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PdN2 crystallizes in the orthorhombic Immm space group. The structure is one-dimensional and consists of two PdN2 ribbons oriented in the (0, 1, 0) direction. Pd2+ is bonded in a linear geometry to two equivalent N1- atoms. Both Pd–N bond lengths are 1.94 Å. N1- is bonded in a linear geometry to one Pd2+ and one N1- atom. The N–N bond length is 1.14 Å.
PdN2(NH3)4(NO2)4 crystallizes in the triclinic P-1 space group. The structure is zero-dimensional and consists of two ammonia molecules, four ammonia molecules, four nitrous acid molecules, and one palladium molecule.