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Design of a High-Assay Low-Enriched Uranium Tri-Structural Isotropic Critical Experiment for Advanced Reactor Validation

High-assay low-enriched uranium (HALEU) fuel is a key component of many small modular reactor designs. Critical experiments are an important way to understand the neutronic performance of systems by obtaining nuclear data validations through measurements. Data reduce uncertainty and risk by showing that systems respond as predicted to changes such as temperature, subsequently advancing the overall technology readiness level of the materials within. Numerous critical experiments have been performed at the National Criticality Experiments Research Center (NCERC) operated by Los Alamos National Laboratory at the Nevada National Security Site since it became operational in 2011. However, the first experiment with HALEU fuel did not occur until 2024. Through extensive engineering, the experiment described in this paper was successfully designed and executed for the Comet vertical lift assembly at NCERC to perform measurements with HALEU tri-structural isotropic fuel that will assist in validation of nuclear data and computational modeling of small modular reactors for years to come.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS

Depletion benchmark for a high-assay low-enriched uranium fuel experiment in the advanced test reactor

Reactor physics depletion benchmarks for high-assay low-enriched uranium (HALEU) fuel are limited in number. In particular, there is limited data for HALEU benchmarks for U-10Mo (uranium-10% molybdenum) plate fuel that is being developed for use in the United States’ high performance research reactors including the Advanced Test Reactor (ATR), Advanced Test Reactor Critical Facility (ATR-C), High Flux Isotope Reactor (HFIR), Massachusetts Institute of Technology Reactor (MITR), University of Missouri Research Reactor (MURR), National Bureau of Standards Reactor (NBSR). These six reactors currently operate with highly enriched uranium dispersed fuel in an aluminum matrix. In support of conversion to a HALEU fuel, qualification of U-10Mo formed into a monolithic foil is being performed. Fuel qualification involves irradiating fuel specimens in the ATR. The irradiation tests provide an opportunity to benchmark depletion capabilities of reactor physics codes in support of the ATR operation, as well as develop benchmarks that can be used by other institutions to benchmark other reactor physics codes. This paper documents the development of a benchmark model of the irradiation of the ATR Full-size plate In center flux trap Position 7 (AFIP-7) experiment using the depletion codes MC21 and Advanced Dimensional Depletion for Engineering of Reactors (ADDER).

Nielsen, Joseph W. [Idaho National Laboratory (INL

Participation in and Assessment of the Second DNCSH Public Workshop

The DOE/NRC Criticality Safety for Commercial-Scale HALEU Fuel Cycle and Transportation (DNCSH) project was established through the Inflation Reduction Act of 2022 (H.R. 5376) to support the US Nuclear Regulatory Commission (NRC) and industry in addressing critical experiment validation gaps that impede the licensing basis and regulatory approval of high-assay low-enriched uranium (HALEU) operations. An initial public workshop was held in February 2024 to address HALEU transportation validation gaps. The resulting call for proposals was released in April and resulted in funding for the execution and/or evaluation of 16 critical experiments. A second public workshop was held in August 2025 to address facility and operational validation gaps, precluding a second call for proposals. A list of attendees is provided in APPENDIX A, Table A-1. A total of 319 participants joined the meeting, which was hosted online via Microsoft Teams as well as in person. The slides from the meeting were uploaded online to the NRC’s Agencywide Documents Access and Management System (ADAMS). The meeting agenda is provided in Table 1-1. In preparation for the meeting, a study was performed to examine expected fissile forms for the fuel cycles of various fuel types at different stages of production and the apparent validation gaps. The resulting report, titled “Benchmark Gap Assessment for the Manufacturing of High-Assay Low-Enriched Uranium Fuels,” provided the foundation for the discussions that took place during the workshop. The discussions and the validation gaps in the report were used to develop the second call for proposals. The present report presents the feedback received before, during, and after the second workshop. All the data presented are based on voluntarily self-reported identification, opinions from workshop participants, and survey responses and are assumed to be as accurate as practically reasonable. The discussions during the workshop and the subsequent survey responses were intended to direct attention to industry-specific areas of interest and to collect feedback on the work performed to date by the DNCSH project.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS

Tensile properties of co-rolled Zr/U-10Mo fuel at ambient and elevated temperatures

The United States High Performance Research Reactor (USHPRR) initiative is currently interested in replacing high-enriched uranium fuel in research reactors with high-assay low-enriched uranium fuel. Here, this work aimed to assist in that mission by providing tensile and bend test data on bare U-Mo and tensile test data on co-rolled Zr/U-10Mo plates at differing thicknesses (0.285 mm, 0.300 mm, and 0.465 mm) and temperatures (293 K, 473 K, and 623 K). Yield strength and ultimate tensile strength values are reported along with an in-depth comparison of how temperature, rolling direction, thickness, and the presence of the Zr-interlayer affect mechanical properties. Results showed that yield strength and ultimate tensile strength in Zr/U-10Mo foils lower as temperature increases by approximately 300 MPa from 293 to 473 K, and another 100 MPa from 473 to 623 K. Additionally it was found that with increased temperature, there is less differentiation in fuel necking and delamination behavior, as well as a greater perceived elongation to fracture. The elastic modulus of co-rolled mini-plates does not follow the volumetric rule of mixtures in terms of averaged strength and is actually lower than the reported moduli of both Zr and U-10Mo.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS

A new HALEU isotopic certified reference material

Candidate certified reference material (CRM) U196 was prepared by gravimetrically mixing and dissolving NNSA NRMP CRM 112-A (natural uranium metal) and CRM 116-A (highly enriched 93.2% 235 U metal) to achieve a high-assay low-enriched uranium (HALEU) isotopic abundance reference material. CRM U196 will be certified for the 233 U/ 238 U, 234 U/ 238 U, 235 U/ 238 U, and 236 U/ 238 U ratios. Gravimetrically determined uranium isotope amount ratios and values derived from the isotope data were calculated from the buoyancy corrected mass data and from certified values for the metal CRMs used to create the solution. The 235 U isotope amount fraction (·100) and expanded uncertainty is 19.5846 ± 0.0028. For attribute verification, total evaporation and modified total evaporation isotope ratio measurements were performed. In conclusion, the reference material is to be distributed as a unit containing 5 mg uranium as dry uranyl nitrate.

High-assay low-enriched uranium

Proceedings for the Workshop on Applied Nuclear Data Activities 2025

The 2025 Workshop for Applied Nuclear Data Activities (WANDA) covered four topic areas in nuclear data: Nuclear Data and Deterrence, Nuclear Data Prioritization for Fusion, High-Assay Low-Enriched Uranium and Novel Moderators for Advanced Reactors, and Data Preservation and Data Workflows. The intention of this workshop is to connect different communities that are invested in nuclear data and have their own unique sets of needs for the purposes of sharing information, fostering collaboration in areas of shared interest, and leveraging synergistic capabilities. The attendance of federal program managers at these workshops is essential in creating awareness of the needs of their respective communities and in providing information to better guide funding investments. In each of these topical sessions, a general description of the nuclear data needs and/or capabilities was presented, along with discussions of existing capabilities that could be leveraged, potential synergistic needs or resources, and challenges that must be overcome for the application space to progress. There are many synergistic nuclear data needs among these application spaces. The discussion largely focused on increasing the accuracy of the nuclear data and better quantifying the data uncertainties that have the greatest impact on applications. The full-day session on data processing and data workflows was by nature intended to be synergistic and applicable to all technical sessions at WANDA. A notable common theme that was highlighted across all sessions was the need for accelerated delivery of nuclear data products across complex and time-consuming workflows.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS

Developing New Fuels for High Performance Research Reactors

The National Nuclear Security Administration (NNSA) Material Management and Minimization (M3) program works globally to minimize the civilian use of highly enriched uranium (HEU), a weapon-usable nuclear material. Supporting this effort, M3’s Office of Reactor Conversion and Uranium Supply is developing new fuels capable of converting research reactors from HEU fuel to high-assay low-enriched uranium (HALEU) fuel. Some of the remaining research and test reactors (RTRs) operating on HEU today have unique designs, fuel configurations, and demanding performance requirements that cannot be met with an existing regulatory-approved low-enriched uranium (LEU) fuel. M3, DOE’s national laboratories, and other industry partners are qualifying new high-density LEU fuels to convert these RTRs while maintaining their unique capabilities supporting a wide variety of science and technology research in areas such as medicine, industry, defense, education, and training. Current efforts are focused on two options for the remaining US high-performance research reactor conversions: a monolithic uranium 10wt% molybdenum (U-10Mo) fuel form and a dispersion uranium silicide fuel form. This paper reviews the history and status of M3’s fuel qualification efforts for the U-10Mo LEU fuel form.

Montgomery, Rose [ORNL] (ORCID:0000000286038936)

Feasibility and strategic implications of deploying nuclear power reactors in Africa

This report assesses the feasibility and strategic implications of deploying nuclear power reactors, including large-scale plants, advanced small modular reactors (SMRs), and microreactors, in African countries. Case studies focus on South Africa, Egypt, Kenya, Ghana, and Nigeria, examining nuclear energy’s role in Africa’s rapidly evolving energy landscape, marked by fast-growing demand, significant electricity access gaps, increasing renewable penetration, and strong policy commitments to industrialization and energy security. Several U.S. reactor technologies and designs are considered based on their development status and readiness for deployment. The analysis finds that nuclear power can provide reliable, clean baseload and flexible generation, as well as high-temperature process heat for desalination, hydrogen production, and industrial applications. However, suitability is highly country-specific, depending on grid size and stability, transmission capacity, cooling water availability, regulatory readiness, and fuel supply chains. Near-term deployment opportunities are strongest for light-water reactors (such as NuScale, BWRX-300, AP300, and SMR-300) that use low-enriched uranium and build on proven technology. More advanced concepts, including gas-cooled, sodium-cooled, molten-salt cooled reactors, and microreactors, will likely be relevant for African deployment in the 2030s or later, contingent on demonstration projects, high-assay low-enriched uranium (HALEU) fuel availability, and mature international licensing frameworks. Economic analysis shows that SMRs are capital-intensive, with projected overnight costs for 300 MWe units in 2025 ranging from approximately 1.4 to 2.6 billion USD per module. The levelized cost of electricity (LCOE) is highly sensitive to the weighted average cost of capital (WACC). Given typically higher financing costs and utility balance-sheet weaknesses in many African countries, bankable project structures will require sovereign guarantees, robust offtake arrangements, and layered financing from export credit agencies, development finance institutions, and vendor nations. Comparisons with recent large nuclear projects in the United Arab Emirates (UAE) and Egypt underscore the central role of state-backed loans, long tenors, and concessional terms. Country case studies illustrate a spectrum of readiness and opportunity. South Africa operates two 920 MWe pressurized light water reactors (totaling 1,840 MWe) at Koeberg and has the most mature regulatory and industrial base, positioning it as a prime candidate for both large reactors and SMRs to replace coal, support desalination, and anchor industrial hubs. Egypt is constructing four VVER-1200 units at El Dabaa with strong state leadership and could later complement this fleet with SMRs for coastal and industrial applications. Kenya and Ghana are advancing through IAEA Milestones with growing institutional capacity and clear interest in SMRs that match their smaller grids and industrialization plans. Nigeria has the largest demand potential but faces acute constraints in grid reliability, project bankability, and regulatory capacity; targeted deployments of large reactors and SMRs near coastal or industrial sites could have high impact if accompanied by major grid upgrades and institutional reforms. The report identifies cross-cutting challenges such as financing, political continuity, public acceptance, nonproliferation and security, waste and back-end management, regulatory capacity, grid adequacy, and long deployment timelines for first-of-a-kind designs, and ANL/NSE-26/3 ii proposes broad directions for resolution. These include stronger multifaceted financing for nuclear, long-term national energy strategies that transcend electoral cycles, proactive stakeholder engagement, strengthened regional and national regulators, and systematic workforce development through centers of excellence and expanded training. The United States should develop partnerships with African countries and offer end-to-end nuclear package similar to those used effectively by competitors: coordinated project development, state-backed financing, long-term fuel services, and durable in-country support through regional offices and sustained workforce/regulatory training. With timely planning, sustained political commitment, and appropriate financing and institutional support, nuclear energy, both large reactors and advanced SMRs, can become a meaningful, though not dominant, pillar of Africa’s future power mix, enhancing energy security, enabling industrial growth, and supporting climate goals.

22 GENERAL STUDIES OF NUCLEAR REACTORS

Assessment of Uranium Isotope Impacts

This report examines the benefits and challenges associated with recycling recovered uranium (RU) from the used nuclear fuel (UNF) discharged from a once-through sodium-cooled fast reactor (SFR) with high-assay low-enriched uranium (HALEU) which has a higher residual U-235 content in the RU. However, there are three minor uranium isotopes that influence the value of the RU. There will be trace quantities of U-232 in RU, which can increase dose rates and, in turn, increase the cost of fuel fabrication. Additionally, the U-234 and U-236 isotopes are found in higher concentration in RU than in NU, and act as neutron poisons, requiring higher U-235 concentrations to compensate for the neutron poisoning effects of these isotopes.

07 ISOTOPE AND RADIATION SOURCES

Modeling a generic TRISO-fueled heat pipe microreactor using SCALE: Depletion, transportation criticality, and shielding

This paper demonstrates the applicability of the SCALE code system to tristructural-isotropic (TRISO)-fueled heat pipe microreactors through depletion, transportation criticality, and shielding analyses of a generic reference design. The study conducted supports US Nuclear Regulatory Commission code readiness efforts for advanced non–light-water reactor technologies and is intended as a code capability demonstration rather than as an optimization of a specific microreactor design. The modeled reactor employs high-assay low-enriched uranium (HALEU) uranium oxycarbide (UCO) TRISO fuel and beryllium oxide (BeO) reflectors and operates at 7.5 MWth with a nominal lifetime of about 3 effective full power years. Representative cases for fresh and irradiated cores were selected to exercise SCALE methods relevant to reactor operation and post-irradiation transport. The discharged-core decay heat is approximately 6% of operating power immediately after shutdown. Transportation criticality calculations show that internal water ingress is the dominant reactivity effect, with fully flooded fresh core and irradiated core configurations remain above the subcriticality criterion, even with the available control mechanisms. Shielding calculations for a simplified transportation package indicate that normal-condition dose rates are governed mainly by shielding thickness and cooling time, whereas the breached hypothetical accident case is governed primarily by cooling time. Overall, the study shows that SCALE supports depletion, transportation criticality, and shielding evaluations efficiently for TRISO-fueled heat pipe microreactors within a single code system.

Criticality

Consequence analyses of sabotage-induced radiological releases in sodium-cooled fast microreactors

Analysis of three sodium-cooled fast microreactors (SFMs) with thermal powers of 10, 30, and 50 MWt showed that smaller reactors result in lower radiological consequences during a postulated sabotage-induced event because of their reduced core inventory. All SFMs used U-10Zr metal fuel enriched to 15 wt% high-assay low-enriched uranium and operated until their respective effective multiplication factor (k eff ) reduced to less than 1 or until the end of their operational lifespan. Sabotage scenarios were simulated at this point, when the fuel inventory within the core contains the highest-level of radioactivity. Radionuclide core inventories were calculated using the SCALE code at shutdown and 3 days post-shutdown. Dose consequence analyses were performed for three sabotage scenarios using the RASCAL tool. As microreactor developers plan for minimal on-site or complete off-site emergency response, it remains essential to evaluate their physical protection needs and potential hazards, including assessing postulated sabotage-induced events that could become more relevant. SFM licensees should identify a credible worst-case, major accident, estimate release source terms, and perform dose consequence analyses to evaluate site-specific physical protection measures. In conclusion, this recommendation supports a risk-informed, performance-based approach, aligning with applicable regulatory requirements, i.e., 10 CFR Parts 100 and 53 rulemaking in the United States.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P

Consequence analyses of sabotage-induced radiological releases in high-temperature helium-cooled prismatic microreactors

Here, this study analyzes the radiological dose consequences of sabotage-induced accidents at three high-temperature helium-cooled prismatic microreactors (HTPMs) with thermal power ratings of 1, 10, and 50 MWt. Each HTPM employs uranium oxycarbide tristructural isotropic fuel enriched to 19.75 wt% high-assay low-enriched uranium. Simulations were conducted to estimate reactor core inventory at the point of fuel discharge––when the effective multiplication factor reduced to less than 1––representing peak radionuclide inventory. Postulated sabotage scenarios leading to reactor shutdown were analyzed at two intervals: immediately post-shutdown (0 h) and 3 days after shutdown using the SCALE code for radionuclide inventories and the RASCAL tool for dose consequences. Results show that although HTPMs benefit from inherent safety features and robust fuel design, radiological consequences scale with reactor power because of increased source term inventories. Smaller microreactors exhibited proportionally lower dose consequences. To support the economic and regulatory feasibility of microreactor deployment, this study emphasizes the value of a risk-informed, performance-based approach, as supported by regulations like 10 CFR Parts 100 and 53 in the United States. Microreactor developers should perform site-specific assessments of potential sabotage or low-probability, high-consequence events, especially when considering minimal on-site or full off-site emergency response.

Consequence

Technoeconomic Design Optimization for Fast Reactors. Part II: Impact of Technoeconomic Constraints on Optimal Design

There is a current drive toward optimizing reactors, particularly small/micro reactors to minimize cost and maximize performance. Previous work has investigated the development of technoeconomic workflows for the design optimization of pool-type fast reactors that aim to deploy into district energy grids. Initial scoping studies verified that the workflow was capable of capturing design trends throughout a variety of design configurations and problem formulations while remaining sufficiently flexible. In this paper, this methodology is applied to understand how cost functions and technoeconomic constraints can drive optimal reactor design. Specifically, the UPu10Zr-fueled fast reactor model from Part I is adapted to include changes in the fissile content limits, control rod worth limits, control rod drive cost, and assumed fuel form. In the case of constraint relaxation at fixed power (fissile content and control rod worth limits), cost sensitivities of 5% to 10% were uncovered. Multi-objective optimization at varying reactor power levels with individualized control rod drives for each assembly (as opposed to one operational and one safety drive) increased cost by $\$10$ to $\$25$ million and substantially altered the optimal core geometry, favoring geometries with substantially fewer control rod placements relative to baseline optimization. Finally, a multi-objective optimization was performed at varying power levels with the fuel form overhauled to metallic, high-assay low-enriched uranium–based U10Zr with more refined fuel cost models. In the case of uranium fueling, the costs increased by at least $50 million relative to the baseline case. Furthermore, economic fuel zoning and lower reactivity swing cores were recovered. Each case serves to demonstrate the value of applying technoeconomic workflows to initial reactor design scoping studies to better understand the trade-off for a proposed concept between different design options.

Argonne Reactor Computation (ARC) codes

Deimos: HALEU TRISO Heated Critical Experiment Data

Deimos was the first critical experiment using high-assay low-enriched uranium (HALEU) TRistructural ISOtropic (TRISO) fuel in over 40 years. HALEU TRISO is the desired fuel form for many of the advanced reactor designs in development; however, very little experimental data are available for this fuel type. Deimos was designed to utilize existing HALEU TRISO fuel in a large graphite moderator to obtain nuclear and reactor physics data to fill the gaps surrounding this fuel type and enrichment. In addition to cold critical data, three separate heated experiments were conducted to measure the temperature reactivity coefficient for this type of system. These measured coefficients were then compared to simulated coefficients to a first level order of fidelity. This comparison showed very good agreement for the experiment where only the inner core was heated and good agreement for the other two configurations, which included heating portions of the outer core. Less agreement when the outer core was heated is attributed to potential heating in the beryllium reflector, which has a positive temperature reactivity coefficient and was unaccounted for in the first-order models. Future heated experiments with Deimos will include temperature monitoring of the beryllium reflector to account for beryllium heating in the simulations.

22 GENERAL STUDIES OF NUCLEAR REACTORS

Assessment of Deep Burnup HALEU Fuel Impact and Requirements

This report explores advancements in nuclear fuel technology, focusing on once-through high-assay low-enriched uranium (HALEU) fuels. It examines the potential for increased fuel residence time in reactors and the fuel cost implications. The study highlights the differences between fast and thermal reactors in terms of fuel enrichment and burnup, emphasizing the complex relationship in fast reactors in which increased core size and fuel density can lead to lower enrichment requirements. Various advances in fuel technologies for light-water reactors (LWR) and sodium-cooled fast reactors (SFR) are presented in this report to provide more comprehensive analysis.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS

Study on Application of Distributed Network of Sensors with List Mode for NMAC Literature Review

Nuclear material accounting and control (NMAC) for nuclear security detects, deters, and resolves questions related to unauthorized removal (i.e. theft) or misuse of nuclear material. NMAC also serves as a key insider threat mitigation measure and aids in recovery of nuclear material that is missing. Effective nuclear security depends on NMAC for timely and accurate information about nuclear material types, quantities, and locations. Bulk nuclear material processing facilities, however, present unique challenges for effective NMAC due to the presence of large quantities of material in-process and the accumulation of residual material holdup within process equipment. These holdup accumulations can obscure accurate physical inventory taking and complicate efforts to resolve NMAC irregularities at the facility level. Bulk material monitoring systems often rely on material balance calculations and indirect measurement techniques, which may mask protracted theft of smaller amounts of nuclear material. These monitoring limitations have generated increased interest in continuous monitoring technologies, including distributed non-destructive assay (NDA) sensor networks capable of providing real-time or near-real-time measurement of material movement and accumulation within bulk processing environments. Recent advancements in distributed networks of NDA radiation detectors and sensing technologies provide an opportunity to address these limitations. Although such distributed sensor networks have been implemented in select facilities for IAEA Safeguards applications, their potential for supporting NMAC functions specifically tailored to nuclear security objectives remains largely unexplored. Furthermore, emerging list-mode data acquisition technologies have reached high technology readiness levels, enabling time-correlated detection of nuclear events across multiple temporal scales. These capabilities provide enhanced opportunities for accurate holdup measurement, continuous process monitoring, and improved detection of material theft or misuse over time. The increasing global expansion of civil nuclear power and development of related bulk material processing facilities, including those supporting high-assay low-enriched uranium (HALEU) and other advanced reactor fuel fabrication, further increases the need for advanced measurement and monitoring strategies for NMAC.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS

Nuclear Security Risks for HALEU Fuels

There is growing interest in high-assay low-enriched uranium (HALEU) for use in advanced nuclear reactors as a high-energy fuel source. The primary objectives of this report are to identify the security risks that directly result from HALEU and to identify the gaps and challenges it presents from a theft and sabotage perspective. This study focuses on HALEU security risks for the front end of the fuel cycle and includes a review of the supply chain, fuel fabrication, and transport for terrestrial reactors.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS