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At least 19 records

Patterns of indoor radon concentrations, radon-hazard potential, and radon testing on a small geographic scale in Utah

Currently, there are no publicly-available estimates of indoor radon concentration at scales smaller than the county. Radon-hazard potential soil maps that reflect underlying geologic factors can be created at small geographic scale and linked to residential and census data. We determined the association between residential radon tests and high radon-hazard potential soil at the residential and block group levels using a large Utah-based dataset. We also identified characteristics of block groups with limited tests in the dataset.

63 RADIATION, THERMAL, AND OTHER ENVIRON. POLLUTAN↗

Intercomparison of Commercially Available Active Radon Measurement Devices in a Discovered Radon Chamber

An unventilated 70 m 3 underground space, with 2.1 m high ceilings and an inner set of concrete walls to damp vibrations, was discovered to have relatively stable radon levels of ~1,080 Bq m -3 over a 1-y period. The addition of radium sources was not required to achieve high and somewhat variable radon levels, as these arise naturally in the space. Several active radon monitoring devices designed for homeowners, radon screeners, radon mitigation professionals, and researchers were tested in the space. These devices were variable in both cost and intended user sophistication. Data were collected at specific time intervals that varied for each device. A cellphone was deployed with an available camera application to periodically capture photographs of the displays of devices not enabled for automatic temporal recording. Attempts were made to alter the radon concentration using fans, radium-laden objects, and radon impermeable sheets. Statistical methods were employed to compare the device's performance under the minor radon transients produced by the addition of 226 Ra sources during the test period. The evaluation of the overall accuracy, noise, and response to transients revealed highly affordable devices that may be useful for future research applications.While unsuitable for precise calibrations at stable radon levels, the space was determined to be adequate as a radon chamber for general research purposes.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Prediction of radon removal efficiency for a flow-through activated charcoal system and radon mitigation characteristics

Activated charcoal was widely used in radon researches and mitigation applications because of good adsorption ability. Here in the paper, a simple model that can predict radon removal efficiency (η) for radon mitigation applications using flow-through activated charcoal system was developed based on the previous works. Experiments were conducted with a flow-through activated charcoal system to validate the model and study the influence of factors on η. The experimental results of η are consistent with the theory to within 4% at the flow rates of 1–3 L/min, but range from 2% to 14% at the flow rates of 4–5 L/min. The equilibrium time of radon linearly decreases with rising flow rate, and η decreases with rising flow rate. With moisture competing with radon for adsorption sites on the activated charcoal, radon reaches the equilibrium concentration more quickly than moisture does. As relative humidity increases, η decreases, but the radon equilibrium concentration increases. The values of η are bigger for those smaller particle sizes with the same type of activated charcoal. The results of this paper are useful for designing activated charcoal systems at indoor environmental conditions and predicting η for radon mitigation applications.

07 ISOTOPE AND RADIATION SOURCES↗

Method for calculating radon activity and radon rejection using a beta-gamma detector

Radon interferes with concentration measurements used by atmospheric radioxenon systems. We demonstrate a method to quantify the amount of radon that is present in the detectors, the impact of radon activity on the minimum-detectable-concentrations, and how to determine the needed radon rejection levels. An example calculation shows a radon rejection level of 10 5 is sufficient to limit impact on the detector sensitivity. We anticipate this method will give analysist a better understanding of radon present in their measurements and allow system designers to tailor their systems’ radon rejection better for its location.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Low Level Radon Concentration and Radon Daughter Dose Monitoring in an Arid-zone Waste Store - 20081

Radioactive waste containing predominantly soil and rubble from the clean-up of a former uranium and thorium minerals processing research facility is currently stored at the Woomera Test Range in South Australia awaiting final disposal. Prior to commencing any manipulation of the nearly 10,000 waste drums (205 L or 55 gallon each), radon concentration monitoring and radon daughter dosimetry has been undertaken to (i) gain understanding of the temporal and spatial variation of radon and its daughters within the storage facility, which could provide insights into the radiological source term and (ii) confirm that radiological risks to workers are below the guideline values. A time series of nearly 12 months of detailed observations shows low level radon concentrations with annual average values that are slightly above the average radon concentrations in Australian homes. Peak values in summer are about three times higher than the annual average based on the CRM measurements. Both radon concentrations and annual effective dose are well below the regulatory limits. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Radon kinetics in a natural indoor radon chamber

An unusual 180 m 3 storage room in the basement of a two-story laboratory building is unventilated, and separated from occupiable rooms by double steel doors. The space completely borders on soil through the concrete floor and two of its concrete walls. The room also contains a separate inner chamber with 1 m thick concrete walls designed to damp vibrations in the room above it. The space boasts a relatively high radon level, 1083 Bq m –3 , which varies with local outdoor environmental conditions. Measurements were made of radon concentrations at various locations and heights within the facility. More than a year of continuous radon concentration data corresponding to a single location are also available, along with measurements of indoor and outdoor pressure, temperature, and humidity. Data were also collected with as many as five fans placed in different locations and cycled on for variable time periods. First order linear kinetic models were created to explain the observed approaches to steady state due to changing conditions and wash-out resulting from intentional ventilation. Results demonstrate a good fit between changes in the radon concentration level and the developed compartmental models. Furthermore, no significant differences were observed between radon concentration at different locations or heights in the chamber.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Quantifying mean, variability, and uncertainty in indoor radon exposure in Pennsylvania using random forest and quantile regression forest models

Radon is a naturally occurring radioactive gas that poses a serious health risk as the primary cause of lung cancer in non-smokers. Despite the well-known adverse association with health outcomes, current radon exposure assessments are limited to county-level or average-level estimates, which fail to capture regional variability. This study uses Machine Learning models, including Random Forest (RF) and Quantile Regression Forest (QRF), to estimate the indoor radon concentrations at the ZCTA (Zip code tabulation area)-level and characterize uncertainties in model estimates. Incorporating geological, meteorological, and building-specific data, the models aim to improve radon risk assessment by capturing mean exposure, variability, and extreme concentration levels. Processed radon test data (n = 718,111) were analyzed using average, variability, and quantile prediction methods. Models that estimate the average radon exposure at the ZCTA-level can yield promising model-fit results, but they do not capture the underlying variability of indoor radon exposure within a ZCTA. We utilize volatility analyses to identify characteristics indicative of high variability of indoor radon exposure. We also show that a QRF model can be used to estimate upper quantiles of residential radon exposure, thereby uncovering localized areas of elevated exposure that were not apparent in mean estimates. The results highlighted the need for a deep characterization of exposure risk and show that regions with moderate average exposure levels could still harbor extreme outliers with implications for evaluating health risks. Utilizing multiple radon exposure models allows for a deeper characterization of radon risk within a geographic area and can better identify high-risk areas. The results from this study provide a foundation for developing mitigation strategies and examining associations between radon exposure and health outcomes at fine scales. Future research should extend the geographic scope and incorporate additional environmental risk factors to establish a comprehensive framework for risk assessment.

Lee, Heechan [ORNL]↗

Performance study of charcoal-based radon reduction systems for ultraclean rare event detectors

The continuous emanation of radon due to trace amounts of uranium and thorium in detector materials introduces radon to the active detection volume of low-background rare event search detectors. 222 Rn produces a particularly problematic background in the physics region of interest by the "naked" beta decay of its 214 Pb daughter nucleus. While charcoal-based adsorption traps are expected to be effective for radon reduction in auxiliary circulation loops that service the warm components of current ton-scale detectors at slow flow rates (0.5-2 SLPM), radon reduction in the entire circulation loop at high flow rates $\mathcal{O}$(100s SLPM) is necessary to reach high sensitivity in future generation experiments. In this article we explore radon dynamics with a charcoal-based radon reduction system in the main circulation loop of time projection chamber detectors. Here, we find that even for perfect radon traps, circulation speeds of 2,000 SLPM are needed to reduce radon concentration in a 10 ton detector by 90%. This is faster by a factor of four than the highest circulation speeds currently achieved in dark matter detectors. We further find that the effectiveness of vacuum swing adsorption systems, which have been employed very successfully at reducing atmospheric radon levels in clean-rooms, is limited by the intrinsic radon activity of the charcoal adsorbent in ultra-low radon environments. Adsorbents with significantly lower intrinsic radon activity than in currently available activated charcoals would be necessary to build effective vacuum swing adsorption systems operated at room temperature for rare event search experiments. If such VSA systems are cooled to about 190 K, this requirement relaxes drastically.

47 OTHER INSTRUMENTATION↗

Radon Kinetics in a Basement Space Measured with Different Devices

Although indoor monitoring of radon and benchmarking of radon measurement devices remain important research topics, few intercomparisons of active radon measurement devices have been performed under realistic conditions, let alone dynamic ones enabling comparison of their transient behavior. Five different radon monitors were therefore placed in a poorly ventilated basement space under three different conditions: 24 h under a steady, elevated radon level, 24 h with fans turned on to produce a radon washout transient, and 9 d with fans turned off for a radon buildup transient. Resulting radon concentrations varied between ~200 and ~2,000 Bq m -3 . Accuracy of the devices were evaluated using root-mean-square error, and ventilation data were fit to first order linear compartmental models. To more accurately model behaviors such as cyclic diurnal variations, the source term corresponding to entry of radon from soil into the basement was considered to be non-constant, as it is likely to vary drastically with both the indoor-outdoor pressure differential and soil concentration variations. Here, the improved radon washout model fit very well with the measurements. Despite a wide variety in list prices, all devices performed similarly during transients and at different radon concentrations.

60 APPLIED LIFE SCIENCES↗

Automated anomalous behaviour detection in soil radon gas prior to earthquakes using computational intelligence techniques

Here in this article, three computational intelligence (CI) models were developed to automatically detect anomalous behaviour in soil radon gas ( 222 Rn) time series data. Data were obtained at a fault line and analysed using three machine learning techniques with the aim at identifying anomalies in temporal radon data prompted by seismic events. Radon concentrations were modelled with corresponding meteorological and statistical parameters. This leads to the estimation of soil radon gas without and with meteorological parameters. The comparison between computed radon concentration and actual radon concentrations was used in finding radon anomaly based upon automated system. The anomaly in radon time series data could be considered due to noise or seismic activity. Findings of study show that under meticulously characterized environments, on exclusion of noise contribution, seismic activity is responsible for anomalous behaviour seen in radon time series data.

58 GEOSCIENCES↗

High-resolution modeling of indoor radon exposure with uncertainty quantification in Utah

Indoor radon accounts for 37% of population-level exposure to ionizing radiation in the United States. However, radon metrics are typically reported at coarse spatial scales, potentially obscuring meaningful local variation. We developed a high-resolution modeling framework to estimate indoor radon concentrations across Utah while explicitly quantifying predictive uncertainty. A total of 19,497 residential radon measurements collected between 2006 and 2017 were combined with environmental and housing characteristics and analyzed using a geospatial neural network that accommodates spatial dependence and nonlinear associations. Predictions were generated on a uniform hexagonal grid at 0.73 km2 resolution (H3 level 8). Out-of-sample predictions aggregated to the H3 level 8 grid showed good agreement with observed concentrations (Pearson r=0.64), while household-level predictions exhibited more moderate agreement (r=0.45). The model produced well-calibrated uncertainty estimates, with 24.1% of held-out observations exceeding the predicted 75th-percentile threshold. Maps of predicted radon concentrations and the probability of exceeding the U.S. EPA action level of 148 Bq/m3 (4 pCi/L) revealed substantial fine-scale spatial heterogeneity that was not apparent in conventional coarse-resolution summaries, with greater local variability observed in densely monitored urban counties than in sparsely sampled regions. High-resolution radon models that explicitly quantify uncertainty provide a useful framework for characterizing the spatial distribution of indoor radon and identifying areas of elevated exceedance risk. These findings highlight the value of fine-scale monitoring data and uncertainty-aware modeling approaches for radon exposure assessment, environmental risk characterization, and radon-related health research.

Wu, Yunhan [ORNL] (ORCID:0000000178842994)↗

Radon Photoionization: Project Technical Report

In most low-background physics experiments, radon is a significant and problematic source of background radiation because it is inert and sufficiently long-lived to pervade laboratory spaces. It may be possible to manipulate (and thus mitigate) radon electromagnetically by taking advantage of its relatively low first ionization energy. When considering ambient-temperature gas phases, only iodine is comparable. The other noble gases, and the most important constituents of breathable air (nitrogen and oxygen), all have higher ionization energies; so it may be possible to selectively manipulate radon in a variety of gas streams by ionizing it with an appropriately low-energy source of photons. Radon’s first ionization energy is in the vacuum UV part of the electromagnetic spectrum, which can be produced using a deuterium lamp. In this report, we present our attempts to manipulate radon via UV photoionization in a laboratory setting. This approach has the potential to increase radon removal efficiency from gases and/or to improve the efficiency of radon detectors. Unfortunately, our experiments suggest that either the life-time of a photoionized radon ion (before it re-neutralizes) is too short to be of much practical use and/or that our low-cost UV-photon source was not sufficiently energetic for efficient photoionization of radon.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

A Review of Variables Impacting the Indoor Inhalation Radon Equilibrium Factor (FEQ)

With radon and its daughter products estimated as the second leading cause of lung cancer in the United States, it is imperative to understand their relative equilibrium inside commercial, community, and residential dwellings. The radon indoor inhalation fractional equilibrium factor (F eq ) quantifies the disequilibrium between radon and its progeny in indoor air, and recent advances have shown how air exchange rates (ACH) influence F eq . These numerically derived ACH-dependent F eq values are incorporated into the U.S. EPA's Radon Vapor Intrusion Screening Level (RVISL) calculator, which assists risk assessors in evaluating radon exposure. To advance the risk assessment science of actinon (Rn-219), thoron (Rn-220), and radon (Rn-222), the impact of variables such as indoor aerosol concentration and composition, outdoor air quality, household-specific characteristics, and environmental/meteorological conditions on the F eq must be examined. The primary objective of this research is to analyze these additional variables to determine the usefulness of incorporating such adjustment factors into the RVISL calculator and to identify areas of future research. Studies regarding the influence of these parameters are presented along with recommendations regarding the adjustment of the numerically derived F eq value. For example, elevated indoor aerosol concentrations, such as those originating from outdoor PM 2.5 or cigarette smoke, increase the abundance of accumulation- mode particles indoors, which in turn raises F eq values by facilitating the attachment of radon progeny to these aerosols. Smoking increases both the bronchial dose and F eq , while regions with high smog levels demonstrate the impact of regional air quality on F eq . In contrast, air cleaning systems and purifiers have been shown to reduce the F eq , suggesting that these systems could help mitigate radon exposure. Additionally, higher F eq values are typically observed during winter when ventilation rates are lower. This paper presents adjustment factors that may be applied to the RVISL F eq , emphasizing the need for further research to refine these variables and ensure accurate risk assessments in diverse environments. Applying these adjustment factors will minimize calculator over- and underestimations, providing a more accurate representation of the real-world risk associated with radon.

54 ENVIRONMENTAL SCIENCES↗