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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Measurement of the 28 Si ⁢(𝑛,𝑛′⁢𝛾) cross section with 𝑛, 𝛾, and correlated 𝑛−𝛾 angular distributions

Silicon has become an unavoidable element in the circuitry central to everyday life. In turn, the interactions of silicon isotopes with neutrons for nuclear physics applications, among other motivations, have become increasingly important to understand. The dominant isotope of silicon, 28 Si, is thus of primary interest for enhanced understanding for neutron transport calculations and related investigations. Unfortunately, the existing measurement database for neutron scattering reactions on 28 Si is minimal, and nuclear data evaluations on this topic have not been updated for decades. This article details new measurements of the 28 Si ⁢(𝑛,𝑛′⁢𝛾) reaction utilizing multiple analysis methods available within the correlated gamma neutron array for scattering (CoGNAC). Specifically, high-precision near-threshold results and high-incident-energy results were obtained using the 𝛾-only and correlated 𝑛−𝛾 techniques. First-ever measurements of the correlated 𝑛−𝛾 angular distribution for particles emitted following population of the first excited state in 28 Si were obtained as well, which provide unique insight into theoretical descriptions of the inelastic neutron scattering reaction mechanism itself and detailed guidance for nuclear reaction models. The results agree well with literature data where they exist, and substantially expand on the current database for neutron reactions on 28 Si .

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Electrical performances of pre-production staves for the ATLAS ITk Strip Detector Upgrade

The ATLAS experiment is currently preparing for an upgrade of the inner tracking detector for the High-Luminosity LHC. The new tracker, ITk, employs an all-silicon detector with outer strip layers. The building block of the ITk strip barrel is the stave which consists of a low-mass support structure hosting the common electrical, optical and cooling services as well as 28 silicon modules. In this contribution, we outline the challenging aspects of the stave pre-production testing phase at Brookhaven National Laboratory. Here, the electrical characterization of these staves, hosting the final design of all ASICs, will be discussed in detail.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2014

Stark shift and field ionization of arsenic donors in {sup 28}Si-silicon-on-insulator structures

We develop an efficient back gate for silicon-on-insulator (SOI) devices operating at cryogenic temperatures and measure the quadratic hyperfine Stark shift parameter of arsenic donors in isotopically purified {sup 28}Si-SOI layers using such structures. The back gate is implemented using MeV ion implantation through the SOI layer forming a metallic electrode in the handle wafer, enabling large and uniform electric fields up to 2 V/μm to be applied across the SOI layer. Utilizing this structure, we measure the Stark shift parameters of arsenic donors embedded in the {sup 28}Si-SOI layer and find a contact hyperfine Stark parameter of η{sub a} = −1.9 ± 0.7 × 10{sup −3} μm{sup 2}/V{sup 2}. We also demonstrate electric-field driven dopant ionization in the SOI device layer, measured by electron spin resonance.

36 MATERIALS SCIENCE↗
DOE OSTI2013

Nuclear Data Sheets for A = 28

Evaluated spectroscopic data and level schemes from radioactive decay and nuclear reaction studies are presented for {sup 28}F, {sup 28}Ne, {sup 28}Na, {sup 28}Mg, {sup 28}Al, {sup 28}Si, {sup 28}P, and {sup 28}S. This evaluation for A=28 supersedes the earlier evaluations by P.M. Endt (1998En04 and 1990En08). However, additional/detailed data for these nuclides can be found in earlier evaluations 1978En02 and 1973EnVA also by P.M. Endt.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

{sup 26}Al production: The Allende meteorite (Chihuahua) stellar nucleosynthesis and solar models

In 1969 a meteorite fell near the small town of Allende, state of Chihuahua in the north of Mexico. Its study yielded information that changed the current understanding of the solar model. In particular traces of {sup 26}Al were found. Abundances of that isotope had been seen in the universe and were related to regions of active heavy nucleosynthesis. Its presence on the solar system was unexpected. It is now understood that cosmic rays induce nuclear reactions on materials to produce {sup 26}Al, on Earth this is well known and it is the basis of many environmental studies, so it is not only the product of some high metalicity star collapse. Taking advantage of the recently reinforced laboratory infrastructure of the Instituto de Física, at UNAM in Mexico City, we proposed to measure the cross section for {sup 26}Al production via some of the most likely reactions, from the nuclear physics point of view (highest Q-values). In this paper the study of the {sup 28}Si(d,α){sup 26} Al nuclear reaction is shown. A target is prepared by a mixture of silicon and aluminum powders. It is irradiated with a deuteron beam (≈1 µA current) at the MV CN-Van de Graaff accelerator laboratory. The number of projectiles is deduced by Rutherford Backscattering Spectrometry (RBS). The produced {sup 26}Al nuclei are then counted at the Accelerator Mass Spectrometry Laboratory.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

Azimuthal correlation and collective behavior in nucleus-nucleus collisions

Various flow effects of nuclear and hadronic origin are investigated in nucleus-nucleus collisions. Nuclear emulsion data collected from {sup 84}Kr + Ag/Br interaction at an incident energy of 1.52 GeV per nucleon and from {sup 28}Si + Ag/Br interaction at an incident energy of 14.5 GeV per nucleon are used in the investigation. The transverse momentum distribution and the flow angle analysis show that collective behavior, like a bounce-off effect of the projectile spectators and a sidesplash effect of the target spectators, are present in our event samples. From an azimuthal angle analysis of the data we also see a direct flow of the projectile fragments and of the produced charged particles. On the other hand, for both data samples the target fragments exhibit a reverse flow, while the projectile fragments exhibit an elliptic flow. Relevant flow parameters are measured.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2014

In-beam γ-ray Spectroscopy of {sup 30}P via the {sup 28}Si({sup 3}He,pγ){sup 30}P Reaction

The level structure of {sup 30}P up to 8.25 MeV was investigated via in-beam γ-ray spectroscopy using the {sup 28}Si({sup 3}He,pγ){sup 30}P reaction at 9 MeV at the University of Tsukuba Tandem Accelerator Complex in Japan. An energy level scheme was deduced from γ-γ coincidence measurements. 47 new transitions have been observed from the previously known states (mostly resonances), thereby reducing the uncertainties in the excitation energies of 17 states from 3 to 10 keV to values of < 1 keV. Furthermore, spin assignments based on measurements of γ-ray angular distributions and γ-γ directional correlation of oriented nuclei (DCO ratios) were made for several observed levels of {sup 30}P.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

Elastic scattering measurements for the system {sup 7}Be+{sup 28}Si at 17.2 MeV

Elastic scattering of {sup 7}Be+{sup 28}Si was studied at several near barrier energies for probing the energy dependence of the optical potential. Our analysis at 17.2 MeV will be presented in this article and discussed, in terms of Continuum Coupled Channel Calculations (CDCC). This research is part of a long term plan concerning the energy dependence of the optical potential for weakly bound projectiles, at near barrier energies and for probing the potential threshold anomaly. The experiment took place at the EXOTIC facility - Laboratori Nationali di Legnaro (LNL), and refers to an angular distribution measurement, using the detector array EXPADES (Exotic Particle Detection System). Results at 9 MeV (Rutherford region) were also analyzed and were used for estimating the solid angle. Our analysis for other energies is under process.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Uniform Silicon Isotope Ratios Across the Milky Way Galaxy

We report the relative abundances of the three stable isotopes of silicon, {sup 28}Si, {sup 29}Si, and {sup 30}Si, across the Galaxy using the v=0,J=1→0 transition of silicon monoxide. The chosen sources represent a range in Galactocentric radii (R{sub GC}) from 0 to 9.8 kpc. The high spectral resolution and sensitivity afforded by the Green Bank Telescope permit isotope ratios to be corrected for optical depths. The optical-depth-corrected data indicate that the secondary-to-primary silicon isotope ratios {sup 29}Si/{sup 28}Si and {sup 30}Si/{sup 28}Si vary much less than predicted on the basis of other stable isotope ratio gradients across the Galaxy. Indeed, there is no detectable variation in Si isotope ratios with R{sub GC}. This lack of an isotope ratio gradient stands in stark contrast to the monotonically decreasing trend with R{sub GC} exhibited by published secondary-to-primary oxygen isotope ratios. These results, when considered in the context of the expectations for chemical evolution, suggest that the reported oxygen isotope ratio trends, and perhaps those for carbon as well, require further investigation. The methods developed in this study for SiO isotopologue ratio measurements are equally applicable to Galactic oxygen, carbon, and nitrogen isotope ratio measurements, and should prove useful for future observations of these isotope systems.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

The {sup 30}P(p, γ){sup 31}S reaction in classical novae: progress and prospects

The unknown thermonuclear rate of the {sup 30}P(p, γ){sup 31}S reaction at classical-nova temperatures currently prohibits the accurate modeling of nova nucleosynthesis in the A ⩾ 30 region. This is hindering the calibration of nova thermometers based on observed O/S, S/Al, O/P, and P/Al abundance ratios in nova ejecta, the calibration of a meter to probe mixing at the core-envelope interface in novae based on the observed Si/H abundance ratio, and the identification of candidate pre-solar nova grains found in primitive meteorites based on laboratory measurements of their {sup 30}Si/{sup 28}Si isotopic ratios. Each of these diagnostics could address key questions in our understanding of classical novae if the {sup 30}P(p, γ){sup 31}S rate were known. We review progress on the determination of the {sup 30}P(p, γ){sup 31}S rate leading to a critical assessment of current interpretations of published data and prospects for future work.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2016

Epitaxially Grown Monoisotopic Si, Ge, and Si{sub 1–x}Ge{sub x} Alloy Layers: Production and Some Properties

The technology of the growth of Si, Ge, and Si{sub 1–x}Ge{sub x} layers by molecular-beam epitaxy with the use of a sublimation source of monoisotopic {sup 30}Si or {sup 28}Si and/or gas sources of monogermane {sup 74}GeH{sub 4} is demonstrated. All of the epitaxial layers are of high crystal quality. The secondary-ion mass spectroscopy data and Raman data suggest the high isotopic purity and structural perfection of the {sup 30}Si, {sup 28}Si, {sup 74}Ge, and {sup 30}Si{sub 1–x}{sup 74}Ge{sub x} layers. The {sup 30}Si layers doped with Er exhibit an efficient photoluminescence signal.

36 MATERIALS SCIENCE↗
DOE OSTI2015

Form factors for dark matter capture by the Sun in effective theories

In the effective theory of isoscalar and isovector dark matter-nucleon interactions mediated by a heavy spin-1 or spin-0 particle, 8 isotope-dependent nuclear response functions can be generated in the dark matter scattering by nuclei. We compute the 8 nuclear response functions for the 16 most abundant elements in the Sun, i.e. H, {sup 3}He, {sup 4}He, {sup 12}C, {sup 14}N, {sup 16}O, {sup 20}Ne, {sup 23}Na, {sup 24}Mg, {sup 27}Al, {sup 28}Si, {sup 32}S, {sup 40}Ar, {sup 40}Ca, {sup 56}Fe, and {sup 59}Ni, through numerical shell model calculations. We use our response functions to compute the rate of dark matter capture by the Sun for all isoscalar and isovector dark matter-nucleon effective interactions, including several operators previously considered for dark matter direct detection only. We study in detail the dependence of the capture rate on specific dark matter-nucleon interaction operators, and on the different elements in the Sun. We find that a so far neglected momentum dependent dark matter coupling to the nuclear vector charge gives a larger contribution to the capture rate than the constant spin-dependent interaction commonly included in dark matter searches at neutrino telescopes. Our investigation lays the foundations for model independent analyses of dark matter induced neutrino signals from the Sun. The nuclear response functions obtained in this study are listed in analytic form in an appendix, ready to be used in other projects.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2016

THE FIRST DISCOVERY OF PRESOLAR GRAPHITE GRAINS FROM THE HIGHLY REDUCING QINGZHEN (EH3) METEORITE

Presolar graphite grains have been extensively studied, but are limited in carbonaceous chondrites, particularly in Murchison (CM2) and Orgueil (CI1), which sampled materials from the oxidizing regions in the solar nebula. Here, we report the first discovery of presolar graphite grains from the Qingzhen (EH3) enstatite chondrite which formed under a highly reducing condition. Eighteen presolar graphite grains were identified by C-isotope mapping of the low-density fraction (1.75–1.85 g cm{sup 3}) from Qingzhen acid residue. Another 58 graphite spherules were found in different areas of the same sample mount using a scanning electron microscope and were classified into three morphologies, including cauliflower, onion, and cauliflower–onion. The Raman spectra of these spherules vary from ordered, disordered, and glassy to kerogen-like, suggestive of a wide range of thermal metamorphisms. NanoSIMS analysis of the C- and Si-isotopes of these graphite spherules confirmed 23 presolar grains. The other 35 graphite spherules have no significant isotopic anomalies, but they share similar morphologies and Raman spectra with the presolar ones. Another three grains were identified during NanoSIMS analysis. Of all the 44 presolar graphite grains identified, six grains show {sup 28}Si-excesses, suggestive of supernovae origins, and four grains are {sup 12}C- and {sup 29,30}Si-rich, consistent with low-metallicity asymptotic giant branch star origins. Another two graphite spherules have extremely low {sup 12}C/{sup 13}C ratios with marginal solar Si-isotopes. The morphologies, Raman spectra, and C- and Si-isotopic distributions of the presolar graphite grains from the Qingzhen enstatite chondrite are similar to those of the low-density fractions from Murchison carbonaceous chondrites. This study suggests a homogeneous distribution of presolar graphite grains in the solar nebula.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2013

Si isotope homogeneity of the solar nebula

The presence or absence of variations in the mass-independent abundances of Si isotopes in bulk meteorites provides important clues concerning the evolution of the early solar system. No Si isotopic anomalies have been found within the level of analytical precision of 15 ppm in {sup 29}Si/{sup 28}Si across a wide range of inner solar system materials, including terrestrial basalts, chondrites, and achondrites. A possible exception is the angrites, which may exhibit small excesses of {sup 29}Si. However, the general absence of anomalies suggests that primitive meteorites and differentiated planetesimals formed in a reservoir that was isotopically homogenous with respect to Si. Furthermore, the lack of resolvable anomalies in the calcium-aluminum-rich inclusion measured here suggests that any nucleosynthetic anomalies in Si isotopes were erased through mixing in the solar nebula prior to the formation of refractory solids. The homogeneity exhibited by Si isotopes may have implications for the distribution of Mg isotopes in the solar nebula. Based on supernova nucleosynthetic yield calculations, the expected magnitude of heavy-isotope overabundance is larger for Si than for Mg, suggesting that any potential Mg heterogeneity, if present, exists below the 15 ppm level.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2017

Structure of the 1d2s Shell from the Data on Single-Nucleon-Transfer Reactions

For the stable silicon isotopes {sup 28}Si and {sup 30}Si, the energies and occupancies of single-particle states of the 1d2s shell are determined by analyzing the combined data for the nucleon stripping and pickup reactions. From the results of analysis and the available experimental data, the variation of the 1d2s proton-shell structure with increasing neutron number for the silicon isotopes with A = 26–34 is discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

Evaluation and Validation of 28,29,30SI Cross Sections in the Resolved Resonance Region

Resonance parameter evaluations of the three stable silicon isotopes 28;29;30 Si, were performed at Oak Ridge National Laboratory in 2002 and the results of those evaluations were restored from the archives in 2018. The evaluations also accounted for the contribution of the direct component of the capture cross sections computed over the neutron resonance range. For the most abundant isotope, 28 Si, the value of the thermal capture cross sections was increased by 10% on the basis of analyses devoted to reevaluating the thermal radiative neutron capture cross sections. The contribution of the direct capture cross sections was recomputed for each isotope, and its energy-dependent behavior improved. Results of benchmark calculations performed at the International Atomic Energy Agency showed an excellent agreement with integral measurements.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗