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Results for “PHOTON EMISSION”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2019

Coherent single-photon emission from colloidal lead halide perovskite quantum dots

Chemically made colloidal semiconductor quantum dots have long been proposed as scalable and color-tunable single emitters in quantum optics, but they have typically suffered from prohibitively incoherent emission. We now demonstrate that individual colloidal lead halide perovskite quantum dots (PQDs) display highly efficient single-photon emission with optical coherence times as long as 80 picoseconds, an appreciable fraction of their 210-picosecond radiative lifetimes. These measurements suggest that PQDs should be explored as building blocks in sources of indistinguishable single photons and entangled photon pairs. Our results present a starting point for the rational design of lead halide perovskite–based quantum emitters that have fast emission, wide spectral tunability, and scalable production and that benefit from the hybrid integration with nanophotonic components that has been demonstrated for colloidal materials.

solar (photovoltaic), solid state lighting, photos↗
DOE OSTI2019

Quantum two-photon emission in a photonic cavity

In this paper, we derive an expression for the two-photon spontaneous emission (TPSE) rate of an excited quantum emitter in the presence of arbitrary bodies in its vicinities. After investigating the influence of a perfectly conducting plate on the TPSE spectral distribution (Purcell effect), we demonstrate the equivalence of our expression with the more usual formula written in terms of the corresponding dyadic Green's function. We establish a convenient relation between the TPSE spectral distribution and the corresponding Purcell factors of the system. Next, we consider an emitter close to a dielectric medium and show that, in the near-field regime, the TPSE spectral distribution is substantially enhanced and changes abruptly at the resonance frequencies. Finally, motivated by the suppression that may occur in the one-photon spontaneous emission of an excited atom between two parallel conducting plates, we discuss the TPSE for this same situation and show that complete suppression can never occur for s → s transitions.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2018

Two-Level Quantum Systems in Two-Dimensional Materials for Single Photon Emission

Single photon emission (SPE) by a solid-state source requires presence of a distinct two-level quantum system, usually provided by point defects. Here we note that a number of qualities offered by novel, two-dimensional materials, their all-surface openness and optical transparence, tighter quantum confinement, and reduced charge screening—are advantageous for achieving an ideal SPE. On the basis of first-principles calculations and point-group symmetry analysis, a strategy is proposed to design paramagnetic defect complex with reduced symmetry, meeting all the requirements for SPE: its electronic states are well isolated from the host material bands, belong to a majority spin eigenstate, and can be controllably excited by polarized light. Here, the defect complex is thermodynamically stable and appears feasible for experimental realization to serve as an SPE-source, essential for quantum computing, with Re Mo V S in MoS 2 as one of the most practical candidates.

36 MATERIALS SCIENCE↗
DOE OSTI2025

Resonant metasurface‐enabled quantum light sources for single‐photon emission and entangled photon‐pair generation

Light encodes information in multiple degrees of freedom (e.g., frequency, amplitude, and phase), enabling high‐speed, high‐bandwidth communication through fiber optics. Unlike classical light, quantum light (single or entangled photons) can transmit quantum states over long distances without loss of coherence, thereby coherently interconnecting quantum nodes for distributed quantum entanglement. Quantum light sources are critical for developing scalable quantum networks aimed at distributed quantum computing, quantum teleportation, and secure quantum communications. However, existing quantum light sources suffer from limited integrability, insufficient spectral and spatial tunability, and inefficiencies in achieving mass‐produced, deterministic, on‐demand quantum light generation. These limitations significantly hinder progress toward direct, on‐chip integration with quantum processing units and detectors – an essential step toward scalable quantum networks. Resonant metasurfaces that leverage photonic modes – such as Mie resonances, guided‐mode resonances, or symmetry‐protected bound states in the continuum – offer strong spatial and temporal confinement of electromagnetic fields, characterized by high quality factors and small mode volumes. These metasurfaces greatly enhance linear and nonlinear light‐matter interactions, making them ideal for efficient on‐chip quantum light generation and manipulation. Here, we describe recent advances in nanoscale quantum light sources and quantum photonic state manipulation enabled by resonant metasurfaces. We also provide an outlook on next‐generation miniaturized quantum light sources achievable through materials innovations in quantum emitters, the co‐design of resonant metasurfaces, and ultimately, the heterogeneous integration of emerging layered van der Waals materials with resonant metasurfaces.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2019

Benchmarking a nonequilibrium approach to photon emission in relativistic heavy-ion collisions

In this study, the production of photons through binary scattering processes is investigated for equilibrated hadronic systems. More precisely, a nonequilibrium hadronic transport approach to describe relativistic heavy-ion collisions is benchmarked with respect to photon emission. Cross sections for photon production in π + ρ → π + γ and π + π → ρ + γ scattering processes are derived from an effective chiral field theory and implemented into the hadronic transport approach, SMASH (Simulating Many Accelerated Strongly-interacting Hadrons). The implementation is verified by systematically comparing the thermal photon rate to theoretical expectations. Further, the impact of form factors is discussed, scattering processes mediated by ω mesons are found to contribute significantly to the total photon production. Several comparisons of the yielded photon rates are performed: to parametrizations of the very same rates as used in hydrodynamic simulations, to previous works relying on different cross sections for the production of direct photons from the hadronic stage, and to partonic rates. Finally, the impact of considering the finite width of the ρ meson is investigated, where a significant enhancement of photon production in the low-energy region is observed. This benchmark is the first step toward a consistent treatment of photon emission in hybrid hydrodynamics + transport approaches and toward a genuine dynamical description.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS1991

Magnetic two-photon scattering and two-photon emission - Cross sections and redistribution functions

The magnetic two-photon scattering cross section is discussed within the framework of QED, and the corresponding scattering redistribution function for this process and its inverse, as well as the scattering source function are calculated explicitly. In a similar way, the magnetic two-photon emission process which follows the radiative excitation of Landau levels above ground is calculated. The two-photon scattering and two-photon emission are of the same order as the single-photon magnetic scattering. All three of these processes, and in optically thick cases also their inverses, are included in radiative transport calculations modeling accreting pulsars and gamma-ray bursters. These processes play a prominent role in determining the relative strength of the first two cyclotron harmonics, and their effects extend also to the higher harmonics.

Alexander, S. G.↗
DOE OSTI2017

Tunable Anisotropic Photon Emission from Self-Organized CsPbBr 3 Perovskite Nanocrystals

In this paper, we report controllable anisotropic light emission of photons originating from vertically aligned transition dipole moments in spun-cast films of CsPbBr 3 nanocubes. By depositing films of nanocrystals on precoated substrates we can control the packing density and resultant radiation pattern of the emitted photons. We develop a technical framework to calculate the average orientation of light emitters, i.e., the angle between the transition dipole moment vector (TDM) and the substrate. This model is applicable to any emissive material with a known refractive index. Theoretical modeling indicates that oriented emission originates from an anisotropic alignment of the valence band and conduction band edge states on the ionic crystal lattice and demonstrates a general path to model the experimentally less accessible internal electric field of a nanosystem from the photoluminescent anisotropy. The uniquely accessible surface of the perovskite nanoparticles allows for perturbation of the normally isotropic emissive transition. Finally, the reported sensitive and tunable TDM orientation and control of emitted light will allow for applications of perovskite nanocrystals in a wide range of photonic technologies inaccessible to traditional light emitters.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
NASA NTRS2006

Improved Photon-Emission-Microscope System

An improved photon-emission-microscope (PEM) instrumentation system has been developed for use in diagnosing failure conditions in semiconductor devices, including complex integrated circuits. This system is designed primarily to image areas that emit photons, at wavelengths from 400 to 1,100 nm, associated with device failures caused by leakage of electric current through SiO2 and other dielectric materials used in multilayer semiconductor structures. In addition, the system is sensitive enough to image areas that emit photons during normal operation.

Vu, Duc↗
DOE OSTI2026

Enhancement of the photon emission rate near the QCD critical point

We compute photon emission rate enhancement near the QCD critical point using an effective theory of dynamic critical phenomena and derive a universal photon spectrum. The emission rate scales similar to conductivity, increasing with the correlation length (𝜉), diverging at the critical point. The spectrum exhibits 𝜔⁢𝑑⁢𝑁 𝛾 /𝑑 3 ⁢𝑘 ∝ 𝜔 −1/2 in the scaling regime, with the transition occurring at a frequency comparable to shear damping rate 𝜔 ∼ 𝛾 𝜂 /𝜉 2 , reflecting the nonequilibrium properties of the near-critical liquid.

dynamic critical phenomena↗
DOE OSTI2022

A full-ring variable-aperture cadmium zinc telluride system for whole-body single photon emission computed tomography: realistic simulations with phantoms

Single photon emission computed tomography (SPECT) is an imaging modality that has demonstrated its utility in a number of clinical indications. Despite this progress, a high sensitivity, high spatial resolution, multi-tracer SPECT with a large field of view suitable for whole-body imaging of a broad range of radiotracers for theranostics is not available. Purpose We have designed a cadmium zinc telluride (CZT) variable-aperture full-ring SPECT scanner instrumented with a broad-energy tungsten collimator intended to fill this technological gap. The final purpose is to provide a multi-tracer solution for brain and whole-body imaging. Our static SPECT scanner breaks the paradigm of the standard dual- and triple-head rotational SPECT systems, utilizing a larger detector area in each scan increasing the sensitivity. We provide a demonstration of the performance of our design using a realistic model of our detector with simulated body-sized 99mTc phantoms. Methods We developed a realistic model of our detector by using a combination of a Geant4 Monte Carlo simulation and a CZT detector response model based on a finite element model. Our approach models the characteristic low-energy tail effect in CZT that noticeably affects the sensitivity and the quality of the scatter correction in CZT detectors. We implement a modified dual energy window scatter correction adapted to include the CZT low-energy tail effect. A dedicated correction is also developed to eliminate the undesirable truncation observed in images given the presence of detector edges and gaps between detectors, due to the non-rotational nature of our device. Corrections for the attenuation, detector response and the presence of collimators are also included. The images are reconstructed using the maximum-likelihood expectation-maximization algorithm implemented in the reconstruction open software STIR. Detector and reconstruction performance are characterized with a Derenzo phantom and a body-sized National Electrical Manufacturers Association (NEMA) Image Quality (IQ) phantom containing 99mTc. Results Our SPECT design can resolve 6.4mm rods in a Derenzo phantom and obtain a good image contrast with the IQ phantom. Explicit testing of the gap and edge correction is provided, showing an excellent performance in eliminating the image truncation artifacts. Our modified scatter correction shows no overestimation of the contrast-recovery ratio for our realistic CZT detector model, as opposed to the cases without correction and with a standard dual-energy window scatter correction. Conclusions In this paper, we further demonstrate the performance of our design for whole-body imaging purposes. This adds to our previous demonstration of improved qualitative and quantitative 99mTc imaging for brain perfusion and 123I imaging for dopamine transport with respect to state-of-the-art NaI dual-head cameras. We show that our design performs similarly to the VERITON SPECT from Spectrum Dynamics, a commercial full-ring CZT SPECT camera, with the potential advantage of the broader energy range of application given by our custom-design tungsten collimators. Here, our device combines high sensitivity and image resolution with a broad-energy imaging application for the purpose of clinical imaging and theranostics of emerging radionuclides.

62 RADIOLOGY AND NUCLEAR MEDICINE↗
DOE OSTI2023

On-demand directional microwave photon emission using waveguide quantum electrodynamics

Routing quantum information between non-local computational nodes is a foundation for extensible networks of quantum processors. Quantum information transfer between arbitrary nodes is generally mediated either by photons that propagate between them or by resonantly coupling nearby nodes. The utility is determined by the type of emitter, propagation channel and receiver. Conventional approaches involving propagating microwave photons have limited fidelity due to photon loss and are often unidirectional, whereas architectures that use direct resonant coupling are bidirectional in principle but can generally accommodate only a few local nodes. Here we demonstrate high-fidelity, on-demand, directional, microwave photon emission. We do this using an artificial molecule comprising two superconducting qubits strongly coupled to a bidirectional waveguide, effectively creating a chiral microwave waveguide. Quantum interference between the photon emission pathways from the molecule generates single photons that selectively propagate in a chosen direction. This circuit will also be capable of photon absorption, making it suitable for building interconnects within extensible quantum networks.

42 ENGINEERING↗
DOE OSTI2017

Tunable and high-purity room temperature single-photon emission from atomic defects in hexagonal boron nitride

Two-dimensional van der Waals materials have emerged as promising platforms for solid-state quantum information processing devices with unusual potential for heterogeneous assembly. Recently, bright and photostable single photon emitters were reported from atomic defects in layered hexagonal boron nitride (hBN), but controlling inhomogeneous spectral distribution and reducing multi-photon emission presented open challenges. Here, we demonstrate that strain control allows spectral tunability of hBN single photon emitters over 6 meV, and material processing sharply improves the single photon purity. We observe high single photon count rates exceeding 7 × 10 6 counts per second at saturation, after correcting for uncorrelated photon background. Furthermore, these emitters are stable to material transfer to other substrates. High-purity and photostable single photon emission at room temperature, together with spectral tunability and transferability, opens the door to scalable integration of high-quality quantum emitters in photonic quantum technologies.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2017

3D Magnetohydrodynamic Models of Nonthermal Photon Emission in the Binary System γ{sup 2} Velorum

Recent reports claiming an association of the massive star binary system γ{sup 2} Velorum (WR 11) with a high-energy γ-ray source observed by Fermi-LAT contrast the so far exclusive role of η Carinae as the hitherto only detected γ-ray emitter in the source class of particle-accelerating colliding-wind binary (CWB) systems. We offer support to this claim of association by providing dedicated model predictions for the nonthermal photon emission spectrum of γ{sup 2} Velorum. We use 3D magnetohydrodynamic modeling (MHD) to investigate the structure and conditions of the wind-collision region (WCR) of γ{sup 2} Velorum including the important effect of radiative braking in the stellar winds. A transport equation is then solved for the entire computational domain to study the propagation of relativistic electrons and protons. The resulting distributions of particles are subsequently used to compute nonthermal photon emission components. In agreement with observation in X-ray spectroscopy, our simulations yield a large shock-cone opening angle. We find the nonthermal γ-ray emission of γ{sup 2} Velorum to be of hadronic origin owing to the strong radiation fields in the binary system, which inhibit the acceleration of electrons to energies sufficiently high for efficient inverse-Compton radiation. We also discuss the strong dependence of a hadronic γ-ray component on the energy-dependent diffusion used in the simulations. Of two mass-loss rates for the WR star found in literature, only the higher rate is able to accommodate the observed γ-ray spectrum with reasonable values for important simulation parameters such as the injection ratio of high-energy particles within the WCR.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1982

Hydrogen two photon emission in the UV spectrum of type 2 supernovae

The continuum emission of Type 2 supernovae demonstrates an ultraviolet (UV) excess when fit by black body emission is attempted. The H two photon emission is advanced as an explanation of the UV excess. A function by which the UV spectra of two Type 2 supernovae (SN 1979c in NGC 4321 and SN 1980k in NGC 6946) are fitted with U,B,V photometric data is presented. The angular velocity of expansion of the supernovae envelope is derived. From this, the linear velocity of expansion and the distances of the parent galaxies are derived. A distance of 17.3 Mpc is obtained for NGC 4321, and a distance of 7.1 Mpc for NGC 6946.

Benvenuti, P.↗
DOE OSTI2018

Red Single-Photon Emission from InAs/AlGaAs Quantum Dots

We report on single-photon emission of InAs/AlGaAs self-assembled quantum dots (QDs) grown by molecular beam epitaxy. By varying the growth conditions the QDs luminescence could be tuned over a wide wavelength range from 0.64 to 1 μm, including red part of the visible spectrum. Emission properties of individual QDs are investigated by micro-photoluminescence (μ-PL) spectroscopy using 500-nm-size etched mesa structures. Autocorrelation functions of photons from single QDs, measured in the wide spectral range demonstrate antibunching effect at zero delay time with a value of g{sup (2)}(0) ~ 0.17 that is a clear evidence of non-classical light.

36 MATERIALS SCIENCE↗