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NASA NTRS1977

Simultaneous holographic and photocurrent studies of the photorefractive effect in LiTaO3 and LiNbO3

In reduced LiNbO3:Mn both the photorefractive sensitivity and the simultaneously measured photocurrent result from drift with a polarization-dependent effective 'internal field' of about 6 kV/cm. In reduced undoped LiTaO3 the observed difference in applied fields of the minimum photorefractive sensitivity and zero photocurrent imply charge transport is by a mechanism that cannot be completely described by diffusion and drift in an electric field. The direct measurement of the harmonic content of phase gratings written in several LiNbO3 and LiTaO3 crystals shows termination of charge-transport results from the space-charge field of the hologram.

Spinhirne, J. M.↗

NASA NTRS1973

Sensitivity and fatigue of LiTaO3 for holographic recording

The sensitivity of crystals of LiTaO3 to hologram formation was observed to vary with impurity concentration from a value comparable to the most sensitive doped LiNbO3 for an impure crystal to a value more than five orders of magnitude smaller for a purer crystal. Fatigue effects were observed upon write-erase cycling. These effects were dependent upon writing and erasure polarization and power and could be virtually eliminated by proper choice of optical parameters.

Spinhirne, J. M.↗

NASA NTRS1974

Sensitivity and fatigue of LiTaO3 for holographic recording

The sensitivity of LiTaO3 crystals to hologram formation has been observed to vary with impurity concentration. For a writing wavelength of 488.0 nm and power density of 1.1 W/sq cm, the sensitivity varied from a value comparable to the most sensitive doped LiNbO3 for an impure crystal to a value more than 5 orders of magnitude smaller for a purer crystal. Fatigue effects were observed upon write-erase cycling. These effects were dependent upon writing and erasure polarization and power density and could be minimized by proper choice of optical parameters.

Spinhirne, J. M.↗

NASA NTRS1978

Development of improved lithium tantalate pyroelectric detectors

A program was undertaken to increase the detectivity of LiTaO3 pyroelectric detectors to meet a performance requirement of D star (500 K, 15 Hz)=4x10 to the 9th power cm Hz1/2W-1. Emphasis was placed on reduction of the thermal conductance of the detector element to its surroundings, thinning the detector wafer to a thickness less than 3 micrometers, and increasing the absorptivity of the standard metallic film coatings. During the program, thermal conductance was reduced 41 percent through the use of reticulated (slotted) structures. Self-supported detector wafers less than 2 micrometers thick were fabricated. Multiple layer coatings, including an AR coating, with 16 percent more absorptance, were designed and fabricated. Later refinements in the multilayer design program have absorptivities of 75-80 percent, but detectors with these coatings had to be more than 2 micrometers thick because of a mismatch in the thermal expansion coefficients with LiTaO3.

Byer, N. E.↗

NASA NTRS1974

Alkali oxide-tantalum oxide and alkali oxide-niobium oxide ionic conductors

A search was made for new cationic conducting phases in alkali-tantalate and niobate systems. The phase equilibrium diagrams were constructed for the six binary systems Nb2O5-LiNbO3, Nb2O5-NaNbO3, Nb2O5-KNbO3, Ta2O5-NaTaO3, Ta2O5-LiTaO3, and Ta2O5-KTaO3. Various other binary and ternary systems were also examined. Pellets of nineteen phases were evaluated (by the sponsoring agency) by dielectric loss measurements. Attempts were made to grow large crystals of eight different phases. The system Ta2O5-KTaO3 contains at least three phases which showed peaks in dielectric loss vs. temperature. All three contain structures related to the tungsten bronzes with alkali ions in non-stoichiometric crystallographic positions.

Roth, R. S.↗

NASA NTRS1984

Pyroelectric materials as electronic pulse detectors of ultraheavy nuclei

The design and testing of ultraheavy-nucleus pulse detectors based on pyroelectric materials are reported, extending the preliminary findings of Tuzzolino (1983) and Simpson and Tuzzolino (1983). Uranium-ion beams of about 240 MeV/u are detected by a 39.5-micron-thick Si detector, degraded to about 175 MeV/u by Al absorbers, and then strike 700-micron-thick polyvinylidene fluoride or 1000-micron-thick LiTaO3 pyroelectric samples. Both detector systems are connected to a coincidence circuit via charge-sensitive preamplifiers, shaping amplifiers with 30-microsec effective time constants, and electronic discriminators. Sample spectra are shown, and the pulse heights measured are found to agree with theoretical calculations to within a factor of about 2. The response of the pyroelectric materials is found to be unaffected by exposure to about 10 Mrad of 2-7-MeV/u heavy ion radiation. With further study and improvement of the detection sensitivity, devices of this type could be applied to large-area space measurements of low ultraheavy-ion fluxes.

Simpson, J. A.↗