimental facility, modeled after the General Atomics Modular High Temperature Gas Reactor (GA-MHTGR) design, was constructed for helium and air mixing experiments. Oxygen sensors and thermocouple probes were installed in all five cavities to measure the concentrations of oxygen (or helium) and the temperature distributions of the gas mixture. The experimental findings highlighted the significant impact of the injected helium jet velocity on the gas mixing process and demonstrated how the direction of the helium jet influences the air-helium temperature profiles within the cavities.

Air-ingress↗

Development and Validation of a Probabilistic Risk Assessment Model for a Generic Modular High Temperature Gas-Cooled Reactor

This study looks to develop and validate a probabilistic risk assessment (PRA) model for the modular high temperature gas-cooled reactor (MHTGR) using INL’s Systems Analysis Programs for Hands-on Integrated Reliability Evaluations (SAPHIRE) software. Validation against a General Atomics design involves matching event and fault trees to historical frequencies, with a goal of under 15% difference. The research aims to deliver a reliable PRA model to assess the safety of MHTGRs for use within high-temperature industrial applications.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Investigation of thermal hydraulic behavior of the High Temperature Test Facility's lower plenum via large eddy simulation

A high-fidelity computational fluid dynamics (CFD) analysis was performed using the Large Eddy Simulation (LES) model for the lower plenum of the High–Temperature Test Facility (HTTF), a ¼ scale test facility of the modular high temperature gas-cooled reactor (MHTGR) managed by Oregon State University. In most next–generation nuclear reactors, thermal stress due to thermal striping is one of the risks to be curiously considered. This is also true for HTGRs, especially since the exhaust helium gas temperature is high. In order to evaluate these risks and performance, organizations in the United States led by the OECD NEA are conducting a thermal hydraulic code benchmark for HTGR, and the test facility used for this benchmark is HTTF. HTTF can perform experiments in both normal and accident situations and provide high-quality experimental data. However, it is difficult to provide sufficient data for benchmarking through experiments, and there is a problem with the reliability of CFD analysis results based on Reynolds–averaged Navier–Stokes to analyze thermal hydraulic behavior without verification. To solve this problem, high-fidelity 3-D CFD analysis was performed using the LES model for HTTF. It was also verified that the LES model can properly simulate this jet mixing phenomenon via a unit cell test that provides experimental information. As a result of CFD analysis, the lower the dependency of the sub-grid scale model, the closer to the actual analysis result. In the case of unit cell test CFD analysis and HTTF CFD analysis, the volume-averaged sub-grid scale model dependency was calculated to be 13.0% and 9.16%, respectively. As a result of HTTF analysis, quantitative data of the fluid inside the HTTF lower plenum was provided in this paper. As a result of qualitative analysis, the temperature was highest at the center of the lower plenum, while the temperature fluctuation was highest near the edge of the lower plenum wall. The power spectral density of temperature was analyzed via fast Fourier transform (FFT) for specific points on the center and side of the lower plenum. FFT results did not reveal specific frequency-dominant temperature fluctuations in the center part. It was confirmed that the temperature power spectral density (PSD) at the top increased from the center to the wake. The vortex was visualized using the well-known scalar Q-criterion, and as a result, the closer to the outlet duct, the greater the influence of the mainstream, so that the inflow jet vortex was dissipated and mixed at the top of the lower plenum. Additionally, FFT analysis was performed on the support structure near the corner of the lower plenum with large temperature fluctuations, and as a result, it was confirmed that the temperature fluctuation of the flow did not have a significant effect near the corner wall. In addition, the vortices generated from the lower plenum to the outlet duct were identified in this paper. It is considered that the quantitative and qualitative results presented in this paper will serve as reference data for the benchmark.

97 MATHEMATICS AND COMPUTING↗

Reactor Performance and Safety Characteristics of Beryllium-Based Composite Moderators as Replacements for Graphite in mHTGRs

Here, this study evaluates beryllium-based two-phase composite moderators as an alternative to graphite in an evaluation of reactor performance and safety characteristics. Historically, modular high-temperature gas-cooled reactors (mHTGRs) use graphite as a moderator because of its high moderating ratio and reasonable thermal properties; however, graphite has unfavorable properties under irradiation, which can require component replacement and a significant radioactive waste burden. In this assessment, we explore advanced moderators comprised of magnesium oxide (MgO) as the host matrix and beryllium metal and/or beryllium oxide (Be and/or BeO) as the entrained moderating phase. For the reactor performance and thermal-hydraulic safety analysis, the core design model of the General Atomics mHTGR-350 was used to demonstrate the feasibility of a “drop-in” replacement of graphite using the beryllium-based moderators. We employed the neutronics code Serpent to analyze the moderating behavior of the composite moderators with comparisons drawn to graphite. We performed a scoping analysis of accidents for mHTGRs using RELAP to show that these moderators do not present impediments to safety and are expected to stay within temperature limits. Measured thermophysical properties of the composite moderators are used in the thermal-hydraulic assessments. Our analysis reveals that the two-phase composite MgO-matrix beryllium-based moderators are a suitable replacement for graphite.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

TRISO Burnup-Dependent Failure Analysis of a HTGR Design-Basis Accident Using BISON

Here, this work assesses the failure behavior of the silicon carbide (SiC) layer in TRIstructural ISOtropic (TRISO) fuel particles with BISON during both steady-state and transient conditions for the MHTGR-350 design by General Atomics. A one-dimensional BISON model for a uranium oxycarbide–bearing TRISO is developed to simulate a power level of 50 mW/particles up to 12.4% fissions per initial metal atom (FIMA). Stress predictions for the materials of interest are presented as a function of burnup, along with the SiC failure probability computed using Weibull statistics under the assumption of realistic SiC quality.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Hazards and Probabilistic Risk Assessments of Advanced Nuclear Reactors Coupled with Industrial Facilities

This report provides a roadmap and tool kit for site specific risk assessments across a broad range of industrial customers co-located with advanced nuclear power plants (ANPP) that are not currently built and operating in the U.S. This report builds upon the body of work sponsored by the Department of Energy (DOE) Integrated Energy Systems Pathway that has produced industrial requirements studies and techno-economic assessments on the topics of feasibility of ANPP supported industrial processes. This report also leverages the DOE Light Water Reactor Sustainability (LWRS) program that has presented hazards assessment and generic probabilistic risk assessments (PRAs) for the addition of a heat extraction system (HES) to light-water reactors (LWRs) co-located with hydrogen production facilities. Many of the hazard assessments and risk assessments performed for the LWRS report are agnostic to whether the nuclear reactor is an ANPP or were adapted to the ANPP focus. The report performs hazards assessments to include industrial facilities: an oil refinery, a methanol plant, a synthetic fuel (synfuel) plant, the production of synthetic gas (syngas) as part of the methanol and synfuel plants, wood pulp and paper mills, and hydrogen production. Hydrogen production facilities are assessed in depth through prior reports in the LWRS program and the results are leveraged in this report. All these facilities are specified through industrial process and requirements research performed by national laboratories, universities, and interaction with industry. Many of the processes used in this report are pre-conceptual designs to use for decarbonization of the current technology facilities. A process of failure modes and effects analysis (what can go wrong) and accidentology (what has historically gone wrong) was used to determine the hazards presented to the nuclear power plant by the addition of the HES and the industrial customer. Chemical properties of feedstocks and products are summarized as part of the hazards assessment. Example analysis procedures are provided for each of the hazard types identified. These deterministic analyses can be used to assess adherence to licensing criteria. They can also be used to meet other safety goals like protection of the public, workers, or industrial facility equipment. A modular high temperature gas-cooled reactor (MHTGR) PRA only existing on paper was modeled and verified in modern PRA software. This will provide a tool for representative ANPP probabilistic analyses for future research.

10 SYNTHETIC FUELS↗

Towards a Benchmark Experiment with the Compact Nuclear Power Source

The Compact Nuclear Power Source (CNPS) was a high-assay low enriched uranium (HALEU) tristructural isotropic (TRISO)-fueled, graphite-moderated microreactor constructed in 1987 at Los Alamos National Laboratory. The reactor, conceived as a power source for short-range radar stations, was designed to be "walk-away safe," and was cooled by heat pipes and ambient air. Though the project was formally cancelled after the fuel and moderator material had been received, its potential to meaningfully advance the body of critical and integral data was evident, and critical experiments with a mock-up of the reactor proceeded at TA-18 until its disassembly in 1991. The reflector and some components of the core would later go on to see service as part of the New Production Reactor Modular High-Temperature Gas-Cooled Reactor (NP-MHTGR) critical experiments. In light of the progress made by groups like Westinghouse and X-Energy towards contemporary graphite-moderated microreactors, the system remains an attractive candidate for the basis of a benchmark experiment even today. Uncertainties remain, however, in some features of the system–inconsistencies in the dimensions and composition of the reactor’s components as described in literature and implemented in current computational models. The identification, quantification, and to the extent possible, the minimization of these uncertainties is a crucial task on the path towards creating a benchmark based on the CNPS system. The present work seeks to initiate this process with a survey of available documentation and improvements to the accuracy of CNPS neutronics models.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

INL Contributions to Draft HTTF Benchmark Specifications

The High-Temperature Test Facility (HTTF) is an integral effects thermal hydraulics test facility at Oregon State University designed as a 1/4 length scale model of the Modular High-Temperature Gas-Cooled Reactor 350 MW core (mHTGR-350). In the spring and summer of 2019, several experiments were conducted at HTTF providing a valuable source of gas-cooled reactor thermal hydraulics data. Idaho National Laboratory (INL), Oregon State University, Argonne National Laboratory, and Canadian Nuclear Laboratories have partnered to use this experimental data to develop a gas-cooled reactor thermal hydraulics benchmark led by INL under the auspices of the Advanced Reactor Technologies (ART) program. This report provides some context on the benchmark, HTTF, and previous Reactor Excursions and Leak Analysis Program (RELAP)5-3D modeling of HTTF. It also provides a draft of the benchmark specifications for the Depressurized Conduction Cooldown problem, which is the INL-led benchmark problem.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

RAVEN Template for Dynamic Representativity Analysis of the High Temperature Test Facility

These slides present a walkthrough of the template that has been developed for using RAVEN to perform representativity analysis using models of the High Temperature Test Facility and the General Atomics Modular High Temperature Gas-cooled Reactor. The presentation provides participants in the HTTF benchmark with a walkthrough on how to use RAVEN for their sensitivity analysis and how to read results from the MHTGR-350 to perform representativity

22 - GENERAL STUDIES OF NUCLEAR REACTORS↗