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Investigation of the approach used in the unresolved resonance region

The typical practice used in Monte Carlo neutron transport codes in the unresolved resonance region (URR) is to take advantage of the probability table (PT) approach. Cross sections are sampled from PTs and used as needed, along with generated average cross sections. The PTs are generated based on cross-section calculations performed using the single-level Breit–Wigner approximation. Although the approach used in the URR seems plausible, a detailed examination was needed to understand the benchmark results obtained using specific tests.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Multiple Critical Unresolved Region Integral Experiment (MCURIE): A Proposed Integral Critical Experimental Framework for Unresolved Region and Intermediate Energies

The Critical Unresolved Region Integral Experiment (CURIE) critical experiment was performed at the National Criticality Experiments Research Center (NCERC) at the Device Assembly Facility (DAF) at the Nevada Nuclear Security Sites (NNSS) in 2020. The objective of CURIE was to improve the quality of integral nuclear data in the uranium-235 ( 235 U) unresolved resonance region (URR) by performing benchmark integral experiments that were sensitive to the URR energy ranges. The CURIE experiment was evaluated for the International Criticality Safety Benchmark Evaluation Project (ICSBEP) handbook and the benchmark evaluation was accepted in 2022. The URR is a region within the intermediate neutron energy range (the intermediate energy ranges from 0.7 eV to 100 keV). The observed resonance structure in neutron cross sections is due to discrete energy levels in the nucleus and are characterized by resonance parameters. In the URR region, the resonance parameters are only partially resolved as the resolution of the experiment techniques becomes comparable to the average width of the resonances themselves, and the resonances are so close to one another that the structure cannot be determined empirically. The ENDF/B-VIII.0 and JEFF-3.3 nuclear data libraries define the URR as beginning at 2.25 keV and continuing until 25 keV. There are minimal intermediate neutron energy benchmarks available in the ICSBEP benchmark handbook, and aside from CURIE there are none that are highly sensitive in the URR energy region. There is a current need for additional experiments sensitive to the URR energy region. There is a new proposed subgroup for the Organization for Economic Co-operation and Development and Nuclear Energy Agency (OECD NEA) Working Party on International Nuclear Data Evaluation Cooperation (WPEC), so any new models or information will need experimental validation and testing. The NEA Working Party on Nuclear Criticality Safety (WPNCS) recent experimental needs and priority list includes intermediate energy 235 U and 238 U experiments, as does the recent Integral Experiments to Address Nuclear Criticality Safety Needs Meeting (May 2023). A variant on the original CURIE experiment called the Multiple Critical Unresolved Region Integral Experiment (MCURIE) is proposed to provide further investigation of the intermediate and URR energy region for uranium. MCURIE will utilize existing fuels at NCERC but use alternative moderators and reflectors to modify the neutron absorption, scattering, and fission spectra of the experiments, allowing for precise targeting of nuclear data sensitivities. The overall goal of MCURIE is to develop a framework for designing and performing integral benchmark experiments with high sensitivities in the intermediate and URR energy regions for nuclear data validation.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

DANCE and NEUANCE measurements of 233 U(n, γ) (Q4 Report to NCSP on FY2022)

Uranium-233 plays an important role in the Th-U fuel cycle, which has been proposed as an alternative to the U-Pu fuel cycle due to its reduced amount of transuranium elements. The available experimental 233 U(n,γ) cross section data in the literature are scarce [1, 2, 3], from which the capture to fission ratio is shown in figure 1. In 2008, the 233 U(n,γ) cross section was investigated at LANL using the DANCE detector combined with a PPAC, however the statistics in the keV regime were inadequate for a reliable extraction of the cross section at 100 keV. Large discrepancies are found between the evaluations, especially in the Unresolved Resonance Region (URR), see figure 1. An accurate measurement of the 233 U(n,γ) cross section is required by the NCSP to complete the neutron-induced cross section data; a new evaluation reported the need of 233 U capture data.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Covariance Data in Unresolved Range [Slides]

This presentation touches on the covariance data in unresolved range. This presentation talks about how the URR has several limitations and the focus on covariance information. The talk briefly outlines the limitations and fosters a discussion that can lead to format proposals.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

On the Uranium and Plutonium Nuclear Data Evaluations [Slides]

This presentation provides overviews of uraniums, 233 U and 235 U, plutonium research including motivations, current status in ENDF/B-VIII.0, the inclusion of sub-thermal data, and the inclusion of LANL ratio capture-to-fission data. Additionally, the preliminary fit of Mosby’s data as reported, fluctuating neutron multiplicities, uncertainty in evaluated libraries, and experimental effects are also presented. The presentation concludes by providing a summary of plans for the U and Pu evaluation work.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

SAMMY Modernization Efforts [Slides]

This presentation discusses SAMMY releases and states that all of its dependencies are freely available. It also discusses version control and confirms that versions will be tagged as needed. Additionally, SAMMY program flow is discussed and states that the program flow was improved to allow for easier external access to SAMMY routines. Modernization of SAMMY is continued with the Doppler and Resolution broadening modules. The presentation concludes by stating that documentation updates are in progress.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Advancements in nuclear data evaluations in the unresolved resonance region [Slides]

Minimal updates to current capabilities (SAMMY/AMPX) and to the ENDF format are proposed to include threshold reaction for outgoing charged-particle channels in the URR formalism. If average resonance parameters are reported, probability tables for newly defined reactions channels may be needed, implemented, and tested. Nuclear data evaluation of n+ 35 Cl reactions can be considered the best case to apply the proposed updates.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Unresolved resonance region cross section measurements and validation [Slides]

This presentation discusses the ENDF format and its implication for experimental data. The effect of self-shielding on measured cross sections some call this effect transmission enhancement (to be explained). Additionally discussed: from experiment to evaluation. And finally, Processing “high energy resolution” transmission for URR evaluation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗