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Measurements of the secondary particle energy spectra in the Space Shuttle
Measurements of the energy spectra of secondary particles produced by galactic cosmic rays and trapped protons due to the nuclear interactions of these particles with the Shuttle shielding provide a powerful tool for validating radiation transport codes. A code validated in this way can be used to better estimate the dose and dose equivalent to body organs, measurements that cannot be made directly. The principal cause of single event upsets in electronic devices in the region of the South Atlantic Anomaly is secondary particles, and even in the region of galactic cosmic radiation a significant fraction is produced by secondary particles. In this paper, we describe the first direct measurements of the energy spectra of secondary protons, deuterons, tritons, 3He and 4He produced by galactic cosmic rays inside the Space Shuttle using a charged particle spectrometer. A comparison of these spectra with radiation transport code HZETRN showed reasonably good agreement for secondary protons. However, the code seriously underestimated the flux of all other light ions. The code has been modified to include pick-up and knock-on processes. The modified code leads to good agreement for deuterons and 3He but not for other light ions. This revised code leads to about 10% higher dose equivalent than the original code under moderate shielding, if we assume that higher charge ion fluxes are correctly predicted by the model.
New Method for the Generation of Secondary Particle Beams at Accelerators
The generation of beams of secondary particles (π and K mesons) at proton accelerators is a difficult scientific and engineering problem. To obtain narrow directional particle beams for experiments, intense extracted proton beams are used, secondary particles (π and K mesons) are generated at an external target, and they are focused and transferred through long magneto-optical channels. In this work, a surprisingly simple method based on a crystal focusing device has been proposed to obtain secondary beams. An experiment on the production of a secondary beam using a crystal has been performed at the U-70 accelerator. Schemes for the formation of beams with energies E ~ 1 TeV have been proposed for large colliders such as the Large Hadron Collider.
Deep Mapping of Small Solar System Bodies with Galactic Cosmic Ray Secondary Particle Showers
We will investigate the use of galactic cosmic ray (GCR) secondary particles to probe the deep interiors of small solar system bodies (SSBs), including comets, asteroids, and geologic structures on the surfaces of airless bodies. Applications include solar system science, planetary defense, and resource utilization. Our Phase I study demonstrated that muons, the long-range charged component of GCR showers, can penetrate SSBs up to a km in diameter, providing information on their interior structure. Muons produced in Earth’s atmosphere have been applied to image the interior of large objects for science and engineering. In Phase I, we found that the production of muons in the solid surfaces of airless bodies is much smaller than in Earth’s atmosphere. Nevertheless, the flux of transmitted muons is sufficient to detect inclusions within an asteroid or comet in a reasonable amount of time, ranging from hours to weeks, depending on the size of the SSB and the density contrast, position and size of the inclusion. For asteroids and comets, large density variations (e.g., porous soil or ice versus solid rock) are relatively easy to detect. The intrinsic spatial resolution of muon radiography (“muography”) is on the scale of a few meters. The spatial resolution that can be achieved in practice depends on signal intensity and integration time (counting statistics), the angular resolution of the muon tracker (hodoscope) and details of data reduction and analysis methodology. Our Phase II project will assess remaining unknowns for the application of muography to determining the interior structure of SSBs, assess risks for implementation, and provide a roadmap for development of SSB muography beyond the NIAC program. To achieve our objectives, we will focus on four interrelated tasks: Task1) Signal and background characterization: Characterize the production and transmission of muons and secondary particle backgrounds made by cosmic ray showers in SSBs; and near-surface features from radiographic and tomographic data; Task2) Imaging studies: Develop methods to determine the density structure of SSB interiors and near-surface features from radiographic and tomographic data; Task3) Instrument design: Using simulations and bench-top laboratory experiments, investigate specific concepts for the design of compact hodoscopes and components; Task4) Synthesis: Combine the results of the first three tasks to determine the range of applicability of the method, identify the steps needed for maturation of the concept, and explore concepts for a pilot muography mission.
Meteoroid impacts on Mars and the secondary particle environment
The degree to which the thin Martian atmosphere filters out meteoroids approaching the Martian surface was calculated by using a model of the meteoroid environment, a model of the Martian atmosphere, and equations of meteor physics. The secondary particle environment on the surface of Mars caused by the material ejected from meteoroid craters was modeled. The model consists of the mass distribution and the speed distribution of the secondary particles. Calculations were made of the penetration flux for aluminum structures on the Martian surface. The penetration hazard on the Martian surface was compared with the penetration hazard in space near Mars and on the lunar surface.
Secondary particle contribution to LET spectra on LDEF
Four experiments utilizing passive detectors (P0006, P0004, A0015, M0004) were flown on LDEF to study the radiation environment. These experiments have been summarized in a companion paper (Benton et al., 1996). One of the experimental goals was to measure LET spectra at different locations and shielding depths with plastic nuclear track detectors (PNTD). It was found that the LET spectra extended well above the LET cutoff imposed by the geomagnetic field on GCR particle penetration into LEO. The high LET particles detected were mostly short-range (range < 2000 m), indicating that they were secondaries produced locally within the PNTD. The presence of these high LET particle fluences is important for the determination of dose equivalent because of the high Quality Factors (Q) involved. A relatively small fraction of particle fluence can contribute a large fraction of dose equivalent. Short-range, inelastic secondary particles produced by trapped protons in the South Atlantic Anomaly (SAA) were found to be a major contributor to the LET spectra above 100 keV/micrometer. The LET spectra were found to extend beyond the approximately 137 keV/micrometer relativistic GCR Fe peak to over 1000 keV/micrometer. The high LET tail of the LET spectra was measured in CR-39 and polycarbonate PNTDs using different techniques. GCR made a relatively modest contribution to the LET spectra as compared to the contributions from short-range secondary particles and stopping protons. LET spectra intercomparisons were made between LDEF measurements and exposures to 154 MeV accelerated proton beams. The similarities support the role of nuclear interactions by trapped protons as the major source of secondary particles in the PNTDs. Also techniques were employed to reduce the range cutoff for detection of the short-range secondaries to approximately 1 micrometer, so that essentially all secondary particles were included in the LET spectra. This has allowed a more realistic assessment of secondary contribution to dose equivalent. Comparisons of measured and calculated LET spectra have been made that demonstrate the need for more accurate modeling of secondary particles in radiation transport codes. Comparisons include preliminary calculations in which attempts have been made to include secondary particles.
Origin of Rapid Delithiation In Secondary Particles Of LiNi 0.8 Co 0.15 Al 0.05 O 2 and LiNi y Mn z Co 1− y − z O 2 Cathodes
Abstract Most research on the electrochemical dynamics in materials for high‐energy Li‐ion batteries has focused on the global behavior of the electrode. This approach is susceptible to misleading analyses resulting from idiosyncratic kinetic conditions, such as surface impurities inducing an apparent two‐phase transformation within LiNi 0.8 Co 0.15 Al 0.05 O 2 . Here, nano‐focused X‐ray probes are used to measure delithiation operando at the scale of secondary particle agglomerates in layered cathode materials during charge. After an initial latent phase, individual secondary particles undergo rapid, stochastic, and largely uniform delithiation, which is in contrast with the gradual increase in cell potential. This behavior reproduces across several layered oxides. Operando X‐ray microdiffraction (‐XRD) leverages the relationship between Li content and lattice parameter to further reveal that rate acceleration occurs between Li‐site fraction ( x Li ) ≈0.9 and ≈0.5 for LiNi 0.8 Co 0.15 Al 0.05 O 2 . Physics‐based modeling shows that, to reproduce the experimental results, the exchange current density ( i 0 ) must depend on x Li , and that i 0 should increase rapidly over three orders of magnitude at the transition point. The specifics and implications of this jump in i 0 are crucial to understanding the charge‐storage reaction of Li‐ion battery cathodes.
Mesoscopic Phase Transition Kinetics in Secondary Particles of Electrode-Active Materials in Lithium-Ion Batteries
Many compounds used as battery storage electrodes undergo large composition changes during use that are accompanied by a first-order phase transition. Most studies of these phase transitions have focused on the unit cell to single-crystallite scale, whereas real battery electrodes are typically composed of mesoscopic assemblies of nanocrystallites, for which phase transformation mechanisms are poorly understood. Here in this work, a systematic study is conducted of the potentiostatic (constant driving force) kinetics of phase transition in secondary particles of representative intercalation compounds: LiFePO 4 , LiMn 1–x Fe x PO 4 , and Li 4 Ti 5 O 7 . Storage kinetics are studied as a function of overpotential, material composition, primary particle size, and temperature. We find that in regimes where phase transformation occurs, the results can be self-consistently explained as nucleation and growth kinetics within the framework of the Johnson–Mehl–Avrami–Kolmogorov model. This implies that despite the common secondary particle topology, the electrochemically driven phase transformations occur by nucleation and growth with little apparent resistance to phase propagation across the grain boundaries. Growth appears to be one-dimensional in nature, consistent with a hybrid growth model in which rapid surface propagation is followed by slower growth into particles.
The cosmic gamma-ray spectrum from secondary particle production in the metagalaxy
Calculated cosmic gamma ray spectrum from secondary particle production in metagalaxy
Separation of primary and secondary particles in mass spectrometric investigations of the upper atmosphere
Primary and secondary particle separation in mass spectroscopy of upper atmosphere
The secondary-particle contribution to the dose from monoenergetic proton beams and the validity of current-to-dose conversion factors
Secondary particle contribution to radiation dose from monoenergetic proton beams and validity of current-to-dose conversion factors
Estimates of primary and secondary particle doses behind aluminum and polyethylene slabs due to incident solar-flare and Van Allen belt protons
Primary and secondary particle radiation doses shielded from solar flare and Van Allen belt protons by aluminum and polyethylene slabs
Charge, energy and LET spectra of high LET primary and secondary particles in CR-39 plastic nuclear track detectors of the P0006 experiment
We have measured the charge, energy and linear energy transfer (LET) spectra of about 800 high LET (LET(sub infinity) H2O greater than 50 keV/micron) particles in CR-39 plastic nuclear track detectors in the P0006 experiment of LDEF. Primary particles with residual range at the reference surface greater than about 2 microns and secondary particles produced in the detector material with total range greater than about 4 microns were measured. We have used a multi-etch technique and an internal calibration to identify and measure the energy of the particles at the reference surface. The LET spectrum was obtained from the charge and energy distribution of the particles.
The Role of Secondary Particle Structures in Surface Phase Transitions of Ni-Rich Cathodes
Nanometer-thick reconstruction layers on layered cathode surfaces have been widely observed on both pristine and cycled materials. However, the mechanisms of reconstruction and the role that these structures play in electrochemical performance are not fully understood. From a crystallographic perspective, such surface reconstruction layers result from cation site-mixing between Li and transition-metal ions, but it remains far from clear as to what the critical factors are that control such cation mixing for various cathode chemistries. In this paper, we report observations on surface transformations during cycling of a Ni-rich cathode-oxide that are governed by direct contact with the liquid electrolyte. Specifically, within a secondary particle, the three-dimensional hierarchical aggregate of primary particles leads to the formation of grain boundaries of different characteristics, including open grain boundaries that allow the permeation of liquid electrolyte, and closed grain boundaries that exclude liquid electrolyte penetration. Upon battery cycling, surfaces in direct contact with the liquid electrolyte showed a surface reconstruction layer while the surfaces that did not have contact with the electrolyte showed no such reconstructions. In addition, the critical role of oxygen in reconstruction of grain boundaries is demonstrated, and the unexpected oxygen depletion at twin boundaries result in severe phase transitions. The present work provides further insights into phase transitions at solid-solid and solid-liquid interfaces within secondary cathode particles and suggests strategies for mitigating surface/interfacial degradation.
Statistical analysis of secondary particle distributions in relativistic nucleus-nucleus collisions
The use is described of several statistical techniques to characterize structure in the angular distributions of secondary particles from nucleus-nucleus collisions in the energy range 24 to 61 GeV/nucleon. The objective of this work was to determine whether there are correlations between emitted particle intensity and angle that may be used to support the existence of the quark gluon plasma. The techniques include chi-square null hypothesis tests, the method of discrete Fourier transform analysis, and fluctuation analysis. We have also used the method of composite unit vectors to test for azimuthal asymmetry in a data set of 63 JACEE-3 events. Each method is presented in a manner that provides the reader with some practical detail regarding its application. Of those events with relatively high statistics, Fe approaches 0 at 55 GeV/nucleon was found to possess an azimuthal distribution with a highly non-random structure. No evidence of non-statistical fluctuations was found in the pseudo-rapidity distributions of the events studied. It is seen that the most effective application of these methods relies upon the availability of many events or single events that possess very high multiplicities.
Spectral characteristics and dose calculations for the primary and secondary particles that result from the interaction of the solar and galactic cosmic-rays with aluminum shields
Spectral characteristics and dose calculations for primary and secondary particles that result from interaction of solar and galactic cosmic rays with aluminum shields
Deep Mapping of Small Solar System Bodies with Galactic Cosmic Ray Secondary Particle Showers
Galactic cosmic rays rain steadily from all directions onto asteroids and comets. The interaction of these high-energy ions produces a cascade of secondary particles, including muons, which can penetrate the solid interiors of small solar system bodies. Muons, which are produced in abundance in Earth's atmosphere, have been used to image large structures on Earth, including the Great Pyramids and the interior of volcanoes. In this study, we demonstrate that the transmitted flux of muons is sensitive to the interior density structure of asteroids and comets, less than a few hundred meters in diameter. Muonography has the potential to fill a critical gap in our knowledge of the deep interiors of small bodies, providing information needed for planetary defense, in situ resource utilization, and planetary science. We use Monte Carlo codes (MCNPX and FLUKA), which accurately model galactic cosmic ray showers, to explore systematic variations in the production of muons in solid surfaces. Results of these calculations confirm the scaling of muon production in Earth's atmosphere to solid regolith materials, as predicted by a simple, semi-empirical model. Muons are primarily produced in the top meter of the regoliths of asteroids and comets. Their rate of production is over three orders of magnitude lower than in Earth's atmosphere and depends strongly on regolith density. In practice, the use of muonography to characterize the interiors of small solar system bodies must overcome their low rate of production and their dependence on regolith density, which can vary over the surface of asteroids and comets. We show that interior contrast can be resolved using a muon telescope (hodoscope) with about 1 sq m aperture with integration times ranging from hours to weeks. Design concepts for a practical hodoscope that could be deployed in situ or on an orbiting spacecraft, are described. Regolith density within the top meter of an asteroid can be determined from radar observations. A concept for a pilot mission that combines remote radar measurements with in situ muonography of a near-Earth asteroid is presented. Perceived challenges and next steps for the development of the concept are described.
Accelerator experiments on the contribution of secondary particles to the production of cosmogenic nuclides in meteorites
Through the interaction of galactic cosmic particle radiation (GCR) a wide variety of cosmogenic nuclides is produced in meteorites. They provide historical information about the cosmic radiation and the bombarded meteorites. An important way to understand the production mechanisms of cosmogenic nuclides in meteorites is to gather information about the depth and size dependence of the build-up of Galactic Rays Cosmic-secondary particles within meteorites of different sizes and chemical compositions. Simulation experiments with meteorite models offer an alternative to direct observation providing a data basis to describe the development and action of the secondary cascade induced by the GCR in meteorites.