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The AI-Base NDA Catalog

The project objective was to create a catalog of NDA capabilities so that as future challenges emerge, potential solutions can be quickly identified. The initial direction was to create a custom database where we would manually add various NDA technologies. During the year, LANL leadership heavily embraced AI tools and established LANL’s Enterprise ChatGPT license. To align with this vision, instead of a database we created a custom GPT to achieve the same capability. We provided a series of references on NDA technologies, the most comprehensive of which is the 2024 “PANDA manual” which is a 700-page textbook. A custom GPT is a semi-isolated version of OpenAI’s GPT model that can be tailored to specific tasks with context documents and instructions. Anyone with a LANL ChatGPT Enterprise account can access the NDA Catalog. Since the GPT exists on the green network, only non-sensitive questions may be asked. The Catalog can be used by simply asking questions in conversational English. We have found the Catalog to be quite accurate, even for heavily technical, complex queries. The Catalog allows the user to describe a measurement problem and it will respond with potential technology solutions.

96 KNOWLEDGE MANAGEMENT AND PRESERVATION

Incorporating the latest Neutron NDA analysis techniques into INCC6

International Neutron Coincidence Counting (INCC6) is the IAEA’s neutron NDA software. With FY25 SGTech support we implemented self-diagnostic features into INCC6. For FY26 we propose to implement advanced analysis methods that have been splintered into custom software for one-off instruments. Incorporating these capabilities in INCC6 will make them available for any new or existing application on the ubiquitous INCC6 platform, increasing safeguards efficiency and effectiveness.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W

New NDA Methods for Thorium Fuel Cycle Safeguards (Final Report)

This project developed portable Neutron Resonance Transmission Analysis (pNRTA) as a new non-destructive assay (NDA) method for thorium fuel cycles safeguards and other applications where multiple isotopes must be measured when present together. pNRTA leverages epithermal neutron resonances to assay multiple safeguards-relevant isotopes (e.g., 233 U and 235 U) when they are present together in a sample. Existing techniques are challenged by this task, driving the need for new active interrogation methods. With selected detectors, pNRTA works in high gamma-ray backgrounds from fission and activation products and 232 U progeny expected in thorium fuel cycle samples. This project leveraged a pNRTA system developed at Pacific Northwest National Laboratory (PNNL) and collaboration with the Massachusetts Institute of Technology (MIT). The system uses a commercially available deuterium-tritium (DT) neutron generator at short standoff (2 m). Key achievements in this project included: first-of-a-kind pNRTA quantitative measurements of 233 U oxide samples, an assessment of neutron detector technologies suitable for pNRTA in high gamma-ray background environments, experimentally demonstrating quantitative assay of samples containing 233 U and 235 U, and modeling studies showing the applicability of pNRTA to a wide range of material forms. Further, a custom algorithm was developed at MIT, which provided mean bias of 9% and relative standard deviation of 36% in assaying 233 U, 235 U, 238 U, and 232 Th content in eight measured samples. These outcomes form a solid technical basis for pNRTA as a new promising capability for international safeguards verification that is portable, non-destructive, quantitative, and isotopic specific.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS

A computational environment for exhaust nozzle design

The Nozzle Design Associate (NDA) is a computational environment for the design of jet engine exhaust nozzles for supersonic aircraft. NDA may be used either to design new aircraft or to design new nozzles that adapt existing aircraft so they may be reutilized for new missions. NDA was developed in a collaboration between computer scientists at Rutgers University and exhaust nozzle designers at General Electric (GE) Aircraft Engines and General Electric Corporate Research and Development. The NDA project has two principal goals: to provide a useful engineering tool for exhaust nozzle design, and to explore fundamental research issues that arise in the application of automated design optimization methods to realistic engineering problems.

Gelsey, Andrew

Distinguishing fissile uranium isotopes using an active well neutron coincidence counter

Proposed thorium-based nuclear fuel cycles are likely to require quantification and verification of 233 U within nuclear material. Because of their similar fission cross sections, active neutron nondestructive assay (NDA) systems may respond similarly to 233 U and 235 U. Traditional safeguards equipment has been optimized for 235 U and 238 U quantification associated with conventional uranium/plutonium fuel cycles and may not be directly applicable to 233 U quantification when mixed with other actinides. This work used models of the large volume active well coincidence counter (LV-AWCC) at Oak Ridge National Laboratory to evaluate the performance of this neutron NDA system to differentiate fissile uranium isotopes. The models were developed to simulate NDA system performance in response to a number of triangular radiation signature training device sources within the central cavity or well. This work predicted that the LV-AWCC can effectively differentiate 233 U from 235 U in certain modes of operation. In active mode, the LV-AWCC with the cadmium liner results in different doubles count rates between the fissile isotopes for a given fissile uranium mass. Without the cadmium liner, the uranium isotopes provide a statistically indistinguishable doubles count rate response for the fissile masses considered in this work (up to approximately 150 g). The cadmium liner serves to harden the neutron interrogation spectrum, which better exploits the notable difference in the 233 U and 235 U fission cross sections at approximately 1 eV. In passive mode, the two fissile isotopes exhibit different doubles and singles count rates regardless of liner presence because the passive source strength of 233 U is approximately 2 orders of magnitude stronger than that of 235 U due to the shorter half-life and correspondingly higher (α, n) yield. We conclude that using neutron interrogation in the LV-AWCC, two measurements are needed to quantify 233 U content in mixed uranium items. The first measurement is used to determine the total fissile uranium mass using a mode that cannot distinguish fissile isotopes (i.e., where a similar response is observed for both fissile uranium isotopes such as active doubles without cadmium or using a thermal neutron interrogation source). In conclusion, the second measurement is used to determine the 233 U content by using a differentiating technique (e.g., passive doubles, passive doubles to singles ratio, active doubles with cadmium).

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND

Validation and demonstration of the AEFC as a practical safeguards tool for inventory verification

The Advanced Experimental Fuel Counter (AEFC) is a nondestructive assay (NDA) instrument designed to determine the residual fissile mass in irradiated fuel assemblies for safeguards verification purposes. This is done by actively interrogating an assembly with a neutron source and measuring the total (Singles) and correlated (Doubles) neutron count rates resulting from induced fissions in the irradiated nuclear fuel and relating those rates to the residual fissile mass using calibration curves. Comprehensive NDA measurements of the irradiated fuel inventory at Israeli Research Reactor 1 (IRR-1) were taken with the AEFC to validate a set of previously developed calibration curves. During the campaign, measurements were acquired of 32 standard fuel assemblies and three control assemblies in just nine days. This is a significant majority of the research reactor's irradiated fuel inventory and the largest data set gathered by the AEFC to date. Many of the fuel assemblies measured during the campaign had much shorter cooling times than those assemblies previously measured with the instrument. Calibration curves developed from previous AEFC deployments were used to determine the residual 235 U mass in the measured standard fuel assemblies. The results of the campaign demonstrated that the AEFC can be used to estimate the 235 U mass remaining in a large number of irradiated fuel assemblies with 1%–5% uncertainty in a reasonable amount of time despite operating in a high dose environment.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P

Evaluation of the Radiological Characterization for Off-Site Source Recovery Program Waste Streams LA-OS-00-01.001, LA-OS-00-03, and LA-OS-00-04

The purpose of this memorandum is to satisfy the requirements of Section 4.4 of the CCP Acceptable Knowledge Documentation procedure CCP-TP-005 (Ref. 1). This evaluation is updating the previously issued memo NEN3:24-045 issued in August 2024. CCP-TP-005 requires an AK Expert and the OSRP group to evaluate the radionuclide characterization of a waste stream and prepare the NDA Memorandum (letter to CCP Records). This NDA memorandum was written with input from the OSRP group, as required by CCP-TP-005. This memo includes a discussion of the limitations for the radiological characterization and a description of the characterization method.

07 ISOTOPE AND RADIATION SOURCES

Study on Application of Distributed Network of Sensors with List Mode for NMAC Literature Review

Nuclear material accounting and control (NMAC) for nuclear security detects, deters, and resolves questions related to unauthorized removal (i.e. theft) or misuse of nuclear material. NMAC also serves as a key insider threat mitigation measure and aids in recovery of nuclear material that is missing. Effective nuclear security depends on NMAC for timely and accurate information about nuclear material types, quantities, and locations. Bulk nuclear material processing facilities, however, present unique challenges for effective NMAC due to the presence of large quantities of material in-process and the accumulation of residual material holdup within process equipment. These holdup accumulations can obscure accurate physical inventory taking and complicate efforts to resolve NMAC irregularities at the facility level. Bulk material monitoring systems often rely on material balance calculations and indirect measurement techniques, which may mask protracted theft of smaller amounts of nuclear material. These monitoring limitations have generated increased interest in continuous monitoring technologies, including distributed non-destructive assay (NDA) sensor networks capable of providing real-time or near-real-time measurement of material movement and accumulation within bulk processing environments. Recent advancements in distributed networks of NDA radiation detectors and sensing technologies provide an opportunity to address these limitations. Although such distributed sensor networks have been implemented in select facilities for IAEA Safeguards applications, their potential for supporting NMAC functions specifically tailored to nuclear security objectives remains largely unexplored. Furthermore, emerging list-mode data acquisition technologies have reached high technology readiness levels, enabling time-correlated detection of nuclear events across multiple temporal scales. These capabilities provide enhanced opportunities for accurate holdup measurement, continuous process monitoring, and improved detection of material theft or misuse over time. The increasing global expansion of civil nuclear power and development of related bulk material processing facilities, including those supporting high-assay low-enriched uranium (HALEU) and other advanced reactor fuel fabrication, further increases the need for advanced measurement and monitoring strategies for NMAC.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS

Wholly Aromatic Ether-imides. Potential Materials for n-Type Semiconductors

We report on the synthesis and characterization of a novel series low-molar-mass ether-imide rod-shaped model compounds. All ether-imides were obtained by terminating the appropriate rigid core dianhydride, i.e. pyromellitic dianhydride (PMDA), 1,4,5,8-naphthalenetetracarboxylic dianhydride (NDA), 3,3',4,4'-biphenyltetracarboxylic dianhydride (BPDA), and 3,3,4,4'-oxydiphthalic dianhydride (ODPA) with three flexible aryl-ether tails of different chain length. The mono-functional aryl-ether amines, i.e. 4-(3-phenoxy-phenoxy)-phenylamine (2) and 4-(3-phenoxy-3-phenoxy-phenoxy)-phenylamine (4), were synthesized using standard fluoro-displacement and Ullmann condensation techniques. The corresponding ether-imide model compounds were obtained in high yields using a one-step solution imidization procedure. Increasing the number of meta-substituted aryl-ether units reduces the melt transition temperatures and at the same time it increases the solubility of the model compounds. Most model compounds are crystalline solids and form isotropic melts upon heating. 2,7-Bis-(-4-phenoxy-phenyl)-benzo[Imn][3,8]phenanthroline1,3,6,8-tetraone (NDA-n0), however, displays a smectic A (SA) when cooled from the isotropic phase, followed by what appears to be either a highly ordered smectic phase or a, columnar phase. This is the first example, known to date, in which a mesophase is detected in a wholly aromatic ether-imide compound. For all compounds we present spectroscopic data and X-ray diffraction data. Cyclic voltammetry was used to determine the redox behavior and pertinent energy levels of the model compounds.

Dingemans, Theo J.

Agentic Diagrammatica: Towards Autonomous Symbolic Computation in High Energy Physics

We present Diagrammatica, a symbolic computation extension to the HEPTAPOD agentic framework, which enables LLM agents to plan and execute multi-step theoretical calculations. Symbolic computation poses a distinctive reliability challenge for LLM agents, as correctness is governed by implicit mathematical conventions that are not encoded in a form that can be easily checked in the computational backend. We identify two complementary remedies, tool-constrained computation and targeted knowledge grounding, and pursue the first as the primary architecture. Concretely, we concentrate the agent's action distribution onto tool calls with convention-fixing semantics, in which the agent specifies a compact, human-auditable diagram specification and a trusted backend performs the symbolic or numerical manipulations exactly. The toolkit provides two complementary calculation paths consuming a shared diagram specification: Naive Dimensional Analysis (NDA) for order-of-magnitude rate estimates and Exact Diagrammatic Analysis (EDA) for tree-level symbolic calculations via automatic FeynCalc code generation, both supplemented by automatic Feynman diagram enumeration and a navigable theory knowledge base. The architecture is validated on two benchmarks: (1) an exhaustive catalog of all tree-level, single-vertex $1\to 2$ partial decay widths across scalar, fermion, and vector parents, with complete massless and threshold limits and Standard Model validation; and (2) an NDA sensitivity study of the muon decay multiplicity $μ^+ \to ν_μ\barν_e + n(e^+e^-) + e^-$, determining the maximum observable $n$ at current and planned muon experiments.

Menzo, Tony [Alabama U.; Fermilab] (ORCID:00000002

Data-Driven Performance Optimization of Gamma Spectrometers With Many Channels

In gamma spectrometers with variable spectroscopic performance across many channels (e.g., many pixels or voxels), a tradeoff exists between including data from successively worse-performing readout channels and increasing efficiency. Brute-force calculation of the optimal set of included channels is exponentially infeasible as the number of channels grows, and approximate methods are required. In this work, we present a data-driven framework for attempting to find near-optimal sets of included detector channels. The framework leverages non-negative matrix factorization (NMF) to learn the behavior of gamma spectra across the detector and clusters similarly-performing detector channels together. Performance comparisons are then made between spectra with channel clusters removed, which is more feasible than brute force. The framework is general and can be applied to arbitrary, user-defined performance metrics depending on the application. We apply this framework to optimizing gamma spectra measured by H3D M400 CdZnTe (CZT) spectrometers, which exhibit variable performance across their crystal volumes. In particular, we show several examples optimizing various performance metrics for uranium and plutonium gamma spectra in non-destructive assay (NDA) for nuclear safeguards, and explore trends in performance versus parameters such as clustering algorithm type. We also compare the NMF + clustering pipeline to several non-machine-learning (ML) algorithms, including several greedy algorithms. Although, we find that the NMF + clustering pipeline tends to find the best-performing set of detector voxels, significantly improving over the unoptimized spectra, but that a greedy accumulation of spectra segmented by detector depth can, in some cases, give similar performance improvements in much less computation time.

Energy resolution

EV Watts Public Database

With the rapid increase in vehicle electrification, there is a need for up-to-date, publicly available national data to understand end user charging and driving patterns, as well as vehicle and infrastructure performance, to inform research planning. Energetics worked with various partners to collect and analyze plug-in electric vehicle (PEV) and electric vehicle supply equipment (EVSE) data from 2019 to 2022. All sensitive attributes have been removed from this publicly available dataset. Researchers from one of the partner national labs under non-disclosure agreement (NDA) can request access to additional attributes by reaching out to evwattsdata@energetics.com.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI

Asynchronous timing and Doppler recovery in DSP based DPSK modems for fixed and mobile satellite applications

While conventional analog modems employ some kind of clock wave regenerator circuit for synchronous timing recovery, in sampled modem receivers the timing is recovered asynchronously to the incoming data stream, with no adjustment being made to the input sampling rate. All timing corrections are accomplished by digital operations on the sampled data stream, and timing recovery is asynchronous with the uncontrolled, input A/D system. A good timing error measurement algorithm is a zero crossing tracker proposed by Gardner. Digital, speech rate (2400 - 4800 bps) M-PSK modem receivers employing Gardner's zero crossing tracker were implemented and tested and found to achieve BER performance very close to theoretical values on the AWGN channel. Nyguist pulse shaped modem systems with excess bandwidth factors ranging from 100 to 60 percent were considered. We can show that for any symmetric M-PSK signal set Gardner's NDA algorithm is free of pattern jitter for any carrier phase offset for rectangular pulses and for Nyquist pulses having 100 percent excess bandwidth. Also, the Nyquist pulse shaped system is studied on the mobile satellite channel, where Doppler shifts and multipath fading degrade the pi/4-DQPSK signal. Two simple modifications to Gardner's zero crossing tracker enable it to remain useful in the presence of multipath fading.

Koblents, B.

The Effects of Compressive Preloads on the Compression-After-Impact Strength of Carbon/Epoxy

A fixture to apply compressive loads to composite specimens during an impact event was used to assess the effect of prestresses on the compression-after-impact (CAI) strength of 16 ply quasi-isotropic carbon/epoxy test coupons. Advanced design of experiments techniques were used to evaluate a range of prestresses and impact energies on two material systems, T300/934 and IM7/8551-7. An instrumented drop tower supplied impact energies between 1 and 9 Joules for the T300/934 material and between 4 and 16 Joules for the IM7/8551-7 material. The prestress values varied between a low of 5.7 Wa and a high of 287 NDa. Results showed some change in CAI strength that could be attributed to the prestresses on the specimens.

Nettles, Alan T.

General Aviation in Nebraska: Nebraska SATS Project Background Paper No. 1

The Nebraska SATS project is a state-level component of NASA's Small Aircraft Transportation System (SATS). During the next several years the project will examine several different factors affecting SATS implementation in Nebraska. These include economic and taxation issues, public policy issues, airport planning processes, information dissemination strategies, and systemic change factors. This background paper profiles the general aviation system in Nebraska. It is written to provide information about the "context" within which SATS will be pursued. The primary focus is thus on describing and providing background information about the current situation. A secondary focus is on drawing general conclusions about the ability of the current system to incorporate the types of changes implied by SATS. First, some brief information on the U.S. aviation system is provided. The next two sections profile the current general aviation aircraft and pilot base. Nebraska's system of general aviation airports is then described. Within this section of the paper, information is provided on the different types of general aviation airports in Nebraska, airport activity levels and current infrastructure. The fourth major section of the background paper looks at Nebraska's local airport authorities. These special purpose local governments oversee the majority of the general aviation airports in the state. Among the items examined are total expenditures, capital expenditures and planning activities. Next, the paper provides background information on the Nebraska Department of Aeronautics (NDA) and recent Federal funding for general aviation in Nebraska. The final section presents summary conclusions.

Smith, Russell

Reliability on ISS Talk Outline

1. Overview of ISS 2. Space Environment and it effects a. Radiation b. Microgravity 3. How we ensure reliability a. Requirements b. Component Selection i. Note: I plan to stay away from talk about Rad Hardened components and talk about why we use older processors because they are less susceptible to SEUs. c. Testing d. Redundancy / Failure Tolerance e. Sparing strategies 4. Operational Examples a. Multiple MDM Failures on 6A due to hard drive failure In general, my plan is to only talk about data that is currently available via normal internet sources to ensure that I stay away from any topics that would be Export Controlled, ITAR, or NDA‐controlled. The operational example has been well‐reported on in the media and those are the details that I plan to cover. Additionally I am not planning on using any slides or showing any photos during the talk.

Misiora, Mike

Non-Destructive Plutonium Assay in Pyroprocessing Bulk Materials with a 3D Boron-Coated-Straw Detector Array

Assessment of plutonium content through all the processing steps is needed and is a challenging task. While several destructive assay methods have been developed for nuclear material accountability, a nondestructive assay (NDA) system for the assessment of plutonium in bulk materials is still needed. This system should withstand pyroprocessing harsh environments and have consistent sensitivity and accuracy despite different fuel form factors. We aim to enable the accurate assessment of the plutonium content of nuclear material during pyroprocessing to improve the separation process and enhance its proliferation resistance. We plan to achieve this goal by developing and demonstrating a new 3D boron-coated-straw neutron detector array (3D-BCSDA) with high efficiency and spatial resolution.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS

Internship overview

Explore the source record for details and available documents.

42 ENGINEERING