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At least 19 records

Testing fast reactor fuels in a thermal reactor: Comparison of transmutation metallic fuel alloys behavior by scanning electron microscopy

To optimize nuclear waste repository performance, the destruction of minor actinide elements, particularly Np and Am, in a neutron fast spectrum reactor is possible by incorporating these elements into nuclear fuel. Evaluating the performance of minor actinide containing fuel is of paramount importance to enabling this technology. However, such a task is challenging without an available domestic fast spectrum test reactor. A comparison of fuel performance tested in an available domestic thermal reactor at the Idaho National Laboratory, the Advanced Test Reactor, and in a fast spectrum reactor in France (Phénix) is presented here in this study. This study evaluates the capability of using a cadmium shrouded test position to mimic the power profile along the fuel radius present in fast spectrum reactors so that thermally driven phenomenon (e.g., constituent redistribution) can be evaluated in a thermal reactor and determined to be prototypical of a fast reactor. Thus, optical microscopy and scanning electron microscopy has been performed on irradiated 35U-29Pu-4Am-2Np-30Zr fuel samples (where the number preceding the element is the weight percent concentration) from the two mentioned reactors that present similar irradiation temperatures and power conditions. The results indicate that fuel performance phenomena are reproducible in the two irradiation conditions. The redistribution of Zr occurred in the same manner for the two samples. Similar partitioning of U-Pu-Zr phases was observed, and the behavior of Am was similar in the analyzed specimens. Finally, the overall microstructure evolution seems not to be affected by minor actinides addition compared to expected behavior of conventional U-19Pu-10Zr ternary metal fuels for both specimens. Slight differences in fuel cladding chemical interaction were, however, observed. This difference is likely driven by difference in cladding composition rather than irradiation conditions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Testing Fast Reactor Fuels in a Thermal Reactor: A Comparison Report

The testing of fast reactor fuels in the thermal-spectrum of the Advanced Test Reactor using cadmium-filtering has been underway since 2003. The objective of this experimental approach to create a temperature profile inside of test fuel rodlets that is nearly prototypic of corresponding fast reactor conditions. This requires, necessarily, that the power generation profile inside of test fuel rodlets also be nearly prototypic of corresponding fast reactor conditions. By doing so, this experimental approach should allow for the study of fast reactor fuel performance phenomena that are primarily dependent upon the conditions of temperature and/or temperature gradient inside the fuel to be possible using a thermal test reactor. Validation of this assertion has been undertaken by both supporting analyses and by comparing fuel performance phenomena observed in fuels irradiated in cadmium-filtered positions in ATR to similar or identical fuels irradiated under similar conditions in genuine fast reactors. This report documents a preliminary comparison of fuel performance data available from the testing of metallic, oxide, and nitride fuels in cadmium-filtered positions in the ATR to the performance of identical or similar fuels irradiated in genuine fast reactors. Although a variety of fuel performance metrics are presented, particular attention is paid to those phenomena that are primarily, or significantly, dependent on conditions of temperature and temperature gradient with the fuel. Although the comparisons presented in this report are at this time limited in scope and preliminary in nature, they do support the assertion that the objectives of the cadmium-filtered testing approach in ATR are both feasible and appear sound. The analyses and comparisons presented in this report show that ATR irradiations performed using cadmium shrouding are sufficiently prototypic that they can be used with confidence in the development and testing of fast reactor fuels.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Testing Fast Reactor Fuels in a Thermal Reactor: A Comparison Report

The testing of fast reactor fuels in the thermal-spectrum of the Advanced Test Reactor using cadmium-filtering has been underway since 2003. The objective of this experimental approach has not been to create testing conditions that are fully prototypic of a fast reactor, but to create a thermal profile inside of test fuel rodlets that is nearly prototypic of corresponding fast reactor conditions. By doing so, this experimental approach should allow for the study of fast reactor fuel performance phenomena that are primarily dependent upon the conditions of temperature and/or temperature gradient inside the fuel to be possible using a thermal test reactor. Validation of this assertion has been undertaken by comparing fuel performance phenomena observed in fuels irradiated in cadmium-filtered positions in ATR to similar or identical fuels irradiated under similar conditions in genuine fast reactors. This report documents a preliminary comparison of limited fuel performance data available from the testing of metallic, oxide, and nitride fuels in cadmium-filtered positions in the ATR to the performance of identical or similar fuels irradiated in genuine fast reactors. Although a variety of fuel performance metrics are presented, particular attention is paid to those phenomena that are primarily, or significantly, dependent on conditions of temperature and temperature gradient with the fuel. Although the comparisons presented in this report are at this time limited in scope and preliminary in nature, they do support the assertion that the objectives of the cadmium-filtered testing approach in ATR are both feasible and appear sound. The available evidence supports the assertion that use of cadmium-filtering creates irradiation conditions in the ATR that are both relevant to, and suitable for, fast reactor fuel performance testing.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Testing Fast Reactor Fuels in a Thermal Reactor: A Comparison Report

The testing of fast reactor fuels in the thermal-spectrum of the Advanced Test Reactor using cadmium-filtering has been underway since 2003. The objective of this experimental approach has not been to create testing conditions that are fully prototypic of a fast reactor, but to create a thermal profile inside of test fuel rodlets that is nearly prototypic of corresponding fast reactor conditions. By doing so, this experimental approach should allow for the study of fast reactor fuel performance phenomena that are primarily dependent upon the conditions of temperature and/or temperature gradient inside the fuel to be possible using a thermal test reactor. Validation of this assertion has been undertaken by comparing fuel performance phenomena observed in fuels irradiated in cadmium-filtered positions in ATR to similar or identical fuels irradiated under similar conditions in genuine fast reactors. This report documents a preliminary comparison of limited fuel performance data available from the testing of metallic, oxide, and nitride fuels in cadmium-filtered positions in the ATR to the performance of identical or similar fuels irradiated in genuine fast reactors. Although a variety of fuel performance metrics are presented, particular attention is paid to those phenomena that are primarily, or significantly, dependent on conditions of temperature and temperature gradient with the fuel. Although the comparisons presented in this report are at this time limited in scope and preliminary in nature, they do support the assertion that the objectives of the cadmium-filtered testing approach in ATR are both feasible and appear sound. The available evidence supports the assertion that use of cadmium-filtering creates irradiation conditions in the ATR that are both relevant to, and suitable for, fast reactor fuel performance testing.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Accelerated Fuel Qualification of Fast Modular Reactor Fuel in a Thermal Reactor: Modeling and Simulation Paired with Irradiation Testing

The accelerated fuel qualification (AFQ) methodology is applied by simulating accelerated fuel tests of the General Atomics Electromagnetic Systems’ fuel system for its 44-MW(electric) gas-cooled, fast-spectrum fast modular reactor (FMR). This fuel is comprised of UO 2 pellets in SiGA® cladding, a silicon carbide ceramic matrix composite. Fast reactors, like the FMR, offer many benefits, including high fuel utilization and flexibility, but may require a lengthy material design process if tests are performed using fast neutron irradiation alone. A thermal neutron irradiation can instead be used to rapidly test how well key components of the current material models extend to high burnup. Thermal neutrons produce a different radial power distribution within the pin than fast neutrons. However, the temperature and burnup values for the two neutron types are comparable, and the differences between the simulated fuel responses are relatively small, demonstrating the weak sensitivity of the physics-based fuel model calculations on the neutron type and the irradiation rate. Furthermore, the deformation of the SiGA cladding saturates after about 1 displacement per atom for both neutron spectra. In an accelerated fuel test, the irradiation time required to reach the target fuel burnup can be reduced by a factor of 3 by using a small rodlet with a 45% smaller pellet diameter while maintaining the same linear power. Therefore, the time for data collection up to high burnup can be significantly reduced while maintaining the same temperature profile, which largely determines the material response. Tests of fuel rodlets of standard and compact size will be carried out in the Idaho National Laboratory’s Advanced Test Reactor (ATR), including full size and compact rodlets with varying gap sizes. By applying physics-based mechanistic modeling and simulation in accordance with the AFQ methodology, this type of compact rodlet testing in a thermal test reactor captures the necessary phenomena to test fuel material models up to high burnup and to simulate the expected impact of fast neutron radiation on the fuel in FMR operations. Finally, this approach to testing fast reactor fuels in existing thermal test reactors, paired with advanced physics-based mechanistic modeling and simulation, is expected to be applicable to a range of advanced fuels and will decrease the overall fuel qualification timeframe from decades to years.

Advanced test reactor (ATR)↗

Variants of Regenerated Fissile Materials Usage in Thermal Reactors as the First Stage of Fuel Cycle Closing

At present, 240 000 t of spent nuclear fuel (SF) has been accumulated in the world. Its long-term storage should meet safety conditions and requires noticeable finances, which grow every year. Obviously, this situation cannot exist for a long time; in the end, it will require a final decision. At present, several variants of solution of the problem of SF management are considered. Since most of the operating reactors and those under construction are thermal reactors, it is reasonable to assume that the structure of the nuclear power industry in the near and medium-term future will be unchanged, and it will be necessary to utilize plutonium in thermal reactors. In this study, different strategies of SF management are compared: open fuel cycle with long-term SF storage, closed fuel cycle with MOX fuel usage in thermal reactors and subsequent long-term storage of SF from MOX fuel, and closed fuel cycle in thermal reactors with heterogeneous fuel arrangement. The concept of heterogeneous fuel arrangement is considered in detail. While in the case of traditional fuel it is necessary to reprocess the whole amount of spent fuel, in the case of heterogeneous arrangement, it is possible to separate plutonium and {sup 238}U in different fuel rods. In this case, it is possible to achieve nearly complete burning of fissile isotopes of plutonium in fuel rods loaded with plutonium. These fuel rods with burned plutonium can be buried after cooling without reprocessing. They would contain just several percent of initially loaded plutonium, mainly even isotopes. Fuel rods with {sup 238}U alone should be reprocessed in the usual way.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Design Studies for a Multiple Application Thermal Reactor for Irradiation Experiments (MATRIX)

The Advanced Test Reactor (ATR) is a high power density test reactor specializing in fuel and materials irradiation. For more than 45 years, the ATR has provided irradiations of materials and fuels testing along with radioisotope production. Should unforeseen circumstances lead to the decommissioning of ATR, the U.S. Government would be left without a large-scale materials irradiation capability to meet the needs of its nuclear energy and naval reactor missions. In anticipation of this possibility, work was performed under the Laboratory Directed Research and Development (LDRD) program to investigate test reactor concepts that could satisfy the current missions of the ATR along with an expanded set of secondary missions. A survey was conducted in order to catalogue the anticipated needs of potential customers. Then, concepts were evaluated to fill the role for this reactor, dubbed the Multi-Application Thermal Reactor Irradiation eXperiments (MATRIX). The baseline MATRIX design is expected to be capable of longer cycle lengths than ATR given a particular batch scheme. The volume of test space in In-Pile-Tubes (IPTs) is larger in MATRIX than in ATR with comparable magnitude of neutron flux. Furthermore, MATRIX has more locations of greater volume having high fast neutron flux than ATR. From the analyses performed in this work, it appears that the lead MATRIX design can be designed to meet the anticipated needs of the ATR replacement reactor. However, this design is quite immature, and therefore any requirements currently met must be re-evaluated as the design is developed further.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Feasibility study of noise analysis methods on virtual thermal reactor subcriticality monitoring

This paper presents the analysis results of Rossi-alpha, cross-correlation, Feynman-alpha, and Feynman difference methods applied to the subcriticality monitoring of nuclear reactors. A thermal spectrum Godiva model has been designed for the analysis of the four methods. This Godiva geometry consists of a spherical core containing the isotopes of H-l, U-235 and U-238, and the H{sub 2}O reflector outside the core. A Monte Carlo code, McCARD, is used in real time mode to generate virtual detector signals to analyze the feasibility of the four methods. The analysis results indicate that the four methods can be used with high accuracy for the continuous monitoring of subcriticality. In addition to that, in order to analyze the impact of the random noise contamination on the accuracy of the noise analysis, the McCARD-generated signals are contaminated with arbitrary noise. It is noticed that, even when the detector signals are contaminated, the four methods can predict the subcriticality with reasonable accuracy. Nonetheless, in order to reduce the adverse impact of the random noise, eight detector signals, rather than a single signal, are generated from the core, one signal from each equally divided eighth part of the core. The preliminary analysis with multiple virtual detector signals indicates that the approach of using many detectors is promising to improve the accuracy of criticality prediction and further study will be performed in this regard. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Identifying and bounding uncertainties in nuclear reactor thermal power calculations

Determination of the thermal power generated in the reactor core of a nuclear power plant is a critical element in the safe and economic operation of the plant. Direct measurement of the reactor core thermal power is made using neutron flux instrumentation; however, this instrumentation requires frequent calibration due to changes in the measured flux caused by fuel burn-up, flux pattern changes, and instrumentation drift. To calibrate the nuclear instruments, steam plant calorimetry, a process of performing a heat balance around the nuclear steam supply system, is used. There are four basic elements involved in the calculation of thermal power based on steam plant calorimetry: The mass flow of the feedwater from the power conversion system, the specific enthalpy of that feedwater, the specific enthalpy of the steam delivered to the power conversion system, and other cycle gains and losses. Of these elements, the accuracy of the feedwater mass flow and the feedwater enthalpy, as determined from its temperature and pressure, are typically the largest contributors to the calorimetric calculation uncertainty. Historically, plants have been required to include a margin of 2% in the calculation of the reactor thermal power for the licensed maximum plant output to account for instrumentation uncertainty. The margin is intended to ensure a cushion between operating power and the power for which safety analyses are performed. Use of approved chordal ultrasonic transit-time technology to make the feedwater flow and temperature measurements (in place of traditional differential-pressure- based instruments and resistance temperature detectors [RTDs]) allows for nuclear plant thermal power calculations accurate to 0.3%-0.4% of plant rated power. This improvement in measurement accuracy has allowed many plant operators in the U.S. and around the world to increase plant power output through Measurement Uncertainty Recapture (MUR) up-rates of up to 1.7% of rated power, while also decreasing the probability of significant over-power events. This paper will examine the basic elements involved in calculation of thermal power using ultrasonic transit-time technology and will discuss the criteria for bounding uncertainties associated with each element in order to achieve reactor thermal power calculations to within 0.3% to 0.4%. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Transition to a U/Pu Fuel Cycle with Fast and Thermal Reactors

The purpose of this study was to analyze the transition from the current U.S. nuclear system to an advanced fuel cycle involving U/Pu continuous recycle in a fleet of fast and thermal reactors. This fuel cycle, known as 'EG29' in the 2014 Nuclear Fuel Cycle Evaluation and Screening (E and S), was identified as one of the four most promising out of a comprehensive list of fuel cycles that were grouped based on similar physics and performance characteristics. The EG29 fuel cycle involves continuously recycling the co-extracted U/Pu from a fleet of fast reactors represented by sodium-cooled fast reactors (SFRs) and burning the surplus amounts in a fleet of thermal reactors represented by pressurized water reactors with full mixed oxide (U,Pu)O{sub 2} cores (MOX-PWRs). The target energy generation ratio of SFRs to MOX-PWRs for the final EG29 system is 70:30. A 1% annual growth in nuclear energy demand was also assumed to be met during the entire scenario, including after EG29 is fully deployed. Therefore, to maintain system-wide mass balance, the SFR was designed to have a Pu inventory ratio (discharged/charged) of 1.4 compared to the MOX-PWR's 0.7. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

A nodal transport method for coupled fast-thermal reactor analysis

We report that for efficient core analyses of coupled fast-thermal reactors, a new deterministic method has been developed based on the variational nodal transport method of VARIANT. A new multigroup cross section generation procedure was devised by combining Monte Carlo lattice calculations for thermal assemblies and the two-step procedure of the MC 2 -3 code for fast assemblies. To reduce assembly homogenization errors in nodal transport calculations, a new nodal equivalence method was developed based on the partial current discontinuity factor (PCDF) and incorporated in VARIANT. A practical procedure to calculate PCDFs with fixed source supercell calculations was also devised. The performance of the proposed method was investigated using a test problem derived from the versatile coupled test reactor (VCTR) design. The new procedure produced multigroup cross sections accurately for all assemblies. VARIANT transport calculations with PCDFs produced accurate multiplication factor and power distribution compared to reference Serpent-2 Monte Carlo solutions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Small CaH{sub 2} Moderated Thermal Reactor for Surface Power Generation I: Conceptual Design

National Aeronautics and Space Administration (NASA) published 'Journey to Mars' on October 8, 2015, stating their plan to send human to Mars for exploration, scientific research and colonization of Mars. Mission time on Martian surface is supposed to be ∼1 year, therefore, a surface power generation system is required for human habitation on Mars. Even though solar power and chemical battery have been used for the past missions, the former cannot generate power during month-scale dust storm on Mars, and the latter is not reliable for long-term use under a cold environment. On the other hand, nuclear power provides stable power even on Mars surface and, since kilowatt class power system is required in the planned mission, a fission power system is better than a radioisotope battery. An 8-year operation is required for the Mars surface power generation system with electrical power of 10 to 100 kWe and specific power of >5 We/kg, which means the system weight needs to be below 2000 kg in the case of 10 to 100 kWe system. In the current study, stretch goals for surface fission power system were set as follows: electric power of 20 kWe and total system weight below 1000 kg. In addition, nuclear security and critical safety are essential features for the surface fission power system considering launch accidents. A sufficient level of nuclear security is needed to prevent terrorists from obtaining nuclear materials even the reactor falls in a geographic area dominated by terrorists. From this view point, it is preferable not to use highly enriched uranium with a space reactor that can be diverted to nuclear weapons. Also, a nuclear reactor core should not reach criticality during a launch accident where the reactor core can be compressed by collision with sea or land. A novel concept of surface power reactor system that satisfies the above requirements is proposed in the current study. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Advanced High-Temperature Sodium-Cooled Thermal Reactors Using Less Than 10% Enriched UO 2 Fuel

Here, this paper presents a 1200-MW(thermal) advanced sodium-cooled thermal reactor concept that uses online refueling of 3.5% to 9.95% enriched UO2 fuel pin bundles; uses either graphite or beryllium oxide (BeO) as a neutron moderator; reaches outlet temperatures of 650°C enabling a thermal efficiency of at least 45%; has a high specific power of 133 W/g U; has average power densities of 16.4 and 43.2 W/cm 3 with graphite and BeO, respectively; reaches an average discharge burnup of 100 MWd/kg U; and generates 52% less spent fuel volume, 28% less fission products, and 47% to 64% less transuranics than a typical large pressurized water reactor for the same amount of electricity produced.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Advanced Reactors Thermal Energy Transport for Process Industries

The operation temperature of advanced nuclear reactors is generally higher than commercial light water reactors and thermal energy from advanced nuclear reactor can be used for various purposes such as liquid fuel production, district heating, desalination, hydrogen production, and other process heat applications, etc. Some of the major technology challenges that must be overcome before the advanced reactors could be licensed on the reactor side are qualification of next generation of nuclear fuel, materials that can withstand higher temperature, improvement in power cycle thermal efficiency by going to combined cycles, SCO2 cycles, successful demonstration of advanced compact heat exchangers in the prototypical conditions, and from the process side application the challenge is to transport the thermal energy from the reactor to the process plant with maximum efficiency (i.e., with minimum temperature drop). The main focus of this study is on doing a parametric study of efficient heat transport system, with different coolants (mainly, water, He, and molten salts) to determine maximum possible distance that can be achieved.

42 ENGINEERING↗

Hot wire needle probe for in-reactor thermal conductivity measurement

Thermal conductivity is a key property that must be known for proper design, test, and application of new fuels and structural materials in nuclear reactors. Thermal conductivity is highly dependent on the physical structure, chemical composition, and the state of the material. Typically, thermal conductivity changes that occur during irradiation are measured out-of-pile by Post Irradiated Examination (PIE) using a “cook and look” approach in hot-cells. Repeatedly removing samples from a test reactor to make out-of-pile measurements is expensive, has the potential to disturb phenomena of interest, and only provides understanding of the sample's end state at the time each measurement is made. There are also limited thermophysical property data for advanced fuels. Such data are needed for simulation design codes, the development of next generation reactors, and advanced fuels for existing nuclear plants. Being able to quickly characterize fuel thermal conductivity during irradiation can improve the fidelity of data, reduce costs of post-irradiation examinations, increase understanding of how fuels behave under irradiation, and confirm or improve existing thermal conductivity measurement techniques. This paper discusses recent efforts to develop and evaluate an in-pile thermal conductivity sensor based on a hot wire needle probe. Testing has been performed on samples with thermal conductivities ranging from 0.2 W/m-K to 22 W-m-K in temperatures ranging from 20 °C to 600 °C. Thermal conductivity values measured using the needle probe match data found in the literature to within 5% for samples tested at room temperature, 5.67% for low thermal conductivity samples tested at high temperatures, and 10% for high thermal conductivity samples tested at high temperatures. Experimental results also show that this sensor is capable of operating in various test conditions and of surviving long duration irradiations.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Bayesian Optimized Deep Ensemble for Uncertainty Quantification of Deep Neural Networks: a System Safety Case Study on Sodium Fast Reactor Thermal Stratification Modeling

Deep neural networks (DNNs) are increasingly important to scientific computing and engineering system simulations. Accurate uncertainty quantification (UQ) for DNNs is critical in safety-sensitive engineering domains. Traditional Deep Ensemble (DE) methods, while easy to implement, frequently suffer from poorly calibrated uncertainty estimates and limited predictive accuracy due to reliance on fixed architectures with varied weight initializations. To address these issues, we introduce a workflow that combines Bayesian Optimization (BO) and DE. The workflow is modular, scalable, and integrates parallel BO initialized with Sobol sequences to individually optimize the hyperparameters of each ensemble member. This method enhances ensemble diversity, improves predictive accuracy, and provides reliable uncertainty estimates. We evaluate the proposed BODE approach in a sodium fast reactor thermal stratification modeling case study, where we used a densely connected convolutional neural network to predict turbulent viscosity during the reactor transient with consideration of data noise. We benchmark its performance against several optimization approaches, including baseline deep ensemble, evolutionary algorithm-optimized ensemble, ensemble formed via random search combined with greedy selection, and a BO ensemble using random initialization. Here, our results demonstrate superior performance of the developed BODE approach. In noise-free scenarios, BODE notably reduces incorrect aleatoric uncertainty and significantly enhances predictive accuracy. Under conditions of 5% and 10% Gaussian noise, BODE adaptively quantifies uncertainty proportional to data noise, achieving up to an 80% reduction in root mean square error compared to baseline methods and producing well-calibrated prediction intervals.

Bayesian optimization↗