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Nuclear Data Sheets for A = 209

The experimental data are evaluated for known nuclides of mass number A = 209 (Au,Hg,Tl,Pb,Bi,Po,At,Rn, Fr,Ra,Ac,Th). Detailed evaluated level properties and related nuclear structure information are presented, with the best values recommended for level energies, half-lives, γ–ray energies and intensities, decay data (energies, intensities and placement of radiations), and other spectroscopic data. This work supersedes the earlier full evaluation of A = 209 by M.J. Martin (1991Ma16)

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Measurements of neutron capture cross section for {sup 207,208}Pb

The neutron capture cross sections for {sup 207,208}Pb have been measured in the neutron energy region from 10 to 110 keV. The γ-rays cascaded from a capture state to the ground state or low-lying states of {sup 208,209}Pb were observed for the first time, using an anti-Compton Nal(Tl) spectrometer and a TOF method. The observed discrete γ-ray energy spectra enabled us to determine neutron capture cross sections for {sup 207,208}Pb with small systematic errors, since we could distinguish γ-ray of {sup 207,208}Pb(n,γ) reactions from background γ-ray with use of the γ-ray spectra. The obtained cross sections include both contributions of resonance and direct capture components different from the previous TOF measurements.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Quasi elastic cross sections for the Bi-209(e, e-prime p) Pb-208 reaction: Jefferson Lab experiment E06007

Quasi elastic cross sections were measured for the first time for both negative and positive missing momenta for the {sup 209}Bi(e,e'p){sup 208}Pb reaction leading to the ground state and hole states of (208)Pb. Experimental cross sections obtained between -0.3 GeV/c to 0.3 GeV/c agree with theoretical calculations using RDWIA techniques both in shape and magnitude for the ground state. The data for the ground state production of {sup 208}Pb are consistent with a theoretical model assuming a single proton(1.06 +- 0.10) in the 1h9/2 orbit in {sup 209}Bi.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Data on photoneutron reactions from various experiments for {sup 133}Cs, {sup 138}Ba and {sup 209}Bi nuclei

Basic methods for determining cross sections for photoneutron partial reactions are examined. They are obtained directly in experiments with quasimonoeneregetic annihilation photons or from the cross section for the (γ, xn) = (γ, 1n) + 2(γ, 2n) + 3(γ, 3n) +... neutron-yield reaction in experiments with bremsstrahlung photons by introducing corrections based on statistical nuclear-reaction theory. The difference in the conditions of these experiments, which leads to discrepancies between their results because of sizable systematic errors, is analyzed. Physical criteria are used to study the reliability of data on the photodisintegration of {sup 133}Cs, {sup 138}Ba, and {sup 209}Bi nuclei. The cross sections for partial and total reactions satisfying the reliability criteria are evaluated within the experimental–theoretical method (σ{sup eval}(γ, in) = F{sub i}{sup theor} × σ{sup expt}(γ, xn)) on the basis of the experimental cross sections σ{sup expt}(γ, xn) and the results of the calculations within the combined model of photonuclear reactions.

74 ATOMIC AND MOLECULAR PHYSICS↗

Impacts of future nuclear power generation on the international monitoring system

Many countries are considering nuclear power as a means of reducing greenhouse gas emissions, and the IAEA (IAEA, 2022) has forecasted nuclear power growth rates up to 224% of the 2021 level by 2050. Nuclear power plants release trace quantities of radioxenon, an inert gas that is also monitored under international agreements as a signature of nuclear weapons tests. To better understand how nuclear energy growth (and resulting Xe emissions) could affect this global nonproliferation architecture, we modeled daily releases of radioxenon isotopes used for nuclear explosion detection in the International Monitoring System (IMS) that is part of the Comprehensive Nuclear Test-Ban Treaty: 131m Xe, 133 Xe, 133m Xe, and 135 Xe to examine the change in the number of radioxenon detections as compared to the 2021 detection levels. If a 40-station IMS network is used, the detections of 133 Xe in 2050 would range from 82% for the low-power scenario to 195% for the high-power scenario, compared to the detections in 2021. If an 80-station IMS network is used, the detections of 133 Xe in 2050 would range from 83% of the 2021 detection rate for the low-power scenario to 209% for the high-power scenario. Essentially no detections of 131m Xe and 133m Xe are expected. The high growth scenario could lead to a six-fold increase in 135 Xe detections, but the total number of detections is still small (on the order of 1 detection per day in the entire network).

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Modern status of photonuclear data

The reliability of experimental cross sections obtained for (γ, 1n), (γ, 2n), and (γ, 3n) partial photoneutron reactions using beams of quasimonoenergetic annihilation photons and bremsstrahlung is analyzed by employing data for a large number of medium-heavy and heavy nuclei, including those of {sup 63,65}Cu, {sup 80}Se, {sup 90,91,94}Zr, {sup 115}In, {sup 112−124}Sn, {sup 133}Cs, {sup 138}Ba, {sup 159}Tb, {sup 181}Ta, {sup 186−192}Os, {sup 197}Au, {sup 208}Pb, and {sup 209}Bi. The ratios of the cross sections of definite partial reactions to the cross section of the neutron-yield reaction, F{sub i} = σ(γ, in)/σ(γ, xn), are used as criteria of experimental-data reliability. By definition, positive values of these ratios should not exceed the upper limits of 1.00, 0.50, 0.33,... for i = 1, 2, 3,..., respectively. For many nuclei, unreliable values of the above ratios were found to correlate clearly in various photon-energy regions F{sub i} with physically forbidden negative values of cross sections of partial reactions. On this basis, one can conclude that correspondent experimental data are unreliable. Significant systematic uncertainties of the methods used to determine photoneutron multiplicity are shown to be the main reason for this. New partial-reaction cross sections that satisfy the above data-reliability criteria were evaluated within an experimental–theoretical method [σ{sup eval}(γ, in) = F{sub i}{sup theor} (γ, in) × σ{sup expt}(γ, xn)] by employing the ratios F{sub i}{sup theor} (γ, in) calculated on the basis of a combined photonuclear-reaction model. It was obtained that cross sections evaluated in this way deviate substantially from the results of many experiments performed via neutron-multiplicity sorting, but, at the same time, agree with the results of alternative activation experiments. Prospects of employing methods that would provide, without recourse to photoneutron-multiplicity sorting, reliable data on cross sections of partial photoneutron reactions are discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Excitations of one-valence-proton, one-valence-neutron nucleus {sup 210}Bi from cold-neutron capture

The low-spin structure of one-proton, one-neutron {sup 210}Bi nucleus was investigated in cold-neutron capture reaction on {sup 209}Bi. The γ-coincidence measurements were performed with use of EXILL array consisted of 16 HPGe detectors. The experimental results were compared to shell-model calculations involving valence particles excitations. The {sup 210}Bi nucleus offers the potential to test the effective proton-neutron interactions because most of the states should arise from the proton-neutron excitations. Additionally, it was discovered that a few states should come from the couplings of valence particles to the 3{sup −} octupole vibration in {sup 208}Pb which provides also the possibility of testing the calculations involving the core excitations.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

The occurrence and impact of carbon-oxygen shell mergers in massive stars

In their final stages before undergoing a core-collapse supernova, massive stars may experience mergers between internal shells where carbon (C) and oxygen (O) are consumed as fuels for nuclear burning. This interaction, known as a C-O shell merger, can dramatically alter the internal structure of the star, leading to peculiar nucleosynthesis and potentially influencing the supernova explosion and the propagation of the subsequent supernova shock. Our understanding of the frequency and consequences of C-O shell mergers remains limited. This study aims to identify, for the first time, early diagnostics in the stellar structure that lead to C-O shell mergers in more advanced stages. We also assess their role in shaping the chemical abundances in the most metal poor stars of the Galaxy. We analyzed a set of 209 stellar evolution models available in the literature, with different initial progenitor masses and metallicities. We then compared the nucleosynthetic yields from a subset of these models with the abundances of odd-Z elements in metal-poor stars. We find that the occurrence of C-O shell mergers in stellar models can be predicted with a good approximation based on the outcomes of the central He burning phase, specifically, from the CO core mass (M CO ) and the 12 C central mass fraction (X C12 ): 90% of models with a C-O merger have X C12 <0.277 and M CO <4.90 M ⊙ , with average values of M CO = 4.02 M ⊙ and X C12 = 0.176. The quantities X C12 and M CO are indirectly affected from several stellar properties, including the initial stellar mass and metallicity. Additionally, we confirm that the Sc-rich and K-rich yields from models with C-O mergers would solve the long-standing underproduction of these elements in massive stars. Our results emphasize the crucial role of C-O shell mergers in enriching the interstellar medium, particularly in the production of odd-Z elements. This highlights the necessity of further investigations to refine their influence on presupernova stellar properties and their broader impact on Galactic chemical evolution.

79 ASTRONOMY AND ASTROPHYSICS↗

SU-D-209-04: Raise Your Table: An Effective Way to Reduce Radiation Dose for Fluoroscopy

Purpose: Patient table height plays an important role in estimating patient skin dose for interventional radiology (IR) procedures, because the patient’s skin location is dependent on the height of table. Variation in table height can lead to as much as 150% difference in skin dose for patient exams with similar air kerma meter readings. In our facility, IR procedural workflow was recently changed to require the IR physicians to confirm the patient table height before the procedure. The patient table height data was collected before and after this workflow change to validate the implementation of this practice. Methods: Table height information was analyzed for all procedures performed in three IR rooms, which were impacted by the workflow change, covering three months before and after the change (Aug 2015 to Jan 2016). In total, 442, 425, and 390 procedures were performed in these three rooms over this time period. There were no personnel or procedure assignment changes during the six-month period of time. Statistical analysis was performed for the average table height changes before and after the workflow change. Results: For the three IR rooms investigated, after the workflow change, the average table heights were increased by 1.43 cm (p=0.004084), 0.66 cm (p=0.187089), and 1.59 cm (p=0.002193), providing a corresponding estimated skin dose savings of 6.76%, 2.94% and 7.62%, respectively. After the workflow change, the average table height was increased by 0.95 cm, 0.63 cm, 0.55 cm, 1.07 cm, 1.12 cm, and 3.36 cm for the six physicians who routinely work in these three rooms. Conclusion: Consistent improvement in table height settings has been observed for all IR rooms and all physicians following a simple workflow change. This change has led to significant patient dose savings by making physicians aware of the pre-procedure table position.

60 APPLIED LIFE SCIENCES↗

Relationships among DNA hypomethylation, Cd, and Pb exposure and risk of cigarette smoking-related urothelial carcinoma

Cigarette smoking and environmental exposure to heavy metals are important global health issues, especially for urothelial carcinoma (UC). However, the effects of cadmium and lead exposure, as well as the levels of DNA hypomethylation, on UC risk are limited. We evaluated the possible exposure sources of Cd and Pb and the relationship among DNA hypomethylation, urinary Cd and Pb levels, and UC risk. We recruited 209 patients with UC and 417 control patients for a hospital-based case–control study between June 2011 and August 2014. We collected environmental exposure-related information with questionnaires. Blood and urine samples were analyzed to measure the Cd and Pb exposure and 5-methyl-2′-deoxycytidine levels as a proxy for DNA methylation. Multivariate logistic regression and 95% confidence intervals were applied to estimate the risk for UC. Study participants with high Cd and Pb exposure in blood or urine had significantly increased risk of UC, especially among the smokers. After adjusting for age and gender, the possible connections of individual cumulative cigarette smoking or herb medicine exposure with the increased levels of Cd and Pb were observed in the controls. Participants with 8.66%–12.39% of DNA hypomethylation had significantly increased risk of UC compared with those with ≥ 12.39% of DNA hypomethylation. Environmental factors including cigarette smoking and herb medicine may contribute to the internal dose of heavy metals levels. Repeat measurements of heavy metals with different study design, detailed dietary information, and types of herb medicine should be recommended for exploring UC carcinogenesis in future studies. - Highlights: • Smoking and herb medicine ingestion is associated with increased urinary Cd and Pb levels. • Urinary levels of Cd and Pb are associated with increased risk of UC. • UC carcinogenesis might have partially resulted from DNA hypomethylation.

60 APPLIED LIFE SCIENCES↗

Transcriptome-wide association analysis identifies candidate susceptibility genes for prostate-specific antigen levels in men without prostate cancer

Deciphering the genetic basis of prostate-specific antigen (PSA) levels may improve their utility for prostate cancer (PCa) screening. Using genome-wide association study (GWAS) summary statistics from 95,768 PCa-free men, we conducted a transcriptome-wide association study (TWAS) to examine impacts of genetically predicted gene expression on PSA. Analyses identified 41 statistically significant (p < 0.05/12,192 = 4.10 × 10 –6 ) associations in whole blood and 39 statistically significant (p < 0.05/13,844 = 3.61 × 10 –6 ) associations in prostate tissue, with 18 genes associated in both tissues. Cross-tissue analyses identified 155 statistically significantly (p < 0.05/22,249 = 2.25 × 10 –6 ) genes. Out of 173 unique PSA-associated genes across analyses, we replicated 151 (87.3%) in a TWAS of 209,318 PCa-free individuals from the Million Veteran Program. Based on conditional analyses, we found 20 genes (11 single tissue, nine cross-tissue) that were associated with PSA levels in the discovery TWAS that were not attributable to a lead variant from a GWAS. Ten of these 20 genes replicated, and two of the replicated genes had colocalization probability of >0.5: CCNA2 and HIST1H2BN. Six of the 20 identified genes are not known to impact PCa risk. Fine-mapping based on whole blood and prostate tissue revealed five protein-coding genes with evidence of causal relationships with PSA levels. Of these five genes, four exhibited evidence of colocalization and one was conditionally independent of previous GWAS findings. These results yield hypotheses that should be further explored to improve understanding of genetic factors underlying PSA levels.

60 APPLIED LIFE SCIENCES↗

Discovery of atomic clock-like spin defects in simple oxides from first principles

Virtually noiseless due to the scarcity of spinful nuclei in the lattice, simple oxides hold promise as hosts of solid-state spin qubits. However, no suitable spin defect has yet been found in these systems. Using high-throughput first-principles calculations, we predict spin defects in calcium oxide with electronic properties remarkably similar to those of the NV center in diamond. These defects are charged complexes where a dopant atom — Sb, Bi, or I — occupies the volume vacated by adjacent cation and anion vacancies. The predicted zero phonon line shows that the Bi complex emits in the telecommunication range, and the computed many-body energy levels suggest a viable optical cycle required for qubit initialization. Notably, the high-spin nucleus of each dopant strongly couples to the electron spin, leading to many controllable quantum levels and the emergence of atomic clock-like transitions that are well protected from environmental noise. Specifically, the Hanh-echo coherence time increases beyond seconds at the clock-like transition in the defect with 209 Bi. Our results pave the way to designing quantum states with long coherence times in simple oxides, making them attractive platforms for quantum technologies.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Doxorubicin-Loaded 70–150 μm Microspheres for Liver-Dominant Metastatic Breast Cancer: Results and Outcomes of a Pilot Study

PurposePatients with breast cancer liver metastasis have a poor prognosis. Local therapy for liver metastasis increases survival. The purpose of this pilot prospective study was to evaluate the efficacy and safety of doxorubicin drug-eluting beads chemoembolization for liver-dominant breast cancer metastasis (LdBM) refractory to chemotherapy.Materials and MethodsAll patients with LdBM refractory to of two or more lines of systemic chemotherapy were screened. Two chemoembolizations at 1-month intervals were scheduled for each patient. Tumor responses were evaluated by MRI every 3 months until progression or death. Adverse events were recorded according to the Common Terminology Criteria for Adverse Events (CTCAE version 4.02) 1 month after each chemoembolization. All patients were free from systemic treatment until progression. Patients with hormone-positive receptors and/or HER-positive disease status continued their targeted therapy.ResultsOut of 23 patients enrolled (mean age: 57.5 ± 11.5 years), 17 completed two chemoembolizations and six underwent only one because of severe adverse events. At 3-month follow-up, the disease control rate was 83 %. The median progression-free survival from the first chemoembolization was 8 months, and the median overall survival was 17 months. Nineteen patients remained free from any systemic chemotherapy for a mean of 209 ± 92 days until progression. Eight grade 3 (asthenia n = 3, anemia n = 2, thrombocythemia n = 2, liver toxicity n = 1) (Rev 1 Comment 1) occurred after the first procedure. No patient died directly due to the procedure.ConclusionWhile chemoembolization with doxorubicin eluding beads for refractory LdBM leads to an 83 % disease control rate, it also causes severe side effects that need to be adequately managed.

62 RADIOLOGY AND NUCLEAR MEDICINE↗

Photon induced Schottky barrier effects in inverse-extraordinary optoconductance structures

We expand upon our previous work and characterize the photo-dependence of the effective Schottky barrier in EOC and I-EOC heterostructures by measuring the open circuit voltage and the change in the reverse bias resistance. Under full illumination by a 5 mW, 632.8 nm HeNe laser, the barrier is effectively eliminated and the Ti-GaAs interface becomes Ohmic. The reverse bias resistance changes by a factor of 209 over an illumination intensity change of 10–5:1. While this work illustrates the behavior of the Schottky interface upon illumination, it also demonstrates the effectiveness of the four-point, van der Pauw measurement fundamental to EOC/I-EOC phenomena at monitoring changes in the active region of the mesa. The resistance is largely unaffected by the photovoltaic, DC offset of the surrounding leads, as indicated by the radial symmetry of 2-D resistance maps obtained by rastering the laser across EOC/IEOC devices.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

The Role of Recti ed Currents in Far-Field RF Sheaths and in SOL Losses of HHFW Power on NSTX

Radio-frequency (RF) rectification is an important sheath phenomenon for wave heating of plasma in fusion devices and is proposed to be the mechanism responsible for converting highharmonic fast-wave (HHFW) power in the National Spherical Torus eXperiment (NSTX) into a heat ux to the divertor. RF rectification has two aspects: current rectification and voltage recti- fication, and, while the latter is emphasized in many application, we demonstrate the importance of current rectification in analysis of the NSTX divertor during HHFW heating. When rectified currents are accounted for in first-principle models for the heat ux to the tiles, we predict a sizeable enhancement for the heat ux in the presence of an RF field: for one case studied, the predicted heat ux increases from 0:103 MW=m2 to 0:209 MW=m2. We also demonstrate how this rectification scales with injected HHFW power by tracking probe characteristics during a HHFW power ramp; the rectified current may be clamped at a certain level. This work is important for minimizing SOL losses of HHFW power in NSTX-U but may also have implications for near-field studies of ICRF antennae: ignoring rectified current may lead to underestimated heat uxes and overestimated rectified voltages.

ICRF HHFW RF rectification Sheaths Divertor↗

Effect of implanted species on thermal evolution of ion-induced defects in ZnO

Implanted atoms can affect the evolution of ion-induced defects in radiation hard materials exhibiting a high dynamic annealing and these processes are poorly understood. Here, we study the thermal evolution of structural defects in wurtzite ZnO samples implanted at room temperature with a wide range of ion species (from {sup 11}B to {sup 209}Bi) to ion doses up to 2 × 10{sup 16} cm{sup −2}. The structural disorder was characterized by a combination of Rutherford backscattering spectrometry, nuclear reaction analysis, and transmission electron microscopy, while secondary ion mass spectrometry was used to monitor the behavior of both the implanted elements and residual impurities, such as Li. The results show that the damage formation and its thermal evolution strongly depend on the ion species. In particular, for F implanted samples, a strong out-diffusion of the implanted ions results in an efficient crystal recovery already at 600 °C, while co-implantation with B (via BF{sub 2}) ions suppresses both the F out-diffusion and the lattice recovery at such low temperatures. The damage produced by heavy ions (such as Cd, Au, and Bi) exhibits a two-stage annealing behavior where efficient removal of point defects and small defect clusters occurs at temperatures ∼500 °C, while the second stage is characterized by a gradual and partial annealing of extended defects. These defects can persist even after treatment at 900 °C. In contrast, the defects produced by light and medium mass ions (O, B, and Zn) exhibit a more gradual annealing with increasing temperature without distinct stages. In addition, effects of the implanted species may lead to a nontrivial defect evolution during the annealing, with N, Ag, and Er as prime examples. In general, the obtained results are interpreted in terms of formation of different dopant-defect complexes and their thermal stability.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

TU-D-209-07: Monte Carlo Assessment of Dose to the Lens of the Eye of Radiologist Using Realistic Phantoms and Eyeglass Models

Purpose: To study how eyeglass design features and postures of the interventional radiologist affect the radiation dose to the lens of the eye. Methods: A mesh-based deformable phantom, consisting of an ultra-fine eye model, was used to simulate postures of a radiologist in fluoroscopically guided interventional procedure (facing the patient, 45 degree to the left, and 45 degree to the right). Various eyewear design features were studied, including the shape, lead-equivalent thickness, and separation from the face. The MCNPX Monte Carlo code was used to simulate the X-ray source used for the transcatheter arterial chemoembolization procedure (The X-ray tube is located 35 cm from the ground, emitting X-rays toward to the ceiling; Field size is 40cm X 40cm; X-ray tube voltage is 90 kVp). Experiments were also performed using dosimeter placed on a physical phantom behind eyeglasses. Results: Without protective eyewear, the radiologist’s eye lens can receive an annual dose equivalent of about 80 mSv. When wearing a pair of lead eyeglasses with lead-equivalent of 0.5-mm Pb, the annual dose equivalent of the eye lens is reduced to 31.47 mSv, but both exceed the new ICRP limit of 20 mSv. A face shield with a lead-equivalent of 0.125-mm Pb in the shape of a semi-cylinder (13cm in radius and 20-cm in height) would further reduce the exposure to the lens of the eye. Examination of postures and eyeglass features reveal surprising information, including that the glass-to-eye separation also plays an important role in the dose to the eye lens from scattered X-ray from underneath and the side. Results are in general agreement with measurements. Conclusion: There is an urgent need to further understand the relationship between the radiation environment and the radiologist’s eyewear and posture in order to provide necessary protection to the interventional radiologists under newly reduced dose limits.

60 APPLIED LIFE SCIENCES↗

SU-E-T-209: Independent Dose Calculation in FFF Modulated Fields with Pencil Beam Kernels Obtained by Deconvolution

Purpose: To obtain the pencil beam kernels that characterize a megavoltage photon beam generated in a FFF linac by experimental measurements, and to apply them for dose calculation in modulated fields. Methods: Several Kodak EDR2 radiographic films were irradiated with a 10 MV FFF photon beam from a Varian True Beam (Varian Medical Systems, Palo Alto, CA) linac, at the depths of 5, 10, 15, and 20cm in polystyrene (RW3 water equivalent phantom, PTW Freiburg, Germany). The irradiation field was a 50 mm diameter circular field, collimated with a lead block. Measured dose leads to the kernel characterization, assuming that the energy fluence exiting the linac head and further collimated is originated on a point source. The three-dimensional kernel was obtained by deconvolution at each depth using the Hankel transform. A correction on the low dose part of the kernel was performed to reproduce accurately the experimental output factors. The kernels were used to calculate modulated dose distributions in six modulated fields and compared through the gamma index to their absolute dose measured by film in the RW3 phantom. Results: The resulting kernels properly characterize the global beam penumbra. The output factor-based correction was carried out adding the amount of signal necessary to reproduce the experimental output factor in steps of 2mm, starting at a radius of 4mm. There the kernel signal was in all cases below 10% of its maximum value. With this correction, the number of points that pass the gamma index criteria (3%, 3mm) in the modulated fields for all cases are at least 99.6% of the total number of points. Conclusion: A system for independent dose calculations in modulated fields from FFF beams has been developed. Pencil beam kernels were obtained and their ability to accurately calculate dose in homogeneous media was demonstrated.

07 ISOTOPE AND RADIATION SOURCES↗