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Hf2OsRu crystallizes in the orthorhombic Immm space group. The structure is one-dimensional and consists of two Hf2OsRu ribbons oriented in the (1, 0, 0) direction. Hf is bonded in a linear geometry to one Os and one Ru atom. The Hf–Os bond length is 2.31 Å. The Hf–Ru bond length is 2.27 Å. Os is bonded in a linear geometry to two equivalent Hf atoms. Ru is bonded in a linear geometry to two equivalent Hf atoms.
Hf2OsRu is Heusler structured and crystallizes in the cubic Fm-3m space group. The structure is three-dimensional. Hf is bonded in a body-centered cubic geometry to four equivalent Os and four equivalent Ru atoms. All Hf–Os bond lengths are 2.82 Å. All Hf–Ru bond lengths are 2.82 Å. Os is bonded in a body-centered cubic geometry to eight equivalent Hf atoms. Ru is bonded in a body-centered cubic geometry to eight equivalent Hf atoms.