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All sourcesNASA NTRSDOE OSTI
NASA NTRS1985

Radiative processes

Solar radiation and the processes that control its deposition in the Earth atmosphere are considered. The published data obtained since 1978 define a reference solar spectral irradiance for use in atmospheric chemical and dynamical studies, while long term satellite measurements are now providing information on variations in the output of the Sun over a range of time scales. As concerns absorption of solar radiation in the atmosphere, new cross section data for molecular oxygen and ozone are now available. Line-by-line calculations used to predict infrared flux divergences, both as regards assumptions made in radiative transfer calculations and in the spectroscopic parameters used as inputs are examined. Also examined are the influence of radiative processes on planetary scale wave activity, photochemical acceleration of radiative damping, and the breakdown of local thermodynamic equilibrium at mesospheric altitudes.

Frederick, J. E.↗
NASA NTRS1993

On possibility of diamond formations in radiation process

The possibility of diamond formation in radiation processes was checked by studying diamond contents in carburanium sample. The diamonds were not found and this result is discussed. At present one possible process of formation of nanometer-size diamond crystals in some meteorites and Earth's diamonds (carbonado), the radiation mechanism, is suggested: the formation of diamonds from carbonaceous matter in tracks of U fragment fissions and heavy fragmentation due to the action of energetic particles of cosmic rays. Bjakov et. al. have carried out the calculations and shown that the volume of formed diamonds in carbonaceous chondrites by radiation processes corresponds to discovery of diamond volume in chondrites. The discovery by Ozima et. al. of the unsupported fission of Xe and Kr in carbonado supports the supposition that carbonado could be formed by radiation processes. The possibility of diamond formation in radiation processes leads to the study of diamond contents in Earth's samples enriched by uranium and carbon. The attempt to release the diamonds from carburanium was undertaken.

Fisenko, A. V.↗
NASA NTRS2010

Experimental Investigation of Space Radiation Processing in Lunar Soil Ilmenite: Combining Perspectives from Surface Science and Transmission Electron Microscopy

Energetic ions mostly from the solar wind play a major role in lunar space weathering because they contribute structural and chemical changes to the space-exposed surfaces of lunar regolith grains. In mature mare soils, ilmenite (FeTiO3) grains in the finest size fraction have been shown in transmission electron microscope (TEM) studies to exhibit key differences in their response to space radiation processing relative to silicates [1,2,3]. In ilmenite, solar ion radiation alters host grain outer margins to produce 10-100 nm thick layers that are microstructurally complex, but dominantly crystalline compared to the amorphous radiation-processed rims on silicates [1,2,3]. Spatially well-resolved analytical TEM measurements also show nm-scale compositional and chemical state changes in these layers [1,3]. These include shifts in Fe/Ti ratio from strong surface Fe-enrichment (Fe/Ti >> 1), to Fe depletion (Fe/Ti < 1) at 40-50 nm below the grain surface [1,3]. These compositional changes are not observed in the radiation-processed rims on silicates [4]. Several mechanism(s) to explain the overall relations in the ilmenite grain rims by radiation processing and/or additional space weathering processes were proposed by [1], and remain under current consideration [3]. A key issue has concerned the ability of ion radiation processing alone to produce some of the deeper- penetrating compositional changes. In order to provide some experimental constraints on these questions, we have performed a combined X-ray photoelectron spectroscopy (XPS) and field-emission scanning transmission electron (FE-STEM) study of experimentally ion-irradiated ilmenite. A key feature of this work is the combination of analytical techniques sensitive to changes in the irradiated samples at depth scales going from the immediate surface (approx.5 nm; XPS), to deeper in the grain interior (5-100 nm; FE-STEM).

Christoffersen, R.↗
NASA NTRS2012

High-Resolution and Analytical TEM Investigation of Space Radiation Processing Effects in Primitive Solar System Materials and Airless Planetary Surface Environments

Energetic ions present in the diverse plasma conditions in space play a significant role in the formation and modification of solid phases found in environments ranging from the interstellar medium (ISM) to the surfaces of airless bodies such as asteroids and the Moon. These effects are often referred to as space radiation processing, a term that encompasses changes induced in natural space-exposed materials that may be only structural, such as in radiation-induced amorphization, or may involve ion-induced nanoscale to microscale chemical changes, as occurs in preferential sputtering and ion-beam mixing. Ion sputtering in general may also be responsible for partial or complete erosion of space exposed materials, in some instances possibly bringing about the complete destruction of free-floating solid grains in the ISM or in circumstellar nebular dust clouds. We report here on two examples of the application of high-resolution and analytical transmission electron microscopy (TEM) to problems in space radiation processing. The first problem concerns the role of space radiation processing in controlling the overall fate of Fe sulfides as hosts for sulfur in the ISM. The second problem concerns the known, but as yet poorly quantified, role of space radiation processing in lunar space weathering.

Christoffersen, R.↗
NASA NTRS2012

2D Radiative Processes Near Cloud Edges

Because of the importance and complexity of dynamical, microphysical, and radiative processes taking place near cloud edges, the transition zone between clouds and cloud free air has been the subject of intense research both in the ASR program and in the wider community. One challenge in this research is that the one-dimensional (1D) radiative models widely used in both remote sensing and dynamical simulations become less accurate near cloud edges: The large horizontal gradients in particle concentrations imply that accurate radiative calculations need to consider multi-dimensional radiative interactions among areas that have widely different optical properties. This study examines the way the importance of multidimensional shortwave radiative interactions changes as we approach cloud edges. For this, the study relies on radiative simulations performed for a multiyear dataset of clouds observed over the NSA, SGP, and TWP sites. This dataset is based on Microbase cloud profiles as well as wind measurements and ARM cloud classification products. The study analyzes the way the difference between 1D and 2D simulation results increases near cloud edges. It considers both monochromatic radiances and broadband radiative heating, and it also examines the influence of factors such as cloud type and height, and solar elevation. The results provide insights into the workings of radiative processes and may help better interpret radiance measurements and better estimate the radiative impacts of this critical region.

Varnai, T.↗
NASA NTRS2004

Tropical Convective Responses to Microphysical and Radiative Processes: A Sensitivity Study With a 2D Cloud Resolving Model

Prognostic cloud schemes are increasingly used in weather and climate models in order to better treat cloud-radiation processes. Simplifications are often made in such schemes for computational efficiency, like the scheme being used in the National Centers for Environment Prediction models that excludes some microphysical processes and precipitation-radiation interaction. In this study, sensitivity tests with a 2D cloud resolving model are carried out to examine effects of the excluded microphysical processes and precipitation-radiation interaction on tropical thermodynamics and cloud properties. The model is integrated for 10 days with the imposed vertical velocity derived from the Tropical Ocean Global Atmosphere Coupled Ocean-Atmosphere Response Experiment. The experiment excluding the depositional growth of snow from cloud ice shows anomalous growth of cloud ice and more than 20% increase of fractional cloud cover, indicating that the lack of the depositional snow growth causes unrealistically large mixing ratio of cloud ice. The experiment excluding the precipitation-radiation interaction displays a significant cooling and drying bias. The analysis of heat and moisture budgets shows that the simulation without the interaction produces more stable upper troposphere and more unstable mid and lower troposphere than does the simulation with the interaction. Thus, the suppressed growth of ice clouds in upper troposphere and stronger radiative cooling in mid and lower troposphere are responsible for the cooling bias, and less evaporation of rain associated with the large-scale subsidence induces the drying in mid and lower troposphere.

Li, Xiao-Fan↗
NASA NTRS1981

Effect of laser frequency on a collision-induced radiative process

A review is presented of the principles of collision induced radiative processes, followed by an examination of the effects of laser frequencies on these processes. A one-dimensional problem involving two electron states is considered, and it is found that the Hamiltonian of the radiation field is dominated by electric-dipole interaction which couples states of different parity. Transitions are noted to be dependent on collisions, and the complexities of three-dimensional systems are expressed as considerations of the angular momentum of the photon, the necessity of treating different states simultaneously, and the fact that a radiation field destroys rotational invariance. Changing the radiation frequency alters the crossing point and offers opportunities to study the interplay of potential surfaces with molecular dynamics. Experiments on Na+A systems are outlined for several collision energies and various laser frequencies. Multiple crossings were obtained, although the total cross-section, at all energies, decreased at 18,350/cm.

Devries, P. L.↗
NASA NTRS1981

Numerical experiments on the role of radiative processes in the development and maintenance of upper level clouds

A time-dependent, two-dimensional Eulerian model is presented whose purpose is to obtain more realistic parameterizations of extended high level cloudiness, and the results of a numerical experiment using the model are reported. The model is anelastic and the Bousinesque assumption is invoked. Unresolved subgrid scale processes are parameterized as eddy diffusion processes. Two phases of water are incorporated and equilibrium between them is assumed. The effects of infrared radiative processes are parametrically represented. Two simulations were conducted with identical initial conditions; in one of them, the radiation term was never turned on. The mean values of perturbation potential temperature at each level in the domain are plotted versus height after 15, 30, and 60 minutes of simulated time. The influence of the radiative term is seen to impose a cooling trend, leading to an increased generation of ice water and an increased generation of turbulent kinetic energy in the cloud layer.

Starr, D. O'C.↗
NASA NTRS1984

Modifications to population rate equations resulting from correlations between collisional and radiative processes

There are many systems of physical interest for which a set of rate equations for level populations can provide insight. If the system has two (or more) different mechanisms for effecting transition between levels, total rates of transfer are usually taken as the sum of rates that the individual mechanisms would cause acting alone. Using the example of a hydrogen atom subjected to (ionic and electronic) collisions and external radiation, it is shown that when these individual mechanisms overlap, the total transfer rates must be modified to account for correlations between collisional and radiative processes. For a broad-band radiation field the modified rates have a simple physical interpretation. In the case of a narrow-band field the overlapping events may cause new coherences to appear and interpretation of the modified 'rates' is more complicated.

Ballagh, R. J.↗
NASA NTRS1996

Gamma-ray pulsars: Radiation processes in the outer magnetosphere

We describe an emission model for gamma ray pulsars based on curvature radiation-reaction limited charges in the outer magnetosphere. We show how pair production on thermal surface flux can limit the acceleration zones. Estimates for the efficiency of GeV photon production eta gamma and the gamma-ray beaming fraction are derived, including their dependence on pulsar parameters. In general eta gamma increases with pulsar age, but is decreased for low magnetic fields and for small magnetic inclinations. We argue that this produces GeV pulse profiles, curvature spectra and detection statistics consistent with the observations. We also describe the optical through X-ray pulsar synchrotron spectrum and the spectral variations with pulsar phase. A test computation for Vela-like parameters reproduces phase-resolved GeV spectra consistent with those observed by EGRET. Finally we comment on very high energy pulsed emission and particle production and note extensions needed to allow a more complete pulsar model.

Romani, Roger W.↗
NASA NTRS1988

Radiative processes in upper tropospheric mixed-phase clouds

The diffusional mass evolution of hydrometeors in upper tropospheric clouds for various radiative conditions in the cloud and for varying ambient moisture supply is simulated using a time dependent microphysical model. Radiation can play an important role in this mass evolution when only one phase is present. When both liquid droplets and ice crystals are situated in a typical upper tropospheric environment and the moisture supply is limited, radiation produces only a minor effect on the mass evolution of the hydrometeors. In these cases ice crystals grow quickly at the expense of the droplets and the droplets evaporate within several minutes, even under water supersaturation conditions. Radiation does not significantly influence the evaporation rates of the droplets in the coexisting cases. In the absence of ice crystals and under certain radiative conditions, the droplets can survive when the environment is subsaturated. For other radiative conditiions, the droplets can evaporate when the environment is supersaturated.

Wesley, Douglas A.↗
NASA NTRS2000

SST Variation Due to Interactive Convective-Radiative Processes

The recent linking of Cloud-Resolving Models (CRMs) to Ocean-Mixed Layer (OML) models has provided a powerful new means of quantifying the role of cloud systems in ocean-atmosphere coupling. This is due to the fact that the CRM can better resolve clouds and cloud systems and allow for explicit cloud-radiation interaction. For example, Anderson (1997) applied an atmospheric forcing associated with a CRM simulated squall line to a 3-D OML model (one way or passive interaction). His results suggested that the spatial variability resulting from the squall forcing can last at least 24 hours when forced with otherwise spatially uniform fluxes. In addition, the sea surface salinity (SSS) variability continuously decreased following the forcing, while some of the SST variability remained when a diurnal mixed layer capped off the surface structure. The forcing used in the OML model, however, focused on shorter time (8 h) and smaller spatial scales (100-120 km). In this study, the 3-D Goddard Cumulus Ensemble Model (GCE; 512 x 512 x 23 cu km, 2-km horizontal resolution) is used to simulate convective active episodes occurring in the Western Pacific warm pool and Eastern Atlantic regions. The model is integrated for seven days, and the simulated results are coupled to an OML model to better understand the impact of precipitation and changes in the planetary boundary layer upon SST variation. We will specifically examine and compare the results of linking the OML model with various spatially-averaged outputs from GCE simulations (i.e., 2 km vs. 10-50 km horizontal resolutions), in order to help understand the SST sensitivity to multi-scale influences. This will allow us to assess the importance of explicitly simulated deep and shallow clouds, as well as the subgrid-scale effects (in coarse-model runs) upon SST variation. Results using both 1-D and 2-D OML models will be evaluated to assess the effects of horizontal advection.

Tao, W.-K.↗
NASA NTRS1991

Determination and impact of surface radiative processes for TOGA COARE

Experiments using atmospheric general circulation models have shown that the atmospheric circulation is very sensitive to small changes in sea surface temperature in the tropical western Pacific Ocean warm pool region. The mutual sensitivity of the ocean and the atmosphere in the warm pool region places stringent requirements on models of the coupled ocean atmosphere system. At present, the situation is such that diagnostic studies using available data sets have been unable to balance the surface energy budget in the warm pool region to better than 50 to 80 W/sq m. The Tropical Ocean Global Atmosphere (TOGA) Coupled Ocean Atmosphere Response Experiment (COARE) is an observation and modelling program that aims specifically at the elucidation of the physical process which determine the mean and transient state of the warm pool region and the manner in which the warm pool interacts with the global ocean and atmosphere. This project focuses on one very important aspect of the ocean atmosphere interface component of TOGA COARE, namely the temporal and spatial variability of surface radiative fluxes in the warm pool region.

Curry, Judith A.↗
NASA NTRS1988

Radiative processes in air excited by an ArF laser

The emission spectrum of air that is excited by an ArF laser has been investigated experimentally and theoretically to determine the conditions under which fluorescence from O2 can be used for the measurement of temperature in aerodynamic flows. In addition to the expected fluorescence from O2, the spectrum from excitation with an intense laser beam is shown to contain significant contributions from the near-resonant Raman fundamental and overtone bands, the four-photon fluorescence excitation of C produced from ambient CO2, and possibly the three-photon excitation of O(2+). The nature of the radiative interactions contributing to these additional features is described.

Laufer, Gabriel↗