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At least 19 records

Development of a Helical Closure for Radioactive Material Shipping Packages

Radioactive Material (RAM) Packagings Used to transport radioactive material • Weapons components • Medical isotopes • Spent nuclear fuel • Etc. • Packages must adhere to 10 CFR 71 which drive to NUREGs, ASME codes, etc. • Transport Index (A2 values) determine if a package is Type A, Type AF, Type B, Type B(U)F

Housley, William M. [Savannah River National Labor↗

Technical Basis Related to the Posture of NASA’s Office of Safety and Mission Assurance for the Launch of Radioactive Material Other than Space Nuclear Systems: Volume 1–Overview of Analysis and Results

NASA has launched and reentered payloads containing radioactive material for over 50 years. The isotopes, their quantity, and their form have varied significantly. The handling of this material prior to its integration into the spacecraft at the launch Center (and after its return to Earth after flight, if applicable) falls under the purview of the Office of the Chief Health and Medical Officer, while after the radioactive material is integrated into the spacecraft at the launch Center, it falls under the purview of the Office of Safety and Mission Assurance’s (OSMA) Nuclear Flight Safety Program. Historically, OSMA concurrence was required for any launch or reentry involving radioactive material. However, OSMA recently revisited this posture due to changes in the Federal policy in this area, and the significant accrued experience. The current report represents the more quantitative study envisioned in the recent change in posture. More specifically, this document addresses the potential risks and other considerations associated with launching small quantities of radioactive material (below the level requiring the Federally-mandated process in National Security Presidential Memorandum- (NSPM-) 20, “Presidential Memorandum on Launch of Spacecraft Containing Space Nuclear Systems” (USG, 2019) to provide the technical basis for when such activities require OSMA concurrence versus notification, as it relates to nuclear flight safety.

Don Helton↗

Development of a Helical Closure for Radioactive Material Shipping Packages

The Savannah River National Laboratory (SRNL) Packaging Technology group proposed a closure design for the outer packaging of a prototype Type B shipping package being developed for the Department of Energy (DOE). The closure design provides an efficient means of securing the containment vessel (CV) within the radioactive material packaging. This design has a simplified operation, requires less components, and less maintenance when compared to current radioactive material package closure methods. This paper will review and discuss the materials, designs, processes, and testing activities that were considered and pursued in the development of the novel closure for the outer packaging of new radioactive material shipping packages.

Housley, William M. [Savannah River National Labor↗

THE DESIGN OF RADIAL HONEYCOMB LATTICES FOR IMPACT ENERGY ABSORPTION IN RADIOACTIVE MATERIALS PACKAGES

In this research we present a variation on the corrugation technique of honeycomb lattices, for cylindrical honeycombs, making them much easier to design for impact energy absorption in radioactive materials packages. This variation, termed radial honeycomb lattices, eliminates the residual strain and saddle effect. The use of honeycomb lattices provides advantages over the typically used foams. While foams are effective at absorbing impact energy, they can burn, their material properties are difficult to control, they can degrade over time, and procurement of raw materials can be dependent on timing of manufacturer batch runs. While the weaknesses of foam are strengths for honeycomb lattices, lattices have a different set of problems. Typically, when cylindrical honeycomb lattices are manufactured, they are manufactured flat, wrapped around a mandrel of the desired radius, and then brazed. This approach introduces residual strains, resulting in the saddle effect, which limits both the radial thickness and cylinder length. The radial honeycomb lattice approach presented here makes the design of thicker and longer cylinder honeycombs possible. To address these issues, we propose a honeycomb lattice which changes in cross-section from the inner to the outer radius of the cylinder. This causes the lattice to automatically wrap into a cylinder as it exits the corrugating gears. The theoretically bounding case, of a square cross-section at the inner radius, transitioning through a hexagon, to a diamond cross-section at the outer radius, results in a maximum thickness of approximately 41% of the inner radius. Full mathematical derivations, implemented in computer code, allow for the design of an entire radial honeycomb lattice, including the corrugating gears. To accomplish this only the radial thickness, inner cross-section shape, cell size, and nominal gear radius need to be specified, making the design of these lattices very efficient. Radial honeycomb lattice prototypes have demonstrated that the honeycomb does indeed wrap into a cylinder as intended, without the saddle effect, and can therefore be used to create thick-walled cylinders of any length. These design improvements make cylindrical honeycomb lattices much more accessible as a design element for radioactive materials packages

Johnson, William R. [Savannah River National Labor↗

Eddy covariance towers as sentinels of abnormal radioactive material releases

Ensuring accurate detection and attribution of abnormal releases of radioactive material is critical for protecting human health and safety. Most commonly, such detection is accomplished via active monitoring approaches involving the collection of physical samples. Further, this is labor intensive and limits the temporal and spatial resolution of any detected events to a relatively coarse level. As an alternative first step towards passive monitoring, we developed an approach using eddy flux tower data records to identify signals from a known abnormal release and quantify the extent to which that signal also occurs at other times in the data record. Through two case studies, one of which targeted the Fukushima nuclear disaster and the other targeting an abnormal release event at a radioisotope production facility in Fleurus, Belgium, we tested our approach and identified several potential heretofore unidentified abnormal events that were consistent with atmospheric circulation patterns and/or wind direction from known release sites. Because our approach is relatively simple and is resistant to systematic errors in the observational record, it has broad applicability beyond specific constituents and ecosystem types to identify a wide variety of limited-duration anomalies in flux tower data to ensure human health and industrial safety.

54 ENVIRONMENTAL SCIENCES↗

Remote detection of radioactive material using a short-pulse CO 2 laser

Detection of radioactive material at distances greater than the radiated particle range is an important goal with applications in areas such as national defense and disaster response. Here, we demonstrate avalanche-breakdown-based remote detection of a 3.6 mCi α-particle source at a standoff distance of 10 m, using 70 ps, long-wave infrared (λ = 9.2 µm) CO 2 laser pulses. This is ∼10 times longer than our previous results using a mid-IR laser. The primary detection method is direct backscatter from microplasmas generated in the laser focal volume. The backscatter signal is amplified as it propagates back through the CO 2 laser chain, enhancing sensitivity by >100 times. Here we also characterize breakdown plasmas with fluorescence imaging, and present a simple model to estimate backscattered signals as a function of the seed density profile in the laser focal volume. All of this is achieved with a relatively long-drive laser focal geometry (f/200) that is readily scalable to >100 m.

43 PARTICLE ACCELERATORS↗

Assessment of Naturally Occurring Radioactive Material (NORM) in Illicit Drugs Using High-Resolution Gamma Spectroscopy

This report documents results assessing the presence of Naturally Occurring Radioactive Material (NORM) in illicit drugs using high-resolution gamma spectroscopy. Specifically, high-purity germanium (HPGe) measurements were conducted at the Drug Enforcement Administration (DEA) South Central Laboratory on 11 samples (referred to as exhibits) including cocaine, fentanyl, heroin, ketamine, LSD, marijuana, methamphetamines, psilocybin mushrooms, and synthetic cannabinoids.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Using radioactive material to evaluate decontamination of contaminated electronics

Electronic materials are used everywhere and can get easily contaminated by their use in the field/laboratory. The goal of this project was to use radioactive material to track the effectiveness of a cleaning procedure using an off-the-shelf cleaning gel. Radioactive potassium bromide (KBr) was used as a model contaminant in four contamination scenarios to gauge the effectiveness of a cleaning gel in the decontamination of contaminated raspberry pi’s. Finally, the investigated decontamination technique was found to be 75–97% effective in removing contamination from the tested electronic devices. 95% of the contaminated electronic devices retained their functionality post-decontamination.

38 - RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCL↗

Explosively Formed Helical Closure for Radioactive Material Packaging

Benefits • Allows for the creation of features in thin-walled metal parts that would otherwise be impossible or impractical to create. • Reduces margin of error during radioactive material package closure. • Increases efficiency of package closure and opening. Applications and Industries • The tooling and method could be used to create closures for any industrial application. There may be use for the geometry produced by the tooling and method that is outside of closures.

Timmons, Darren↗

Automated technologies needed to prevent radioactive materials from reentering the atmosphere

Project SIREN (Search, Intercept, Retrieve, Expulsion Nuclear) was created to identify and evaluate the technologies and operational strategies needed to rendezvous with and capture aerospace radioactive materials (e.g., a distressed or spent space reactor core) before such materials can reenter the terrestrial atmosphere and then to safely move these captured materials to an acceptable space destination for proper disposal. A major component of the current project SIREN effort is the development of an interactive technology model (including a computerized data base) that explores, in building-block fashion, the interaction of the technologies and procedures needed to successfully accomplish a SIREN mission. The SIREN model will include appropriate national and international technology elements--both contemporary and projected into the next century. To obtain maximum flexibility and use, the SIREN technology data base is being programmed for use on 286-class PC's. The major technical elements for a successful SIREN mission include: ground and space-based tracking, launch vehicles of needed payload capacity, telerobotic systems, sensors, capture technologies, and space transport and disposal. However, Project SIREN also will impose specialized requirements including the use of dextrous aerospace systems capable of properly functioning in intense radiation and thermal environments.

Buden, David↗

Automated technologies needed to prevent radioactive materials from reentering the atmosphere

Project SIREN (Search, Intercept, Retrieve, Expulsion Nuclear) has been created to identify and evaluate the technologies and operational strategies needed to rendezvous with and capture aerospace radioactive materials (e.g., a distressed or spent space reactor core) before such materials can reenter the terrestrial atmosphere and then to safely move these captured materials to an acceptable space destination for proper disposal. A major component of the current Project SIREN effort is the development of an interactive technology model (including a computerized data base) that explores in building block fashion the interaction of the technologies and procedures needed to successfully accomplish a SIREN mission. This SIREN model will include appropriate national and international technology elements-both contemporary and projected into the next century. To permit maximum flexibility and use, the SIREN technology data base is being programmed for use on 386-class PC's.

Buden, David↗

Transfer functions for Q A /Q B international regulatory limits for the safe transport of radioactive materials

This paper presents a proposed revision of the International Atomic Energy Agency transport regulations, related to the A 1 and A 2 limit values used to determine the radioactive transport classification. Based on the 'Q system', a novel methodology was introduced to derive Q A and Q B values related to scenarios involving external exposure from a distant source. These values are key parameters that respectively represent the total effective dose and total equivalent dose to the skin, from all primary and secondary particles contributing to radiation exposure. The International Working Group (WG A 1 /A 2 ) is established and associated with the TRANSSC Technical Expert Group on Radiation Protection. A review of the A 1 and A 2 values is performed in response to identified limitations within the existing Q system. The followed approach is based on Monte Carlo simulations that enabled the development of transfer functions aimed at reducing computational time and increasing the flexibility of dose evaluations for any radionuclide with known particle emission spectra. This method allows updating the Q A and Q B values to account for future data evolutions (decay data, fluence-to-dose conversion coefficients) and standardizing the calculation of regulation limits across all referenced radionuclides and scenarios related to external exposure. The transfer functions are established using three Monte Carlo simulation codes—FLUKA, Geant4, and MCNP—and address the previous limitations of the 'Q system', reflecting the latest International Commission for Radiation Protection recommendations and improvements in calculation techniques. The results of the WG show consistent agreement across the codes, with minor discrepancies observed at low primary energies due to statistical uncertainties and different handling of stopping power for electrons/positrons in the codes. This revised approach aligns with current standards and recommendations, ensuring that the radiological consequences of transport accidents are acceptable for the new A 1 and A 2 limits from a radiological protection perspective.

61 RADIATION PROTECTION AND DOSIMETRY↗

Low radioactivity material for use in mounting radiation detectors

Two materials, sapphire and synthetic quartz, have been found for use in Ge detector mounting assemblies. These materials combine desirable mechanical, thermal, and electrical properties with the radioactive cleanliness required to detect minimal amounts of K, Th, and U.

Fong, Marshall↗

Evaluation of the Radioactive Material Released in the Harborview Research and Training Building and Some Implications for Emergency Response

On 2 May 2019, during the 137 Cs source recovery operation, a source capsule in a research irradiator containing approximately 77.1 TBq was breached. Based on a geometric reconstruction analysis of the damage to the capsule, approximately 46.3 GBq (0.04%) was impacted by the chop saw (grinder) inside a mobile hot cell on the loading dock at the University of Washington Harborview Research and Training (HRT) Building. A very small fraction of the material impacted, less than 1%, was released from the mobile hot cell and then to the rest of the HRT Building. The objectives of this project were to assess the accidental release of 137 CsCl and its implications related to emergency response methods and the ramifications of 137 CsCl transport. The phenomenology of this event was also compared with past alkali halide dispersal events. The vast number of measurements and samples collected by the remediation contractors, the Department of Energy’s Nuclear Emergency Support Team, and the small number of retrospective samples collected by the authors informed the analysis. The techniques included (1) autoradiography and electron microscopy of samples collected from the HRT Building and the irradiator, (2) 3D visualization of deposition on surfaces and within the ventilation system, and (3) a study of the damage to the source capsule to evaluate the Cs particle size and particle composition due to the grinding accident. Subsequently, the cesium contaminant transport through the numerous pathways in the building was reconstructed to assess the deposition on surfaces as a function of particle size. Furthermore, the implications for emergency response are relevant to data quality and management. A Data Quality Objective guides data collection methods so that they have appropriate accuracy and precision for the intended application. Recommendations were made with respect to the sample collection protocols and archiving of samples.

46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN↗

Evaluation of the Radioactive Material Release in the Harborview Research and Training Building and Implications for Emergency Response

On May 2, 2019, during the 137 Cs source recovery operation, a source capsule in a research irradiator containing approximately 77.1 TBq was breached. Based on a geometric reconstruction analysis of the damage to the capsule, approximately 46.3 GBq (0.04%) was impacted by the chop saw (grinder) inside a Mobile Hot Cell (MHC) on the loading dock at the University of Washington Harborview Research and Training (HRT) Building. A very small fraction of the material impacted, less than 1%) was released from the Mobile Hot Cell and then to the rest of the HRT Building. The objectives of this project were to assess the accidental release of 137 CsCl and its implications related to emergency response methods and the ramifications of 137 CsCl transport. The phenomenology of this event was also compared with past alkali halide dispersal events. The vast number of measurements and samples collected by the remediation contractors, the Department of Energy's Nuclear Emergency Support Team, and the small number of retrospective samples collected by the authors informed the analysis. The techniques included (1) autoradiography and electron microscopy of samples collected from the HRT Building and the irradiator, (2) 3D visualization of deposition on surfaces and within the ventilation system, and (3) a study of the damage to the source capsule to evaluate the Cs particle size and particle composition due to the grinding accident. Subsequently, the cesium contaminant transport through the numerous pathways in the building was reconstructed to assess the deposition on surfaces as a function of particle size. The implications for emergency response are relevant to data quality and management. A Data Quality Objective (DQO) guides data collection methods so that they have appropriate accuracy and precision for the intended application. Recommendations were made with respect to the sample collection protocols and sample archival.

61 RADIATION PROTECTION AND DOSIMETRY↗