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At least 19 records

Enhancement of Second-Order Nonlinear-Optical Signals by Optical Stimulation

Second-order nonlinear optical interactions such as sum- and difference-frequency generation are widely used for bioimaging and as selective probes of interfacial environments. However, inefficient nonlinear optical conversion often leads to poor signal-to-noise ratio and long signal acquisition times. We demonstrate the dramatic enhancement of weak second-order nonlinear optical signals via stimulated sum- and difference-frequency generation. We present a conceptual framework to quantitatively describe the interaction and show that the process is highly sensitive to the relative optical phase of the stimulating field. To emphasize the utility of the technique, we demonstrate stimulated enhancement of second harmonic generation (SHG) from bovine collagen-I fibrils. Using a stimulating pulse fluence of only $3\text{ }\text{ }\mathrm{nJ}/{\mathrm{cm}}^{2}$, we obtain an SHG enhancement >${10}^{4}$ relative to the spontaneous signal. The stimulation enhancement is greatest in situations where spontaneous signals are the weakest—such as low laser power, small sample volume, and weak nonlinear susceptibility—emphasizing the potential for this technique to improve signal-to-noise ratios in biological imaging and interfacial spectroscopy.

42 ENGINEERING↗

Coherent (photon) vs incoherent (current) detection of multidimensional optical signals from single molecules in open junctions

The nonlinear optical response of a current-carrying single molecule coupled to two metal leads and driven by a sequence of impulsive optical pulses with controllable phases and time delays is calculated. Coherent (stimulated, heterodyne) detection of photons and incoherent detection of the optically induced current are compared. Using a diagrammatic Liouville space superoperator formalism, the signals are recast in terms of molecular correlation functions which are then expanded in the many-body molecular states. Two dimensional signals in benzene-1,4-dithiol molecule show cross peaks involving charged states. The correlation between optical and charge current signal is also observed.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Spectral and temporal properties of optical signals with multiple sinusoidal phase modulations

Optical signals generated by multiple sinusoidal temporal phase modulations (multi-FMs) applied to a monochromatic field are studied from the viewpoint of their optical spectrum and temporal modulations arising from spectral impairments. Statistical analysis based on the central limit theorem shows that the signals' optical spectrum converges to a normal distribution as the number of modulations increases, allowing one to predict the frequency range containing a given fraction of the total energy with the associated cumulative density function. The conversion of frequency modulation to amplitude modulation is analyzed and simulated for arbitrary multi-FM signals. These developments are of theoretical and practical importance for high-energy laser systems, where optical pulses are phase modulated in the front end to smooth out the on-target beam profile and prevent potentially catastrophic damage to optical components.

Dorrer, C.↗

Optical signal quality improvement due to nonlinear interaction between spectral channels

This paper examines stimulated Brillouin scattering (SBS) suppression in multichannel DWDM systems owing to nonlinear cross interaction between the channels and its effect on optical signal quality (1/OSNR{sub R}) in a communication link. We present an experimental study of single-, three- and five-channel systems with 10 Gbit s{sup −1} NRZ channels. The optical signal quality in the three- and five-channel systems is shown to be better than that in the single-channel system. The reason for this is that cross-phase modulation broadens the spectrum of the signal and raises the SBS threshold. This in turn ensures a more pronounced optical signal quality improvement due to self-phase modulation. (paper)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Silicon technology compatible photonic molecules for compact optical signal processing

Photonic molecules (PMs) based on multiple inner coupled microring resonators allow to surpass the fundamental constraint between the total quality factor (Q{sub T}), free spectral range (FSR), and resonator size. In this work, we use a PM that presents doublets and triplets resonance splitting, all with high Q{sub T}. We demonstrate the use of the doublet splitting for 34.2 GHz signal extraction by filtering the sidebands of a modulated optical signal. We also demonstrate that very compact optical modulators operating 2.75 times beyond its resonator linewidth limit may be obtained using the PM triplet splitting, with separation of ∼55 GHz.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Encoding the complete electric field of an ultraviolet ultrashort laser pulse in a near-infrared nonlinear-optical signal

We introduce a variation on the cross-correlation frequency-resolved optical gating (XFROG) technique that uses a near-infrared (NIR) nonlinear-optical signal to characterize pulses in the ultraviolet (UV). Using a transient-grating XFROG beam geometry, we create a grating using two copies of the unknown UV pulse and diffract a NIR reference pulse from it. We show that, by varying the delay between the UV pulses creating the grating, the UV pulse intensity-and-phase information can be encoded into a NIR signal. We also implemented a modified generalized-projections phase-retrieval algorithm for retrieving the UV pulses from these spectrograms. We performed proof-of-principle measurements of chirped pulses and double pulses, all at 400 nm. This approach should be extendable deeper into the UV and potentially even into the extreme UV or x-ray range.

47 OTHER INSTRUMENTATION↗

Effect of alpha and Gaussian refractive index profiles on the design of highly nonlinear optical fibre for efficient nonlinear optical signal processing

We propose an index profiled, highly nonlinear ultra-flattened dispersion fibre (HN-UFF) with appreciable values of fibre parameters such as dispersion, dispersion slope, effective area, nonlinearity, bending loss and splice loss. The designed fibre has normal zero flattened dispersion over S, C, L, U bands and extends up to 1.9857 μm. The maximum dispersion variation observed for this fibre is as low as 1.61 ps km{sup −1} nm{sup −1} over the 500-nm optical fibre transmission spectrum. This fibre also has two zero dispersion wavelengths at 1.487 and 1.9857 μm and the respective dispersion slopes are 0.02476 and 0.0068 ps nm{sup −2} km{sup −1}. The fibre has a very low ITU-T cutoff wavelength of 1.2613 μm and a virtuous nonlinear coefficient of 9.43 W{sup −1} km{sup −1}. The wide spectrum of zero flattened dispersion and a good nonlinear coefficient make the designed fibre very promising for different nonlinear optical signal processing applications. (fibre optics)

42 ENGINEERING↗

Nonlinear effects in optical signal transmission using a multimode fibre with weak coupling

We present the results of numerical simulation of nonlinear propagation of an optical signal in multimode gradient- and step-index fibres with weak coupling. It is found that when signals propagate in different modes, the system quality factor ( Q -factor) for a gradient-index fibre increases with the number of the modes involved. The quality degradation of the transmitted data with increasing the number of the involved modes is demonstrated for the case when the signals in different modes travel at the same velocity. It is shown that the use of a step-index fibre may significantly deteriorate the signal quality due to the presence of a mode with a small dispersion parameter. (fibre-optic communication)

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Application of combined optical signal processing methods to compensate for nonlinear effects in fibre-optic communication links

We report on the use of complex quadrature amplitude signal processing methods based on a combination of static neural networks and special modulation techniques. The conditions are found that allow one to construct the most effective combination of signal processing methods for transmitting signals with considerable power (in the nonlinear regime). Using analytical methods, it is shown how the statistical properties of a signal affect the efficiency of combined processing methods. (paper)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

On the ability of resonant diffraction gratings to differentiate a pulsed optical signal

The passage of an optical pulse through a resonant grating is considered. The conditions under which the resonant grating differentiates the envelope of the incident pulse are determined. It is shown that the necessary condition for computing the k-order derivative is the presence of k resonances in the transmission spectrum of the grating in the vicinity of the central frequency of the incident pulse. A method is described for constructing the stacked structure for computing the kth derivative on the basis of repetition of the structure for computing the first derivative. The results of numerical simulation of diffraction of the pulse from the analyzed structure for computing the first, second, and third derivative are presented.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Analog optical signal transmission for HEP experiments

A critical element in all high-energy physics experiments is the signal transmission from the active elements to the data acquisition system. It is especially challenging in large volume detectors based on noble liquids that are extensively being used for dark matter and neutrino detection.The topic of this contribution is the optical signal transmission of the signals acquired with silicon photomultipliers, which is able to satisfy many stringent experimental requirements. It is RF-noise immune and operates in cryogenic liquids and in high-electric fields.This transmission system is based on commercially available electronics components and customized Fabry-Perot laser diodes.I will talk about encountered challenges, breakthrough, and advances from the original concept of this system up to final validation tests, demonstrating progressive developments.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

All-optical signal processing at 10 GHz using a photonic crystal molecule

We report on 10 GHz operation of an all-optical gate based on an Indium Phosphide Photonic Crystal Molecule. Wavelength conversion and all-optical mixing of microwave signals are demonstrated using the 2 mW output of a mode locked diode laser. The spectral separation of the optical pump and signal is crucial in suppressing optical cross-talk.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Superbolts: The Most Powerful Optical Signals Generated by Lightning [Slides]

The most powerful optical lightning events are termed “superbolts." Superbolts can arise from physical lightning phenomena or radiative transfer effects. The most intense superbolts are caused by long-horizontal “megaflashes” in stratiform clouds that are particularly effective optical emitters. The scale, intensity, and rarity of superbolts and megaflashes make them difficult to observe. RF-powerful events recently labeled “superbolts” are a different phenomenon.

54 ENVIRONMENTAL SCIENCES↗

Rod-like plasmonic nanoparticles as optical building blocks: how differences in particle shape and structural geometry influence optical signal

Gold nanoparticles, particularly those with an anisotropic shape, have become a popular optical probe for experiments involving work on the nanoscale. However, to carry out such delicate and intricate experiments, it is first necessary to understand the detailed behavior of individual nanoparticles. In this series of experiments, optical and electron microscopy were utilized for the characterization of individual nanoparticles and small assemblies of nanoparticles. In the first experiment, gold nanorods were investigated. Single, isolated nanorods exhibit two maxima of localized surface plasmon resonance (LSPR), which are associated with the two nanorod axes. Upon the physical rotation of a nanorod at one of its LSPR wavelengths under polarized illumination, the optical behavior varies in a sinusoidal fashion. A dimer of nanorods exhibits optical behavior quite similar to a nanorod, except the LSPR maxima are shifted and broader. Under differential interference contrast (DIC) microscopy, a pair of nanorods separated by a distance below the diffraction limit can be distinguished from a single nanorod due to its optical behavior upon rotation. Dark field microscopy is unable to distinguish the two geometries. For the second set of experiments, the optical behavior of single gold nanorods at non-plasmonic wavelengths was investigated. The same nanorod was rotated with respect to a polarized light source under DIC, dark field, and polarized light microscopy. DIC microscopy was found to produce diffraction pattern peaks at non-plasmonic wavelengths, which could be altered by adjusting the setting of the polarizer. In the third set of experiments, the optical behavior of a single gold dumbbell and several simple dumbbell geometries were investigated with microscopy and simulations. The single dumbbell displayed behavior quite similar to that of a nanorod, but dumbbells exhibit a shift in both LSPR wavebands. Moreover, the shape of dumbbell particles allows them to interlock with one another quite easily. The dimers that form as a result display optical behavior that differs from what has been previously reported about nanorod dimers. Simulated surface charge density patterns reveal that hybridization of LSPR modes occurs readily along the lobes of individual dumbbells in some situations. A pentamer of dumbbells also displays hybridization of modes, and “hot spots” are observed at junctions between pairings of dumbbells. In the final set of experiments, the assembly behavior of nanoparticles in solution was observed in real time. In general, large assemblies of nanoparticles display backbone-like rigidity, but an interesting variety of movements is permitted within the larger structures.

36 MATERIALS SCIENCE↗

TH-AB-209-03: Overcoming Resolution Limitations of Diffuse Optical Signals in X-Ray Induced Luminescence (XIL) Imaging Via Selective Plane Illumination and 2D Deconvolution

Purpose: To evaluate the resolution and sensitivity of XIL imaging using a surface radiance simulation based on optical diffusion and maximum likelihood expectation maximization (MLEM) image reconstruction. XIL imaging seeks to determine the distribution of luminescent nanophosphors, which could be used as nanodosimeters or radiosensitizers. Methods: The XIL simulation generated a homogeneous slab with optical properties similar to tissue. X-ray activated nanophosphors were placed at 1.0 cm depth in the tissue in concentrations of 10{sup −4} g/mL in two volumes of 10 mm{sup 3} with varying separations between each other. An analytical optical diffusion model determined the surface radiance from the photon distributions generated at depth in the tissue by the nanophosphors. The simulation then determined the detected luminescent signal collected with a f/1.0 aperture lens and back-illuminated EMCCD camera. The surface radiance was deconvolved using a MLEM algorithm to estimate the nanophosphors distribution and the resolution. To account for both Poisson and Gaussian noise, a shifted Poisson imaging model was used in the deconvolution. The deconvolved distributions were fitted to a Gaussian after radial averaging to measure the full width at half maximum (FWHM) and the peak to peak distance between distributions was measured to determine the resolving power. Results: Simulated surface radiances for doses from 1mGy to 100 cGy were computed. Each image was deconvolved using 1000 iterations. At 1mGy, deconvolution reduced the FWHM of the nanophosphors distribution by 65% and had a resolving power is 3.84 mm. Decreasing the dose from 100 cGy to 1 mGy increased the FWHM by 22% but allowed for a dose reduction of a factor of 1000. Conclusion: Deconvolving the detected surface radiance allows for dose reduction while maintaining the resolution of the nanophosphors. It proves to be a useful technique in overcoming the resolution limitations of diffuse optical imaging in tissue. C. S. acknowledges support from the NIH National Institute of General Medical Sciences (Award number R25GM109439, Project Title: University of Chicago Initiative for Maximizing Student Development, IMSD). B. Q. and P. L. acknowledge support from NIH grant R01EB017293.

60 APPLIED LIFE SCIENCES↗

Millisecond-long suppression of spectroscopic optical signals using laser filamentation

Ultrashort laser pulse filamentation in air can extend the delivery of focused laser energy to distances greatly exceeding the Rayleigh length. In this way, remote measurements can be conducted using many standard methods of analytical spectroscopy. The performance of spectroscopic techniques can be enhanced by temporal gating, which rejects the unwanted noise and background. In the present work, we investigate the thermal relaxation of air in the wake of single-filament plasmas using shadowgraphy. Here, we demonstrate that the transient change in refractive index associated with relaxation of the gas can be used to reject both continuous and time-varying spectroscopic signals, including emission from laser-produced plasmas. This method can augment temporal gating of simple optical detectors.

47 OTHER INSTRUMENTATION↗

Response of a matrix photodetector into components of an optical signal with different spatial frequencies

We have used the method of direct evaluation of energy incident on each pixel of a photosensitive array to assess the distortions of a matrix photodetector response into a sinusoidal spatial signal. Using the data obtained, we have formulated recommendations for selecting a resolution of a matrix photodetector as a function of a maximum spatial frequency in the recorded interference pattern, as well as for matching of the resolutions of an objective and a photodetector of a digital camera or camcorder. (paper)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗