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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

Advancing extreme pulsed lasers through measurements: summary of the pulsed laser metrology workshop

In this report we present consensus findings produced during the pulsed laser metrology (PLM) workshop (Boulder, CO, USA, August 2025). The workshop was a meeting of 35 scientists from private industry, academia, and U.S. government to compile a list of the metrology needs to support extreme pulsed laser development and implementation. We define ‘extreme pulsed lasers’ loosely as those with peak powers above 1 TW or multi-Joule pulse energies. Such lasers are being increasingly used and investigated for use in high energy particle acceleration, short wavelength radiation generation, laser-based fusion, etc. The rapid growth of these fields and the proliferation of extreme lasers for these applications, coupled with the extreme electric fields they generate and relative scarcity of such lasers, presents unique challenges to accuracy in their measurement. The PLM workshop was a two-day event designed to hear from users, developers, and researchers on the current state of optical metrology associated with these extreme pulsed lasers. The goal was to identify the most important measurement challenges limiting development and implementation of these lasers in practical applications. We report here the conclusions and recommendations of this workshop. The hope is that this document will become the first of many iterations which track the status of measurement needs supporting extreme pulsed lasers.

Lasers↗
DOE OSTI2026

Robust direct laser acceleration of electrons with flying-focus laser pulses

Direct laser acceleration (DLA) offers a compact source of high-charge, energetic electrons for generating secondary radiation or neutrons. While DLA in high-density plasma optimizes the energy transfer from a laser pulse to electrons, it exacerbates nonlinear propagation effects, such as filamentation, that can disrupt the acceleration process. Here, we show that superluminal flying-focus pulses (FFPs) mitigate nonlinear propagation, thereby enhancing the number of high-energy electrons and resulting x-ray yield. Three-dimensional particle-in-cell simulations show that, compared to a Gaussian pulse of equal energy (1 J) and intensity (2 × 10 20 W/cm 2 ), an FFP produces 80 × more electrons above 100 MeV, increases the electron cutoff energy by 20%, triples the high-energy x-ray yield, and improves x-ray collimation. These results illustrate the ability of spatiotemporally structured laser pulses to provide additional control in the highly nonlinear, relativistic regime of laser-plasma interactions.

Laser-produced plasmas↗
DOE OSTI2026

Microscopy X-ray imaging enriched with small angle X-ray scattering for few nanometer resolution reveals shock waves and compression in intense short pulse laser irradiation of solids

Understanding how laser pulses compress solids into high-energy-density states requires diagnostics that simultaneously resolve macroscopic geometry and nanometer-scale structure. Here we present a combined X-ray imaging (XRM) and small-angle X-ray scattering (SAXS) approach that bridges this diagnostic gap. Using the Matter in Extreme Conditions end station at LCLS, we irradiated 25 μm copper wires with 45 fs, 0.9 J, 800 nm pulses at 3.5 × 10 19 W/cm 2 while probing with 8.2 keV XFEL pulses. XRM visualizes the evolution of ablation, compression, and inward-propagating fronts with ∼ 200 nm resolution, while SAXS quantifies their nanometer-scale sharpness via the time-resolved evolution of scattering streaks. The joint analysis reveals that an initially smooth compression steepens into a nanometer-sharp shock front after t sh ≈ (18 ± 3) ps, consistent with an analytical steepening model and hydrodynamic simulations. The front reaches a velocity of c sh ≈ 25 k m / s and a lateral width of several tens of microns, demonstrating direct observation of shock formation and decay at solid density for the first time with few-nanometer precision. This integrated XRM–SAXS method establishes a quantitative, multi-scale diagnostic of laser-driven shocks in dense plasmas relevant to inertial confinement fusion, warm dense matter, and planetary physics.

Kluge, Thomas [Helmholtz-Zentrum Dresden-Rossendor↗
DOE OSTI2025

Particle Beam Acceleration Using 3 Petawatt Laser Pulses

The Zettawatt-Equivalent Ultrashort pulse laser System (ZEUS) is presently operational at the Gerard Mourou Center for Ultrafast Optical Science (CUOS) at the University of Michigan. ZEUS is a significant upgrade of the previous high power laser systems at CUOS and consists of two beamlines thatoperate in perfect synchronization. The 500 TW beamline became operational in 2023, 2 PW operation started in 2025 and full 3 PW power levels will be available in 2026. It is presently the highest power laser system in the US. In this grant the high field science group at CUOS has leveraged this unique high power laser facility to investigate laser wake field acceleration (LWFA) in ultra-high power laser plasma interactions and have shown how this can scale for future electron–positron colliders at high energy. The dual beam experimental configuration enables flexibility for many frontier experiments in laser-driven acceleration research, in particular, enabling extended channelling/acceleration experiments, positron generation/acceleration experiments and proof-of-principle transverse pumping “dephasingless” electron acceleration experiment and theory. LWFA may be able to miniaturize particle accelerators for high energy physics and also enable new sources of ultrafast, extreme brightness and precise x-rays for a wide variety of applications. In laser wake field acceleration, an electron bunch “surfs” on the electron plasma wave (the “wake field”) generated by the ponderomotive force of an intense laser. The plasma wave has a strong longitudinal electric field that stays in phase with the relativistic driver. A relativistic charged particle may, therefore, remain in phase with the accelerating field over long distances and gain ultra-relativistic energies. The accelerating electric field strength that the plasma wave can support can be many orders of magnitude higher than that of conventional accelerators, which makes laser wakefield acceleration an exciting prospect as an advanced accelerator concept. In this research project we have investigated the scaling of this mechanism to laser powers of 2 PW and have measured the x-ray emission and radio frequency emission resulting from the acceleration process. We have also performed theoretical investigation of mechanisms to scale laser driven accelerators to much higher energy using dephasingless acceleration processes.

43 PARTICLE ACCELERATORS↗
DOE OSTI2024

Study of ablation and shock generation across three orders of magnitude of laser intensity with 100 ps laser pulses

The laser ablation and subsequent shock generation in solid targets plays an important role in a variety of research topics from equation of state models for materials to inertial confinement fusion. One of the long-standing issues is the knowledge of ablation depth in the picosecond time regime. Here, we report on a direct technique for determining the ablation depth in aluminum using x-ray diffraction data from Linac Coherent Light Source at the Stanford Linear Accelerator Center. This technique gives a direct measurement of the shock wave propagation in the bulk target, enabling an ability to discern early timescale physics from late timescale effects not available in postmortem analysis. We find that the ablation depths only vary by 0.2 μm across three orders of magnitude of laser intensity, while the pressure increased by a factor of 10 following a square root dependence on laser pulse energy. We further observe that the ablation depth in this intensity range (10 11 –10 13 W/cm 2 in intensity, corresponding to 0.8–80 J/cm 2 in fluence) cannot be modeled by a universal scaling law, given the complexity of the mechanisms governing laser ablation in this intensity regime.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Reliable Determination of Pulses and Pulse-Shape Instability in Ultrashort Laser Pulse Trains Using Polarization-Gating and Transient-Grating Frequency-Resolved Optical Gating Using the RANA Approach

Devices that measure the presence of instability in the pulse shapes in trains of ultrashort laser pulses do not exist, so this task necessarily falls to pulse-measurement devices, like Frequency-Resolved Optical Gating (FROG) and its variations, which have proven to be a highly reliable class of techniques for measuring stable trains of ultrashort laser pulses. Fortunately, multi-shot versions of FROG have also been shown to sensitively distinguish trains of stable from those of unstable pulse shapes by displaying readily visible systematic discrepancies between the measured and retrieved traces in the presence of unstable pulse trains. However, the effects of pulse-shape instability and algorithm stagnation can be indistinguishable, so a never-stagnating algorithm—even when instability is present—is required and is generally important. In previous work, we demonstrated that our recently introduced Retrieved-Amplitude N-grid Algorithmic (RANA) approach produces highly reliable (100%) pulse-retrieval in the second-harmonic-generation (SHG) version of FROG for thousands of sample trains of pulses with stable pulse shapes. Further, it does so even for trains of unstable pulse shapes and thus both reliably distinguishes between the two cases and provides a rough measure of the degree of instability as well as a reasonable estimate of most typical pulse parameters. Here, we perform the analogous study for the polarization-gating (PG) and transient-grating (TG) versions of FROG, which are often used for higher-energy pulse trains. We conclude that PG and TG FROG, coupled with the RANA approach, also provide reliable indicators of pulse-shape instability. In addition, for PG and TG FROG, the RANA approach provides an even better estimate of a typical pulse in an unstable pulse train than SHG FROG does, even in cases of significant pulse-shape instability.

47 OTHER INSTRUMENTATION↗
DOE OSTI2026

Structural and Electrocatalytic Studies of Pulsed Laser Deposited Epitaxial RuO 2 Thin Films

Two sets of high-quality epitaxial ruthenium oxide (RuO 2 ) thin films with different thicknesses were synthesized in situ on cost-competitive sapphire substrates by using a pulsed laser deposition technique. The first set of films, with a thickness of 40 nm and a sheet resistance of 15.7 Ω/□, was prepared using 2100 laser pulses, while the second set of films, with a thickness of 87 nm and a sheet resistance of 6.7 Ω/□, was prepared using 4800 laser pulses. All other deposition parameters were kept the same. The post-deposition structural and morphological measurements showed that both sets of films grew at the same growth rate, had the same crystallinity, similar grain boundary density, and slightly different surface roughness. The thicker RuO 2 films achieved an overpotential of 280 mV for the oxygen evolution reaction at a current density of 100 μA/cm 2 , comparable to or exceeding the performance of films grown on more expensive substrates. Comparatively, the thinner RuO 2 films, which have a significantly higher charge transfer resistance (250 Ω versus 100 Ω for thick films), display a higher overpotential of 320 mV. These results indicate that the lower electrical resistance of thicker films promotes charge transfer through the film body, leading to superior electrocatalytic properties.

charge-transfer↗
DOE OSTI2025

Effects of non-equilibrium ionization and excitation on radiation absorption in plasma plumes induced by ablation of metal targets with nanosecond laser pulses

Ionization and radiation absorption in nanosecond laser-induced plasma plumes are routinely modeled using the Saha–Boltzmann equilibrium ionization model (EQM). However, the equilibrium assumption can be inaccurate during the laser pulse when non-equilibrium effects significantly impact radiation absorption. In the present work, the EQM and non-equilibrium collisional-radiative model (CRM) are compared to reveal the effect of plasma non-equilibrium on radiation absorption in non-homogeneous plumes and degree of plasma shielding. Simulations of plume expansion induced by irradiation of a copper target in 1 atm argon background gas with a 10 ns Gaussian pulse at a fluence from 8 Jcm −2 to 14 Jcm −2 are performed with a hybrid computational model that couples a lumped particle direct simulation Monte Carlo method with either CRM or EQM. The simulations show that the EQM strongly underestimates the effects of ionization and radiation absorption compared to CRM and, contrary to the CRM, predict strong ionization of the background gas. The differences between the models are explained by the qualitatively different coupling between plume expansion and dynamics of ionization and exitation processes in the CRM and EQM under conditions when the characteristic times for most radiation- and electron-induced processes are longer than the pulse duration. The CRM-based predictions are also found to agree much better with available experimental data. In conclusion, these results indicate that the model of Saha–Boltzmann equilibrium cannot be used for reliable prediction of the degree of plasma shielding in plumes induced by nanosecond laser pulses or for processing results of spectroscopic measurements at early stages of expansion of such plumes.

Physics - Plasma physics↗
DOE OSTI2025

Demonstration of full-scale spatiotemporal diagnostics of solid-density plasmas driven by an ultra-short relativistic laser pulse using an X-ray free-electron laser

Understanding the complex plasma dynamics in ultra-intense relativistic laser–solid interactions is of fundamental importance for applications of laser–plasma-based particle accelerators, the creation of high-energy-density matter, understanding planetary science, and laser-driven fusion energy. However, experimental efforts in this regime have been limited by the lack of accessibility of over-critical densities and the poor spatiotemporal resolution of conventional diagnostics. Over the last decade, the advent of femtosecond brilliant hard X-ray free-electron lasers (XFELs) has opened new horizons to overcome these limitations. Here, for the first time, we present full-scale spatiotemporal measurements of solid-density plasma dynamics, including preplasma generation with tens of nanometer scale length driven by the leading edge of a relativistic laser pulse, ultrafast heating and ionization at the main pulse arrival, the laser-driven blast wave, and transient surface return current-induced compression dynamics up to hundreds of picoseconds after interaction. These observations are enabled by utilizing a novel combination of advanced X-ray diagnostics including small-angle X-ray scattering, resonant X-ray emission spectroscopy, and propagation-based X-ray phase-contrast imaging simultaneously at the European XFEL-HED beamline station.

Huang, Lingen [Helmholtz-Zentrum Dresden-Rossendor↗
DOE OSTI2025

Arbitrary-velocity laser pulses in plasma waveguides

Space-time structured laser pulses feature an intensity peak that can travel at an arbitrary velocity while maintaining a near-constant profile. These pulses can propagate in uniform media, where their frequencies are correlated with continuous transverse wave vectors, or in structured media, such as a waveguide, where their frequencies are correlated with discrete mode numbers. Here, we demonstrate the formation and propagation of arbitrary-velocity laser pulses in a plasma waveguide where the intensity can be orders of magnitude higher than in a solid-state waveguide. The flexibility to control the velocity of the peak intensity in a plasma waveguide enables new configurations for plasma-based sources of radiation and energetic particles, including THz generation, laser wakefield acceleration, and direct laser acceleration.

42 ENGINEERING↗
DOE OSTI2025

Active control of laser beam pointing for the Zettawatt-Equivalent Ultrashort pulse laser System: a proof-of-principle study with 16-inch optics

We present a proof-of-principle study of active beam-pointing control for the Zettawatt-Equivalent Ultrashort pulse laser System (ZEUS) using a piezo-actuated 16-inch mirror. To the best of our knowledge, this is the largest actively controlled mirror reported in a high-power laser system. A simple proportional feedback control was implemented based on a field-programmable gate array, which reduced the standard deviation of beam-pointing fluctuations by 91% to 0.075 μrad in the horizontal direction and by 78% to 0.25 μrad in the vertical direction. We also demonstrated the elimination of long-term pointing jitter caused by temperature drift using the same apparatus.

laser pointing control↗
DOE OSTI2025

Pausing ultrafast melting by timed multiple femtosecond-laser pulses

An intense femtosecond-laser excitation of a solid induces highly nonthermal conditions. In materials like silicon, laser-induced bond-softening leads to a highly incoherent ionic motion and eventually nonthermal melting. But is this outcome an inevitable consequence, or can it be controlled? Here, we performed ab initio molecular dynamics simulations of crystalline silicon after timed multiple femtosecond-laser pulse excitations with fluence above the nonthermal melting threshold. Our results demonstrate an excitation mechanism that pauses nonthermal melting and creates a metastable state instead, with an electronic structure similar to the ground state. This mechanism can be generalized to other materials, potentially enabling structural and/or electronic transitions to metastable phases in the high-excitation regime. In addition, our approach could be used to switch off nonthermal contributions in experiments, allowing reliable electron-phonon coupling constants to be obtained more easily.

47 OTHER INSTRUMENTATION↗
DOE OSTI2025

Versatile system for ion energy measurements generated by pulsed laser ionization: Insights into electron-ion dynamics

Ion energy distributions generated by pulsed laser interactions with materials are essential for applications ranging from materials science to oncology. Ion energy characterization is particularly important for an emerging mass spectrometry technique called virtual-slit cycloidal mass spectrometry (VS-CMS). The ion energy distribution influences the design and performance of VS-CMS instruments, as well as the efficacy of laser-driven ionization methods in various fields. Several established techniques, including the retarding potential method, time-of-flight (TOF) analysis, and electrostatic energy analyzers, have been employed to measure ion energy distributions. The wide range of ion energies reported highlights the strong dependence of ion energy on laser parameters, target materials, and experimental conditions, as well as the necessity of making independent measurements of the ion energy distribution for specific laser systems and materials. This paper presents the design and characterization of a simple TOF-based apparatus for measuring ion energy distributions from pulsed laser ionization without external fields. This approach minimizes perturbation of electron-ion dynamics and enables simultaneous energy measurements at multiple spatial positions. Here, the apparatus was tested using a nanosecond pulsed Nd:YAG laser operating at 1064 nm, 532 nm, and 266 nm on solid copper sheets at various laser fluences. Simultaneous measurements at different distances provide new insights into ion-electron interactions post-ionization and demonstrate the influence of laser wavelength and fluence on ion energy distributions.

Ion energy↗
DOE OSTI2026

The Focus of an Ultraintense Laser Pulse

Back in 1885, von Lommel studied the diffraction of a circular opening. His study was one step further than the Airy diffraction model (describing patterns in the focal plane) because von Lommel’s model was able to describe what the light distribution before and after the focus is. Today’s extreme lasers have a flat-top profile whose diffraction pattern in the vicinity of the focus is very much reminiscent of von Lommel’s description. In the present Chapter, we will compute, based on a Huygens-Fresnel integral method, the laser field distribution around the focus. This modelling is particularly important because the intensity distribution before and after the focal plane (where the Airy disk exists) is very relevant to many contemporary experiments, and is key to the ionization of atoms and the dynamics of liberated electrons. For clarity, we are going to analyze three cases corresponding to three f-numbers: f/10, f/1.8, and f/1.1. Our computed results reveal the present-day significance of von Lommel’s pioneering results. Here, they help us understand the light distribution in the entire focal region of an ultraintense laser pulse including the full vectorial fields, not just the focal plane.

Roso, Luis [Universidad de Salamanca (Spain)]↗
DOE OSTI2025

Enhanced quantum radiation with flying-focus laser pulses

The emission of a photon by an electron in an intense laser field is one of the most fundamental processes in electrodynamics and underlies the many applications that utilize high-energy photon beams. This process is typically studied for electrons colliding head-on with a stationary-focus laser pulse. Here, we show that the energy lost by electrons in the quantum regime and the yield of emitted photons can be substantially increased by replacing a stationary-focus pulse with an equal-energy flying-focus pulse whose focus co-propagates with the electrons. Furthermore, these advantages of the flying focus result from the energy loss and the photon yield scaling more favorably with the interaction time than the laser intensity in the quantum regime, with the latter also holding in the classical regime. Monte Carlo simulations of electrons colliding with equal-energy stationary and flying-focus laser pulses demonstrate these advantages.

Compton scattering↗
DOE OSTI2025

Electron acceleration by exponentially chirped laser pulses

Single-electron acceleration in vacuum by exponentially chirped plane-wave and tightly focused Gaussian laser pulses is investigated. Numerical calculations and particle-in-cell simulations, employing the chirped fields, demonstrate that GeV net energy gain, over sub-millimeter excursion distances, is possible from PW-class femtosecond laser pulses.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Quantitative phase imaging around water vapor microbubbles under pulsed laser illumination

We measured water temperature around a self-oscillating water vapor-rich bubble using diffraction phase microscopy equipped with a pulsed laser. The water vapor-rich bubble, which causes a strong water flow around it, was generated by locally heating degassed water through the photothermal conversion properties of an FeSi2 thin film. The generation of the flow is related to the self-oscillation of the bubble at sub-MHz frequencies and the temperature distribution around it. Here, the refractive index of the surrounding water was measured using a pulsed laser with a 3.5-ns pulse duration, which guarantees a time resolution of less than 1/200 of the oscillation cycle of the bubble. The temperature distribution around the bubble was calculated from the measured refractive index.

Narihira, Kyoshiro [Kyoto University, Japan]↗
DOE OSTI2024

System and method for large-area pulsed laser melting of metallic powder in a laser powder bed fusion application

The present disclosure relates to systems and methods for performing large area laser powder bed fusion (LBPF) to form a plurality of layers of a 3D part in a layer-by-layer fashion using meltable powder particles. In one implementation the system makes use of a first light source, which may be a diode laser subsystem, for generating a first light pulse of a first duration. The first light is used to preheat a substrate underneath a new layer of powder particles, wherein the substrate is formed from a previously fused quantity of the powder particles. A second light source, which may be a pulse laser, generates a second light pulse subsequent to the first light pulse. The second light pulse has a second duration shorter than the first duration by a factor of at least about 10, and fully melts the new layer of powder particles in addition to the substrate, to achieve a smooth printed layer. The wavelength of the first light pulse also differs from a wavelength of the second light pulse.

Khairallah, Saad A.↗