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16 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Melting of magnesium oxide up to two terapascals using double-shock compression

Constraining the melting behavior of magnesium oxide, a major constituent of gaseous and rocky planets, is key to benchmarking their evolutionary models. Using a double-shock technique, we extended the MgO melt curve measurements to 2 TPa; this is twice the pressure achieved by previous melting experiments on any material. A temperature plateau is observed between 1218 and 1950 GPa in the second shock states, which is attributed to latent heat of melting. At 1950 GPa, the measured melting temperature is 17,600 K, 17% lower than recent theoretical predictions. Furthermore, the melting curve is steeper than that of MgSiO 3 , indicating that MgO is likely solid in the interior of Saturn-sized gas giants and extra-solar super-Earth planets.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Diamond formation in double-shocked epoxy to 150 GPa

We present measurements of diamond formation in doubly shocked Stycast 1266 epoxy (comprising C, H, Cl, N, and O) using in situ x-ray diffraction. Epoxy samples were reshocked against a LiF window to pressures between 80 and 148 GPa in experiments at the Omega Laser Facility. Furthermore, the pressure and temperature conditions were diagnosed in situ using velocimetry and optical pyrometry, respectively. X-ray diffraction patterns of the compressed epoxy are consistent with cubic diamond (Fd3¯m), indicating that diamond can precipitate not only from twice-shocked CH polystyrene [Kraus et al. Nat. Astron. 1, 606 (2017)] at these conditions but also from twice-shocked CH polymers with the addition of oxygen, nitrogen, and chlorine. These results, in combination with previous works on CH, CH 2 , CH 4 , and methane hydrate, support that diamond often, but not always, forms from CH-based compounds at extreme pressures and temperatures, indicating that the chemical composition, thermodynamic compression path, and kinetics play an important role.

36 MATERIALS SCIENCE↗
NASA NTRS1972

Interplanetary double-shock ensembles with anomalous electrical conductivity

Similarity theory is applied to the case of constant velocity, piston-driven, shock waves. This family of solutions, incorporating the interplanetary magnetic field for the case of infinite electric conductivity, represents one class of experimentally observed, flare-generated shock waves. This paper discusses the theoretical extension to flows with finite conductivity (presumably caused by unspecified modes of wave-particle interactions). Solutions, including reverse shocks, are found for a wide range of magnetic Reynolds numbers from one to infinity. Consideration of a zero and nonzero ambient flowing solar wind (together with removal of magnetic considerations) enables the recovery of earlier similarity solutions as well as numerical simulations. A limited comparison with observations suggests that flare energetics can be reasonably estimated once the shock velocity, ambient solar wind velocity and density, and ambient azimuthal Alfven Mach number are known.

Dryer, M.↗
DOE OSTI2026

Efficacy of Gadolinium Gallium Garnet (GGG) as a High-Impedance Optical Window for Shock Wave Experiments

We conducted a series of plate impact experiments to examine the efficacy of < 111>-oriented gadolinium gallium garnet (GGG) single crystals as high-impedance optical window for Photonic Doppler velocimetry (PDV) under shock and double-shock loading. At ~ 123 GPa, shocked GGG remains fully transparent to 1550 nm light for at least 250 ns without any signal degradation. Above 135 GPa, PDV data measured through GGG exhibit a gradual loss of fringe contrast following shock entrance, which eventually leads to transparency loss. The duration for which shocked GGG remains transparent decreases with increasing pressure, and at ~ 148 GPa, it becomes opaque within ~ 20–30 ns. This limits the use of GGG as an interferometry window between ~ 110–140 GPa under single shock loading. Within this pressure range, the refractive index of GGG increases linearly with density: n = 1.552 + 0.054ρ. In contrast to single shock loading, where GGG becomes opaque rapidly above ~ 140 GPa, double-shocked GGG remains optically transparent for over 100 ns when it is first shocked to ~ 123 GPa and then reshocked to significantly higher pressures (215–233 GPa). Our findings raise the exciting possibility of GGG being used as a high-impedance optical window in multi-shock and shock-ramp loading experiments.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS1972

Pioneer 7 observations of the August 29, 1966, interplanetary shock-wave ensemble.

The detailed plasma (except for electrons) and magnetic field data from Pioneer 7 are presented for a proposed double-shock ensemble. The Ames Research Center plasma probe data are compared with that of the MIT probe. These data are compared with MHD theory to show that the discontinuities themselves satisfy the magnetic Hugoniot equations. The data are also compared with the theoretical predictions for the double-shock structure. The theory requires as input only the forward shock velocity, the original ambient solar wind conditions, and a reasonable assumption regarding the density and azimuthal magnetic field in the 'new' solar wind which is detected after passage of the reverse shock. A unique solution is then obtained for the theoretical piston and reverse shock positions as well as for the temporal plasma behavior for both infinite and finite electrical conductivities.

Dryer, M.↗
NASA NTRS1979

Second sound shock waves and critical velocities in liquid helium 2

Large amplitude second-sound shock waves were generated and the experimental results compared to the theory of nonlinear second-sound. The structure and thickness of second-sound shock fronts are calculated and compared to experimental data. Theoretically it is shown that at T = 1.88 K, where the nonlinear wave steepening vanishes, the thickness of a very weak shock must diverge. In a region near this temperature, a finite-amplitude shock pulse evolves into an unusual double-shock configuration consisting of a front steepened, temperature raising shock followed by a temperature lowering shock. Double-shocks are experimentally verified. It is experimentally shown that very large second-sound shock waves initiate a breakdown in the superfluidity of helium 2, which is dramatically displayed as a limit to the maximum attainable shock strength. The value of the maximum shock-induced relative velocity represents a significant lower bound to the intrinsic critical velocity of helium 2.

Turner, T. N.↗
DOE OSTI2022

Simulation and analysis of the 3D double shock-induced recompression of spall using a hybrid PAGOSA with FLIP+MPM

In this work, an innovative hybrid algorithm PAGOSA with FLIP + MPM is first presented by coupling PAGOSA with the particle FLIP + MPM, and applied to systematically exploring the 3D recompression of spall induced by double-shock waves in ductile materials as the few existing studies are currently limited to the pure longitudinal recompression of spall, and ignore the 3D effects. This algorithm solves the difficulties the grid-based methods encounter when applied to capturing the fracture in material. We first validate the capabilities of PAGOSA with FLIP + MPM to predict different fracture/fragmentation cases by solving two benchmark problems and comparing with the analytical solutions or the experiment results. The convergences and the infinity-norm errors are also investigated. Subsequently, the 3D effects are demonstrated by simulating the spallation in material using PAGOSA with FLIP + MPM and comparing with those in the longitudinal cases. Additionally, some factors that affect the spallation with 3D effects are also discussed. Finally, the recompressions of spall in material with/without 3D effects are systematically simulated and analyzed. The recompression of spall driven by a high explosive is also simulated to show the ability of PAGOSA with FLIP + MPM to handle this kind of problem. The conditions that can lead to a recompression of spall are explored. Also, numerical results show that PAGOSA with FLIP + MPM can accurately predict different fracture cases, that the 3D effects play an important role in fracture/fragmentation, and the recompression of spall is very sensitive to the occurrence conditions, shows great differences when considering 3D effects in real applications. Moreover, the present hybrid method can be easily extended to other grid-based techniques employed for fracture in materials.

3D effects↗
DOE OSTI2020

Dynamic experiments to study the α - ε phase transition in cerium

The ability to understand and predict the response of matter at extreme conditions requires knowledge of a material’s equation-of-state including the location of phase boundaries, transition kinetics, and the evolution of material strength. Cerium is a material with a complex phase diagram that continues to attract significant scientific interest. Recent dynamic experiments have provided information on the low-pressure γ–α phase transition, sound speed, and Hugoniot data for the higher-pressure α phase, as well as the incipient shock melt transition. Despite these efforts, there are still regions of the phase diagram that are largely unexplored dynamically, including the high-pressure region below the melt boundary. Along a room temperature isotherm, diamond anvil cell data report a transition to the ϵ phase between 13 and 17 GPa. At higher temperatures, similar diamond anvil cell data show significant disagreement regarding the existence, location, and slope of the ϵ-phase boundary. In this work, double-shock loading was used to access the α–ϵ region of the phase diagram to obtain equation-of-state information and to determine the location of the ϵ-phase boundary for shock loading.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2024

Extreme Metastability of Diamond and its Transformation to the BC8 Post-Diamond Phase of Carbon

Diamond possesses exceptional physical properties due to its remarkably strong carbon–carbon bonding, leading to significant resilience to structural transformations at very high pressures and temperatures. Despite several experimental attempts, synthesis and recovery of the theoretically predicted post-diamond BC8 phase remains elusive. Through quantum-accurate multimillion atom molecular dynamics (MD) simulations, we have uncovered the extreme metastability of diamond at very high pressures, significantly exceeding its range of thermodynamic stability. We predict the post-diamond BC8 phase to be experimentally accessible only within a narrow high pressure–temperature region of the carbon phase diagram. The diamond to BC8 transformation proceeds through premelting followed by BC8 nucleation and growth in the metastable carbon liquid. Here we propose a double-shock compression pathway for BC8 synthesis, which is currently being explored in experiments at the National Ignition Facility.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Release dynamics of nanodiamonds created by laser-driven shock-compression of polyethylene terephthalate

Laser-driven dynamic compression experiments of plastic materials have found surprisingly fast formation of nanodiamonds (ND) via X-ray probing. This mechanism is relevant for planetary models, but could also open efficient synthesis routes for tailored NDs. We investigate the release mechanics of compressed NDs by molecular dynamics simulation of the isotropic expansion of finite size diamond from different P-T states. Analysing the structural integrity along different release paths via molecular dynamic simulations, we found substantial disintegration rates upon shock release, increasing with the on-Hugnoiot shock temperature. We also find that recrystallization can occur after the expansion and hence during the release, depending on subsequent cooling mechanisms. Our study suggests higher ND recovery rates from off-Hugoniot states, e.g., via double-shocks, due to faster cooling. Laser-driven shock compression experiments of polyethylene terephthalate (PET) samples with in situ X-ray probing at the simulated conditions found diamond signal that persists up to 11 ns after breakout. In the diffraction pattern, we observed peak shifts, which we attribute to thermal expansion of the NDs and thus a total release of pressure, which indicates the stability of the released NDs.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Evaluation of RMI Ejecta Sourcing from Reconstructed Interfaces in 2D FLAG Flyer-Plate Simulations

This study investigates the performance of RMI ejecta sourcing from a reconstructed interface in two-dimensional FLAG ejecta flyer-plate simulations. Enabling the RMI ejecta model to operate on reconstructed interfaces has been a longstanding challenge in FLAG, limiting its applicability to experiments in which interface reconstruction is not required. Addressing this limitation is therefore an important step toward expanding the model’s predictive capability. The first phase of this effort focused on identifying a flyer-plate/target configuration that produces large ejecta clouds from two distinct shocks using the standard RMI ejecta model. A series of simulations examined the effects of flyer composition, layer thickness, and mesh resolution on shock structure and ejecta formation. VISAR traces were used to evaluate shock timing and identify configurations that produced a clear double-shock response. A copper middle-layer flyer with a doubled tin layer yielded the most favorable shock characteristics and was selected as the baseline configuration. After confirming this configuration performed as expected when running a reference FLAG version, it became the basis for three simulations: (1) a standard two-dimensional ejecta flyer-plate calculation using a reference FLAG version, (2) the same calculation with the reconstructed interface option enabled, and (3) a calculation employing ALE strategies to force the ejecta model to operate on the reconstructed interface. While the baseline simulation produced the expected ejecta response, the reconstructed interface approach did not result in measurable ejecta, indicating that this capability remains under development. These results highlight both the progress made and the remaining challenges in extending the RMI ejecta model to reconstructed interfaces.

36 MATERIALS SCIENCE↗
NASA NTRS1985

Persistence of shocks to large distances in the solar wind

Present hydrodynamic models of solar wind streams predict that interactions will cause interplanetary shocks to decay and large-scale structures to coalesce and smooth out, with a decay length of 10-15 AU for moderate or small-amplitude shocks. The Pioneer 10 plasma data, extending 1-30 AU, are examined in the light of such predictions. It is found that coalescence of streams into a single stream per solar rotation does occur, in general, but that considerable structure remains by 30 AU. The leading edge of a stream often exhibits a velocity jump of greater than 20 km/s; many of these may be shocks. There is a characteristic velocity-density-temperature signature of these distant streams which differs from the close-in double-shock signature. A unique transient was seen in July 1982, at 28 AU, with a velocity jump of about 235 km/s.

Kayser, S. E.↗
DOE OSTI2020

Shocking Cerium into a New Phase

A material's equation of state (EOS) - which indicates its state under various conditions of pressure, temperature, volume, and energy, and relates them to various phases - is a vital part of understanding the material’s behavior and response in different environments and applications. However, determining the EOS and complete phase diagrams of some materials can pose daunting challenges. One of these materials is cerium, for which some regions of the phase diagram have proven elusive. Investigators from the U.S. Department of Energy’s (DOE’s) Los Alamos National Laboratory (LANL) employed the U.S. DOE’s Advanced Photon Source (APS) to probe the high-pressure solid phase of cerium through shock-wave experiments that provided a detailed look at the cerium's transition from the α-ϵ phases. Their work, which provides the first evidence that an α-ϵ phase transition can be shock-induced in cerium, was published in the Journal of Applied Physics.

36 MATERIALS SCIENCE↗