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All sourcesNASA NTRSDOE OSTI
DOE OSTI2011

Nuclear Data Sheets for A = 133

Evaluated nuclear structure and decay data for all nuclei within the A=133 mass chain are presented. The experimental data are evaluated and best values for level and gamma-ray energies, quantum numbers, lifetimes, gamma-ray intensities, and other nuclear properties are recommended. Inconsistencies and discrepancies that exist in the literature are noted. This work supersedes the earlier evaluation by S. Raab (1995Ra12), published in Nuclear Data Sheets75, 491 (1995).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

Reactor Fuel Isotopics and Code Validation for Nuclear Applications

Experimentally measured isotopic concentrations of well characterized spent nuclear fuel (SNF) samples have been collected and analyzed by previous researchers. These sets of experimental data have been used extensively to validate the accuracy of depletion code predictions for given sets of burnups, initial enrichments, and varying power histories for different reactor types. The purpose of this report is to present the diversity of data in a concise manner and summarize the current accuracy of depletion modeling. All calculations performed for this report were done using the Oak Ridge Isotope GENeration (ORIGEN) code, an internationally used irradiation and decay code solver within the SCALE comprehensive modeling and simulation code. The diversity of data given in this report includes key actinides, stable fission products, and radioactive fission products. In general, when using the current ENDF/B-VII.0 nuclear data libraries in SCALE, the major actinides are predicted to within 5% of the measured values. Large improvements were seen for several of the curium isotopes when using improved cross section data found in evaluated nuclear data file ENDF/B-VII.0 as compared to ENDF/B-V-based results. The impact of the flux spectrum on the plutonium isotope concentrations as a function of burnup was also shown. The general accuracy noted for the actinide samples for reactor types with burnups greater than 5,000 MWd/MTU was not observed for the low-burnup Hanford B samples. More work is needed in understanding these large discrepancies. The stable neodymium and samarium isotopes were predicted to within a few percent of the measured values. Large improvements were seen in prediction for a few of the samarium isotopes when using the ENDF/B-VII.0 libraries compared to results obtained with ENDF/B-V libraries. Very accurate predictions were obtained for 133 Cs and 153 Eu. However, the predicted values for the stable ruthenium and rhodium isotopes varied as much as 10% of the measured values, and 109 Ag was consistently over-predicted by as much as 170%. In general, there is a larger uncertainty for modeling radioactive fission products when compared to either the actinides or the stable fission products in SNF. The relative C/E ratios ranged from a few percent for 137 Cs up to 60% and 100% for 106 Ru and 125 Sb, respectively. Limited or no radioactive fission products data exist in the current data sets for reactor types other than PWRs and BWRs. More work is needed in obtaining a greater diversity of radioactive fission product data. While performing this survey, issues leading to inconsistencies in nuclear fission yield data were discovered that specifically impacted the fission product noble gases. Emphasis was given to this legacy data, and corrective actions were taken as described in this report. After the fission yield data were corrected, the stable xenon and krypton fission products were predicted to within 5% of their measurements. However, preliminary results not explicitly given in this report indicate that the relative C/E ratio for the radioactive isotope 85 Kr varied as much as 10%. Due to the complex migration and the difficulty in measuring noble gases in the fuel, a more thorough investigation is needed to understand how accurately depletion codes can calculate these gas concentrations.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2013

Low background HPGe spectrometer in investigations of 2β decay

The low background high sensitive HPGe spectrometer called OBELIX is briefly described. The calibration measurements using {sup 152}Eu, {sup 133}Ba and La{sub 2}O{sub 3} sources in different geometries, the obtained efficiency curves for OBELIX HPGe detector, the results of measurements of radioactivity of the NEMO-3 sources ({sup 100}Mo, {sup 150}Nd) as well as future plans for OBELIX detector (e.g. 0νEC/EC decay of {sup 106}Cd) are presented.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2013

Study of Rayleigh–Taylor growth in laser irradiated planar SiO{sub 2} targets at ignition-relevant conditions

Rayleigh–Taylor (RT) growth experiments were performed on the OMEGA laser [T. R. Boehly et al., Opt. Commun. 133, 495 (1997)] using planar SiO{sub 2} targets seeded with a single mode 60-μm wavelength perturbation driven at peak laser intensities up to 9 × 10{sup 14} W/cm{sup 2}. These are the first RT measurements in SiO{sub 2} at conditions relevant to direct-drive inertial confinement fusion ignition. The measured average modulation growth rates agree with the 2-D hydrodynamics code DRACO, providing an important step in the development of target ablators that are robust to RT growth and hot- electron preheat considerations when driven at the intensities required to achieve thermonuclear ignition.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2011

Atomic mix in directly driven inertial confinement implosions

Directly driven implosions on the Omega laser [T. R. Boehly et al., Opt. Commun. 133, 495 (1997)] have measured the presence of atomic mix using D+T neutron yield rates from plastic capsules with and without deuterated layers, and a nearly pure tritium fuel containing 0.7% deuterium. In 15, 19, and 24 {mu}m thick plastic shells, D+T neutron yields increased by factors of 86, 112, and 24 when the 1.2 {mu}m thick inner layer was deuterated. Based on adjusting a fully atomic mix modvfel to fit yield degradation in the un-deuterated capsule and applying it to the capsule with the deuterated layer, atomic mixing accounts for 40-75% of the yield degradation due to mix. For the first time, the time dependence of mixed mass was measured by the ratio of the yield rates from both types of capsules. As expected, the amount of mix grows throughout the D+T burn.

36 MATERIALS SCIENCE↗
DOE OSTI2013

Polar-drive implosions on OMEGA and the National Ignition Facility

Polar-drive (PD) experiments on the OMEGA [Boehly et al., Opt. Commun. 133, 495 (1997)] laser are described. Continuous pulse shapes, where a low-power foot is followed by a rise to the main pulse, and triple-picket pulse shapes, where three pickets precede the main pulse, are used to irradiate warm plastic shell capsules. Both of these pulse shapes set the target on a low, ignition-relevant adiabat of ∼3.5. The areal density is modeled very well in these implosions indicating that shock timing is well modeled in PD geometry. It is shown that the symmetry can be predictably varied by changing the beam pointings. Symmetry is also well reproduced across the two pulse shapes. Limitations of OMEGA experiments are discussed. Preliminary designs for PD implosion experiments on the NIF, with the goal of addressing ignition-relevant issues for PD, including symmetry are presented.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2013

Improving cryogenic deuterium–tritium implosion performance on OMEGA

A flexible direct-drive target platform is used to implode cryogenic deuterium–tritium (DT) capsules on the OMEGA laser [Boehly et al., Opt. Commun. 133, 495 (1997)]. The goal of these experiments is to demonstrate ignition hydrodynamically equivalent performance where the laser drive intensity, the implosion velocity, the fuel adiabat, and the in-flight aspect ratio (IFAR) are the same as those for a 1.5-MJ target [Goncharov et al., Phys. Rev. Lett. 104, 165001 (2010)] designed to ignite on the National Ignition Facility [Hogan et al., Nucl. Fusion 41, 567 (2001)]. The results from a series of 29 cryogenic DT implosions are presented. The implosions were designed to span a broad region of design space to study target performance as a function of shell stability (adiabat) and implosion velocity. Ablation-front perturbation growth appears to limit target performance at high implosion velocities. Target outer-surface defects associated with contaminant gases in the DT fuel are identified as the dominant perturbation source at the ablation surface; performance degradation is confirmed by 2D hydrodynamic simulations that include these defects. A trend in the value of the Lawson criterion [Betti et al., Phys. Plasmas 17, 058102 (2010)] for each of the implosions in adiabat–IFAR space suggests the existence of a stability boundary that leads to ablator mixing into the hot spot for the most ignition-equivalent designs.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗