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SiCl2 crystallizes in the orthorhombic P2_12_12_1 space group. The structure is zero-dimensional and consists of four dichlorosilane molecules. Si is bonded in a distorted water-like geometry to two equivalent Cl atoms. Both Si–Cl bond lengths are 2.06 Å. Cl is bonded in a single-bond geometry to one Si atom.
CSiCl3(SiCl2)2 crystallizes in the monoclinic C2/c space group. The structure is zero-dimensional and consists of sixteen dichlorosilane molecules, eight methane molecules, and eight trichlorosilane molecules.
(CH3CN)2(SiCl2)5 is Magnesium tetraboride-like structured and crystallizes in the orthorhombic Pbcn space group. The structure is zero-dimensional and consists of eight acetonitrile molecules and twenty dichlorosilane molecules.