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Results for “INTERNAL CONVERSION COEFFICIENT”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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13 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Fine structure in the α decay of $^{179}$Hg and $^{177}$Au

Abstract The$$\upalpha $$ α -decay fine structure of$$^{179}$$ 179 Hg and$$^{177}$$ 177 Au was studied by means of decay spectroscopy. Two experiments were performed at the Accelerator Laboratory of the University of Jyväskylä (JYFL), Finland, utilizing the recoil separator RITU and a digital data acquisition system. The heavy-ion induced fusion-evaporation reactions$$^{82}_{36}$$ 36 82 Kr + $$^{100}_{44}$$ 44 100 Ru and$$^{88}_{38}$$ 38 88 Kr + $$^{92}_{42}$$ 42 92 Mo were used to produce the$$^{179}$$ 179 Hg and$$^{177}$$ 177 Au nuclei, respectively. Studying the evaporation residues (ER, recoils)-$$\alpha _1$$ α 1 -$$\alpha _2$$ α 2 correlations and$$\upalpha $$ α -$$\gamma $$ γ coincidences, a new$$\upalpha $$ α decay with E$$_\alpha $$ α = 6156(10) keV was observed from$$^{179}$$ 179 Hg. This decay populates the (9/2$$^-$$ - ) excited state at an excitation energy of 131.3(5) keV in$$^{175}$$ 175 Pt. The internal conversion coefficient for the 131.3(5) keV transition de-exciting this state was measured for the first time. Regarding the$$^{177}$$ 177 Au nucleus, a new$$\upalpha $$ α decay with E$$_\alpha $$ α = 5998(9) keV was observed to populate the 156.1(6) keV excited state in$$^{173}$$ 173 Ir. Two de-excitation paths were observed from this excited state. Moreover, a new 215.7(13) keV transition was observed to depopulate the 424.4(13) keV excited state in$$^{173}$$ 173 Ir. Properties of the$$^{179}$$ 179 Hg and$$^{177}$$ 177 Au$$\upalpha $$ α decays were examined in a framework of reduced widths and hindrance factors. For clarity and simplicity, the spin and parity assignments (e.g.$$J^{\pi }$$ J π ) are presented without brackets throughout the text.

Physics↗
NASA NTRS2007

Transient Numerical Modeling of Catalytic Channels

This paper presents a transient model of catalytic combustion suitable for isolated channels and monolith reactors. The model is a lumped two-phase (gas and solid) model where the gas phase is quasi-steady relative to the transient solid. Axial diffusion is neglected in the gas phase; lateral diffusion, however, is accounted for using transfer coefficients. The solid phase includes axial heat conduction and external heat loss due to convection and radiation. The combustion process utilizes detailed gas and surface reaction models. The gas-phase model becomes a system of stiff ordinary differential equations while the solid phase reduces, after discretization, into a system of stiff ordinary differential-algebraic equations. The time evolution of the system came from alternating integrations of the quasi-steady gas and transient solid. This work outlines the numerical model and presents some sensitivity studies on important parameters including internal transfer coefficients, catalytic surface site density, and external heat-loss (if applicable). The model is compared to two experiments using CO fuel: (1) steady-state conversion through an isothermal platinum (Pt) tube and (2) transient propagation of a catalytic reaction inside a small Pt tube. The model requires internal mass-transfer resistance to match the experiments at lower residence times. Under mass-transport limited conditions, the model reasonably predicted exit conversion using global mass-transfer coefficients. Near light-off, the model results did not match the experiment precisely even after adjustment of mass-transfer coefficients. Agreement improved for the first case after adjusting the surface kinetics such that the net rate of CO adsorption increased compared to O2. The CO / O2 surface mechanism came from a sub-set of reactions in a popular CH4 / O2 mechanism. For the second case, predictions improved for lean conditions with increased external heat loss or adjustment of the kinetics as in the first case. Finally, the results show that different initial surface-species distribution leads to different steady-states under certain conditions. These results demonstrate the utility of a lumped two-phase model of a transient catalytic combustor with detailed chemistry.

Struk, Peter M.↗
NASA NTRS1998

Prelaunch Calibrations of the Clouds and the Earth's Radiant Energy System (CERES) Tropical Rainfall Measuring Mission and Earth Observing System Morning (EOS-AM1) Spacecraft Thermistor Bolometer Sensors

The Clouds and the Earth's Radiant Energy System (CERES) spacecraft scanning thermistor bolometer sensors measure earth radiances in the broadband shortwave solar (O.3 - 5.0 micron and total (0.3 to 100 microns) spectral bands as well as in the 8-12 microns water vapor window spectral band. On November 27, 1997, the launch of the Tropical Rainfall Measuring Mission (TRMM) spacecraft placed the first set of CERES sensors into orbit, and 30 days later, the sensors initiated operational measurements of the earth radiance fields. In 1998, the Earth Observing System morning (EOS-AM1) spacecraft will place the second and third sensor sets into orbit. The prelaunch CERES sensors' count conversion coefficients (gains and zero-radiance offsets) were determined in vacuum ground facilities. The gains were tied radiometrically to the International Temperature Scale of 1990 (ITS-90). The gain determinations included the spectral properties (reflectance, transmittance, emittance, etc.) of both the sources and sensors as well as the in-field-of-view (FOV) and out-of-FOV sensor responses. The resulting prelaunch coefficients for the TRMM and EOS-AM1 sensors are presented. Inflight calibration systems and on-orbit calibration approaches are described, which are being used to determine the temporal stabilities of the sensors' gains and offsets from prelaunch calibrations through on-orbit measurements. Analyses of the TRMM prelaunch and on-orbit calibration results indicate that the sensors have retained their ties to ITS-90 at accuracy levels better than /- 0.3% between the 1995 prelaunch and 1997 on-orbit calibrations.

Lee, Robert B., III↗
DOE OSTI2024

Transfer functions for Q A /Q B international regulatory limits for the safe transport of radioactive materials

This paper presents a proposed revision of the International Atomic Energy Agency transport regulations, related to the A 1 and A 2 limit values used to determine the radioactive transport classification. Based on the 'Q system', a novel methodology was introduced to derive Q A and Q B values related to scenarios involving external exposure from a distant source. These values are key parameters that respectively represent the total effective dose and total equivalent dose to the skin, from all primary and secondary particles contributing to radiation exposure. The International Working Group (WG A 1 /A 2 ) is established and associated with the TRANSSC Technical Expert Group on Radiation Protection. A review of the A 1 and A 2 values is performed in response to identified limitations within the existing Q system. The followed approach is based on Monte Carlo simulations that enabled the development of transfer functions aimed at reducing computational time and increasing the flexibility of dose evaluations for any radionuclide with known particle emission spectra. This method allows updating the Q A and Q B values to account for future data evolutions (decay data, fluence-to-dose conversion coefficients) and standardizing the calculation of regulation limits across all referenced radionuclides and scenarios related to external exposure. The transfer functions are established using three Monte Carlo simulation codes—FLUKA, Geant4, and MCNP—and address the previous limitations of the 'Q system', reflecting the latest International Commission for Radiation Protection recommendations and improvements in calculation techniques. The results of the WG show consistent agreement across the codes, with minor discrepancies observed at low primary energies due to statistical uncertainties and different handling of stopping power for electrons/positrons in the codes. This revised approach aligns with current standards and recommendations, ensuring that the radiological consequences of transport accidents are acceptable for the new A 1 and A 2 limits from a radiological protection perspective.

61 RADIATION PROTECTION AND DOSIMETRY↗
NASA NTRS1994

Dynamics and efficiency of type III solar radio emission

Existing calculations of nonlinear coupling coefficients for fundamental and harmonic emission via three-wave interactions are refined and used to calculate the conversion efficiency of Langmuir energy into electromagnetic waves when the Langmuir waves have the observed bursty form. Resulting field strengths for harmonic emission are found to be consistent with typical International Sun Earth Explorer 3 (ISSE 3) observations at 1 AU. Fundamental emission at 1 AU is found to proceed only when stimulated by the presence of a source of ion sound waves. However, it is argued that electrostatic decay of Langmuir waves can supply the necessary waves provided the driving electron beam is sufficiently fast. Under these conditions, the predicted fundamental field strengths can account for both the highest and typical fields observed; they also dominate the predicted harmonic fields, consistent with observations. This mechanism is also consistent with previous observations that fundamental emission generally occurs early in type III events, when the beam is fastest. For typical parameters it is shown that neither fundamental nor harmonic emission saturates its respective source instability, contrary to previous assumptions. However, saturation cannot be ruled out under particularly favorable conditions.

Robinson, P. A.↗
DOE OSTI2024

Why Perovskite Thermal Stress is Unaffected by Thin Contact Layers

Metal halide perovskite photovoltaics have emerged as a high efficiency, low-cost alternative that can potentially rival or enhance conventional silicon technology. Despite exceptional initial power conversion efficiencies, achieving compliance with international standards and widespread adoption requires further enhancements to their operational stability. Notably, addressing mechanical strain and stress in brittle perovskites has emerged as a pivotal approach to mitigate chemical degradation and improve reliability during thermal cycling. Here, in this study, a popularized strain engineering strategy is investigated in which a high coefficient of thermal expansion (CTE) hole transport layer (i.e., PDCBT) is cast onto inorganic perovskite (CsPbI 2 Br) at 100 °C. Contrary to previously published results, the X-ray diffraction (XRD):Sin 2 ψ and substrate curvature measurement techniques show that the hole transport layer has no discernible impact on perovskite strain. The accuracy of the XRD:Sin 2 ψ method for measuring strain is highlighted in contrast to an analysis based on shifts of single XRD peaks which can be influenced by multiple artifacts. The findings in this study are in accordance with mechanics theory: thin layers are unable to induce significant strain changes in perovskite thin films as the force they apply is negligible compared to that applied by a thick and stiff substrate.

14 SOLAR ENERGY↗
DOE OSTI2024

Evaluation of Dose Coefficients Implemented in MACCS

A variety of dose conversion factor files (DCF files) have been supplied for use with the MACCS code since it was initially released. For MACCS 4.2, the MACCS DCF files have been updated to include coefficients used in the computation of acute skin doses from within the MACCS software to increase functionality and to add a pseudo-organ to represent the total effective dose equivalent (TEDE) (as defined in 10 CFR 20.1003) based on International Commission on Radiological Protection (ICRP) Publication 30. This report provides a description of how these changes have been implemented and a summary of the various DCF files supplied with MACCS 4.2. The report also provides supplemental discussions to assist the reader in understanding the technical basis for the MACCS DCFs. These supplemental discussions include a summary of basic dosimetry modeling concepts and a brief review of the Federal Guidance Reports (FGRs) upon which MACCS dose coefficients have historically been based.

97 MATHEMATICS AND COMPUTING↗
NASA NTRS1981

High power densities from high-temperature material interactions

Thermionic energy conversion (TEC) and metallic-fluid heat pipes (MFHPs), offering unique advantages in terrestrial and space energy processing by virtue of operating on working-fluid vaporization/condensation cycles that accept great thermal power densities at high temperatures, share complex materials problems. Simplified equations are presented that verify and solve such problems, suggesting the possibility of cost-effective applications in the near term for TEC and MFHP devices. Among the problems discussed are: the limitation of alkali-metal corrosion, protection against hot external gases, external and internal vaporization, interfacial reactions and diffusion, expansion coefficient matching, and creep deformation.

Morris, J. F.↗
NASA NTRS1977

An automated consultant for MACSYMA

A consultant is necessary whenever on is faced with a problem solving situation in a domain one does not fully understand. The lack of knowledge may be incidental, as it is when the domain or device is fairly simple but time constraints make it impossible for the user to learn all that is necessary. Computer systems like MACSYMA in which the level of commands is so close to the level of the task environment that the user is apt to confuse a simply defined procedure (like COEFF) with its mathematical counterpart (here coefficient) that it at best approximates. A computer program is described which has the capability of conversing with its user in English about a difficulty he has encountered, and providing information tailored to his need. The MACSYMA Advisor is a program distinct from MACSYMA with its own separate data base and expertise. For convenience the program can be called directly from MACSYMA and can access the user's data structures contained therein. The Advisor described here deals only with the "straightline" or nested use of MACSYMA commands and not loops or user-defined functions. The implementation of the Advisor relies heavily on an explict, internal "model" of the user's state of knowledge, his goals, and his "plan" for achieving them.

Genesereth, M. R.↗
NASA NTRS2022

Experimental Heat Transfer Results and Flow Visualization of Vertical Upflow Boiling in Earth Gravity with Subcooled Inlet Conditions – In Preparation for Experiments Onboard the International Space Station

Since 2012, researchers at the Purdue University Boiling and Two-Phase Flow Laboratory (PU-BTPFL) and NASA Glenn Research Center have been collaborating on a long-term effort to study flow boiling and condensation in microgravity. The ultimate goal has been to develop the Flow Boiling and Condensation Experiment (FBCE) for the International Space Station (ISS). Based on the findings from prior flow boiling experiments both at different orientations in Earth gravity and onboard parabolic flights simulating short durations of microgravity, a final refined experiment design, construction, and operating procedure have been arrived at for long-duration microgravity flow boiling experiments onboard the ISS. This study investigates flow boiling of n-Perfluorohexane with subcooled inlet in a rectangular channel of dimensions 114.6 mm heated length, 2.5 mm width, and 5 mm height. These pre-launch experiments (Mission Sequence Testing) were conducted in vertical upflow orientation in Earth gravity using the same experimental rig that was launched to the ISS in August 2021. The various operating parameters varied are heating configuration (single- and double-sided), mass velocity (180 – 3200 kg/m2s), inlet subcooling (+0 – 32°C, encompassing both highly subcooled and near-saturated inlet conditions), and inlet pressure (119 – 191 kPa). High-speed video flow visualization images are presented to explain the two-phase interfacial physics within the channel’s heated section. Heat transfer results in terms of flow boiling curves, streamwise profiles of wall temperature and heat transfer coefficient, and averaged heat transfer coefficients are analyzed and parametric effects elucidated. Severe temporal thermodynamic equilibrium is observed for near-saturated inlet at very low velocities. Nucleate boiling degradation starts at larger heat fluxes for single-sided heating than double sided at low mass velocities with highly subcooled inlet, and conversely at high mass velocities with near-saturated inlet. Nucleate boiling degradation can be delayed to higher heat fluxes by highly subcooling the inlet and increasing mass velocity. The entire local heat transfer coefficient profiles are degraded at higher heat fluxes for near-saturated inlet, but only the downstream part for highly subcooled inlet. This study also confirmed reliability of the upcoming ISS experimental data for subcooled inlet conditions and the collected Earth-gravity data will be used for comparison against the ISS data.

flow boiling↗