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Ultra-pure nickel for structural components of low-radioactivity instruments

The next generation of nuclear and particle physics rare-event search experiments demand structural materials combining ultra-low levels of radioactive contamination with exceptional mechanical strength. Here, this study evaluates chemical vapor deposition (CVD) nickel as a low radioactive background candidate structural material for such applications. Manufacturer-supplied CVD Ni grown on aluminum substrates was assayed via inductively coupled plasma mass spectrometry (ICP-MS) employing isotope-dilution. These material assays produced measured bulk concentration of 232 Th, 238 U, and nat K at the levels of ~70 ppq, ≲100 ppq, and ~900 ppt, respectively, which is the lowest reported in nickel. Surface-etch profiling uncovered higher concentrations of these contaminants extending ~10 μ m beneath the surface, likely associated with the aluminum growth substrate. Additionally, the CVD Ni underwent tensile testing alongside standard Ni samples. CVD Ni exhibited a planar tensile strength of ~600 MPa, significantly surpassing standard nickel. However, heat treatment was found to reduce the tensile strength to levels comparable to standard Ni, with implications for high-temperature weld joining methods. The results reported are compared to the one other well documented usage of CVD Ni in a low radioactive background physics research experiment and a discussion is provided on how the currently reported results may arise from changes in CVD fabrication or testing process. These results establish CVD Ni as a promising low-radioactivity structural material, while outlining the need for further development in surface cleaning and weld-joining techniques to fully realize its potential in large-scale, low radioactive background rare-event search experiments.

47 OTHER INSTRUMENTATION

Ultra-sensitive radon assay using an electrostatic chamber in a recirculating system

Rare event searches such as neutrinoless double beta decay and Weakly Interacting Massive Particle detection require ultra-low background detectors. Radon contamination is a significant challenge for these experiments, which employ highly sensitive radon assay techniques to identify and select low-emission materials. This work presents the development of ultra-sensitive electrostatic chamber (ESC) instruments designed to measure radon emanation in a recirculating gas loop, for future lower background experiments. Unlike traditional methods that separate emanation and detection steps, this system allows continuous radon transport and detection. This is made possible with a custom-built recirculation pump. A Python-based analysis framework, PyDAn, was developed to process and fit time-dependent radon decay data. Radon emanation rates are given for various materials measured with this instrument. A radon source of known activity provides an absolute calibration, enabling statistically-limited minimal detectable activities of 20 µBq. These devices are powerful tools for screening materials in the development of low-background particle physics experiments.

47 OTHER INSTRUMENTATION

Ultra-sensitive radon assay using an electrostatic chamber in a recirculating system

Rare event searches such as neutrinoless double beta decay and Weakly Interacting Massive Particle detection require ultra-low background detectors. Radon contamination is a significant challenge for these experiments, which employ highly sensitive radon assay techniques to identify and select low-emission materials. This work presents the development of ultra-sensitive electrostatic chamber (ESC) instruments designed to measure radon emanation in a recirculating gas loop, for future lower background experiments. Unlike traditional methods that separate emanation and detection steps, this system allows continuous radon transport and detection. This is made possible with a custom-built recirculation pump. A Python-based analysis framework, PyDAn, was developed to process and fit time-dependent radon decay data. Radon emanation rates are given for various materials measured with this instrument. A radon source of known activity provides an absolute calibration, enabling statistically-limited minimal detectable activities of 20 uBq. These devices are powerful tools for screening materials in the development of low-background particle physics experiments.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND

Radioactivity-in-materials lead for nEXO (Final Scientific Report)

Abstract, introduction, and summary of work completed and products produced by DOE award SC002466. Primary products were six peer-reviewed publications and two PhD theses. This award also supported the operation of an underground HPGe detector and several radioassay measurements: one in a stand alone publication in Phys. Rev. C and the others in an upcoming nEXO radioassay summary paper. The nEXO collaboration aims to demonstrate the Majorana nature of the neutrino by observing the neutrinoless double-beta decay of 136 Xe with a next-generation experiment. The University of Kentucky nEXO group (UKY) operates a world-leading ultra-low-background γ-ray spectrometer as part of the nEXO radioactive background control R&D effort. The nEXO project is a proposed ton-scale neutrinoless double-beta decay experiment. The UKY PI is leading the radioactivity content assessment for all materials required by the nEXO project. As a subset of this task, UKY is also responsible for project-wide management of all low-background γ-ray spectrometry measurements; material assays with these types of instruments, together with ICP-MS, neutron-activation-analysis, and α-spectrometry, are critical to ensuring that the nEXO project can achieve its design sensitivity

73 NUCLEAR PHYSICS AND RADIATION PHYSICS

High-bandwidth frequency domain multiplexed readout of transition-edge sensors for neutrinoless double beta decay searches

The next-generation of cryogenic neutrinoless double-beta decay experiments require increasingly fast readout in order to improve background discrimination. These experiments, operated as cryogenic calorimeters at ∼ 10 mK, are usually read out by high-impedance neutron transmutation doped (NTD) thermistors, which provide good energy resolution, but are limited by ∼ 1 ms response times. Superconducting detectors, such as transition-edge sensors (TESs) with a time resolution of ∼ 100 μs, offer superior timing performance over NTD semiconductor bolometers. To make this technology viable for an application to a thousand or more channels, multiplexed readout is necessary in order to minimize the thermal load and radioactive contamination induced by the readout. Frequency-domain multiplexing readout (fMUX) for TESs, previously developed at Berkeley Lab and McGill University, is currently in use for mm-wave telescopes with detector sampling rates in the order of 100 Hz. We demonstrate a new readout system, based on the McGill/Berkeley digital fMux readout, to satisfy the higher bandwidth and noise requirements of the next generation of TES-instrumented cryogenic calorimeters. Each multiplexing readout module comprises 10 superconducting resonators in the 1–5 MHz range and a DC superconducting quantum interference device (DC-SQUID), interfaced to high-speed field programmable gate array (FPGA)-based electronics for digital signal processing and low-latency SQUID feedback. The new readout samples detectors at 156 kHz, three orders of magnitude faster than its cosmology-oriented predecessor, and demonstrates a stable feedback bandwidth of 3 kHz in a real TES-based system.

47 OTHER INSTRUMENTATION

Characterization of Precipitation-Induced Radon Progeny Deposition Events Using a City-Scale Sensor Network

Networks of radiation detectors provide a platform for real-time radioactive source detection and identification in urban environments. Detection algorithms in these systems must adapt to naturally-occurring changes in background, which requires well-characterized relationships between precipitation events and their corresponding radiological signature. Here, we present a quantitative and qualitative description of rain-induced radon progeny deposition events occurring in Chicago from September 2023 to February 2024. We measure ambient gamma radiation levels, precipitation rate, temperature, pressure, and relative humidity in a network of sensor nodes. For each identified precipitation period, we decompose spectra into static- and radon-associated components as defined by a non-negative matrix factorization (NMF) algorithm. We find a consistent power-law relationship between a precipitation-dependent peak of the radon progeny proxy (RPP) and the peak strength of the radon-associated NMF component for most precipitation events. We conduct a case study of a rainfall period with abnormally high levels of implied radon progeny concentration and describe its temporal and spatial evolution. We hypothesize that this phenomenon is due to the air mass path that intersects a uranium-rich region of Wyoming. Finally, we cluster precipitation events into three distinct categories. One category roughly corresponds to events with deep low-pressure systems and high relative radon concentration, while another is characteristic of light stratiform rain with slightly higher temperatures and intermediate relative radon concentration. The third category appears to contain weak-gradient or lake breeze convection showers with intermittent precipitation and low relative radon concentration. These findings suggest that radiological anomaly detection could be improved by training unique background models corresponding to each category of meteorological event.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND

Benchmarking the design of the cryogenics system for the underground argon in DarkSide-20k

DarkSide-20k (DS-20k) is a dark matter detection experimentunder construction at the Laboratori Nazionali del Gran Sasso (LNGS)in Italy. It utilises ∼ 100 t of low radioactivity argon from anunderground source (UAr) in its inner detector, with half serving astarget in a dual-phase time projection chamber (TPC). The UArcryogenics system must maintain stable thermodynamic conditionsthroughout the experiment's lifetime of over10 years. Continuous removal ofimpurities and radon from the UAr is essential for maximising signalyield and mitigating background. We are developing an efficient andpowerful cryogenics system with a gas purification loop with atarget circulation rate of1000 slpm. Central to itsdesign is a condenser operated with liquid nitrogen which is pairedwith a gas heat exchanger cascade, delivering a combined coolingpower of more than 8 kW. Here wepresent the design choices in view of the DS-20k requirements, inparticular the condenser's working principle and the coolingcontrol, and we show test results obtained with a dedicatedbenchmarking platform at CERN and LNGS. We find that the thermalefficiency of the recirculation loop, defined in terms of nitrogenconsumption per argon flow rate, is95 % and the pressure in the testcryostat can be maintained within±(0.1–0.2) mbar. Wefurther detail a 5-day cool-down procedure of the test cryostat,maintaining a cooling rate typically within-2 K/h, as required for theDS-20k inner detector. Additionally, we assess the circuit's flowresistance, and the heat transfer capabilities of two heat exchangergeometries for argon phase change, used to provide gas forrecirculation. We conclude by discussing how our findings influencethe finalisation of the system design, including necessarymodifications to meet requirements and ongoing testing activities.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND