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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2019

Spatially dependent embedded self-shielding method for nonuniform temperature distribution

The embedded self-shielding method (ESSM) is simple and robust, and applicable to any geometrical configuration to account for resonance self-shielding by performing fixed source transport calculations. ESSM is very similar to the subgroup method, which has been successful in the MPACT neutronics code developed by CASL. The subgroup method introduces errors in a least-squares fitting process that is used to generate subgroup quadrature sets and cannot be applied to thermal energy groups, as ESSM introduces error for spatially dependent self-shielded cross sections inside the fuel. This study focused on integrating the conventional ESSM with an improved Stoker-Weiss method to obtain spatially dependent resonance self-shielded cross sections for a nonuniform fuel temperature distribution. Here, the proposed method would serve as a substitute for the subgroup method in high fidelity simulations using CASL’s VERA. Benchmark results show that this new, spatially dependent ESSM (SDESSM) is an appropriate candidate to replace the subgroup method.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2018

Thermopolarization Effect in Linear Polyethylene Oxide upon Crystallization from Melt

The correlation between crystallite structural changes and polarization properties of a linear crystallized [–CH{sub 2}CH{sub 2}O–]{sub n} polyethylene oxide polymer is studied. The average spherulite radius and polarization of polyethylene oxide are inspected as functions of molecular weight of polymer and crystallization temperature from melt in a nonuniform temperature field.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2017

Extreme Two‐Phase Cooling from Laser‐Etched Diamond and Conformal, Template‐Fabricated Microporous Copper

Abstract This paper reports the first integration of laser‐etched polycrystalline diamond microchannels with template‐fabricated microporous copper for extreme convective boiling in a composite heat sink for power electronics and energy conversion. Diamond offers the highest thermal conductivity near room temperature, and enables aggressive heat spreading along triangular channel walls with 1:1 aspect ratio. Conformally coated porous copper with thickness 25 µm and 5 µm pore size optimizes fluid and heat transport for convective boiling within the diamond channels. Data reported here include 1280 W cm −2 of heat removal from 0.7 cm 2 surface area with temperature rise beyond fluid saturation less than 21 K, corresponding to 6.3 × 10 5 W m −2 K −1 . This heat sink has the potential to dissipate much larger localized heat loads with small temperature nonuniformity (5 kW cm −2 over 200 µm × 200 µm with <3 K temperature difference). A microfluidic manifold assures uniform distribution of liquid over the heat sink surface with negligible pumping power requirements (e.g., <1.4 × 10 −4 of the thermal power dissipated). This breakthrough integration of functional materials and the resulting experimental data set a very high bar for microfluidic heat removal.

Palko, James W.↗
DOE OSTI2020

Completion Effects on Diagnosing Multistage Facture Treatments with Distributed Temperature Sensing

Summary Distributed temperature sensing (DTS) is a valuable tool to diagnose multistage hydraulic fracture treatments. When a stage interval is shut in, the clusters that take more fluid during pumping warm up more slowly. Therefore, the fluid volume injected into each cluster can be quantitatively interpreted by numerical inversion of the warm-back temperature behavior. This general concept assumes that the different warm-back behavior is controlled by only the injected fluid volume; however, recent observations of DTS data indicate that completion configurations significantly influence the warm-back behavior. This paper investigates the completion effects on the DTS interpretation. In ideal conditions, when a stage is fractured, the upstream stage intervals should show an almost uniform temperature that is close to the injected fluid temperature. This is due to the high fluid velocity of injected fluid in the wellbore, and the upstream intervals have not been perforated (noncommunicating intervals), so the only heat transfer is heat conduction between the wellbore fluid and the surrounding reservoir. But the field DTS data show considerably irregular variations in temperature along the upstream stage intervals. These variations are caused by the completion effects. The nonuniform temperature profile is caused by different heat transfer behavior induced by completion hardware along the production casing string, such as joints, clamps, and blast protectors, and by the sensing cable location in the cement, as well as the cement quality. Because the varying heat transfer behavior impacts the warm-back behavior as well as the temperature profile, the completion effects need to be considered in DTS interpretation. A method of DTS interpretation considering the completion effects to diagnose multistage fracture treatments was developed. Because the heat transfer between a wellbore and a reservoir depends on the overall heat transfer coefficient describing heat conduction through the completion in a forward model, this parameter needs to be tuned all along the wellbore. To calibrate the completion effect, the temperature inversion is conducted using the temperature measured at a stage interval that is upstream of a stage interval currently being treated. Because the interpreted stage interval is not perforated at that time, the thermal behavior at the noncommunicating interval is governed by only the heat conduction through the completion environment. Once the effective values of the overall heat transfer coefficient are estimated along the interpreted stage interval, they can be assumed to be constant physical parameters. Then, the fluid volume distribution is interpreted by using the effective overall heat transfer coefficient profile along each interval. This study provides a field application of the developed interpretation method. The new interpretation method provides more accurate diagnosis of fracture treatments by DTS interpretation.

Engineering↗
DOE OSTI2025

Multifrequency eddy-current detection of fast transient thermal signatures for in situ monitoring applications

Eddy-current (EC) nondestructive evaluation has a long history of use in a variety of ex situ defect monitoring applications because of its exquisite sensitivity to local material variations. Due to the relationship between a material's conductivity and its temperature, EC methods have also been used to investigate quasistatic, long-range temperature variations in casting applications. However, these techniques remain underutilized for the measurement of rapidly varying, spatially nonuniform temperature distributions. In this work, we construct a model system capable of generating repeatable temperature transients in steel plates and measure real-time eddy-current signals with millisecond time resolution and spatial resolution of the order of 1 mm. Using a combination of Multiphysics simulations, fast thermal imaging, and time-resolved holographic interferometry, we tease apart contributions to the eddy-current signals arising from temperature variations and transient plate deformation. Finally, we perform a systematic study in which we vary the plate thickness and the eddy-current excitation frequency to demonstrate that eddy-current techniques can provide information about a three-dimensional, time-varying, subsurface thermal distribution, which is inaccessible to the traditional thermal imaging techniques.

Rosenberg, Ethan R. [Lawrence Livermore National L↗
DOE OSTI2020

Underpotential lithium plating on graphite anodes caused by temperature heterogeneity

Rechargeability and operational safety of commercial lithium (Li)-ion batteries demand further improvement. Plating of metallic Li on graphite anodes is a critical reason for Li-ion battery capacity decay and short circuit. It is generally believed that Li plating is caused by the slow kinetics of graphite intercalation, but in this paper, we demonstrate that thermodynamics also serves a crucial role. We show that a nonuniform temperature distribution within the battery can make local plating of Li above 0 V vs. Li 0 /Li + (room temperature) thermodynamically favorable. This phenomenon is caused by temperature-dependent shifts of the equilibrium potential of Li 0 /Li + . Supported by simulation results, we confirm the likelihood of this failure mechanism during commercial Li-ion battery operation, including both slow and fast charging conditions. This work furthers the understanding of nonuniform Li plating and will inspire future studies to prolong the cycling lifetime of Li-ion batteries.

25 ENERGY STORAGE↗
DOE OSTI2021

NRC Multiphysics Analysis Capability Deployment (FY2021 - Part 2)

This report details the progress and activities of Idaho National Laboratory (INL) on the Nuclear Regulatory Commission (NRC) project “Development and Modeling Support for Advanced Non-Light Water Reactors.” Task 4b was completed for this report. INL developed a sample problem showing how to use Serpent 2 to calculate macroscopic cross sections for use in Griffin for a typical sodium fast reactor Unprotected Loss of Flow (ULOF) transient. The complicating factor is the relatively large axial gradient of the coolant (and hence fuel) temperature and its evolution during the transient. A 3D Griffin model of the Advanced Burner Test Reactor (ABTR) is coupled to the System Analysis Module (SAM) to perform the ULOF transient. The model includes various explicit feedback mechanisms for fast reactors, including Doppler, radial expansion from the displacement of the support plate, and axial expansion from the displacement of the fuel pins. The results for the ULOF transient are consistent with published values. We observed small effects in the transient results that arise from the superhomogenization equivalence correction of uniform and nonuniform temperature data sets, but they diminish as more dominant reactivity mechanisms are added to the model. Potential improvements to the neutronics model include: adding the differential control rod and sodium feedback mechanisms, implementing cross section re-homogenization based on the partial volume of the various materials, and enhancing the kinetics parameters. Furthermore, the fluids model only includes four subchannels to represent the entire active core due to performance limitations in SAM when attempting to model one subchannel per assembly.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2021

Understanding the Cold Season Arctic Surface Warming Trend in Recent Decades

Abstract Whether sea‐ice loss or lapse‐rate feedback dominates the Arctic amplification (AA) remains an open question. Analysis of data sets based upon observations reveals a 1.11 K per decade surface warming trend in the Arctic (70°–90°N) during 1979–2020 cold season (October–February) that is five times higher than the corresponding global mean. Based on surface energy budget analysis, we show that the largest contribution (∼82%) to this cold season warming trend is attributed to changes in clear‐sky downward longwave radiation. In contrast to that in Arctic summer and over tropics, a reduction in lower‐tropospheric inversions plays a unique role in explaining the reduction of the downward longwave radiation associated with atmospheric nonuniform temperature and corresponding moisture changes. Our analyses also suggest that Arctic lower‐tropospheric stability should be considered in conjunction with sea‐ice decline during the preceding warm season to explain AA.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Universal time-dependent Ginzburg-Landau theory

We study the hydrodynamics of superconductors within the framework of Schwinger-Keldysh effective field theory (EFT). We show that in the vicinity of the superconducting phase transition the most general leading-order EFT satisfying the local Kubo-Martin-Schwinger condition is described by a version of the time-dependent Ginzburg-Landau (TDGL) equations augmented with stochastic terms. This version of TDGL is applicable in the gapless regime independent of any microscopic details. Within this approach, it is possible to include systematically the effects of nonuniform temperature and heat conductivity, as well as explicit or spontaneous breaking of time reversal. Here, we also introduce a thermal version of the Josephson relation and use it to construct an exotic hydrodynamics describing a phase of matter where heat can flow without dissipation.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2020

A New Approach to Indoor Characterization of PV Module Energy Yield Parameters

Temperature and solar irradiance are among the most relevant parameters that affect the energy yield of photovoltaic cells and modules. A rise in the module temperature leads to a significant decrease in the open circuit voltage and a small increase in the short circuit current. Here we use a new tool to determine temperature coefficients as well as to assess power rating of multi c-Si, mono c-Si, CdTe, and CIGS-based PV modules in controlled indoor conditions per IEC 60891 and IEC 61853-1. We use the tool to explore how nonuniformities in module temperature affect the accuracy of the temperature coefficients.

14 SOLAR ENERGY↗
DOE OSTI2026

Spatially resolved phase transformation mapping in 410 stainless steel during additive manufacturing visualized via real-time infrared data

Here, in this study, we demonstrate that spatially resolved cooling curves derived from real-time infrared (IR) thermography during additive manufacturing (AM) can capture spatial variations in phase transformation temperatures through cooling curve analysis (CCA). Using this approach, we show that during laser hot-wire deposition of 410 stainless steel (410SS), the martensite start temperature (M s ) evolves dynamically throughout the build. The M s temperature is spatially nonuniform, ranging from 185 °C to 348 °C, with the lowest values toward the build center and higher values toward the upper region of the deposit. In the lower portion of the build, no M s inflection is detected via CCA, consistent with transformation occurring earlier during thermal cycling followed by tempering during subsequent thermal cycles. These trends in M s are corroborated by characterizing the microstructure by electron backscatter diffraction (EBSD). Traditionally, M s is assumed to be constant, and a single interpass temperature is applied during both deposition and residual stress modeling. Our results demonstrate that IR-derived cooling curves provide a route to spatially and temporally resolved transformation temperature tracking for dynamic interpass control and improved residual-stress modeling.

Additive manufacturing↗
DOE OSTI2022

Understanding thermal and mechanical effects on lithium plating in lithium-ion batteries

Lithium plating is one of the main concerns for cell durability, as cyclable lithium and cell capacity are decreased during the process. Thermal and mechanical loads can influence cell behavior, including lithium plating driving forces, as suggested by the Arrhenius equation and the Bruggeman relation, respectively. Hence, a 1D and a 3D model are employed to study the thermal and mechanical effects on lithium plating in a lithium-ion battery with a high areal capacity (4 mAh/cm 2 ). The 1D model assumes uniform mechanical and temperature profile, while the 3D model is capable of capturing the nonuniformity of stress and temperature in the cell. Further, the effects of mechanical deformation and different temperatures on the process of lithium plating are investigated in this study. With the help of the 1D charging simulations, it is observed that lower temperatures increase the risk of lithium plating and the presence of mechanical deformations can accelerate its initiation. Furthermore, 3D charging simulations indicated that folds and boundaries of jellyrolls are more susceptible to lithium plating due to the higher stress concentration and lower temperature, respectively.

25 ENERGY STORAGE↗
DOE OSTI2018

Numerical Modeling of RBMK-1000 Graphite Stack Distortion

Engineering and detailed three-dimensional models of the RBMK-1000 graphite stack for modeling of its distortions caused by the appearance of longitudinal cracks in the blocks owing to the nonuniformity of the temperature and fluence distributions are described. As the neutron fluence accumulates and the limit longitudinal deflection of the graphite columns is reached, the graphite stack is repaired by cutting the graphite blocks. The developed models make it possible to evaluate the accumulation of deflection of the columns before and after repairs and the effectiveness of various repair schemes. The developed models are used to calculate the maximum deflection of the stack columns in the No. 1 unit of the Leningradskaya NPP for different operating conditions after repairs.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2021

Steady-State Mechanical Analysis for Target Assembly in the Material Plasma Exposure eXperiment Facility

The Material Plasma Exposure eXperiment (MPEX) steady-state linear plasma facility is currently under design at Oak Ridge National Laboratory to expose target specimens to fusion divertor regimes. The neutron-irradiated target is actively cooled and remote handled in the MPEX facility for conducting plasma-material–interaction (PMI) experiments. Here, the steady-state stresses in the target and target assembly system are investigated using two-dimensional (2-D) and three-dimensional (3-D) models to provide expected stresses/strains under the heat loads to which various system components would be exposed during MPEX operation. The calculated temperatures from the 2-D axisymmetric mechanical model were found to be in excellent agreement with those from the full 3-D thermohydraulic model, providing a strong model validation. Numerical simulation results for the steady-state mechanical model indicate nonuniform distributions for the temperature, stress, and deformation within the critical components. For the initial design, the deformation results indicate possible gap openings between contacting surfaces below the plasma-facing materials. To reduce the possibility of interfacial gap opening, the target assembly was slightly changed and evaluated using the 2-D stress model. Numerical simulation results indicate that the interfacial gap openings can be minimized without drastically changing the entire target assembly. The stress-strain conditions for the target will be further used to assess the appropriate operation during MPEX experiments and gain insight into materials science phenomena during PMI.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Simulation and measurement of beam-induced heating of ceramic vacuum chambers

In this article, we summarize recent theoretical and experimental studies of the impedance and beam-induced heating of titanium-coated ceramic vacuum chambers used in the NSLS-II injection kickers. The impedance was calculated using the field matching theory assuming planar approximation and compared with the mpedanceake2 code. For the coating thickness of a few microns, we demonstrated that the beam-induced power is dissipated in the titanium coating and that the longitudinally averaged two-dimensional power density is approximated by an analytical expression, thus allowing the use of a simplified model of the power density as input for the code to simulate the temperature distribution with realistic nonuniform thickness of the Ti coating. For a few values of the NSLS-II beam current, we measured the beam-induced heating of two ceramic chambers using thermal sensors installed along the chamber and compared the measurement results with the simulations. Published by the American Physical Society 2024

36 MATERIALS SCIENCE↗
DOE OSTI2022

Dispersion relation and instability for an anisotropic nonuniform flowing plasma

A generalized formula for wave instability is developed for an anisotropic nonuniform plasma with finite flows and temperatures. Six-moment fluid equations are solved to give the analytic expression for wave instability in arbitrarily nonuniform plasmas. The analytic formula explicitly states the dependence of wave instability on the nonuniformities of number density, flow velocity, and anisotropic or isotropic pressure. The accuracy of the formalism is verified by a numerical calculation of implicit dispersion relations in complex Fourier space. The analysis shows that nonuniformity plays a critical role in plasma instability, while the flow velocity and anisotropic pressures determine the growth rate of the instability. Lastly, the instability diagram and associated instability criterion for anisotropy-driven instability are introduced as applications of the formalism.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2019

Temperature control to reduce capacity mismatch in parallel-connected lithium ion cells

The temperature and capacity of individual cells affect the current distribution in a battery pack. Non uniform current distribution among parallel-connected cells can lead to capacity imbalance and premature aging. This paper develops models that calculate the current in parallel-connected cells and predict their capacity fade. The model is validated experimentally for a nonuniform battery pack at different temperatures. The paper also proposes and validates the hypothesis that temperature control can reduce capacity mismatch in parallel-connected cells. Three Lithium Iron Phosphate cells, two cells at higher initial capacity than the third cell, are connected in parallel. The pack is cycled for 1500 Hybrid Electric Vehicles cycles with the higher capacity cells regulated at 40 C and the lower capacity cell at 20 C. As predicted by the model, the higher capacity and temperature cells age faster, reducing the capacity mismatch by 48% over the 1500 cycles. A case study shows that cooling of low capacity cells can reduce capacity mismatch and extend pack life.

25 ENERGY STORAGE↗
DOE OSTI2024

Reaction Pathways and Energy Consumption in NH 3 Decomposition for H 2 Production by Low Temperature, Atmospheric Pressure Plasma

Pathways for NH 3 decomposition to N 2 and N 2 H 4 by atmospheric pressure nonthermal plasma are analyzed using a combination of molecular beam mass spectrometry measurements and zero-dimensional kinetic modeling. Experimental measurements show that NH 3 conversion and selectivity towards N 2 formation scale monotonically with the specific energy input into the plasma with ~ 100% selectivity to N 2 formation achieved at specific energy inputs above 0.12 J cm −3 (3.1 eV (molecule NH 3 ) −1 ). The kinetic model recovers these trends, although it underpredicts N 2 selectivity at low specific energy input. These discrepancies can be explained by the underestimation of reaction rate coefficients for reactions that consume N 2 H x species in collisions with H radicals and/or radial nonuniformities in power deposition, gas temperature, and species concentrations that are not represented by the plug flow approximation used in the model. The kinetic model shows that N 2 formation proceeds through N 2 H x decomposition pathways rather than NH x decomposition pathways in low temperature, atmospheric pressure plasma. Higher selectivity toward N 2 production can be achieved by operating at higher NH 3 conversion and with a higher gas temperature. Furthermore, the high energy cost of NH 3 decomposition by atmospheric pressure nonthermal plasma found in this work (25–50 eV (molecule NH 3 converted) −1 ; 17–33 eV (molecule H 2 formed) −1 ) is a result of the energy requirement for electron-impact dissociation of NH 3 and the significant re-formation of NH 3 by three-body recombination reactions between NH 2 and H.

Nonthermal plasma↗