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A three-dimensional laser ray-tracing methodology for radiation-hydrodynamics simulations

We report on a methodology for performing laser ray-tracing in three spatial dimensions for radiation-hydrodynamics simulation codes. Our method, which is an extension of that developed in Haines et al., Comput. Fluids 201, 104478 (2020), utilizes an automatically generated separate mesh for the laser ray-tracing from the radiation-hydrodynamics mesh. This enables the laser mesh to be tailored to minimize ray noise with significantly fewer rays than would be required when the ray-tracing is performed on the radiation-hydrodynamics mesh, primarily by allowing the use of high-aspect-ratio cells that are not suitable for hydrodynamics solvers. For a planar target, we show that our method provides a ≈ 100× reduction in computational expense to achieve a fixed level of ray noise relative to ray-tracing directly on the radiation-hydrodynamics mesh. The relatively low ray requirement also enables efficient computation of cross-beam energy transfer. Each cell in the logically cubic laser mesh is a non-convex dodecahedron with triangular sides, and numerical integration of the ray trajectories and inverse bremsstrahlung is performed by mapping each cell to the unit cube. We will describe our methodology in detail as well as its implementation in the xRAGE radiation-hydrodynamics code, discuss performance, and present the results from applying the methodology to test problems with analytic solutions for laser ray-tracing through a quadratic density gradient with an analytic solution as well as for a laser-driven heat front. In 3D radiation-hydrodynamics simulations of laser-driven experiments performed on the National Ignition Facility, laser ray-tracing with our methodology uses less than 1% of total computational time while introducing acceptably low levels of ray noise.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Coupling laser physics to radiation-hydrodynamics

In order to accurately model implosion hydrodynamics in a radiation-hydrodynamics code, it is essential to include accurate accounting for energy deposition physics. In inertial confinement fusion (ICF), where capsules are driven by lasers or laser-driven x-rays, energy deposition profiles and energy transport have a strong impact on the development and evolution of capsule dynamics and hydrodynamic instabilities. Nevertheless, accurately modeling laser beam propagation in radiation-hydrodynamics codes presents unique challenges associated with disparate resolution requirements, the potential to seed spurious noise in highly unstable systems, and computational expense. We discuss a new method for coupling laser ray-tracing physics to a radiation hydrodynamics code, developed in the process of implementing the Mazinisin laser ray-trace into the xRAGE radiation hydrodynamics code. In contrast to previous approaches, in which laser ray-tracing is performed on the radiation-hydrodynamics mesh, our method involves a mesh generation and evolution strategy that addresses the unique requirements of the laser ray-trace in a separate mesh, enabling performance enhancements and strategies to reduce noise seeded by the discretization of beams into computational rays. In addition, we have employed several methods to ensure that spurious mesh imprinting is minimized. These involved optimizing the laser and radiation-hydrodynamics meshes as well as interpolation between them and requires the use of an exact initialization method for the radiation-hydrodynamics mesh. Furthermore, these techniques have enabled efficient computation of laser-driven implosions and other experiments with minimal introduction of spurious noise.

47 OTHER INSTRUMENTATION↗

Expansion-Driven Self-Magnetization of High-Energy-Density Plasmas

Understanding plasma self-magnetization is one of the fundamental challenges in both laboratory and astrophysical plasmas. Self-magnetization can modify plasma transport properties, altering the dynamical evolution of plasmas. Multiple high-energy-density (HED) experiments have observed the formation of ion-scale magnetic filaments of megagauss strength, though their origin remains debated. Here, in this study, we conduct 2D collisional particle-in-cell (PIC) simulations with a laser ray-tracing module for a fully self-consistent simulation of the plasma ablation, expansion, and magnetization. The simulations use a planar geometry, effectively suppressing the Biermann magnetic fields, to focus on anisotropy-driven instabilities. The laser intensity is varied between 10 13 and 10 14 W/cm 2 , which is relevant to HED and inertial fusion experiments where collisions must be considered. We find that, above a critical intensity, the plasma rapidly self-magnetizes via an expansion-driven Weibel process, producing a plasma beta of 100 (𝛽 = 8⁢𝜋⁢𝑘 𝐵 ⁢𝑛 𝑒 ⁢𝑇 𝑒 /𝐵 2 ) and Hall parameter 𝜔 ce ⁢𝜏 𝑒 >1 within the first few hundred picoseconds. The magnetic field is sufficiently strong to modify plasma heat transport, and simulations with an artificially suppressed magnetic field show noticeably different temperature profiles.

Lezhnin, K. V. [Princeton Plasma Physics Laborator↗

Developing nonlinear laser-plasma instability models for high-fidelity, multi-physics simulation capability for ICF/HED (IC Report) [Slides]

Modeling nonlinear effects of laser plasma instabilities (LPI) is critically important for ICF/HED experiments. Our project has the following goals: • Develop physics-based nonlinear LPI models using PIC simulations • Couple the nonlinear LPI effects to macroscopic modeling of ICF/HED exp. through laser ray-tracing (LRT).

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Laser heating system at the Extreme Conditions Beamline, P02.2, $\mathrm{PETRA III}$

A laser heating system for samples confined in diamond anvil cells paired with in situ X-ray diffraction measurements at the Extreme Conditions Beamline of PETRA III is presented. The system features two independent laser configurations (on-axis and off-axis of the X-ray path) allowing for a broad range of experiments using different designs of diamond anvil cells. The power of the continuous laser source can be modulated for use in various pulsed laser heating or flash heating applications. An example of such an application is illustrated here on the melting curve of iron at megabar pressures. The optical path of the spectroradiometry measurements is simulated with ray-tracing methods in order to assess the level of present aberrations in the system and the results are compared with other systems, that are using simpler lens optics. Based on the ray-tracing the choice of the first achromatic lens and other aspects for accurate temperature measurements are evaluated.

47 OTHER INSTRUMENTATION↗

An imaging refractometer for density fluctuation measurements in high energy density plasmas

In this work, we report on a recently developed laser-probing diagnostic which allows direct measurements of ray-deflection angles in one axis, whilst retaining imaging capabilities in the other axis. This allows us to measure the spectrum of angular deflections from a laser beam which passes though a turbulent high-energy-density plasma. This spectrum contains information about the density fluctuations within the plasma, which deflect the probing laser over a range of angles. We create synthetic diagnostics using ray-tracing to compare this new diagnostic with standard shadowgraphy and schlieren imaging approaches, which demonstrates the enhanced sensitivity of this new diagnostic over standard techniques. We present experimental data from turbulence behind a reverse shock in a plasma and demonstrate that this technique can measure angular deflections between 0.06 and 34 mrad, corresponding to a dynamic range of over 500.

47 OTHER INSTRUMENTATION↗

Frequency-Selectable Laser Source (FLS) for Cosmic Microwave Background Experiments

Cosmic Microwave Background (CMB) experiments measure remnant radiation from the early universe and use that data to determine fundamental properties of the universe. We can constrain key parameters, such as \textit{r}, the cosmic tensor-to-scalar ratio, and $N_\text{eff}$, the effective number of relativistic species, by analyzing the CMB power spectra. Improving our measurements of the CMB requires improving our instrument systematics, one of the most important of which is detector bandpass. Current experiments use a Fourier Transform Spectrometer (FTS) to measure bandpass. However, the FTS is systematics limited, and cannot achieve the accuracy needed to make improved CMB measurements. For this reason, we are developing a new instrument, the Frequency-Selectable Laser Source (FLS) to decrease the uncertainty in bandpass by an order of magnitude. In this paper, we describe work completed to support the version 2 upgrade to the FLS. Using ray-tracing software, we modeled the FLS optics to set physical tolerances for the new design. We also discuss the laser calibration, and future work to be completed in further development of the FLS upgrade.

Rosen-Turits, Gabriel M.↗

Frequency-Selectable Laser Source for Cosmic Microwave Background Experiments

Cosmic Microwave Background (CMB) experiments measure remnant radiation from the early universe and use that data to determine fundamental properties of the universe. We can constrain key parameters, such as \textit{r}, the cosmic tensor-to-scalar ratio, and $N_\text{eff}$, the effective number of relativistic species, by analyzing the CMB power spectra. Improving our measurements of the CMB requires improving our instrument systematics, one of the most important of which is detector bandpass. Current experiments use a Fourier Transform Spectrometer (FTS) to measure bandpass. However, the FTS is systematics limited, and cannot achieve the accuracy needed to make improved CMB measurements. For this reason, we are developing a new instrument, the Frequency-Selectable Laser Source (FLS) to decrease the uncertainty in bandpass by an order of magnitude. In this paper, we describe work completed to support the version 2 upgrade to the FLS. Using ray-tracing software, we modeled the FLS optics to set physical tolerances for the new design. We also discuss the laser calibration, and future work to be completed in further development of the FLS upgrade.

Rosen-Turits, Gabriel M. [Fermilab]↗

Geometric optics model of Thomson scattering enhanced by parametric coupling

We formulate a theory of Thomson scattering (TS) from inhomogeneous plasmas using a ray-tracing approach. The scattered radiation is described within the eikonal approximation, including convective gain arising from scattering instabilities driven by the TS probe laser. In the limit of a weak probe and vanishing gain, the theory recovers the standard TS cross section and scattered power due to volumetric particle noise. The ray-tracing formalism is implemented in a TS fitting framework, enabling accurate analysis of inhomogeneous plasmas whose background profiles can be provided by large-scale hydrodynamic simulations or experimental diagnostics. Here, several examples of synthetic TS spectra are presented, and further extensions of the theory are discussed.

Carleton, D. E. [University of Alberta, Edmonton, ↗

Simulations of Radiation Hydrodynamics in Strongly Coupled Plasmas (Final Report)

Radiation propagates throughout the Universe and is often the only information we have from distant astronomical objects. Additionally, radiation plays a key role in systems ranging from the interior of stars to the establishment of shocks at the edges of forming galaxies to neutron star mergers. Here radiative processes, absorption, emission, and scattering, are fundamental to transport of momentum and energy, as well as, the overall evolution of these and other astrophysical systems. In some cases, radiation-dominant systems are also sufficiently dense and ionized, such that, the ions are strongly coupled (ie electrostatic energy >> thermal energy or Γ >> 1), which will affect radiative processes and the transport of radiation. During this project, we developed a computational ray-tracing algorithm to study radiation transport through a simulated neutron star capsule implosion under conditions relevant to Omega-60 laser experiments.

79 ASTRONOMY AND ASTROPHYSICS↗

Accurate and efficient predictions of keyhole dynamics in laser materials processing using machine learning-aided simulations

The keyhole phenomenon has been widely observed in laser materials processing, including laser welding, remelting, cladding, drilling, and additive manufacturing. Keyhole-induced defects, primarily pores, dramatically affect the performance of final products, impeding the broad use of these laser-based technologies. The formation of these pores is typically associated with the dynamic behavior of the keyhole. So far, the accurate characterization and prediction of keyhole features, particularly keyhole depth, as a function of time, has been a challenging task. In situ characterization of keyhole dynamic behavior using the synchrotron X-ray technique is informative but complicated and expensive. Current simulations are generally hindered by their poor accuracy and generalization abilities in predicting keyhole depths due to the lack of accurate laser absorptance data. In this study, we develop a machine learning-aided simulation method that accurately predicts keyhole dynamics, especially in keyhole depth fluctuations, over a wide range of processing parameters. In two case studies involving titanium and aluminum alloys, we achieve keyhole depth prediction with a mean absolute percentage error of 10 %, surpassing those simulated using the ray-tracing method with an error margin of 30 %, while also reducing computational time. This exceptional fidelity and efficiency empower our model to serve as a cost-effective alternative to synchrotron experiments. Our machine learning-aided simulation method is affordable and readily deployable for a large variety of materials, opening new doors to eliminate or reduce defects for a wide range of laser materials processing techniques.

Computational fluid dynamics↗

Absolute calibration of the conical crystal configuration of the zinc spectrometer (ZSPEC) at the OMEGA laser facility

In this study, we present the absolute calibration of the conical crystal for the zinc spectrometer (ZSPEC), an x-ray spectrometer at the OMEGA laser facility at the Laboratory for Laser Energetics. The ZSPEC was originally designed to measure x-ray Thomson scattering using flat or cylindrically curved highly oriented pyrolytic graphite crystals centered around Zn He-alpha emission at 9 keV. To improve the useful spectral range and collection efficiency of the ZSPEC, a conical highly annealed pyrolytic graphite crystal was fabricated for the ZSPEC. The conically bent crystal in the Hall geometry produces a line focus perpendicular to the spectrometer axis, corresponding to the detector plane of electronic detectors at large scale laser facilities such as OMEGA, extending the useful range of the spectrometer to 7–11 keV. Further, using data collected using a microfocus Mo x-ray source, we determine important characteristics of ZSPEC such as the dispersion, spatial resolution, and absolute sensitivity of the instrument. A ray-trace model of ZSPEC provides another point of agreement in calculations of the ZSPEC dispersion and crystal response.

47 OTHER INSTRUMENTATION↗

Design of a Multi-Monochromatic X-ray Imager (MMI) for Kr K-shell line emission

We report the Multi-Monochromatic X-ray Imager (MMI) is a time-gated spectrometer used in implosion experiments at the OMEGA laser facility. From the data, electron temperature and density spatial distributions can be obtained at different implosion times. Previous MMI designs used Ar K-shell emission (3–6 keV) as a spectroscopic tracer and provided a spectral resolution of around 20 eV. However, Ar K-shell line emission becomes less useful at electron temperatures above 2 keV due to over-ionization. Kr K-shell (12–16 keV) has been shown to be an attractive alternative to diagnose hot implosion cores in recent publications. The purpose of this paper is to show a new point design that allows the MMI to detect this higher photon energy range with suitable spectral resolution. The algorithm used to find the optimal design couples a ray-tracing code and an exhaustive parameter space search. This algorithm may be useful as a tool to find optimal MMI designs for other purposes, i.e., other spectral regions for other spectroscopic tracers. So, the main change between the two designs is the replacement of the multi-layer mirror with a flat Bragg Ge (220) crystal. The final Kr K-shell MMI design has a photon energy range from 12 to 16.1 keV.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Implementation of compound refractive lenses for large field-of-view x-ray phase-contrast imaging during hypervelocity impact experiments

Synchrotron x-ray phase-contrast imaging (XPCI) offers time-resolved visualization of dynamic compression phenomena, but its intrinsically small field-of-view (FOV) limits the time that key features remain in frame. A novel approach to enlarge the FOV is achieved by positioning a two-dimensional parabolic compound refractive lens (CRL) upstream of the sample to deliberately defocus the white beam. Ray-tracing simulations and XPCI measurements show that this CRL configuration can expand the beam by ∼50% vertically and ∼15% horizontally based on the full width at half-maximum of the beam. Implementing the CRL, however, attenuates the photon flux and lowers signal-to-noise ratio (SNR). Task-based analysis using a calibration grid (30 μm dots) showed that both setups fail to consistently meet the Rose criterion (SNR ≥ 5) for features of this size in single-bunch imaging. Extrapolating the measured SNR Rose values suggests that the minimum consistently detectable feature lies closer to 30–40 μm for the standard XPCI setup and above 40 μm for CRL-XPCI. Despite this limitation, the CRL configuration nearly doubles the illuminated area, enabling simultaneous tracking of front and rear observations of boron carbide targets subjected to rod and sphere impacts at 1.0–2.6 km/s. Image tracking algorithms and photonic Doppler velocimetry were used to measure penetration and rear-surface velocity histories. Together, these measurements capture crack fronts, penetration, and material breakout, offering new benchmark data for validating high-strain-rate constitutive models of ceramic materials.

Ceramic materials↗

Towards performing high-resolution inelastic X-ray scattering measurements at hard X-ray free-electron lasers coupled with energetic laser drivers

High-resolution inelastic X-ray scattering is an established technique in the synchrotron community, used to investigate collective low-frequency responses of materials. When fielded at hard X-ray free-electron lasers (XFELs) and combined with high-intensity laser drivers, it becomes a promising technique for investigating matter at high temperatures and high pressures. This technique gives access to important thermodynamic properties of matter at extreme conditions, such as temperature, material sound speed, and viscosity. The successful realization of this method requires the acquisition of many identical laser-pump/X-ray-probe shots, allowing the collection of a sufficient number of photons necessary to perform quantitative analyses. Here, a 2.5-fold improvement in the energy resolution of the instrument relative to previous works at the Matter in Extreme Conditions (MEC) endstation, Linac Coherent Light Source (LCLS), and the High Energy Density (HED) instrument, European XFEL, is presented. Some aspects of the experimental design that are essential for improving the number of photons detected in each X-ray shot, making such measurements feasible, are discussed. A careful choice of the energy resolution, the X-ray beam mode provided by the XFEL, and the position of the analysers used in such experiments can provide a more than ten-fold improvement in the photometrics. The discussion is supported by experimental data on 10 µm-thick iron and 50 nm-thick gold samples collected at the MEC endstation at the LCLS, and by complementary ray-tracing simulations coupled with thermal diffuse scattering calculations.

36 MATERIALS SCIENCE↗