Nuclear Fission Dynamics: Past, Present, Needs, and Future
Not Available
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
SEARCH · Engineering Papers
Results for “adiabatic collective motion”
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.
Generative deep-learning reveals collective variables of Fermionic systems
Complex processes of fermionic systems ranging from protein folding to nuclear fission often follow a low-dimensional reaction path parametrized in terms of a few collective variables. In nuclear theory, variables related to the shape of the nuclear density in a mean-field picture are key to describing the large amplitude collective motion of the neutrons and protons. Exploring the adiabatic energy landscape spanned by these degrees of freedom reveals the possible reaction channels while simulating the dynamics in this reduced space yields their respective probabilities. Unfortunately, this theoretical framework breaks down whenever the systems encounters a quantum phase transition with respect to the collective variables. Here, in this study, we introduce a novel generative deep-learning algorithm designed to build reaction paths that ensure that the many-fermion wave function stays differentiable with respect to the collective variables. This approach is applicable to any fermionic system described by a coherent state. We use the case of potential energy curves in the 16 O nucleus within the Hartree-Fock theory to illustrate its main features.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Unified theory of spin and charge in a ferromagnet
Here, we derive a unified theory of spin and charge degrees of freedom in a ferromagnet. The spin-transfer torque and spin electromotive force are examined from the coarse-grained perspective of collective coordinates. The resulting equations of motion reflect a balance of conservative, gyroscopic (Berry-phase), and dissipative forces. We then expand the space of collective coordinates by adding the electric charge. The adiabatic spin-transfer torque and spin electromotive force (emf) turn out to be a gyroscopic force; their nonadiabatic counterparts are a dissipative force.
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
Spin–vibronic coherence drives singlet–triplet conversion
Design-specific control over the transitions between excited electronic states with different spin multiplicities is of the utmost importance in molecular and materials chemistry. Previous studies have indicated that the combination of spin-orbit and vibronic effects, collectively termed the spin-vibronic effect, can accelerate quantum-mechanically forbidden transitions at non-adiabatic crossings. However, it has been difficult to identify precise experimental manifestations of the spin-vibronic mechanism. Here we present coherence spectroscopy experiments that reveal the interplay between the spin, electronic and vibrational degrees of freedom that drive efficient singlet-triplet conversion in four structurally related dinuclear Pt(II) metal-metal-to-ligand charge-transfer (MMLCT) complexes. Photoexcitation activates the formation of a Pt-Pt bond, launching a stretching vibrational wavepacket. The molecular-structure-dependent decoherence and recoherence dynamics of this wavepacket resolve the spin-vibronic mechanism. Further, we find that vectorial motion along the Pt-Pt stretching coordinates tunes the singlet and intermediate-state energy gap irreversibly towards the conical intersection and subsequently drives formation of the lowest stable triplet state in a ratcheting fashion. This work demonstrates the viability of using vibronic coherences as probes to clarify the interplay among spin, electronic and nuclear dynamics in spin-conversion processes, and this could inspire new modular designs to tailor the properties of excited states.
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗